基于表面等离子体激元效应的可调制滤波器

针对常用的光学滤波器滤波波长不可变的特点,提出一种利用表面等离子体激元效应实现可调制滤波的方法.该方法根据金属邻近电介质的介电常数发生改变时,金属与入射光波的表面等离子体激元耦合共振模式发生改变,以此实现滤波波长调制.在加工有亚波长纳米孔阵列的Au薄膜上制作了一可见光滤波器,实验中采用空气、酒精和油作为介质对器件进行调制.结果表明:相对于常用的光学滤波器,该器件由于可以方便地改变临近介质的介电常数,因此具有滤波波长连续可调、快速方便、波长变化精度高等特点.     

介电常数近零模式与表面等离激元模式耦合实现宽带光吸收

介电常数为零或近零模式在微纳结构中提供了一个新的方式调控光与物质的相互作用.本文首先利用金属圆盘阵列结构激发了表面等离激元共振,在共振频率处实现了光的局域效果;然后通过在金属-绝缘体-金属超表面微纳结构中加入掺杂半导体材料,利用上层金属圆盘阵列激发的表面等离激元共振诱导介电常数近零模式的产生,从而使得介电常数近零模式与表面等离激元模式发生耦合,在中红外波段实现了一个470 nm的宽带吸收效果;数值模拟结果显示,在宽带吸收处存在光场的强局域效果.与窄带吸收相比,宽带吸收有更广泛的应用,比如吸收器、传感器、滤波器、微测辐射热计、光电探测器、相干热发射器、太阳能电池、指纹识别和能量收集装置等.     

Enhanced optical transmission through a nanoslit by coupling light between periodic strips and metal film

Surface plasmon resonance （SPR） is obtained by exciting the surface plasmon （SP） at the metal and dielectric interface, which can greatly enhance the extraordinary optical transmission （EOT） through a nanoslit milled in the metal film. We present a structure with a 50-nm-wide silver nanoslit for EOT by coupling light into the dielectric interlayer between periodic strips and a metal film. When the period of the metallic strips is equal to the wavelength of the SPR, the transmission efficiency of 187.6 through the nanoslit is enhanced. The metallic strip width over the nanoslit is optimized to improve transmission efficiency, and the maximal efficiency of 204.3 is achieved.     

各向异性特异材料波导中表面等离子体的共振性质

使用时域有限差分法,研究了各向异性特异材料(AMM)作为包层的AMM/介质/AMM波导中表面等离子体的共振性质.色散关系表明,当特异材料为负磁导率的always-cutoff型时,AMM/介质/AMM波导支持TE极化的表面等离子体,表面等离子体的波长随着中间介质层的厚度和特异材料磁等离子体频率的减小而变短.在有限长度AMM/介质/AMM波导中,由于两端界面的反射,表面等离子体模在波导中形成Fabry-Perot共振,而实现亚波长的表面等离子体微腔.在共振频率,电场强度在微腔的中部达到最大值,而磁场分别在两端界面处达到最大,电磁能强局域在中间介质层中,这一性质将在可调的具有强局域特性的亚波长微腔及腔量子电动力学中具有潜在的应用.     

Outcoupling surface plasmons into propagation modes using a subwavelength dielectric grating for device applications

Coupling of surface plasmon polaritons to radiation modes by use of a one-dimensional subwavelength dielectric grating on a thin metal slab is discussed. The surface plasmon waves obtained in Kretschmann configuration are resonant outcoupled to radiation modes by using a subwavelength dielectric grating. A peak outcoupling efficiency is predicted to be 74.57% with rigorous coupled-wave analysis. In addition, potential applications of these results in the design and improvement of various optoelectronic devices, such as polarizers, wavelength filters and biochemical sensors are discussed.     

Photonic bandgap structures for long-range surface plasmon polaritons

Propagation of long-range surface plasmon polaritons (LR-SPPs) along periodically thickness-modulated metal stripes embedded in dielectric is studied both theoretically and experimentally for light wavelengths in the telecom range. We demonstrate that symmetric (with respect to the film surface) nm-size thickness variations result in the pronounced band gap effect, and obtain very good agreement between measured and simulated (transmission and reflection) spectra. This effect is exploited to realize a compact wavelength add-drop filter with the bandwidth of 20 nm centered at 1550 nm. The possibilities of achieving a full bandgap (in the surface plane) for LR-SPPs are also discussed.     

多组分金属聚合体的光学纳米复合体系(英文)

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Dielectric layer-dependent surface plasmon effect of metallic nanoparticles on silicon substrate

The electromagnetic interaction between Ag nanoparticles on the top of the Si substrate and the incident light has been studied by numerical simulations. It is found that the presence of dielectric layers with different thicknesses leads to the varied resonance wavelength and scattering cross section and consequently the shifted photocurrent response for all wavelengths. These different behaviours are determined by whether the dielectric layer is beyond the domain where the elcetric field of metallic plasmons takes effect, combined with the effect of geometrical optics. It is revealed that for particles of a certain size, an appropriate dielectric thickness is desirable to achieve the best absorption. For a certain thickness of spacer, an appropriate granular size is also desirable. These observations have substantial applications for the optimization of surface plasmon enhanced silicon solar cells.     

Infrared absorption by surface phonons and surface plasmons in small crystals

A continuum model is developed which describes the infrared absorption of interacting spheres very much smaller than the wavelength of light. A mode with uniform polarization inside the sphere is assumed responsible for the absorption. The frequency of this mode in a small isolated sphere can be greatly shifted from the bulk value due to the surface polarization charge. If the particles are not isolated, this frequency is also influenced by the dipolar interaction of neighboring particles. We find that it is possible to define an average dielectric function for a layer of small interacting, absorbing spheres which has the Lorentz form for either phonon or plasmon excitations. If both plasmon and phonon excitations are possible in the same particle, the absorption coefficient of the coupled system displays two resonances and an antiresonance.     

Sub‐wavelength interference pattern from volume plasmon polaritons in a hyperbolic medium

Inside of a hyperbolic medium, the principal components of the permittivity tensor have opposite signs causing the medium to exhibit a ‘metallicbr’ type of response to light wave sin one direction, and a ‘dielectric’ response in the other. Our study shows that inside hyperbolic media, volume plasmon polaritons (VPPs) propagate along the characteristic planes, forming distinct, directionally dependent optical responses. This is similar to the propagation of conventional surface plasmon polaritons (SPPs) along the planar interfaces separating the isotropic dielectrics and metallic slabs. Interestingly, the plasmon polariton propagates along the resonance cone in a volume of hyperbolic metamaterial crossing the interfaces of the constitutive materials. The Young's double‐slit scheme is used to study the spatially‐confined diffraction in a hyperbolic slab, made of many thin planar layers of a metal and dielectric, to obtain the sub‐wavelength interference pattern at the output interface. Proof‐of‐concept systems for producing such patterns applicable to nanolithography and subwavelength probes are demonstrated.     

光纤表面等离子体波传感器的温度特性的研究

本文从粒子振动的角度讨论了光纤表面等离子体波传感器对于温度的敏感特性。对于金属 /介质的表面等离子体波传感器 ,在界面处产生的等离子体振动实质是大量电子的集体振荡。在某一特定的波长的P光激励下 ,电子吸收了光子的能量而改变了原来的运动方式 ,当激励的光信号与电子群的固有振荡频率一致时 ,大量的电子振动变为一种谐振。由于界面处的电子密度与温度是密切相关的 ,不同的温度时密度不同———温度越高 ,电子的密度越大 ,而电子群的集体振荡又与电子的密度密切相关。所以温度的变化将对等离子体的共振频率产生非常重要的影响。利用了这一效应来补偿环境介质的温度变化 ,可以克服环境温度对测试所带来的影响。此外 ,本文也讨论了采用光纤SPW传感器可以进行多参数的测量。     

基于金属表面等离子激元控制光束的新进展

表面等离子激元(Surface plasmon polaritons,SPPs)是一种在金属-介质界面上激发并耦合电荷密度起伏的电磁振荡,具有近场增强、表面受限、短波长等特性,在纳米光子学的研究中扮演着重要角色。近年来表面等离子光学和基于SPPs的纳米光子器件的研究引起了国际上科学家们的广泛关注。讨论了SPPs的基本原理和在亚波长结构下的光学特性,介绍了基于亚波长金属结构的表面等离子激元在空间光束准直与聚焦、平面内光束聚焦与传导和在近场纳米光束的控制等方面的研究情况,以及在纳米光子学器件中的潜在应用。     

Plasmon modes of a superlattice — Classical vs quantum limits

The collective plasmon excitations of a superlattice are investigated in both the classical and quantum limits. Using a model that is applicable to superlattices whose constituent layers are either semiconductor- semiconductor, semiconductor-metal, or metal-metal, we show that the surface plasmon interface modes of each layer (slab) couple via the long range Coulomb interaction into two bands of plasmons with dispersion along the superlattice axis. Results for plasmon dispersion are presented for the classical limit (de Broglie wavelength less than the layer width) where the response is treated via a solution of Maxwell's equations using the bulk 3-D dielectric constant to describe each intervening layer. These results are compared to the plasmon dispersion in the quantum regime where the wave-vector frequency dependent dielectric constant of the superlattice is calculated taking into account quantization effects (subband structure). The relationship between the modes in both limits is derived.     

金纳米球壳表面等离激元共振波长调谐特性研究

理论研究了金纳米球壳的几何结构参数, 及物理参量对局 域表面等离激元共振波长调谐特性的影响. 结果表明, 随着壳层厚度的增大, 球壳消光共振峰先蓝移后红移, 高阶峰转向时对应的壳层厚度比低阶峰大, 且该厚度与球壳内径的比值随内径尺寸的增大而减小, 随内核材料或外界环境介电常数的增大而增大, 散射共振峰也有类似的移动规律. 利用电子杂化效应和相位延迟效应对该现象进行了理论解释.     

Propagation oscillations in the near-field response of traveling surface waves launched by metallic nanoapertures

We discuss the implications of a frequency-dependent complex dielectric function ε(ω) of a metal for the interpretation of scanning near-field optical microscopy (SNOM) measurements in the vicinity of metallic nanoapertures. For subwavelength slits in gold films we observe distinct spatial intensity oscillations in the near-field signal for specific wavelengths in the visible spectrum. These oscillations of the SNOM signal far away from the nanoslit are ascribed to a constructive interference between the propagating surface plasmon (SP) with light scattered parallel to the gold–air interface. In these spatial SNOM-signal oscillations information about the surface plasmon dielectric function is encoded which can be extracted, for example, in surface plasmon interferometry for applications as sensors or waveguides.     

Influence of amount of CTAB and ascorbic acid concentration on localized surface plasmon resonance property of gold nanorod

Gold nanorods (AuNRs) are prepared through seeded growth approach. Synthesis parameters of the amount of cetyltrimethylammonium bromide (CTAB), and concentration of ascorbic acid (AA) were studied. We were aiming for an aspect ratio of 3 which could be achieved by a nanorod feature in the range of 45 nm length and 15 nm width. The absorption spectra are observed with an UV–visible NIR spectrophotometer and analysed theoretically. It is known that there are two plasmon resonance peaks for gold nanorod corresponding to transverse surface plasmon resonance (TSPR) and longitudinal surface plasmon resonance (LSPR), respectively. It is found that as the concentration of CTAB increases, the yield of NRs increases. As the concentration of AA increased from 0.05 to 0.2 M, LSP shifts to longer wavelength but upon further increasing the concentration, LSP shifts back to shorter wavelength. A linear relationship between LSPR wavelength and surrounding medium dielectric constant is obtained, which is in good agreement with the theoretical results.     

表面等离子体激元微盘的优化设计及应用

表面等离子体激元(SPP)微腔具有很高的品质因子和极小的模式体积,在光电子器件研究方面具有重要的应用价值。采用有限元法对表面等离子体激元的金属覆盖介质微盘谐振腔进行理论模拟,研究考虑微盘底半径、介质层厚度及金属膜厚度等参数对微盘表面等离子体模的品质因子及模体积的影响。研究表明,在光通信波段1550nm附近获得高品质因子(1000以上),极低模式体积的表面等离子体微盘。最后研究了利用优化设计的微盘进行折射率传感的应用,获得了高达300nm/RIU的折射率传感灵敏度。     

Tunable optical sorting and manipulation of nanoparticles via plasmon excitation

We numerically investigate the optical forces exerted by an incident light beam on Rayleigh metallic particles over a dielectric substrate. In analogy with atom manipulation, we identify two different trapping regimes depending on whether the illumination is performed within the plasmon band or out of it. By adjusting the incident wavelength, the particles can be selectively guided, or immobilized, at the substrate interface.     

功能光学纳米Ag薄膜的制备及其光学特性研究

对以热蒸发法制备的超薄Ag薄膜,扫描电子显微镜结果显示其呈纳米尺度的颗粒状,由透射谱测量发现其具有表面等离子体激元特征.检测到不同条件制备纳米Ag薄膜的表面等离子体共振吸收峰的位移规律,且纳米Ag材料具有选择性的透过、反射特性.通过不同的制备条件,得到了在长波范围内透过率超过90％、在表面等离子体共振峰值位置处反射率接近50％且峰位可调的光学薄膜材料.这种薄膜材料有望成为应用在薄膜太阳电池中间层中具有潜在性光管理功能的光学薄膜材料. 关键词： 热蒸发 纳米Ag薄膜 表面等离子体激元 光管理