原子核的形状相变

简要回顾原子核形状相变研究的现状，并将相干态理论与角动量投影方法相结合，在不区分质子玻色子和中子玻色子的相互作用玻色子模型（IBM-1）框架下，对角动量驱动的轴对称情况下的具有U（5）、SU（3）对称性以及两种对称性之间过渡区的原子核的形状相变进行了具体研究。We review the status of the research of nuclear shape phase transitions in this paper. Meanwhile, by taking the coherent state theory and angular momentum projection method, we study the shape phase transitions of axially symmetric even-even nuclei with U（5） symmetry, SU（3） symmetry and those in the transitional region of the two symmetries in the framework of Interacting Boson Model-1 （IBM-1）, which does not distinguish the proton bosons from neutron bosons.     

原子刚性转子散射几率的密耦合波包法计算

本文分别在方向固定于空间的质心坐标系(以下简称SF坐标系)和随体坐标系(以下简称BF坐标系)两种坐标系中,详细地讨论了最近发展起来的密耦合波包理论,以He-H₂为碰撞体系,计算了其态-态跃迁几率,结果表明:(1)在两种坐标系中建立的理论是等价的,其计算结果与标准的密耦合(以下简称CC)法计算的结果符合良好;(2)如果耦合项数增加,则在BF坐标系中密耦合波包法的计算效率将明显高于在SF坐标系中密耦合波包法的计算效率。 关键词：     

Size control of charge-orbital order in half-doped manganite La0.5Ca0.5MnO3

Motivated by recent experimental results, we study the effect of size reduction on half-doped manganite, La(0.5)Ca(0.5)MnO(3), using the combination of density-functional theory (DFT) and dynamical mean-field theory (DMFT). We find that upon size reduction the charge-ordered antiferromagnetic phase, observed in bulk, is destabilized, giving rise to the stability of a ferromagnetic metallic state. Our theoretical results, carried out on a defect-free nanocluster in isolation, establish the structural changes that follow upon size reduction to be responsible for this. Our study further points out the effect of size reduction to be distinctively different from application of hydrostatic pressure. Interestingly, our DFT+DMFT study additionally reports the correlation-driven stability of the charge-orbitally ordered state in bulk La(0.5) Ca(0.5) MnO(3), even in the absence of long-range magnetic order.     

弯曲振动引致的过渡态的混沌

从单摆运动的特征出发 ,指出分子的过渡态 (包括解离时的态 ) ,如分子内弯曲振动引致结构变化的过渡态 ,必然伴随着混沌现象 ,而且和Chirikov的多重共振会导致混沌的观点有关 .并以从HCN、HNC和其非局域态的高激发振动态的能级拟合得到的弯曲模式的性质说明这个观点 .最后 ,提出一个处理弯曲振动引致的过渡态的混沌的物理模型 .     

Quantal phases, disorder effects, and superconductivity in spin-Peierls systems

In view of recent developments in the investigation on cuprate high- T(c) superconductors and the spin-Peierls compound CuGeO3, we study the effect of dilute impurity doping on the spin-Peierls state in quasi-one-dimensional systems. We identify a common origin for the emergence of antiferromagnetic order upon the introduction of static vacancies and superconductivity for mobile holes.     

Analytical solutions describing the phase separation driven by a free energy functional containing a long-range interaction term

We are primarily concerned with the variational problem with long-range interaction. This functional represents the Gibbs free energy of the microphase separation of diblock copolymer melts. The critical points of this variational problem can be regarded as the thermodynamic equilibrium state of the phase separation phenomenon. Experimentally it is well-known in the diblock copolymer problem that the final equilibrium state prefers periodic structures such as lamellar, column, spherical, double-diamond geometries and so on. We are interested in the characterization of the periodic structure of the global minimizer of the functional (corresponding to the strong segregation limit). In this paper we completely determine the principal part of the asymptotic expansion of the period with respect to epsilon (interfacial thickness), namely, we estimate the higher order error term of the period with respect to epsilon in a mathematically rigorous way in one space dimension. Moreover, we decide clearly the dependency of the constant of proportion upon the ratio of the length of two homopolymers and upon the quench depth. In the last section, we study the time evolution of the system. We first study the linear stability of spatially homogeneous steady state and derive the most unstable wavelength, if it is unstable. This is related to spinodal decomposition. Then, we numerically investigate the time evolution equation (the gradient flow of the free energy), and see that the free energy has many local minimizers and the system have some kind of sensitivity about initial data. (c) 1999 American Institute of Physics.     

Local moment and ferromagnetic state formation in dilute,degenerate d-electron alloys: Ferromagnetic versus antiferromagnetic interactions

In this note the Kim [1] non-degenerate Anderson model (NDAM) of random dilute alloys treatment of local moment and ferromagnetic state formation is generalized to the ten-fold degenerate Anderson model (TDAM) of Siegel and Kemeny [2], Siegel [3,4] and Moriya [12]. We first determine how an impurity state is modified by neighboring impurities. For a simple binary alloy the local electron state at each impurity site depends upon the local distribution of other impurities. Second we derive a TDAM general relationship for the occurrence of a local moment on one impurity and the ferromagnetic ordering of the total impurity spins. Lastly we derive the impurity-impurity TDAM magnetic interaction; for the direct transfer interaction the impurity-impurity magnetic interaction can be ferromagnetic or antiferromagnetic depending upon the fractional occupation of impurity states. At each stage we compare our results with those of Kim's NDAM treatment.     

非全熔合反应裂变角分布

采用核固体径迹探测器测量了¹⁶O+¹⁵⁹Tb、¹⁶O+¹⁹⁷)Au和¹⁶O+²⁰⁹Bi反应碎片角分布,扣除中等质量碎片(IMF)的贡献,用过渡态统计模型(TSM)和单个自旋标准理论拟合实验的裂变角分布,提取裂变核的自旋. 讨论了它随质心系入射能量的变化.     

Characteristics of helium DC plasma jets at atmospheric pressure with multiple cathodes

A novel DC plasma torch with multiple cathodes is developed for generating laminar, transitional and turbulent plasma jets. The jet's characteristics, including jet appearance, voltage fluctuation, thermal efficiency, specific enthalpy, and distributions of temperature, pressure, and velocity, are experimentally investigated. The results show that as the gas flow rate increases, the plasma jet transforms first from the laminar state to the transitional state and second to the turbulent state. Compared with the transitional/turbulent jet, the laminar jet possesses not only a better stability and a longer hightemperature zone but also a higher average/core temperature and a higher specific enthalpy at the nozzle's outlet. With the change of jet states from the laminar to the turbulent flow, the core pressure and velocity at the nozzle's outlet increase,while the decaying rates of temperature/pressure/velocity along the jet's axial direction increase sharply. Furthermore, applications of laminar, transitional and turbulent jets for zirconia spray coating are described. The test results indicate that the long laminar jet is favorable for the deposition of a high-quality coating because the powder particles injected into the laminar jet may have better heating and lower kinetic energy.     

Carrier-mediated ferromagnetism in N co-doped (Zn, Mn)O-based diluted magnetic semiconductors

Mn-doped ZnO is anti-ferromagnetic spin glass state, however, it becomes half-metallic ferromagnets upon hole doping. In this Letter we report a theoretical study of (Zn, Mn)O system codoped with N, and show that this codoping can change the ground state from anti-ferromagnetic to ferromagnetic. We have carried out the first-principles electronic structure calculations and report total energy to estimate whether the ferromagnetic state was stable or not. Our approach is based on the spin-polarized relativistic Korringa–Kohn–Rostoker (SPR–KKR) density functional theoretical (DFT) method, within the coherent potential approximation (CPA). Self-consistent electronic structure calculations were performed within the local density approximation, using the Vosko–Wilk–Nusair parameterization of the exchange-correlation energy functional. Our results for energy difference between ferromagnetic sate and spin glass state as well as their dependence on concentrations were presented and discussed.     

反扭曲向列相液晶盒中的引流

根据Erickson-Leslie流体动力学方程,研究了反扭曲向列相液晶盒.该液晶盒只有在有外场的情况下才会扭曲.通过计算模拟得出指向矢构形和流速与时间的关系.在外加电压情况下,由于存在引流效应导致指向矢分布不正常.     

原子核过渡区的量子相变

在相互作用玻色子模型(IBM) 基础上用O(6) 高阶项代替传统的SU(3) 四极-四极相互作用来研究原子核从振动到转动过渡区的量子相变行为。利用U(5)-SU(3) 和UQ 两种方案,在玻色子数分别为N = 8 和N = 20 不同情况下,研究了原子核的一些低激发态的能级比和电四极跃迁比。结果表明:随着玻色子数N 的增大,系统的量子相变行为得到加强;两种方案都可以用来描述从振动到转动过渡区的原子核的量子相变特征且O(6) 高阶项方案下量子相变行为更为明显。在此基础上,进一步应用这两种方案具体讨论了152Sm 核的低激发态能级和电四极跃迁性质并与实验数据进行对比分析。结果表明,用O(6) 高阶项可以更为合理地描述带内跃迁及不同带之间的带间跃迁性质。With the framework of Interacting Boson Model(IBM), transitional patterns from the spherical to the axially deformed limit of the IBM with a schematic Hamiltonian are studied by replacing the SU(3) quadrupole-quadrupole term with O(6) cubic interaction. But, we use the two schemes to investigate some energy ratios and B(E2) ratios for different bosons N = 8 and N = 20. The results show that with the increasing of the numbers of bosons, the transitional behaviors can be enhanced; the transitional behaviors are very similar in the two schemes. However, there are some distinctive differences for some quantities across the entire transitional region, such as energy levels and ratios, B(E2) values and ratios, and expectation values of the shape variables. Generally speaking, the transition is smoother and the nuclear shape is less well defined in the new scheme. Then we apply the two schemes to the critical point symmetry candidate, such as 152Sm, and find the overall fitting quality of the UQ scheme is better than that of the U(5)-SU(3) scheme, especially for the inter-band E2 transitions in 152Sm.     

Half-metallicity induced by out-of-plane electric field on phosphorene nanoribbons

Exploring the half-metallic nanostructures with large band gap and high carrier mobility is a crucial solution for developing high-performance spintronic devices. The electric and magnetic properties of monolayer zigzag black-phosphorene nanoribbons (ZBPNRs) with various widths are analyzed by means of the first-principles calculations. Our results show that the magnetic ground state is dependent on the width of the nanoribbons. The ground state of narrow nanoribbons smaller than 8ZBPNRs prefers ferromagnetic order in the same edge but antiferromagnetic order between two opposite edges. In addition, we also calculate the electronic band dispersion, density of states and charge density difference of 8ZBPNRs under the action of out-of-plane electric field. More interesting, the addition of out-of-plane field can modulate antiferromagnetic semiconductor to the half metal by splitting the antiferromagnetic degeneracy. Our results propose a new approach to realize half-metal in phosphorene, which overcomes the drawbacks of graphene/silicene with negligible band gap as well as the transitional metal sulfide (TMS) with low carrier mobility.     

基于三维简并四波混频的PDT光敏剂HA瞬态光栅特性研究

竹红菌甲素(hypocrellin A,HA)具有丰富的激发态特性,有可能在新型光动力疗法(PDT)光敏剂、激光染料和新型光电器件方面有一定的应用前景。利用瞬态光栅技术研究了竹红菌甲素分别在不同极性和粘度溶剂中以及溶剂本身的瞬态光栅特性,把其瞬态光栅的超快过程归结为竹红菌甲素质子转移形成的过渡态TS*的衰减,得出过渡态TS*瞬态光栅的寿命为10.5 ps。竹红菌甲素分子的质子转移过渡态TS*瞬态光栅寿命不受溶剂极性和粘度的影响。     

Study of the <Superscript>190</Superscript>Hg Nucleus: Testing the Existence of U(5) Symmetry

In this paper, we have considered the energy spectra, quadrupole transition probabilities, energy surface, charge radii, and quadrupole moment of the¹⁹⁰Hg nucleus to describe the interplay between phase transitions and configuration mixing of intruder excitations. To this aim, we have used four different formalisms: (i) interacting boson model including configuration mixing, (ii) Z(5) critical symmetry, (iii) U(6)-based transitional Hamiltonian, and (iv) a transitional interacting boson model Hamiltonian in both interacting boson model (IBM)-1 and IBM-2 versions which are based on affine \( \widehat{SU\left(1,1\right)} \) Lie algebra. Results show the advantages of configuration mixing and transitional Hamiltonians, in particular IBM-2 formalism, to reproduce the experimental counterparts when the weight of spherical symmetry increased.     

Diffusion of poly(diallyldimethylammonium chloride) in aqueous solutions with added salt

The peculiarities of the fluctuation motions of diallyldimethylammonium chloride polyions (PDADMAC) in 0.01M, 0.025M, and 0.05M NaCl aqueous solutions were studied depending on the polyion concentration by means of dynamic and static light scattering. The behavior of the system in a transitional region between dilute and unentangled semidilute solutions was investigated. The nature of the fastest and slowest motion modes is discussed; additional modes observed upon scattering in semidilute solutions were attributed to interaction modes.     

Parallel Detection of Multiple Transitional Spectral Patterns Using Optical Spectrogram Scope

In measurement of ultrafast phenomena caused by several photochemical reactions, multiple transitional spectral patterns contained in a signal pulse are directly associated with different interactions, allowing us to identify individual interactions from these patterns. We propose a new method by which we can detect multiple transitional spectral patterns contained in a signal pulse in parallel using optical spectrogram scope (OSS). In the experimental demonstration, we used an arrayed filter composed of matched filters recording three kinds of transitional spectral patterns in the OSS system, and we directly detected two different patterns contained in a signal pulse in parallel.     

Properties of QBist State Spaces

Every quantum state can be represented as a probability distribution over the outcomes of an informationally complete measurement. But not all probability distributions correspond to quantum states. Quantum state space may thus be thought of as a restricted subset of all potentially available probabilities. A recent publication (Fuchs and Schack, , 2009) advocates such a representation using symmetric informationally complete (SIC) measurements. Building upon this work we study how this subset—quantum-state space—might be characterized. Our leading characteristic is that the inner products of the probabilities are bounded, a simple condition with nontrivial consequences. To get quantum-state space something more detailed about the extreme points is needed. No definitive characterization is reached, but we see several new interesting features over those in Fuchs and Schack (, 2009), and all in conformity with quantum theory.     

Large-eddy simulation of flows past a flapping airfoil using immersed boundary method

The numerical simulation of flows past flapping foils at moderate Reynolds numbers presents two challenges to computational fluid dynamics: turbulent flows and moving boundaries. The direct forcing immersed boundary(IB) method has been developed to simulate laminar flows. However,its performance in simulating turbulent flows and transitional flows with moving boundaries has not been fully evaluated. In the present work,we use the IB method to simulate fully developed turbulent channel flows and transitional flows past a stationary/plunging SD7003 airfoil. To suppress the non-physical force oscillations in the plunging case,we use the smoothed discrete delta function for interpolation in the IB method. The results of the present work demonstrate that the IB method can be used to simulate turbulent flows and transitional flows with moving boundaries.     

场冷条件下超导块材的吸引力与排斥力

基于K im临界态模型,通过考虑超导块材内部屏蔽电流的穿透历史过程,其计算了不同场冷条件下高温超导悬浮系统的悬浮力。其计算结果与实验结果吻合很好。结果显示:超导块材的最大吸引力随场冷高度的升高呈指数关系减小;达到最大吸引力的悬浮高度随场冷高度的增加近似呈线性关系增长。最大排斥力随场冷高度的变化曲线存在临界值:当场冷高度小于临界值时,最大排斥力呈线性关系增加;反之,最大排斥力呈指数关系增长。悬浮力与场冷高度的这些变化规律可以用超导块材内部屏蔽电流的穿透情况进行很好地解释,为超导块材的实际工业应用提供了重要的理论依据。