Raman-gain,linewidth, and effectiveg-value with spin-flip-Raman scattering in inSb

In this paper we report on measurements of spin-flip-Raman gain inn-InSb as a function of the magnetic field. The measurements were carried out at temperatures of 1.8 K and 4.2 K and at a carrier concentration of 1.35×10¹⁵ cm^?3. The Raman cross sections obtained from these results, e.g. 1.25×10^?20 cm²/sr at a magnetic field of 10 kG and a pump frequency of 1884.35 cm^?1, agree very well with those theoretically predicted by Wherrett and Wolland. Furthermore, these measurements yield line shapes and linewidths of the spontaneous scattering (100–1500 MHz) and allow the determination of the effectiveg-value with an accuracy known from ESR-investigations. These results are discussed in terms of already published theoretical investigations.     

Magneto-Raman scattering inp-type indium antimonide

We report for the first time stimulated magneto-Raman scattering inp-type InSb. Two different Raman scattering processes were observed. The first one has a Raman shift of about 2cm⁻¹/kG and is observed at magnetic fields up to 30kG. The other one is observable only at high magnetic fields above 30kG and shows Raman shifts between 1.2cm⁻¹ and 3.0cm⁻¹ with a tuning rate of about 0.2cm⁻¹/kG. The first process can be interpreted either as spin-flip Raman scattering by photo-excited electrons in the conduction band or as Raman scattering by holes in the valence band involving transitions from heavy to light hole states. The other Raman shift observed seems to occur on account of transitions between the heavy hole ladders.     

Measurement of spin-flip raman gain,effectiveg-value and absorption of radiation under transient electric field conditions in insb

We studied the change in Spin-flip Raman (SFR) gain and behaviour of the effectiveg-value as a function of pulsed electric fields inn-type InSb. The samples were held at 1.8 K in magnetic fields up to 1.4 T. Varying the strength of a pulsed electric field applied to the samples parallel to the magnetic field we found a direct correlation between the increase in electron temperature and the decrease of the Raman gain. Measurements of the Raman gain and spontaneous line width at different times after the starting of the electric pulse and during its fall time with a time resolution of 10 ns give no indication of a motional narrowing of the SFR line and of an increase of the gain during the decrease of the electric field pulse. These two predictions were made by Mooradian et al. (1972) to explain the observed transient increase of the intensity of the stimulated SFR Stokes radiation after an electric field across the sample was switched off. With our direct measurement of the Raman gain we could establish that at any time during and after the electric field pulse, the gain is less or equal to the value without electric field. In the electric field region from 0.3 V/cm up to 0.6 V/cm the Raman gain shows several maxima, originating from SFR scattering between different spin splitted conduction band levels. The electron distribution under pulsed electric field conditions give rise to a dynamically varying absorption mechanism of transmitted radiation. Time resolved transmission measurements explain the observed increase of stimulated SFR Stokes radiation during the switch-off time of electric field pulses by a lower absorption of radiation and not by a larger gain.     

Spin-other-orbit interaction in highly excited configurations with p and g electrons in outer shells

The matrix of the operator of the spin-other-orbit interaction energy is constructed for npn’g and np ⁵ n’g configurations. The matrix elements of this operator are calculated in the single-configuration approximation with wave functions in the LSJM representation and in the representation of uncoupled angular momenta using the known general formulas. The spin-other-orbit interaction is represented by three direct and three exchange radial Marvin spin interaction integrals.     

Stimulated brillouin scattering in SF6 with a free-running XeCl laser as pump

A XeCl laser system without dispersive elements is used to investigate near threshold reflectivity and phase-conjugation (PC) fidelity of stimulated Brillouin scattering (SBS) mirrors with SF₆ as the active medium. Using different focal-length lenses to focus the broadband laser radiation into the Brillouin medium, it was found that at threshold the effective interaction length for SBS is equal to the confocal parameter and that the SBS gain is equal to its steady-state value for monochromatic pumping. High PC-fidelity values ranging from 0.8–1.0 were found under most of the experimental conditions investigated.     

Constrained current algebras and g/u(1) conformal field theories

Operator quantization of the WZNW theory invariant with respect to an affine Lie algebra with a constrained subalgebra is performed using Dirac's procedure. Upon quantization the initial energy-momentum tensor is replaced by the g/u(1)^d coset construction. The WZNW theory with a constrained current is equivalent to the su(2)/u(1) conformal field theory.     

Determination of temperature and concentration of molecular nitrogen,oxygen and methane with coherent anti-stokes raman scattering

Temperature and concentration measurements by Coherent Anti-Stokes Raman Scattering (CARS) of molecular nitrogen, oxygen and methane were carried out. A comparison of corrected thermocouple and CARS temperature measurements in a high-temperature furnace up to 2000 K is presented. The temperature dependent CARS spectra of N₂ and O₂ are evaluated by a simulation program. Agreement between CARS and thermocouple temperatures is obtained within 40 K for N₂ and 80 K for O₂. Good agreement is found between measurements and calculations of the decrease of CARS intensity with temperature. Various quick-fit methods for N₂-and O₂-temperature measurements from temperature sensitive spectral parameters were tested. Temperature dependent CARS spectra of thev ₁-fundamental of methane are recorded and the methane CARS intensity as function of temperature is measured.     

Optical properties and g factors of GaAs quantum rods

The Hamiltonian of the zinc-blende quantum rods in the framework of eight-band effective-mass approximation in the presence of external homogeneous magnetic field is given. The electronic structure, optical properties and electron g factors of GaAs quantum rods are investigated. We found that the electron g factors are very sensitively dependent on the dimensions of the quantum rods. As some of the three dimensions increase, the electron g factors decrease. The more the dimensions increase, the more the electron g factors decrease. The dimensions perpendicular to the direction of the magnetic field affect the electron g factors more than the other dimension.     

Influence of gas circulation on stimulated Raman scattering and amplification of ultrashort laser pulses in methane

Applying gas recirculation in a high pressure cell, laser pulses of 1 ps at 400 nm and with a repetition rate of 1 kHz were frequency shifted by stimulated Raman scattering and amplification in methane gas at high pressure. We studied the influence of gas recirculation on the conversion efficiencies into the Stokes and anti-Stokes components as well as on their spatial distributions and spectral shapes using generator and generator-amplifier arrangements. For high pump energies, recirculation in the generator cell decreases conversion efficiency into the first Stokes component whereas it increases conversion into higher Stokes and anti-Stokes components. It results in a significantly improved spatial characteristics of the frequency-shifted radiation, however, is accompanied by a substantial spectral broadening. Using gas recirculation in the generator-amplifier arrangement we achieved a conversion efficiency into the first Stokes component of about 50% with highly improved spatial and spectral characteristics.     

Holographic scattering lines observed with photorefractive BaTiO3

We investigate holographic scattering processes in BaTiO₃ pumped by two coherent copropagating waves. Four lines are observed on a screen behind the sample. The experimental results are well described by a model taking into account parametric mixing of four copropagating waves and limitations of optically induced space charge fields because of the finite trap density.     

Coherent anti-Stokes Raman scattering velocimetry with nearly degenerate pumps

The time evolution of the anti-Stokes signal produced from the non-linear interaction of a short Stokes pulse and two long pump pulses that are nearly degenerate in frequency has been investigated. It is shown that this approach allows us to specify the accuracy of CARS (coherent anti-Stokes Raman scattering) velocimetry and to extend the range of operation of the method. In addition, an original optical scheme capable of delivering short visible pulses with good spatial and spectral properties is reported. The optical bench has been used for the characterisation of a low-pressure laminar Mach-10 flow. Received: 24 October 2001 / Revised version: 8 January 2002 / Published online: 14 March 2002     

Performance of a Nd: YAG oscillator/ampflifier with phase-conjugation via stimulated Brillouin scattering

Phase conjugation via stimulated Brillouin scattering in CH₄ gas has been used to correct amplifier aberrations in a Nd: YAG oscillator/amplifier system. The single amplifier stage has been used in two-pass and four-pass arrangements. Using the four-pass arrangement incorporating compensation for thermal birefringence, a single-frequency diffraction-limited output of 350 mJ, in a compressed 6 ns pulse is achieved at 15 Hz repetition rate.     

Selective laser heating and nonlinear light scattering in a homogeneous medium

Observation of light scattering on the laser-produced temperature inhomogeneities, the centres of which are connected with some absorbing molecules, is reported. The experimentally observed scattering intensity agrees well theory.     

Determination of temperature by stimulated raman scattering of molecular nitrogen,oxygen, and carbon dioxide

We have determined the temperature from SRS spectra of N₂-N₂, N₂-CO₂, O₂-O₂, and CO₂-CO₂ recorded in wide pressure and temperature ranges. The fitting procedure takes simultaneously into account the Dicke effect and motional narrowing. We have quantified the accuracy of the MEG and ECS-P models for rotational relaxation. The temperature extracted from each model is compared with thermocouple measurements. The influence of vibrational broadening and shifting is discussed in detail.     

Efficient multi-frequency generation of ultrashort light pulses using stimulated Raman scattering and optical parametric amplification

Optical parametric amplification of multi-frequency seed pulses generated in a mixture of compressed hydrogen and methane by stimulated Raman scattering of 1 ps, 1 kHz laser pulses at 395.8 nm has been studied. Efficient generation of spectrally narrow ultrashort pulses with a spatial distribution close to the Gaussian profile of the pump beam was obtained in the visible and near infrared ranges.     

Off-resonant excitation of molecular vibrations in liquids,investigated by picosecond probe scattering

The coherent excitation of molecular vibrations in liquids via off-resonant stimulated Raman amplification is shown to consist of two parts with vastily different spectral and temporal properties. One component situated at the frequency difference _L –e _S of the driving fields follows almost instantaneously the system response function. The second part at the eigenfrequency e ₀ carries information on the vibrational dephasing. Detecting both frequency components simultaneously by coherent anti-Stokes probe scattering a novel 2-channel method is demonstrated. The vibrational dephasing time of thev ₃-mode of CH₃I is directly measured to beT ₂=2.6±0.15 ps. This result gives experimental support to the deconvolution techniques required in conventional spectroscopy.     

Transient conical parametric scattering of two orthogonally polarized waves in BaTiO3

The strength of the transient parametric scattering in BaTiO₃ is shown to be strongly dependent on the initial conditions of the sample illumination. It is shown that the effect can be explained by a considerable increase of the seeding radiation intensity after pre-exposure of the sample to the ordinarily polarized pump beam. Received: 27 March 2000 / Published online: 16 June 2000     

Tunable middle infrared radiation with HgGa2S4 crystal

Optical properties of orange phased HgGa₂S₄ crystal is investigated. Generation of tunable middle infrared radiation by second harmonic of tunable CO₂ laser radiation has been demonstrated. Second harmonic conversion efficiency with respect to other infrared crystal has also been discussed.