Coexistence of superconductivity and magnetism

A model consisting of the B.C.S.-Hamiltonian and Zener's s-d exchange interaction is solved rigorously in the thermodynamic limit. Coexistence of superconductivity and magnetism is only possible for an impurity spin concentration smaller than a half at T ≠ 0.     

Coexistence problem of magnetism and superconductivity

The recent development of the problem of coexistence of magnetism and superconductivity will be reviewed. The possible coexistence of superconductivity with various types of magnetism carried by localized magnetic moments and itinerant electrons is critically discussed in connection with several existing materials such as rare earth ternary compounds [(RE)Mo₆S₈, (RE)Mo₆Se₈ and (RE)Rh₄B₄], newly synthesized organic superconductors [(TMTSF)₂X] and Y₉Co₇. In order to obtain a coherent picture for the understanding the rich phenomena associated with the interplay between two mutually exclusive types of long-range order, a unified point of view based on a key concept of the partial gapping model proposed by the author is introduced as a working hypothesis.     

Coexistence of superconductivity and magnetism theoretical predictions and experimental results

Superconductivity and ferromagnetic ordering are two antagonistic types of ordering, and their mutual influence leads to many interesting phenomena which have been studied recently in ternary compounds. Theoretical analysis of ferromagnetic materials which are type II superconductors near the superconducting transition point T _cl shows that they become type I near the magnetic transition point T _M. The proposed theory constructed for the case T _M « T _cl predicts the formation of a transverse domain-like (DS phase) magnetic structure below T _M. The electronic spectrum appears to be gapless in the DS phase of clean compounds with a re-entrant transition. The change from type II to type I behaviour as the sample is cooled to T _M has been observed in ErRh₄B₄. Experimental data for HoMo₆S₈, HoMo₆Se₈ and ErRh₄B₄ give evidence for the coexistence of super-conductivity and non-uniform magnetic ordering below T _M. Mutual influence of superconducting and magnetic orderings is also studied.     

Coexistence of magnetism and superconductivity in the hole doped FeAs-based superconducting compound

The magnetic and superconducting properties of the Sm-doped FeAs-based superconducting compound were investigated under wide ranges of temperature and magnetic field. After the systematical magnetic ion substitution, the superconducting transition temperature decreases with increasing magnetic moment. The hysteresis loop of the La_0.87?xSm_xSr_0.13FeAsO sample shows a superconducting hysteresis and a paramagnetic background signal. The paramagnetic signal is mainly attributed to the Sm moments. The experiment demonstrates that the coexistence of magnetism and superconductivity in the hole doped FeAs-based superconducting compounds is possible. Unlike the electron doped FeAs-based superconducting compounds SmFeAsOF, the hole doped superconductivity is degraded by the substitution of La by Sm. The hole-doped and electron-doped sides are not symmetric.     

Coexistence of superconductivity and ferromagnetism in ferromagnet/superconductor proximity structures

The Nambu spinor Green's function approach is applied to calculating the density of states (DOS) and superconducting order parameter in normal-metal/insulator/ferromagnet/superconductor (NM/I/FM/SC) junctions. It is found that the s-wave superconductivity and ferromagnetism can coexist near the FM/SC interface, which is induced by proximity effect. On the SC side, the spin-dependent DOS appears both within and without the energy gap. On the FM side, the superconducting order parameter displays a damped oscillation and the DOS exhibits some superconducting behavior. The calculated result for the DOS in FM for “0 state” and “π state” can reproduce recent tunneling spectra in Al/Al₂O₃/PdNi/Nb tunnel junctions. Received 1st July 2002 Published online 19 November 2002     

Coexistence of magnetism and superconductivity in the iron-based compound Cs0.8(FeSe0.98)2

We report on muon-spin rotation and relaxation (μSR), electrical resistivity, magnetization and differential scanning calorimetry measurements performed on a high-quality single crystal of Cs(0.8)(FeSe(0.98))(2). Whereas our transport and magnetization data confirm the bulk character of the superconducting state below T(c)=29.6(2) K, the μSR data indicate that the system is magnetic below T(N)=478.5(3) K, where a first-order transition occurs. The first-order character of the magnetic transition is confirmed by differential scanning calorimetry data. Taken all together, these data indicate in Cs(0.8)(FeSe(0.98))(2) a microscopic coexistence between the superconducting phase and a strong magnetic phase. The observed T(N) is the highest reported to date for a magnetic superconductor.     

Pyroelectric coupling in thin film photovoltaics

We propose a theory of thin film photovoltaics in which one of the polycrystalline films is made of a pyroelectric material grains such as CdS. That film is shown to generate strong polarization improving the device open circuit voltage. Implications and supporting facts for the major photovoltaic types based on CdTe and CuIn(Ga)Se₂ absorber layers are discussed.

     

Coexistence of ferromagnetism and superconductivity in normal mental/superconductor/ferromagnet structures

<正>We extend the Blonder,Tinkham and Klapwijk theory to the study of the inverse proximity effects in the normal mental/superconductor/ferromagnet structures.In the superconducting film,there are the gapless superconductivity and the spin-dependent density of states both within and without the energy gap.It indicates an appearance of the inverse-proximity-effect-induced ferromagnetism and a coexistence of ferromagnetism and superconductivity near the interface.The influence of exchange energy in the ferromagnet and barrier strength at the superconductor/ferromagnet interface on the inverse proximity effects is discussed.     

Superconductivity in Pb-PbTe thin film structures

The critical temperatures of thin superconducting films of Pb in intimate contact with PbTe have been measured resistively. The films were formed by sequential deposition and by co-evaporation of Pb and PbTe. The results show a depression of the critical temperature.     

Magnetic nonuniformity and thermal hysteresis of magnetism in a manganite thin film

We measured the chemical and magnetic depth profiles of a single crystalline (La(1-x)Pr(x))(1-y)Ca(y)MnO(3-δ) (x=0.52±0.05, y=0.23±0.04, δ=0.14±0.10) film grown on a NdGaO(3) substrate using x-ray reflectometry, electron microscopy, electron energy-loss spectroscopy, and polarized neutron reflectometry. Our data indicate that the film exhibits coexistence of different magnetic phases as a function of depth. The magnetic depth profile is correlated with a variation of chemical composition with depth. The thermal hysteresis of ferromagnetic order in the film suggests a first-order ferromagnetic transition at low temperatures.     

N掺杂SiO2纳米薄膜的制备及其磁性

利用射频磁控反应溅射技术,制备了氮掺杂的SiO₂纳米薄膜.发现N掺杂SiO₂体系纳米薄膜具有铁磁性.较小的氮化硅颗粒均匀分布在氧化硅基质中有利于磁有序的形成.基底温度为400℃时,样品薄膜具有最大的饱和磁化强度和矫顽力,分别为35 emu/cm³和75 Oe.薄膜的磁性可能产生于氮化硅和氧化硅的界面.理论计算表明,N掺杂SiO₂体系具有净自旋.同时,由氮化硅和氧化硅界面之间的电荷转移导致的轨道磁矩也会对样品的磁性有贡献 关键词： 2薄膜')" href="#">N掺杂SiO₂薄膜 射频磁控反应溅射 界面磁性 基底温度     

Coexistence of s-wave superconductivity and antiferromagnetism

We study the phase diagram of a new model that exhibits a first order transition between s-wave superconducting and antiferromagnetic phases. The model, a generalized Hubbard model augmented with competing spin-spin and pair-pair interactions, was investigated using the projector quantum Monte Carlo method. Upon varying the Hubbard U from attractive to repulsive, we find a first order phase transition between superconducting and antiferromagnetic states.     

Coexistence of superconductivity and magnetic order

Experimental work on systems showing evidence of the coexistence of superconductivity and magnetic order is reviewed. The presently known systems are shown to be “superconducting spin glasses” rather than “ferromagnetic superconductors”. In those systems where the magnetic order is expected to be long-ranged (up to now) superconductivity vanishes as soon as the magnetic order appears. But it is not excluded that magnetic order with a correlation length larger than the superconductive coherence length can coexist with superconductivity.     

Coexistence of superconductivity and magnetic order

The microscopic theory of simple antiferromagnetic superconductors is extended to structures where the magnetic order is described by a spin-density wave. For the case where the magnetic system is inherently ferromagnetic, the free energy of the combined system is minimized with respect to the amplitude and the wave vector of the spin-density wave. It is found that the wave vector depends very weakly on temperature. We apply the theory to the coexistence region in ErRh₄B₄, finding a first-order re-entry transition.     

Competitions of magnetism and superconductivity in FeAs-based materials

Using the numerical unrestricted Hartree--Fock approach, we study the ground state of a two-orbital model describing newly discovered FeAs-based superconductors. We observe the competition of a (0, π) mode spin-density wave and the superconductivity as the doping concentration changes. There might be a small region in the electron-doping side where the magnetism and superconductivity coexist. The superconducting pairing is found to be spin singlet, orbital even, and coexisting s_xy + d_x²-y² wave (even parity).     

Coexistence of ferromagnetism and superconductivity in NiBi-binary alloy

We investigate the effects of the antiferromagnetic exchange coupling between the Nickel and Bismuth2 atoms (J_int2 < 0) on the magnetizations of the NiBi-binary alloy versus temperature and external magnetic field by means of the effective field theory. We find that the magnetization of the Ni, Bi1, Bi2 and total NiBi-binary alloy has two different magnetic phase transitions for the J_int2 < 0. One of them is a first-order phase transition (FOPT) at T_t = 0.349 and the other is a second-order phase transition (SOPT) at T_c = 0.791. We also study the hysteresis behaviors and we find that the values of the coercive field points of the Bi2 are higher than those of the Ni and Bi1. Moreover, Ni, Bi1 and Bi2 components have ferromagnetic hysteresis behaviors whereas the total NiBi has type II superconducting behavior. Therefore, we suggest that ferromagnetism and superconductivity coexist in the NiBi-binary alloy that is qualitatively good agreement with the some experimental and theoretical works.     

Coexistence of superconductivity and itinerant-antiferromagnetism in CrRe alloys

Zero field Re NMR of CrRe alloy with more than 18%Re in superconducting state has been observed. The nuclear spin-lattice relaxation time (T₁) of Re in the vortex state increases exponentially with decreasing temperature as in the case of BCS superconductor. The result shows a coexistence of superconductivity and itinerant-electron antiferromagnetism.     

Coexistence of superconductivity and ferromagnetism in two dimensions

Ferromagnetism is usually considered to be incompatible with conventional superconductivity, as it destroys the singlet correlations responsible for the pairing interaction. Superconductivity and ferromagnetism are known to coexist in only a few bulk rare-earth materials. Here we report evidence for their coexistence in a two-dimensional system: the interface between two bulk insulators, LaAlO(3) (LAO) and SrTiO(3) (STO), a system that has been studied intensively recently. Magnetoresistance, Hall, and electric-field dependence measurements suggest that there are two distinct bands of charge carriers that contribute to the interface conductivity. The sensitivity of properties of the interface to an electric field makes this a fascinating system for the study of the interplay between superconductivity and magnetism.     

Coexistence of superconductivity and ferromagnetism in ferromagnetic metals

We address the question of coexistence of superconductivity and ferromagnetism. Using a field theoretical approach we study a one-fermion effective model of a ferromagnetic superconductor in which the quasiparticles responsible for the ferromagnetism form the Cooper pairs as well. For the first time we solve self-consistently the mean-field equations for the superconducting gap and the spontaneous magnetization. We discuss the physical features which are different in this model and the standard BCS model and consider their experimental consequences.