Isomeric ratios in photonuclear reactions of molybdenum isotopes induced by bremsstrahlung in the giant dipole resonance region

We have determined the isomeric ratios of isomeric pairs ^97m,gNb, ^95m,gNb and ^91m,gMo produced in ⁹⁸Mo(γ, p)^97m,gNb, ⁹⁶Mo(γ, p)^95m,gNb and ⁹²Mo(γ, n)^91m,gMo photonuclear reactions in the giant dipole resonance (GDR) region by the activation method. The results were analyzed, discussed and compared with the similar data from literature to examine the role of excitation energy, neutron configuration, channel effect and direct and pre-equilibrium processes in (γ, p) photonuclear reactions. In this work the isomeric ratios for ^97m,gNb from 14 to 19 MeV, for ^195m,gNb from14 to 24 MeV except 20 and 23.5 MeV and for ^91m,gMo at 14 and 15 MeV are the first time measurements.     

Isomeric cross-section ratios for (n, 2n) reactions induced by 14.7 MeV neutrons in In and Sb

Isomeric cross section ratios were measured for (n, 2n) reactions induced by 14.7 MeV neutrons in In and Sb isotopes. Experimental results were compared with the theoretical calculations performed with the Huizenga and Wandenbosch method.     

Near-barrier fusion reactions induced by α on197Au,193Ir,191Ir,185Re,181Ta,121Sb and69Ga nuclei

Fusion-evaporation cross-sections for the α-induced reactions upon¹⁹⁷Au,¹⁹³Ir,¹⁹¹Ir,¹⁸⁵Re,¹⁸¹Ta,¹²¹Sb and⁶⁹Ga nuclei at bombarding energies near the Coulomb barrier have been measured by off-line observation of the γ-rays emitted in the radioactive decay of the residual nuclei using stacked foil technique. The total fusion cross-section for the systems have been compared with simple statistical model calculations using the code ALICE/91 as well as with the coupled channel calculations that include the β₂ and ν₄ slatic deformations and dynamic couplings of the vibrational/rotational states of the target and the projet tile using the code CCDEF.     

Hyperfine interactions of light Ir,Re isotopes in iron

The technique of On-line Nuclear Orientation has been applied to light Ir and Re isotopes. Using both¹⁹²IrFe and⁵⁴MnNi thermometers, orientation as a function of temperature was measured over the range 10–100 mK. Pulsed implantation methods were used to obtain spectra with gamma transitions well identified and clear of contaminant activities. Magnetic moment/oriented state spin combinations were obtained for^180,182,183Ir and for^180,179Re. The results are briefly discussed.     

Energetic neutrons and gamma rays measured on the Aryabhata satellite

An experiment to measure energetic neutrons and gamma rays in space was launched in the first Indian scientific satellite,Aryobhata, on April 19, 1975. From this experiment, the first measurements in space of the Earth’s albedo fiux of neutrons of energy between 20 and 500 MeV have been made; the values obtained for two mean geomagnetic vertical cut-off rigidities of 5.6 and 17.0 GV are (6.3±0.4)×10⁻² and (1.4±0.3)×10⁻² neutrons cm⁻² sec⁻¹ respectively. These measurements confirm that protons arising from cosmic ray albedo neutron decay, can adequately account for the protons in the inner radiation belt. Observations on gamma rays of energy between 0.2 and 24 MeV have enabled the determination of the total background gamma ray flux in space as a function of latitude. This in turn has permitted useful information on the diffuse cosmic gamma rays. We have also observed four events that showed sudden increases in the gamma ray counting rates between 0.2 and 4.0 MeV. Observational details of these events are given.     

Cross sections of fast neutron induced reactions on molybdenum isotopes

Cross sections of (n, p), (n, α), and (n, 2n) reactions on molybdenum isotopes have been measured, in the neutron energy range from 13 MeV to 17 MeV, and interpreted in terms of evaporation from the compound nucleus and preequilibrium emission.     

Cross sections of fast neutron induced reactions on selenium isotopes

Cross sections for^{74, 76, 77, 78}Se(n, p)^{74, 76, 77, 78}As,⁷⁶,Se(n,2n)⁷⁵Se and⁸⁰Se(n, α)⁷⁷,Ge reactions have been measured in the energy range from 13.0 to 16.6 MeV by the activation technique using Ge(Li) detectorγ-ray spectroscopy. Samples of selenium of natural isotopic composition were used as targets. The measurements provide information on the evolution of the (n, p) excitation functions with the increasing target neutron number (isotopic effect). The reaction model combining the compound nucleus and the preequilibrium emission processes is used to interpret these three types of reactions. The isotopic trend for the (n, p) reactions due to the neutron-proton competition in the compound nucleus is satisfactorily reproduced. However, a further experimental and theoretical work is needed for a better understanding of the origins of discrepancies which are suggested to be related to the precompound aspects of the assumed reaction model.     

The COMPLIS experiment on neutron deficient Au, Pt and Ir isotopes

The COMPLIS (COllaboration for spectroscopic Measurements using a Pulsed Laser Ion Source) experiment is carried out at the ISOLDE Booster facility at CERN. The aim is to measure the hyperfine structure and the isotope shift of a series of radioactive laser desorbed atoms by multiple step laser ionization. This technique is especially suitable for refractory elements not directly available as beams from the isotope separator. By collecting a primary radioactive beam, it is possible to delay the laser desorption as long as necessary to obtain the particular daughter of interest. Laser spectroscopy measurements have been carried out on very neutron deficient gold, platinum and iridium isotopes. Magnetic moments μ_I, spectroscopic quadrupole moments and changes of the nuclear mean square charge radius along each isotopes series have been extracted. From some results, a detailed comparison with the predictions of the models is presented. This revised version was published online in August 2006 with corrections to the Cover Date.     

Isomeric yield ratios of 87m,gY from different nuclear reactions

We investigate the parity-violating nucleon-nucleon potential as obtained in chiral effective field theory. By using resonance saturation we compare the chiral potential to the more traditional one-meson-exchange potential. In particular, we show how parameters appearing in the different approaches can be compared with each other and demonstrate that analyses of parity violation in proton-proton scattering within the different approaches are in good agreement. In the second part of this work, we extend the parity-violating potential to next-to-next-to-leading order. We show that generally it includes both one-pion- and two-pion-exchange corrections, but the former play no significant role. The two-pion-exchange corrections depend on five new low-energy constants which only become important if the leading-order weak pion-nucleon constant h _π turns out to be very small.     

Activation cross sections and isomeric ratios in reactions induced by 14.5 MeV neutrons on152Sm,154Sm and178Hf

Cross sections for the reactions¹⁵²Sm(n, p)^152g,m1,m2 Pm,¹⁵⁴Sm(n, p)^154g,m Pm,¹⁷⁸Hf(n, p)^178m,g Lu,¹⁵⁴Sm(n, d)¹⁵³Pm and¹⁵²Sm(n, α)¹⁴⁹Nd were measured at 14.5 MeV neutron energy by the activation method. On the basis of these cross sections, the associated isomeric ratios in¹⁵⁴Pm,¹⁵²Pm,¹⁷⁸Lu and the comparison with the predictions of different compound and precompound models, conclusions are drawn about the role of the preequilibrium processes in 14.5 MeV neutron induced reactions. Calculations for equal angular momentum removal by equilibrium and preequilibrium emitted particles better reproduced the experimental isomeric ratios, than for higher angular momentum removal in the preequilibrium phase. The isomeric ratios may be used as a source of additional information about the spin of the isomeric states in¹⁵²Pm and¹⁵⁴Pm for which the spectroscopic information is uncertain.     

Incoherent scattering functions of 145 keV gamma rays by K-shell electrons in Y,Ag and Au

The values of incoherent scattering functions are determined experimentally for 145 keV gamma rays in elements Au, Ag and Y at scattering angles 40°, 70° and 100°, using a x-ray gamma coincidence technique. The corresponding theoretical values are obtained from the tabulations of Hubbellet al, and computed from the models of Jauch and Rohrlich and Shimizuet al. A comparison between the theoretical and experimental results showed that the non-relativistic approach adopted in the theory of Shimizuet al is inapplicable to the present cases. A gross agreement is noticed between the present experimental results and the other theoretical values.     

Evidence of new isotopes:169, 170Ir,166, 167, 168Re

At the Darmstadt UNILAC newα-emitting nuclei were produced in the bombardment of⁸⁹Y and⁹³Nb targets using⁸⁴Kr ions with energies in the range of 5.1 to 5.5 MeV/u, and 5.8 to 6.4 MeV/u, and using⁸⁶Kr ions with energies in the range of 5.6 to 6.0 MeV/u. Reaction recoils emitted from the targets were stopped and transported with argon to a collection site. Using three alpha detectors and spectrum multiscaling, energies and half-lives were measured. Ir and Re isotopes were identified by cross bombardments, excitation function data andα-systematics. The decay characteristics of the new species are as follows: Estimates onα-branching ratios have been obtained for^{169, 170}Os and^{166, 167, 168}Re.     

Isomeric ratios of the cross sections for Sn(p, xpyn)X reactions

In proton-nucleus reactions, the ratios of the cross sections for 18 isomeric pairs were measured by the induced-activity method as functions of the initial-proton energy and of the number of emitted nucleons. The isotopic effect and the cross sections for charge-exchange reactions are discussed. The experimental values of the cross sections for disintegration reactions like (p, xpyn) are compared with the theoretical values calculated on the basis of the cascade-evaporation model.     

<Emphasis Type="Italic">T</Emphasis>-odd angular correlations in the emission of prompt gamma rays and neutrons in nuclear fission induced by polarized neutrons

Study of the T-odd three-vector correlation in the emission of prompt neutrons from ²³⁵U fission by polarized cold neutrons has been continued at the facility MEPHISTO of the FRM II reactor (Technical University of Munich). The sought correlation was not found within experimental error of 2.3 × 10⁻⁵. The upper limit for the asymmetry coefficient has been set to |D _n | < 6 × 10⁻⁵ at 99% confidence level, whereas for ternary fission correlation coefficient D _α = (170±20) × 10⁻⁵. This limit casts doubt on a model that explains the three-vector correlation in ternary fission by the Coriolis mechanism. At the same time, five-vector correlation in the emission of prompt fission neutrons has been measured, which describes the rotation of the fissioning nucleus at the moment it breaks (ROT effect). At the angle 22.5° to the fission axis, the correlation coefficient was found to be (1.57 ± 0.20) × 10⁻⁴, while at the angle of 67.5° it is zero within the experimental uncertainty. The existence of ROT effect in the emission of prompt fission neutrons can be explained by the anisotropy of neutron emission in the rest frame of the fragment (fission fragments are aligned with respect to the axis of deformation of the fissioning nucleus), similar to the mechanism of ROT effect in the emission of prompt γ-rays.     

The decay of the isotopes176Ir and177Ir

^176,177Ir were produced by irradiation of¹⁴¹Pr with⁴⁰Ar. β-delayed γ-rays of^176,177Ir were observed for the first time. From γγ-coincidence data decay schemes could be constructed. A new half-life of¹⁷⁷Ir was obtained yielding t_1/2=30 (2) s. α-branching ratios of 3.1(6) % for¹⁷⁶Ir and 0.06(1)% for¹⁷⁷Ir were measured.     

The decay of the isotopes179Ir and180Ir

The probability for non-radiative (n.r.) excitations in muonic²⁰⁹Bi was determined from a ( ^–,)-measurement by comparing the intensities of muonic X-ray transitions in single and coincidence spectra. The values of P_n.r(3p1s)=(17.9±2.0)% and P_n.r.(3d1s)=(3.0±2.2)% were measured for the first time. The strength of the n.r. decay of the 2p-level was found to be (4.2±2.2)%. The n.r. transition probabilities of two subcomplexes of the (2p1s)-transition leading to different mean excitation energies are (3.2±1.8)% and (5.0±2.0)%, respectively.We are indebted to the following institutes or organizations for financial support: Bundesministerium ffir Forschung und Technologic der Bundesrepubfik Deutschland contract number 06 BN 271 (HP, PD, HH, FR, CR), Foundation for Fundamental Research on Matter (FOM) and the Netherlands Organization of the Advancement of Pure Research (NWO) (JK, CTAMdL, WL, AT) and the Schweizer Nationalfonds (LS).     

Statistical decay of gamma rays in (nth, γ) reactions

Isomer ratios obtained in doubly even targets in the (n_th, γ) reaction are calculated using realistic level densities and spin cut-off parameters. The calculations were performed using the Monte Carlo method and the general agreement between the present calculations and experimental data is satisfactory. In one case the shape of the γ-ray spectrum was calculated and good agreement with experimental data was obtained.     

Multiparticle break-up of 10B induced by fast neutrons

The reaction $\text{n}\text{+}{}^{10}\text{B}\text{→ α + α +}\text{d}\text{+}\text{n}$ induced by 14.4 MeV neutrons has been investigated in a kinematically complete experiment. Several final-state interactions have been observed in the sequential decay of the n + ¹⁰B system. The angular distribution of the ¹⁰B(n, ⁶Li₁)⁵He₀ reaction, leading to two unstable particles and consequently measurable only in a kinematically complete experiment, has been measured. It has been analysed in the framework of DWBA as a pick-up process with the transfer of the five-nucleon cluster ⁵Li. The presence of quasifree scattering and quasifree reaction with the deuteron as spectator has also been observed.