Temperature dependent narrow-band terahertz pulse generation in periodically poled crystals via difference frequency generation

Femtosecond optical pulse is used to generate narrow-band terahertz pulses depending on a quasi-phase-matched condition in periodically poled lithium niobate (PPLN) and stoichiometric lithium tantalate (PPSLT) crystals by difference frequency generation. The origin of narrow-band THz generation proved that the two frequency components of the fs pulse contribute to the frequency mixing. By cryogenic cooling, the absorption of THz waves in the crystal is significantly reduced which results in efficient THz generation. Simultaneously generated forward and backward THz pulses were 1.38 and 0.65 THz with as narrow as the bandwidth of 32 GHz in the PPSLT sample. Temperature dependence of the generated THz waveforms had good agreement with the simulation result using one dimensional plane-wave propagation model.     

Selection rules for indirect transitions in crystals with a zinc blende structure

Selection rules have been obtained for transitions between various irreducible combination of states and for intervalley transitions in crystals with a zinc blende structure, taking account of spin-orbit and time-reversal effects.In conclusion the author thanks V. A. Chaldyshev and N. V. Kudryavtsev for their constant interest in the work and for their valuable advice.     

基于闪锌矿晶体中受激电磁耦子散射产生可调谐太赫兹波的理论研究

基于受激电磁耦子散射原理,采用已报道的利用非线性光学参量振荡方法产生可调谐太赫兹波的实验条件作为理论分析的实验模型,以GaAs,GaP, InP,ZnTe晶体为代表,计算分析了在闪锌矿晶体中参量振荡产生太赫兹波的吸收、增益特性,对输出THz波的调谐特性给出了详尽分析.分析太赫兹波高效耦合输出的腔型结构,并与掺氧化镁铌酸锂晶体组成的太赫兹波参量振荡器做对比. 关键词： 太赫兹波 太赫兹波参量振荡 电磁耦子 闪锌矿晶体     

The effect of microsegregation on the generation of dislocations in zinc single crystals

The applicability of Tiller's considerations on the production of dislocations is proved. The density of dislocations appearing during impurity microsegregation increases with increasing rate of growth as a consequence of the corresponding change in the effective distribution coefficient. The real value of C at the microsegregation boundaries is at least twice as great as the average value of the concentration of impurities in the crystal in question.

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Zeeman effect of the direct exciton in zinc blende under uniaxial stress

Zeeman splitting of the direct exciton in zinc blende crystal under uniaxial stress is calculated. The simultaneous application of stress and a magnetic field will allow a precise determination of the electron and hole gyromagnetic factors.     

On the theory of the linear electro-optical effect in cubical crystals

The linear electro-optical effect in cubical crystals of acentric classes is considered by an approximate covariant method. Simple analytic expressions for the induced optic axes and for the eigenvalues and eigenvectors of the inverse dielectric tensor are obtained for all directions of the electric field in these crystals. The method used enables one to determine the above quantities with a high degree of accuracy. The cases where the electric field rotates in planes orthogonal to the crystallographic directions and in the planes of symmetry of the crystal are considered in detail.     

ZnTe晶体中光学整流产生的THz辐射及其电光探测研究

借助抽运-探测技术研究了ZnTe晶体中光学整流产生的太赫兹(THz)辐射，利用ZnTe晶体的线性电光效应探测THz辐射场分布，观察到了较窄(约为0.2 ps)的THz场分布及相应较宽(响应超过4 THz，半峰宽约为2.4 THz)的THz频谱，并运用琼斯矩阵对实验结果进行了理论拟合. 研究了飞秒激光脉冲波长(750—850 nm)、脉冲宽度(56—225 fs)和晶体旋转与THz辐射产生的关系. 同时改变探测光偏振方向进行偏振调制，并从理论上分析了偏振调制对THz辐射探测的影响. 关键词： THz辐射 光学整流 电光探测 ZnTe     

The effect of phototautomerism on the nonlinearity of the liquid crystals

The nonlinearity of hydroxy-azo dye doped liquid crystals is investigated and the effect of tautomerism is considered. The results indicate that, the nonlinearity of guest-host system can be affected by control of phototautomerism and incident light modulation. In special conditions, the variation of nonlinearity can be stable, so it can generate a stable refractive index pattern because of the optical reorientation of liquid crystal molecules.     

The generation of terahertz radiation via optical rectification in the self-induced transparency regime

The possibility of efficient terahertz generation via optical rectification in electro-optic crystal doped with the two-level resonant impurities is demonstrated. Under conditions of the self-induced transparency regime the laser pulses slows down to achieve the phase matching condition. The terahertz generation is accompanied by periodic modulation and spectral deformation of the laser pulse. The most efficient generation occurs under condition of small negative detuning from the resonant frequency of the two-level system.     

Two-color laser wavelength effect on intense terahertz generation in air

Near-IR femtosecond lasers have been proposed to produce high-field terahertz radiation in the air via the laser-plasma interaction, but the physical mechanism still needs to be further explored. In this work, we theoretically investigate the effect of the two-color laser wavelength on the terahertz generation in the air based on a transient photocurrent model.We show that the long wavelength laser excitation can greatly enhance the terahertz amplitude for a given total laser intensity. Furthermore, we utilize a local current model to illustrate the enhancement mechanism. Our analysis shows that the terahertz amplitude is determined by the superposition of contributions from individual ionization events, and for the long wavelength laser excitation, the electron production concentrates in a few ionization events and acquires the larger drift velocities, which results in the stronger terahertz radiation generation. These results will be very helpful for understanding the terahertz generation process and optimizing the terahertz output.     

Generating terahertz radiation via optical rectification in nonlinear crystals: Theory and experimental results

Key principles of terahertz radiation generation via laser pulse optical rectification are reviewed. The development of theoretical concepts is considered in connection with recent experimental results. The usability of resonant effects and metamaterials for the further development of this technique of generation is analyzed.     

Magnetic-field induced generation of A-like centers in Cz-Si crystals

The effect of the constant magnetic-field induced generation of oxygen–vacancy defects in Czochralski-grown silicon crystals was detected for the first time. The qualitative theory of the effect is given. It assumes that the effect arises from excitation of the Si–O bond of interstitial oxygen and is valid for both constant and pulsed magnetic fields. Experimental verification of the theory in the combined constant and pulsed fields strongly confirmed it.     

基于GaSe和ZnGeP2晶体差频产生可调谐太赫兹辐射的理论研究

基于非线性光学频率变换理论,采用已报道的利用非线性光学差频方法产生可调谐太赫兹波的实验条件作为理论分析的实验模型,计算模拟出在不同相位匹配条件下,GaSe和ZnGeP2晶体差频的相位匹配角、走离角、允许角和有效非线性系数,并对计算结果进行了分析比较,总结出对应输出不同太赫兹波长的最佳相位匹配方式.计算结果为利用非线性晶体差频产生可调谐太赫兹辐射的实验研究提供深入和全面的理论基础.     

The superprism effect in lithium niobate photonic crystals for ultra-fast, ultra-compact electro-optical switching

We numerically analyze ultra-refraction and slow-light in lithium niobate photonic crystals in order to investigate and then optimize the efficiency of a tunable photonic crystal superprism. In contrast to a passive superprism 1-to-N demultiplexer, we describe a tunable bandpass filter with only three output ports. The electro-optic effect in lithium niobate is used to achieve tunability, with the filter bandwidth shifting in wavelength as the refractive index of the superprism is modified by an externally applied electric field. Such a device could be used to realize a compact and fast wavelength multiplexer/demultiplexer for telecommunications or optical interconnect applications. We calculate constant frequency dispersion contours (plane-wave expansion) to identify initial configurations that show significant ultra-refraction, and verify the expected behavior of light propagation inside the structure using 2D FDTD (finite difference time domain) simulations. We show that the voltage requirements of such an electro-optically tunable superprism could potentially be relaxed by exploiting the enhancement of the electro-optic effect recently discovered by our group [M. Roussey, M.-P. Bernal, N. Courjal, D. Van Labeke, F.I. Baida, Electro-optic effect exaltation on lithium niobate photonic crystals due to slow photons. Appl. Phys. Lett. 89 (24) (2006) 241110], which we believe to be due to the presence of slow-light in the nanostructure. We present a methodology that readily identifies superprism design points showing both strong ultra-refraction as well as low group velocity. However, we find that this improved voltage efficiency comes at the cost of reduced operating bandwidth and increased insertion losses due to proximity to the band-edge.     

Optical second harmonic generation induced by picosecond terahertz pulses in centrosymmetric antiferromagnet NiO

Optical second harmonic generation at the photon energy of 2?ω = 2eV in the model centrosymmetric antiferromagnet NiO irradiated with picosecond terahertz pulses (0.4–2.5 THz) at room temperature is detected. The analysis of experimental results shows that induced optical second harmonic generation at the moment of the impact of a terahertz pulse arises through the electric dipole mechanism of the interaction of the electric field of a pump pulse with the electron subsystem of NiO. Temporal changes in optical second harmonic generation during 7 ps after the action of the pulse are also of an electric dipole origin and are determined by the effects of propagation of the terahertz pulse in a NiO platelet. Coherent oscillations of spins at the antiferromagnetic resonance frequency induced by the magnetic component of the terahertz pulse induce a relatively weak modulation of magnetic dipole optical second harmonic generation.     

Interplay between nonlocality and nonlinearity in nematic liquid crystals

Spatial nonlocality has a crucial role in the optical response of bulk liquid crystals. With specific reference to one-dimensional modulation instability, we demonstrate the tuning of transverse nonlocality in the nonlinear response of nematics.