De Haas-van Alphen oscillations in the quasi-two-dimensional organic metal (BEDO-TTF)5[CsHg(SCN)4]2

The magnetization oscillations in the quasi-two-dimensional organic metal (BEDO-TTF)₅[CsHg(SCN)₄]₂ are thoroughly investigated over a wide range of magnetic field directions at different temperatures down to 0.4 K. The results obtained are in good agreement with the shape and sizes of the Fermi surface calculated from the x-ray diffraction data. Apart from the fundamental frequencies, the combination frequencies are found in the magnetization oscillation spectrum. It is demonstrated that these combination frequencies are governed by the motion of charge carriers along the real closed orbits inside the network of magnetic breakdown orbits formed under the action of the magnetic field. It is uniquely established that the combination frequencies previously revealed in the magnetoresistance oscillation spectrum of the same metal are associated with the quantum interference effect. The angular dependences of the oscillation amplitude exhibit minima, which are explained by the spin splitting of the Landau levels.     

Inverse magnetoresistance in (FeCoB)-(Al<Subscript>2</Subscript>O<Subscript>3</Subscript>) magnetic granular composites

The magnetoresistance, magnetization, and microstructure of granular composites with the general formula (Fe₄₀Co₄₀B₂₀)_x(Al₂O₃)_100?x were studied for contents of the amorphous metallic component both above and below the percolation threshold (x≈43). The low-temperature transverse magnetoresistance of the composites is negative at x=41 and practically zero for x=49. For metal contents below the percolation threshold (x=31), a noticeable (7–8%) positive magnetoresistance, reached in magnetic fields of about 17 kOe, was observed. Possible mechanisms of the generation of inverse (positive) magnetoresistance are discussed.     

Hydrostatic-Pressure-Induced Reentrance of the Metallic State in the κ-(ET)2Hg(SCN)2Cl Quasi-Two-Dimensional Organic Conductor

On cooling below 30 K, the κ-(ET)₂Hg(SCN)₂Cl quasi-two-dimensional organic metal, which is in the quantum spin liquid state at liquid helium temperatures, undergoes a transition to the Mott insulator state. The application of a hydrostatic pressure p = 0.7 kbar stabilizes the metallic state and makes it possible to study the behavior of the interlayer magnetoresistance at liquid helium temperatures. The field dependence of the magnetoresistance exhibits an unlimited power-law growth, which indicates that the polaron mechanism contributes to the interlayer transport. The spectrum of observed magnetoresistance oscillations corresponds to the Fermi surfaces characteristic of conducting layers with the κ-type structure.

     

Electric and magnetic properties of the perovskites Ba2(FeMo)O x (5.88 ≤ x 6.01)

The purpose of this work is to establish the relation between the magnetic, electric, and magnetotransport properties and the oxygen nonstoichiometry of the compounds Ba₂(FeMo)O _x (5.88 ≤ x ≤ 6.01). The investigations established the behavior of the magnetization, resistance, and magnetoresistance of samples in this series. It is shown that the behavior of the magnetization can be described by assuming that the iron ions become divalent (Fe³⁺→ Fe²⁺) as a result of the reduction of the samples and the molybdenum ions become hexavalent (Mo⁵⁺ → Mo₆₊) as a result the oxidation of the samples. It is established that there are two contributions to the magnetoresistance which arise as result of magnetic ordering of the intragranular interlayer and intergranular transfer of spin-polarized charge carriers. It is inferred that electric transport in samples of this series is determined by percolation processes between granules with metallic conductivity separated by a dielectric interlayers.     

Anomalies of magnetoresistance of compounds with atomic clusters RB12 (R = Ho, Er, Tm, Lu)

The magnetoresistance and magnetization of single-crystal samples of rare-earth dodecaborides RB₁₂ (R = Ho, Er, Tm, Lu) have been measured at low temperatures (1.8–35 K) in a magnetic field of up to 70 kOe. The effect of positive magnetoresistance that obeys the Kohler’s rule Δρ/ρ = f(ρ(0, 300 K)H/ρ(0, T)) is observed for the nonmagnetic metal LuB₁₂. In the magnetic dodecaborides HoB₁₂, ErB₁₂, and TmB₁₂, three characteristic regimes of the magnetoresistance behavior have been revealed: the positive magnetoresistance effect similar to the case of LuB₁₂ is observed at T > 25 K; in the range T _N ≤ T ≤ 15 K, the magnetoresistance becomes negative and depends quadratically on the external magnetic field; and, finally, upon the transition to the antiferromagnetic phase (T < T _N ), the positive magnetoresistance is again observed and its amplitude reaches 150% for HoB₁₂. It has been shown that the observed anomalies of negative magnetoresistance in the paramagnetic phase can be explained within the Yosida model of conduction electron scattering by localized magnetic moments. The performed analysis confirms the formation of spin-polaron states in the 5d band in the vicinity of rare-earth ions in paramagnetic and magnetically ordered phases of RB₁₂ and makes it possible to reveal a number of specific features in the transformation of the magnetic structure of the compounds under investigation.     

Frequency combinations in the magnetoresistance oscillations spectrum of a linear chain of coupled orbits with a high scattering rate

The oscillatory magnetoresistance spectrum of the organic metal (BEDO)₅Ni(CN)₄. 3C₂H₄(OH)₂ has been studied up to 50 T, in the temperature range from 1.5 K to 4.2 K. In high magnetic field, its Fermi surface corresponds to a linear chain of quasi-two-dimensional orbits coupled by magnetic breakdown (MB). The scattering rate consistently deduced from the data relevant to the basic α and the MB-induced β orbits is very large which points to a significant reduction of the chemical potential oscillation. Despite of this feature, the oscillations spectrum exhibits many frequency combinations. Their effective masses and (or) Dingle temperature are not in agreement with either the predictions of the quantum interference model or the semiclassical model of Falicov and Stachowiak.     

Low temperature magnetization and magnetoresistance studies on the layered manganite system La1.2Sr1.8Mn2−xRuxO7 (x=0, 0.1, 0.5, 1.0)

We report the detailed results of magnetization and magnetoresistance measurements in the Ru doped layered manganite system La_1.2Sr_1.8Mn_2−xRu_xO₇ (x=0, 0.1, 0.5, 1.0). High-resolution measurements of magnetization and magnetoresistance were carried out as functions of temperature, magnetic field and time. We find evidence for the existence of competing ferromagnetic and antiferromagnetic interactions resulting in the formation of a frustrated spin-glass-like state at low temperatures. The time dependent magnetization follows the relation very well. We find that Ru doping enhances the coercive field and drives the system towards a magnetically mixed phase at low temperatures. Large negative magnetoresistance values are observed in all samples and at low temperatures the magnetoresistance varies as the square root of the applied magnetic field.     

Existence of two-dimensional closed orbits and delocalized carriers in the spin-ordered state of quasi-one-dimensional (TMTSF)2PF6

The magnetoresistance in spin-ordered state of quasi-one-dimensional (TMTSF)₂PF₆ has been studied. Both the frequency and anisotropy of the magnetoresistance oscillations are found to be independent of temperature; this proves the temperature independence of the geometry of two-dimensional closed contours at the Fermi level. At the same time, the oscillation amplitude decreases with the temperature, indicating the depopulation of the closed contours in the T = 0 limit. An explanation for the above seemingly controversial results has been proposed.     

Magnetic oscillations in the 2D network of compensated coupled orbits of the organic metal (BEDT-TTF) 8 Hg 4 Cl 12 (C 6 H 5 Br) 2

Interlayer magnetoresistance and magnetisation of the quasi-two dimensional organic metal (BEDT-TTF)₈Hg₄Cl₁₂(C₆H₅Br)₂ have been investigated in pulsed magnetic fields extending up to 60 T and 33 T, respectively. About fifteen fundamental frequencies, composed of linear combinations of only three basic frequencies, are observed in the oscillatory spectra of the magnetoresistance. The dependencies of the oscillation amplitude on the temperature and on the magnitude and orientation of the magnetic field are analyzed in the framework of the conventional two-dimensional Lifshitz-Kosevitch (LK) model. This model is implemented by damping factors which accounts for the magnetic breakthrough occurring between electron and hole orbits yielding conventional Shubnikov-de Haas closed orbits (model of Falicov and Stachowiak) and quantum interferometers. In particular, a quantum interferometer enclosing an area equal to the first Brillouin zone area is evidenced. The LK model consistently accounts for the temperature and magnetic field dependence of the oscillation amplitude of this interferometer. On the contrary, although this model formally accounts for almost all of the observed oscillatory components, it fails to give consistent quantitative data in most other cases. Received 4 September 2002 / Received in final form 14 November 2002 Published online 27 January 2003 RID="a" ID="a"e-mail: audouard@insa-tlse.fr RID="b" ID="b"UMR 5830: Unité Mixte de Recherche CNRS - Université Paul Sabatier - INSA de Toulouse RID="c" ID="c"UMS 5642: Unité Mixte de Service CNRS - Université Paul Sabatier - INSA de Toulouse     

Existence of two-dimensional closed orbits and delocalized carriers in the spin-ordered state of quasi-one-dimensional (TMTSF)2PF6

The magnetoresistance in spin-ordered state of quasi-one-dimensional (TMTSF)₂PF₆ has been studied. Both the frequency and anisotropy of the magnetoresistance oscillations are found to be independent of temperature; this proves the temperature independence of the geometry of two-dimensional closed contours at the Fermi level. At the same time, the oscillation amplitude decreases with the temperature, indicating the depopulation of the closed contours in the T = 0 limit. An explanation for the above seemingly controversial results has been proposed. The text was submitted by the authors in English.     

Coulomb blockade anisotropic magnetoresistance effect in a (Ga,Mn)As single-electron transistor

We observe low-field hysteretic magnetoresistance in a (Ga,Mn)As single-electron transistor which can exceed 3 orders of magnitude. The sign and size of the magnetoresistance signal are controlled by the gate voltage. Experimental data are interpreted in terms of electrochemical shifts associated with magnetization rotations. This Coulomb blockade anisotropic magnetoresistance is distinct from previously observed anisotropic magnetoresistance effects as it occurs when the anisotropy in a band structure derived parameter is comparable to an independent scale, the single-electron charging energy. Effective kinetic-exchange model calculations in (Ga,Mn)As show chemical potential anisotropies consistent with experiment and ab initio calculations in transition metal systems suggest that this generic effect persists to high temperatures in metal ferromagnets with strong spin-orbit coupling.     

Metastable structure and properties of (La0.73Bi0.27)0.67Ca0.33MnO3

The electrical transport and magnetic properties of high Bi doped (La_0.73Bi_0.27)_0.67Ca_0.33MnO₃ are studied at the temperature and magnetic field ranges from 10 to 300 K and 0 to 3 T. Significant temperature and magnetic field hystereses are observed in both resistivity and magnetization measurements. Meanwhile, an enhanced magnetoresistance effect, within a wide temperature window, is obtained in the (La_0.73Bi_0.27)_0.67Ca_0.33MnO₃. The hysteresis and enhanced magnetoresistance are discussed based on an inhomogeneous metastable structure related to the Bi dopant.     

Effect of oxygen non-stoichiometry on magnetic and electrical transport properties of La0.67Sr0.33MnO3

The effect of oxygen deficiency and oxygen excess on the magnetic and electrical transport properties of La_0.67Sr_0.33MnO₃ has been investigated. The thermal and isothermal magnetization measurement results show that the Curie temperature and saturation magnetization of oxygen deficient sample (defined as A) are higher than those oxygen excess sample (defined as B). The electrical resistivity of A is lower than that of B in studied temperature range. The magnetoresistance (MR) of B is larger than that of A in the temperature range from 280 to 360 K, which agrees with the magnetic field needed full spin polarization at room temperature. The colossal MR (CMR) around transition temperature from ferromagnetic metal to paramagnetic insulator (T_MI) for A is larger than that for B, which arises from assistance of stronger lattice deformation for A.     

Magnetoresistance of carbon-covered Co nanowires

We have investigated the magnetoresistance of carbon-coated Co nanowires with various widths down to w=32 nm at low temperatures (T=4.2 K). The nanowires and their non-magnetic contact pads are prepared by means of a three-step electron beam lithography (EBL) process in a LEO secondary electron microscope. We obtain wires with highest quality by using specifically customized resist systems with undercut. The longitudinal magnetoresistance shows pronounced features at the coercive fields H_c—where H_c increases with decreasing wire width as —indicating a magnetization reversal process accomplished by domain nucleation and traversal. In contrast, the transverse and perpendicular magnetoresistance continuously decrease to their saturation values which can be understood in terms of a coherent rotation of the magnetization using the anisotropic magnetoresistance.     

The electric conductivity of a laminated metal system (alternating magnetic and nonmagnetic layers)

A set of kinetic equations for the distribution functions of carriers differing both by the energy spectrum and by the spin projection is used to investigate the conductivity of a multilayer sample (alternating layers of magnetic (m) and nonmagnetic (_n) metals). The boundary conditions on the interlayer surfaces are derived in an approximation in which the surface scattering is divided into “specular” and “diffuse” scattering and is characterized by scattering parameters (reflection and transmission) which are related to each other by relations dependent on spin projections and on the type of spectrum. The problem on the longitudinal (with respect to the layers) current is treated; situations are analyzed in which the variation in conductivity due to the change of mutual orientation of magnetization in successive m layers from antiparallel to parallel may be of the order of the values of the conductivity proper (the so-called giant magnetoresistance effect). This is possible only in the case of thin (compared with the free path) n layers (in m layers, the ratios of the characteristic dimensions may be arbitrary) and in the mandatory presence of specular surface scattering. Results are given for different possible ratios of Fermi momenta of electron groups and for different fractions of specular and diffuse scattering. The possibility of realizing the effects of both signs is demonstrated.     

Magnetic and magnetotransport properties of nanocrystalline (Fe2B)0.20X0.80 (X=Ag or Cu) alloys prepared by mechanical alloying

The magnetic and magnetotransport properties of nanocrystalline (Fe₂B)_0.20X_0.80 (X=Ag or Cu) alloys have been studied by Mössbauer, magnetization and magnetoresistance (MR) techniques. The samples were prepared by mechanical alloying the nanostructured Fe₂B alloy and Ag or Cu chemical elemental powders in a high-impact mill machine. The Mössbauer spectroscopy and magnetic measurements of as-milled (Fe₂B)_0.20Ag_0.80 and annealed (Fe₂B)_0.20Cu_0.80 alloys indicate the presence of small Fe and Fe₂B magnetic particles. The magnetoresistance curves of (Fe₂B)_0.20X_0.80 (X=Ag or Cu) alloys show a non-saturated behavior, an indication of a spin-glass-like state generated by the magnetic coupling between these magnetic particles. The non-saturated effect is more pronounced in the alloy with Ag, where the MR values decrease linearly with the external magnetic field, even at 7 T. The magnetoresistance values, at 4.2 K and for a magnetic field of 7 T, are 4.0% and 4.5%, for (Fe₂B)_0.20Ag_0.80 and (Fe₂B)_0.20Cu_0.80 samples, respectively.     

Magneto-transport and magnetic properties of (1-x)La0.7Ca0.3MnO3+xAl2O3 composites

We report magneto-transport and magnetic properties of (1-x)La_0.7Ca_0.3MnO₃+xAl₂O₃ composites synthesized through a solid-state reaction method combined with a high energy milling method. Most interestingly, the effective magnetic anisotropy is found to decrease with increase in the non-magnetic insulating Al₂O₃ phase fraction in the composites. In addition, we observed that the magnitude of low-field magnetoresistance arising from spin-polarized tunneling of conduction electrons, as well as that of high-field magnetoresistance, displays a Curie-Weiss law-like behavior. Finally, we found that the temperature dependence of low and high-field magnetoresistance is controlled predominantly by the nature of temperature response of surface magnetization of the particles.     

钙钛矿(La1-yTby)0.67Sr0.33MnO3的超巨磁电阻效应

采用固相反应烧结法制成了钙钛矿(La_1-yTb_y)_0.67Sr_0.33MnO₃(y=0—1)多晶样品.研究了样品的微观结构,常温、低温下的磁性,样品的磁电阻随温度、成分的变化关系,电阻随温度变化特性等.并在y=0.40样品中,170K附近、最大磁化场为7T时,观察到了900%的巨磁电阻. 关键词：     

Highly oriented La2/3Ca1/3MnO3 films grown on silicon-on-insulator substrates by pulsed laser deposition

High quality La_2/3Ca_1/3MnO₄(LCMO) thin films have been deposited on silicon-on-insulator (SOI) substrates only buffered by yt tria-stabilized zirconia (YSZ) by using the pulsed laser deposition (PLD) technique. The results obtained from X-ray diffraction (XRD), reflection high energy electron diffraction (RHEED), scanning electron microscopy (SEM) and magnetization investigations indicate that the LCMO films are highly oriented both in-plane and out-of-plane. The Curie temperature T _c is close to 260 K and the insulator–metal (I–M) transition appears around 220 K. The conducting mechanism at low temperatures is dominated by the electron–magnon scattering. A tensile stress from the film–substrate lattice mismatch results in magnetic ‘easy axes’ in the film plane and the magnetic anisotropy energy increases with cooling. A maximum magnetoresistance (MR) is observed near 190 K, with the external magnetic field either parallel or vertical to the LCMO film plane. Moreover, the large intrinsic high-field magnetoresistance (HFMR) and the very small extrinsic low-field magnetoresistance (LFMR) again reveal that the LCMO films on SOI substrates are highly oriented thin films of good crystallinity.     

High-frequency spin-dependent tunnelling in magnetic nanocomposites: Magnetorefractive effect and magnetoimpedance

Since the dielectric permittivity is linear with frequency-dependent conductivity, high-frequency properties for any kind of magnetic materials with the high magnetoresistance depend on magnetization. It manifests as magnetorefractive effect (MRE) in the infrared region of spectrum and as magnetoimpedance (MI) in the frequency range between radio and microwaves. The main mechanism of both MRE and MI in nanocomposites with tunnel-type magnetoresistance is high-frequency spin-dependent tunnelling. We report on recent results of theoretical and experimental investigations of MRE and MI in nanocomposites Co_51.5Al_19.5O₂₉, Co_50.2Ti_9.1O_40.7, Co_52.3Si_12.2O_35.5 and (Co_0,4Fe_0,6)₄₈(MgF)₅₂. Most of the obtained experimental data for MRE and MI are consistent with the theory based on considering the tunnel junction between adjacent granules in percolation cluster as a capacitor.