量子点激子超辐射的条件和量子点集合的相干辐射

半导体量子点的激子超辐射出现的条件是本文激子超辐射的理论研究中的重点,我们的理论推导结果揭示要观测到半导体量子点的激子超辐射必须采用短于百飞秒的激发源。我们用ZnO单量子点观察到激子超辐射,同时测量和分析讨论了量子点集合的相干辐射性质,发现单量子点超辐射的二次方泵浦与辐射强度关系被大量量子点间的线性递增所掩盖。     

Population inversion in a single InGaAs quantum dot using the method of adiabatic rapid passage

Preparation of a specific quantum state is a required step for a variety of proposed quantum applications. We report an experimental demonstration of optical quantum state inversion in a single semiconductor quantum dot using adiabatic rapid passage. This method is insensitive to variation in the optical coupling in contrast with earlier work based on Rabi oscillations. We show that when the pulse power exceeds a threshold for inversion, the final state is independent of power. This provides a new tool for preparing quantum states in semiconductor dots and has a wide range of potential uses.     

Electrical control of hole spin relaxation in charge tunable InAs/GaAs quantum dots

We report on optical orientation of singly charged excitons (trions) in charge-tunable self-assembled InAs/GaAs quantum dots. When the charge varies from 0 to -2, the trion photoluminescence of a single quantum dot shows up and under quasiresonant excitation gets progressively polarized from zero to approximately 100%. This behavior is interpreted as the electric control of the trion thermalization process, which subsequently acts on the hole-spin relaxation driven in nanosecond time scale by the anisotropic electron-hole exchange. This is supported by the excitation spectroscopy and time-resolved measurements of a quantum dot ensemble.     

Photoluminescence of single quantum wires and quantum dots

The results of a study into the photoluminescence spectra of a set of quantum dots based on GaAs enclosed in AlGaAs nanowires are presented. The steady state and time resolved spectra of photoluminescence under optical excitation both from an array of quantum wires/dots and a single quantum wire/dot have been measured. In the photoluminescence spectra of single quantum dots, emission lines of excitons, biexcitons and tritons have been found. The binding energy of the biexciton in the studied structures was deduced to be 8 meV.     

Growth and time-resolved photoluminescence study of self-organized CdSe quantum dots in ZnSe

Employing two different growth methods: standard molecular beam epitaxy (MBE) and low-temperature atomic layer epitaxy (ALE) with subsequent annealing, we have obtained high-quality quantum dot structures consisting of CdSe embedded in ZnSe. Single dot emission lines are observed in micro-luminescence. The samples have been investigated by further optical methods including time-resolved photoluminescence under resonant excitation at 4.2 K. Distinct properties of systems with three-dimensional confinement are observed such as the suppression of the interaction between isolated quantum dots (QDs). In standard quantum wells tunneling/hopping processes generally lead to a pronounced red shift of the luminescence over time due to a lateral localization of excitons in potential fluctuations. A much less pronounced red shift is observed for the QDs reflecting only the different lifetimes of single dots and higher excited states. The red shift completely vanishes under resonant excitation that selectively excites only a few QDs of the ensemble in the layer. Typical behaviour is also observed from the halfwidth of the quantum dot emission.     

Magneto optics of single photons emitted from single InAs/GaAs self-assembled quantum dots in a planar microcavity

We fully characterize the fine spectral structure of neutral and negatively charged single microcavity quantum dot excitons, using polarization-sensitive magneto-photoluminescence spectroscopy. We show that the microcavity allows the simultaneous detection of both the bright and dark excitons using Faraday configuration. Thus, we were able to fully determine the fine structure and the g-factors of the neutral and negatively charged single exciton states within the same single quantum dot. Our measurements are in excellent agreement with novel, many carrier model calculations, which take into account Coulomb and exchange interactions among all the confined e–h pair states.     

Another model for a multiexcitonic quantum dot in an optical microcavity

Very recently, a multiexcitonic quantum dot in an optical microcavity have been theoretically studied [Herbert Vincka, Boris A. Rodriguez, and Augusto Gonzalez, Physica E, 2006, 35: 99–102]. However, due to the inevitable damping losses through the microcavity, in this work, we will present a more precise and sound model in the Lindblad form master equation to investigate the photonic properties of a single quantum dot (QD) in an optical microcavity system, in which the QD may confine the multiexcitons and be in resonant interaction with a single photonic mode of an optical microcavity. The excitation energies, and the properties of the emission photon from the QD microcavity are computed as functions of the exciton-photon coupling strength, detuning, and pump rate. We further compare our results with their results, and find that the calculated intensity of the emitted photon and the spectra crucially depend on the exciton-photon coupling strength g, the photon detuning, and the number of excitons in the QD. Finally, we will give a physical mechanism of the dressed-state picture for the strong coupling between the single mode of an optical microcavity and the QD emitters to explain the details of the emission photon spectra. Our study establishes useful guidelines for the experimental study of such multiexcitonic quantum dot in an optical microcavity system.      

Dynamics of confined excitons and biexcitons of CuCl quantum dots

We investigated the dynamics of confined excitons and biexcitons in CuCl quantum dots in an NaCl matrix by using subpicosecond pump and probe absorption spectra, and time-resolved luminescence spectra. Then temporal changes of the absorption, optical gain, and luminescence are interpreted in relation to the exciton dynamics. The optical nonlinearity is discussed in terms of the exciton-exciton interaction in the quantum dot.     

Emission from neutral and charged excitons in a single quantum dot in a magnetic field

We report on optical spectroscopy of self-assembled InAs quantum dots in a magnetic field. We describe how we measure the emission characteristics of a single quantum dot (QD) in high magnetic fields at low temperature using a miniature, fiber-based confocal microscope. Example results are presented on a QD whose charge can be controlled using a field-effect device. For the uncharged, singly and doubly charged excitons we find a diamagnetism and the spin Zeeman effect. In contrast, for the triply-charged exciton we find a fundamentally different behavior. Anti-crossings in magnetic field imply that confined states of the QD are hybridized with Landau-like levels associated with the two-dimensional continuum.     

Charge oscillations in a double quantum dot in the Coulomb blockade regime

The two-electron dynamics in a symmetric double quantum dot placed in a onstant electric field is considered. It is shown that, despite the Coulomb blockade, interdot electron-density oscillations are possible. In these oscillations, a charge equal to the charge of a single electron is periodically transferred from one quantum dot to the other.     

Lifetime dispersion in a single quantum dot

We present a decay formula for photoluminescence of a single quantum dot. We apply the formula to time-resolved photoluminescence (PL) measurements for a single InAs/GaAs quantum dot. The formula works very well for the PL decays of excitons and biexcitons in the system. The physical basis of the formula originates from the temporal dispersion of lifetimes. PACS 78.67.Hc; 78.47.+p; 78.55.Cr; 71.35.-y     

Photoluminescence of charged magneto-excitons in InAs single quantum dots

We calculated the photoluminescence spectra of charged magneto-excitons in single two-dimensional parabolic quantum dots, using an unrestricted Hartree–Fock method. The calculated luminescence spectra explain well the observed red shifts of transition energies of InAs/GaAs single quantum dot by additional electron capture in a dot. The magnetic-field-induced transition of the ground state configuration of trapped electrons causes drastic change in the photoluminescence spectra. The dependence of photoluminescence intensities of charged excitons on the excess energies of photogenerated carriers above the bulk GaAs energy gap is studied phenomenologically, by calculating the steady state electron population probability in a dot.     

Quantum optical studies on individual acceptor bound excitons in a semiconductor

We demonstrate the generation of triggered single photons at a predetermined and well defined energy using the radiative recombination of single nitrogen-bound excitons in a semiconductor. The nitrogen atoms are embedded in a ZnSe quantum well structure and were excited by nonresonant optical pumping (82 MHz) at low temperature (4 K). We find resolution-limited photoluminescence lines (280 micro eV) which display photon antibunching under continuous optical pumping. Our results also suggest that single nitrogen-bound excitons are well suited for cavity quantum electrodynamics experiments.     

Energy spectra and lifetimes of quasiparticles in an open quantum dot surrounded by identical barriers in a cylindrical quantum wire

A theory of quasi-stationary states and lifetimes of electrons, holes, and excitons in an open cylindrical semiconductor quantum wire containing a quantum dot surrounded by two identical antidots (with potential barriers of finite height) is developed using the scattering matrix method. The energy spectra and lifetimes of electrons, holes, and excitons in a β-HgS/β-CdS/β-HgS/β-CdS/β-HgS nanoheterosystem are calculated and analyzed as functions of the geometric parameters of the quantum dot involved. It is demonstrated that an increase in the height of the quantum dot leads to a decrease in the energy of quasi-stationary exciton states of the Breit-Wigner type and to an increase in their lifetimes. The lifetime of exciton states is long enough for these states to be observed in the experiment.     

Charge and current beats in T-shaped qubit–detector systems

The time evolution of a charge qubit coupled electrostatically with different detectors in the forms of single, double and triple quantum dot linear systems in the T-shaped configuration between two reservoirs is theoretically considered. The correspondence between the qubit quantum dot oscillations and the detector current is studied for different values of the inter-dot tunneling amplitudes and the qubit–detector interaction strength. We have found that even for a qubit coupled with a single QD detector, the coherent beat patterns appear in the oscillations of the qubit charge. This effect is more evident for a qubit coupled with double or triple-QD detectors. The beats can be also observed in both the detector current and the detector quantum dot occupations. Moreover, in the presence of beats the qubit oscillations hold longer in time in comparison with the beats-free systems with monotonously decaying oscillations. The dependence of the qubit dynamics on different initial occupations of the detector sites (memory effect) is also analyzed.     

The electronic and optical properties of a triexciton in CdSe/ZnS core/shell quantum dot nanocrystals

In the study, we aim to investigate the electronic and optical properties of single excitons, biexcions and triexcitons in a CdSe/ZnS core/shell quantum dot nanocrystal. The electronic structure has been determined by solving of the Poisson–Schrödinger equations self-consistently. In calculations, the exchange-correlation effects between identical particles have been taken into account in the frame of the local density approximation. We have demonstrated that the optical properties of triexciton systems are remarkably different from the single and biexciton systems. Absorption peaks or transition energies of the triexciton system are well separated from those of single- and bi-exciton systems. We have observed that the core-radius dependent transition energy variations of triexcitons are higher when compared with single- and bi-excitonic systems. The transition energy shifts of double and triple excitons with respect to the single exciton have been calculated as a function of the core radius and we have shown that the energy shifts are inversely proportional with the radius. We have also investigated the radius-dependent changes in binding energies and lifetimes of the structures and the comparative results have been discussed in a detail manner.     

Impurity-modulated Aharonov–Bohm oscillations and intraband optical absorption in quantum dot–ring nanostructures

In this work we study the electronic states in quantum dot–ring complex nanostructures with an on-center hydrogenic impurity. The influence of the impurity on Aharonov–Bohm energy spectra oscillations and intraband optical absorption is investigated. It is shown that in the presence of a hydrogenic donor impurity the Aharonov–Bohm oscillations in quantum dot–ring structures become highly tunable. Furthermore, the presence of the impurity drastically changes the intraband absorption spectra due to the strong controllability of the electron localization type.     

Evolution of entanglement between distinguishable light states

We investigate the evolution of quantum correlations over the lifetime of a multiphoton state. Measurements reveal time-dependent oscillations of the entanglement fidelity for photon pairs created by a single semiconductor quantum dot. The oscillations are attributed to the phase acquired in the intermediate, nondegenerate, exciton-photon state and are consistent with simulations. We conclude that emission of photon pairs by a typical quantum dot with finite polarization splitting is in fact entangled in a time-evolving state, and not classically correlated as previously regarded.     

Coherent photonic coupling of semiconductor quantum dots

We report a new type of coupling between quantum dot excitons mediated by the strong single-photon field in a high-finesse micropillar cavity. Coherent exciton coupling is observed for two dots with energy differences of the order of the exciton-photon coupling. The coherent coupling mode is characterized by an anticrossing with a particularly large line splitting of 250 microeV. Because of the different dispersion relations with temperature, the simultaneous photonic coupling of quantum dot excitons can be easily distinguished from cases of sequential strong coupling of two quantum dots.     

Optically probing spin and charge interactions in a tunable artificial molecule

We optically probe and electrically control a single artificial molecule containing a well defined number of electrons. Charge and spin dependent interdot quantum couplings are probed optically by adding a single electron-hole pair and detecting the emission from negatively charged exciton states. Coulomb- and Pauli-blockade effects are directly observed, and tunnel coupling and electrostatic charging energies are independently measured. The interdot quantum coupling is shown to be mediated by electron tunneling. Our results are in excellent accord with calculations that provide a complete picture of negative excitons and few-electron states in quantum dot molecules.