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1.
在自旋-轨道劈裂阵模型下,通过类铜的内壳层激发组态计算了类镍Gd的双电子复合速率系数,其中考虑了共振和非共振辐射平衡跃迁对自电离能级的影响,而忽略了因碰撞跃迁引起的电子俘获,非共振辐射平衡跃迁在低电子温度条件下主要影响双电子复合过程;本文讨论了双电子复合系数及双电子伴线强度比随电子温度的变化.  相似文献   

2.
在自旋-轨道劈裂阵模型下,通过类铜的内壳层激发组态计算了类镍氙的双电子复合速率系数,其中考虑了共振和非共振辐射平衡跃迁对自电离能级的影响,而忽略了因碰撞跃迁引起的电子俘获,非共振辐射平衡跃迁在低电子温度条件下主要影响双电子复合过程;本文讨论了双电子复合系数及双电子伴线强度比随电子温度的变化.  相似文献   

3.
焦荣珍  冯晨旭 《中国物理 B》2008,17(5):1845-1847
This paper analyses the effect of configuration complex on dielectronic recombination (DR) process in highly ionized plasmas (Xe^26+, Dy^38+, W^46+) by using the multiconfiguration relativistic Hartree-Fock method. Resonant and nonresonant radiative stabilizing transitions and decays to autoionizing levels followed by radiative cascades are included. Collisional transitions following electron capture are neglected. The remarkable difference between the isoelectronic trend of the rate coefficients for DR through 3d^94l4l′ and through 3d^94l5l′ is emphasized. The trend of DR through 3d^94l4l′ shows irregularities at relatively low temperature due to the progressive closing of DR channels as atomic number Z increases.  相似文献   

4.
杨天丽  蒋刚  朱正和 《中国物理》2004,13(6):850-854
The rate coefficients α^{DR} of dielectronic recombination (DR) for Cu-like Au^{50+} ion collided with the incident free electron are calculated based on the quasi-relativistic multi-configuration Hartree-Fock theory. The results clearly show that the α^{DR} of all recombination channels exhibits resonance characters with electron temperature. At lower temperatures, the recombination for electrons caused by 4s excitation is dominant through outer electron radiative transitions among the intermediate doubly excited autoionizing levels, in which the most components come from 3d^{10}5pns states, whereas with increasing electron temperature, DR caused by 3d excitation turns out to be dominant, and the contribution from the 3d^94s4fnf state to the total rate coefficient of electron 3d is the largest with α^{DR}=1.15×10^{- 11} cm^3·s^{-1} at an electron temperature of T_e=0.35 keV. Under this condition, there exists a strong competition between the two types of recombination channels.  相似文献   

5.
利用全相对论组态相互作用方法,详细研究了W44+ 离子从基组态3s23p63d104s2俘获一个电子形成双激发态(3s23p63d104s2)nln′l′(n = 4 ~ 6,n′= 4 ~7) 的双电子复合(DR) 过程。通过比较不同壳层电子激发的DR 速率系数,得知4s 电子激发和3d 电子激发的DR 速率系数分别在低温和中高温度时给出了主要贡献,得到了主要的电子激发DR通道。在1 eV~50 keV 温度范围内,计算了n = 4~18 的DR速率系数,并外推到了n= 100,得到总DR 速率系数。比较总DR 速率系数、三体复合(TBR) 以及辐射复合(RR) 速率系数,结果表明DR 速率系数在研究的温度范围内远大于TBR 和RR 速率系数,其将明显地影响ITER 等离子体的电离平衡和离化态布居。Based on the fully relativistic configuration interaction method, theoretical calculations are carried out to research the dielectronic recombination (DR) processes, in which W44+ ions in the ground state 3s23p63d104s2 trap an electron to form doubly excited states (3s23p63d104s2)nln’l’(n =4~6,n′= 4~7). The comparison of the DR rate coefficients of different shells shows that DR approach is as follow: the 4s subshell excitation dominates to DR at low temperature, but 3d subshell excitation attributes to DR at high temperature. Total DR rate coefficients from n=4~18 are evaluated directly, and the results are extrapolated up to n = 100 in the temperature range from 1 to 5×104 eV, and thus get the total DR rate coefficients. Compared total DR rate coefficients to three-body recombination (TBR) rate coefficients and radiative recombination (RR) rate coefficients, it showed that the total DR rate coefficients obviously significantly greater than other two recombination rate coefficients, and thus it obviously influence ionization equilibrium and ionization state population of ITER plasma.  相似文献   

6.
符彦飙  王旭东  苏茂根  董晨钟 《物理学报》2016,65(3):33401-033401
复杂结构离子的双电子复合(DR)速率系数在核聚变、极紫外光刻光源等应用研究的等离子体谱模拟中具有重要的价值.利用基于全相对论组态相互作用理论的FAC程序包,详细计算了Au~(34+)离子的双电子复合速率系数.研究分析了激发、辐射通道,组态相互作用,级联退激对DR速率系数的影响.其中,级联退激对DR速率系数的贡献必须予以考虑.对双电子复合、辐射复合以及三体复合速率系数做了比较,在温度大于1 eV范围,双电子复合都大于辐射复合以及三体复合速率系数,相应的DR过程对于等离子体离化态分布和能级布居以及光谱模拟都极为重要.对基态和第一激发态的DR速率系数进行了参数拟合,拟合值与计算值的偏差小于1.73%.研究结果将为复杂结构离子双电子复合过程的进一步研究提供参考.  相似文献   

7.
The results of calculations of the ionization equilibrium and radiative energy loss rates for C, N and O ions in low-density plasmas are presented for electron temperatures in the range 104–107 °K (~1–103 eV). The ionization structure is determined using the steady-state corona model, in which electron impact ionization from the ground states is balanced by direct radiative and dielectronic recombination. Using an improved theory, detailed calculations are carried out for the dielectronic recombination rates in which account is taken of all radiative and autoionization processes involving a single-electron electricdipole transition of the recombining ion. The radiative energy loss processes considered are electron-impact excitation of resonance line emission, direct radiative recombination, dielectronic recombination, and electron-ion bremsstrahlung. For all three elements, resonance line emission resulting from 2s?2p transitions produces a broad maximum in the energy loss rate near 105°K(~ 10 eV).  相似文献   

8.
类铜Dy37+离子的双电子复合速率研究   总被引:2,自引:2,他引:0       下载免费PDF全文
在自旋轨道劈裂阵模型(SOSA)下,通过类锌组态,理论计算出类铜Dy37+的双电子复合速率系数,得出其在电子温度0.02 keV~5.0 keV范围内的变化规律,分析了不同离化度离子的能级特征,并分析了影响双电子复合速率系数的主要因素是相应的中间自电离态旁观电子主量子数、旁观电子角动量和电离能,这为实现等离子体的诊断提供了重要的参数.  相似文献   

9.
 在自旋轨道劈裂阵模型下,通过类铜组态理论计算出类镍Gd36+的双电子复合速率系数,得出其在电子温度 0.02~5keV 范围内的变化规律,并分析了影响双电子复合速率系数的主要因素是相应的自电离系数和离化势,这为等离子体的诊断提供了一种新的方法。  相似文献   

10.
The X-ray emission spectra of nickel plasma were simulated under the collisional radiative model (CRM) by using the flexible atomic code (FAC). The dynamical processes including collisional excitation (CE), radiative recombination (RR), dielectronic recombination (DR), collisional ionization (CI) and resonance excitation were considered in the model, and the rate coefficients of DR, RR as well as CI were consistent with previous results within 15%. It was found that the contributions to spectra from cascades and indirect processes could not be ignored. The intensities of spectral lines for lithium-like nickel L-shell ions are sensitive to the electron temperature. The good agreement between present spectral peaks and earlier observed results can be taken as a measure of the accuracy of the present work.  相似文献   

11.
 利用全相对论组态相互作用理论方法,研究了类铷W37+离子从基组态3s23p63d104s24p64d经过双激发态(3s23p63d104s24p64d)-1nln′l′(n,n′=4,5)的双电子复合过程,得到了该离子在温度为1~5×104 eV范围内的总双电子复合速率系数。分析比较了不同电子激发的双电子复合速率系数,结果表明:4p电子激发的双电子复合速率系数在低温时给出了主要贡献,而3d的贡献在高温时突出。由于强组态相互作用,两电子一光子跃迁对双电子复合速率系数的贡献不可忽略,其中辐射跃迁4p54d5d5f-4p64f5d的贡献是双激发态4p54d5d5f总的双电子复合速率系数的5%。对双电子复合、辐射复合以及三体复合速率系数的比较表明,在所研究的温度范围内双电子复合速率系数最大。  相似文献   

12.
Based on the multi-configuration Dirac-Fock method, theoretical calculations are carried out for the dielectronic recombination (DR) rate coefficients and the collision excitation rate coefficients of Sn^10+ ions. It is found that the total DR rate coefficient has its maximum value between 10eV and 100eV and is greater than either the radiative recombination or three-body recombination rate coefficients (the number of free electrons per unit is 10^21 cm^3) for the ease of Te 〉 1 eV. Therefore, DR can strongly influence the ionization balance of laser produced multi-charged tin ions. The related dieleetronie satellite cannot be ignored at low temperature Te 〈 5 eV.  相似文献   

13.
利用基于全相对论组态相互作用理论的FAC程序包, 详细研究了温度在0.1~1650 eV范围内Xe8+离子的双电子复合(DR)过程。 通过比较4s, 4p和4d壳层电子激发的双电子复合速率系数, 发现温度在10 eV以上时, 内壳层4p电子激发的双电子复合速率数对总双电子复合速率系数有很重要的贡献, 而4s电子激发对总双电子复合速率数贡献小于7.5%。 给出了△n=0, 1和2 三类芯激发对总双电子复合速率系数的贡献以及自由电子俘获到不同主量子数的双电子复合速率系数, 发现△n=2的芯激发和n′>15的DR速率系数对总DR速率系数的贡献也很重要。 进一步给出了△n=0, 1和2 三类芯激发和总DR速率系数的拟合参数, 拟合结果和计算值符合, 偏差小于1%。 通过对双电子复合、 辐射复合以及三体复合速率系数的比较得知, 在温度高于1 eV时, DR过程是Xe8+离子的主要复合过程。Based on the fully relativistic configuration interaction method, theoretical calculations are carried out for the dielectronic recombination (DR) rate coefficients of Xe8+ ions in the temperature region from 0.1 to 1 650 eV. The comparison of the DR rate coefficients from 4s, 4p and 4d subshell excitations shows that 4d subshell excitation dominates in the whole temperature region. The contribution from 4p subshell excitation is very important at temperature above 10 eV and the contributions from 4s subshell excitation is lower than 7.5% in the whole temperature region. Similarly, the comparison of the DR rate coefficients through △n=0, 1 and 2 core excitation shows that the contribution from △n=2 core excitation can not be neglected, the contributions from n′>15 can also not be neglected. The DR rate coefficients of △n=0, 1 and 2 core excitation and the total DR rate coefficients are fitted with some parameters, which are in good agreement with theoretical calculations values (within 1% difference). The total DR rate coefficients are greater than radiative recombination (RR) and three body recombination (TBR) rate coefficients at temperature above 1 eV. Therefore, the DR process can strongly influence the ionization balance of laser produced xenon plasmas.  相似文献   

14.
牟致栋  魏琦瑛 《物理学报》2007,56(3):1358-1364
用HFR波函数对低密度类氢Ni27+等离子体与电子相互作用的KLn和KMn共振激发的双电子复合过程进行了细致的理论计算研究.根据可能的重要辐射衰变通道,分析了Ni27+等离子体Kα 型和Kβ 型辐射衰变的双电子复合速率系数随旁观电子主量子数n和轨道角动量量子数l与电子温度的变化行为,计算了Ni27+等离子体双电子复合过程的总速率系数.研究结果表明,在低密度条件下,Kα 型和Kβ型辐射衰变的分支双电子复合速率系数与旁观电子主量子数n和轨道角动量量子数l有重要关系,前者的分支速率系数远大于后者. 关键词: 27+离子')" href="#">Ni27+离子 Kα型和Kβ型辐射衰变')" href="#">Kα型和Kβ型辐射衰变 双电子复合 速率系数  相似文献   

15.
王巍  蒋刚 《物理学报》2010,59(11):7815-7823
讨论了稠密等离子体中双电子复合速率系数的计算方法,推导出了在双激发态间跃迁过程和关于双激发态的碰撞电离和自电离过程的影响下双电子复合速率系数作为关于电子密度函数的计算公式,并以类氖镍离子为例进行了计算.计算结果展示了双电子复合速率系数随电子密度增大的具体变化趋势.此外,还给出了在不同原子过程影响下双电子复合速率系数的数据,并进行了分析.  相似文献   

16.
The dielectronic recombination (DR) rate coefficient αDR is explicitly calculated for the Si, Ar, Fe and Mo target ions of the Mg isoelectronic sequence with twelve electrons. Both the 3s, Δn ≠ 0 and 3s, Δn = 0 transitions are considered in detail. An explicit LS coupling scheme was applied to all the dominant transitions of these ions. Results of αDR with different free electron temperatures are also discussed  相似文献   

17.
复杂结构离子的双电子复合速率系数在极紫外光刻光源、核聚变等应用研究的等离子体光谱模拟和诊断中具有重要的应用价值。利用全相对论组态相互作用方法,详细计算了基组态为4p64d9的Re30+离子经双激发态(4p64d9)-1nln'l'(n=4~6,n'=4~23)的双电子复合(DR)过程。研究分析了激发、辐射通道,组态相互作用,级联退激对DR速率系数的影响。其中内壳层4p电子激发的DR速率系数是总DR速率系数的28.2%~44.9%,所以内壳层4p电子激发的贡献不可以忽略。级联退激对DR速率系数的最大贡献为12.9%,也必须要予以考虑。通过对双电子复合、辐射复合、以及三体复合速率系数的比较,辐射复合速率系数的最大值为DR速率系数的22.6%,三体复合速率系数的最大值仅为DR速率系数的0.3%。因此,DR速率系数远远大于辐射复合和三体复合速率系数。该结果表明DR过程对于等离子体离化态分布、能级布居以及光谱模拟都极为重要。为了方便应用,对基态和第一激发态的总DR速率系数进行了参数拟合。该研究结果将为Re激光等离子体的光谱模拟及复杂结构离子DR过程的进一步研究提供参考。Dielectronic recombination (DR) rate coefficients of complex ions are very important in some application research, such as extreme ultraviolet lithography and nuclear fusion. Based on the fully relativistic configuration interaction method, theoretical calculations are carried out to research the DR processes, in which Re30+ ions in the ground state 4p64d9 to (4p64d9)-1nln'l'(n=4~6, n'=4~23). Influence of excitation and radiation channels, configuration interaction, the effect of decays to autoionizing levels possibly followed by radiative cascades (DAC) are analyzed. The contributions through 4p subshell excitations to the total rate coefficient are 28.2%~44.9% in the whole temperature region. Hence the contributions from inner-shell electron excitation are very important. The contributions from the DAC transitions increase smoothly with the increasing temperature and are about 12.9% at 50 000 eV. The contributions of DAC can not be neglected. By means of compared total DR rate coefficients to radiative recombination rate coefficients and three-body recombination rate coefficients, it shows that the maximum value of the radiation recombination rate coefficient is 22.6% of the DR rate coefficient and the maximum value of the three-body recombination rate coefficient is only 0.3% of the DR rate coefficient. The total DR rate coefficient is greater than either the radiative recombination or three-body recombination coefficients in the whole temperature range. The corresponding DR process is very important for plasma ionization distribution, population level and spectrum simulation. In addition to facilitate the application, the total DR rate coefficients for the ground state and the first excited state are fitted to an empirical formula. These results will provide the reference for the further analyses of rhenium laser plasma spectrum simulation and the complex structures ions DR process.  相似文献   

18.
董晨钟  邹宇  王建国  李家明 《物理学报》1995,44(11):1712-1718
双电子复合是一种共振辐射复合过程,在这一过程中,一个具有特定能量的自由电子与电离度为q的离子A~(+q)碰撞,形成有两个电子激发的自电离态n_(?)l_(?)nl,该自电离态进一步发射光子,复合成A~(+(q-1))离子,一系列n(?)l_(?)nl自电离态(n_(?)l_(?)l固定,n从有限到无限变化)形成一个通道,本文在相对论单组态理论基础上,具体探讨了类氦铁离子(3s_(1/2)~nP_(1/2))J=(?)通道中,双电子复合速率随n的变化规律,根据本文得到的规律,可以很方便地计算任意离子的任意一 关键词:  相似文献   

19.
The dielectronic recombination (DR) rate coefficient αDR is explicitly calculated for the Mo, Fe, Ar, and Ox target ions of the Be-sequence with four electrons, in the isolated resonance approximation. This work extends the previous study of the Mo38+ ions at 1.4, 2.8, and 5.6 keV electron temperatures. Both Δn≠0 and Δn = 0 transitions are considered in detail. The Δn≠0 contribution still dominates, but the Δn = 0 effect becomes quite large for heavy ions. An explicit LS coupling scheme is employed throughout for the dominant transitions calculated here, and contributions from many other intermediate states and cascade transitions are included by comparing the dominant contribution with the more complete Mo38+ case and proportionately scaling their effect. Nonrelativistic Hartree-Fock wave functions are used in the evaluation of the Auger and radiative amplitudes, and the continuum wave functions are calculated using the Hartree-Fock direct potential and explicit nonlocal exchange potential. The scaling property of αDR and its breakdown are examined, and an improved form of the phenomenological formula is proposed.  相似文献   

20.
We describe the general analytic derivation of the dielectronic recombination (DR) rate coefficient for multielectron ions in a plasma based on the statistical theory of an atom in terms of the spatial distribution of the atomic electron density. The dielectronic recombination rates for complex multielectron tungsten ions are calculated numerically in a wide range of variation of the plasma temperature, which is important for modern nuclear fusion studies. The results of statistical theory are compared with the data obtained using level-by-level codes ADPAK, FAC, HULLAC, and experimental results. We consider different statistical DR models based on the Thomas–Fermi distribution, viz., integral and differential with respect to the orbital angular momenta of the ion core and the trapped electron, as well as the Rost model, which is an analog of the Frank–Condon model as applied to atomic structures. In view of its universality and relative simplicity, the statistical approach can be used for obtaining express estimates of the dielectronic recombination rate coefficients in complex calculations of the parameters of the thermonuclear plasmas. The application of statistical methods also provides information for the dielectronic recombination rates with much smaller computer time expenditures as compared to available level-by-level codes.  相似文献   

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