双光子抽运随机激光器中辐射光能量的演化

基于非相干反馈随机激光器的扩散方程理论，将扩散方程中的增益项改写为饱和形式，并利用有限差分方法，研究了双光子抽运随机激光器中辐射光能量随时间演化特性.对扩散方程的数值求解给出了系统辐射光能量由自发辐射开始，经历小信号增益状态得到放大，再到由于增益饱和形成稳态输出的整个演化过程.表明介质的无序导致了在较低能量情况下也能获得饱和增益这样的非线性效应.结果为研究获得双光子抽运随机激光器的稳态输出提供了理论依据. 关键词： 随机激光器 双光子抽运 饱和效应 无序介质中的光学效应     

光抽运双光子激光朗之万量子理论

本文采用朗之万量子理论获得光抽运双光子激光具有双光子损耗时的朗之万方程,进一步获得稳态平均光子数、频率牵引、线宽和动态斯塔克效应,对激光增益来源的分析表明,非相干抽运仅有单双光子两步过程有贡献,而相干抽运,除上述过程外还有单双光子一步过程有贡献,而且,上述两个过程都受到负反馈和饱和因子的制约,线宽与稳态平均光子数无关。 关键词：     

Effects of absorption saturation in colloidal quantum dots as fluorophores for multiphoton fluorescence microscopy

It is shown that colloidal semiconductor nanocrystals (quantum dots), which are promising fluorophores for multiphoton fluorescence microscopy, exhibit a two-photon absorption saturation effect at moderate powers (not exceeding 10 mW) of femtosecond pumping radiation. An analytical expression for the power of two-photon fluorescence of quantum dots as a function of the average pumping power is obtained. With this expression, the deviation of the found dependence from the quadratic law is explained by two factors, i.e., a large two-photon absorption cross section of quantum dots and their slow (compared to the typical pumping pulse-repetition period) relaxation to an unexcited state. Using an LSM 510 Carl Zeiss laser scanning microscope equipped with a Ti:Sa tunable femtosecond laser, a series of model experiments is performed to reveal the saturation effect in a solution of commercially available quantum dots. Good agreement is obtained between the measured dependence of the power of two-photon fluorescence on the average pump power and the theoretical calculation results. It is also experimentally demonstrated that, under fluorescence saturation conditions, the spatial resolution of the method of multiphoton fluorescence microscopy is lost; this effect is analyzed numerically.     

Effective control over the dual-color emitted light waves from one-dimensional random media pumped by Femtosecond-Lasing Pulses

The spectral property of dual-color random laser is investigated by simultaneously solving Maxwell’s equations and rate equations of electronic population in which the pumping rate is described by a time function with duration of hundreds of femtoseconds. Results show that the delay time and peak intensity of the emitted light depends strongly on the pumping process. An effective optimization method is proposed to exercise control over the dual-color laser emission from the dye solution with scattering nano-particles. It is demonstrated numerically that the controllable single mode operation of a dual-color random laser by choosing the proper pump profile and pumping region. The present work enriches the knowledge about random lasers and offers more guidance for relevant experiments.     

Single- and two-photon excitation of a GaAs random laser

We have demonstrated an anti-Stokes random laser emission at lambda approximately 885 nm in micrometer-size powder of GaAs. The maximal pumping wavelength, lambda=1,300 nm, exceeded the lasing wavelength by nearly 50%. We conclude that both one- and two-photon pumping contribute to optical excitation of the material, with the two-photon pumping being a key process in creating the population inversion and gain.     

Absorption and subsequent emission saturation of two-photon excited materials: theory and experiment

The saturation of two-photon absorption and the subsequent photoluminescence of matter under ultrafast laser pulse excitation are studied. For this purpose the experimental results of using two organic conjugated polymers as model substances are discussed theoretically. One model is based on the commonly used hyperbolic approach, whereas the new theory introduced correctly describes the saturation in two-photon spectroscopy and fits the experiment closely. The new model permits microscopic analysis of the absorption saturation process and makes possible an estimate of the two-photon absorption coefficient from the saturation intensity.     

Two-photon pumping of random lasers by picosecond and nanosecond lasers

We experimentally demonstrated two-photon pumping of random lasers using picosecond and nanosecond pump lasers. The picosecond laser pumping experiment was performed with 400 ps laser pulses at 770 nm, and the gain media was a Coumarin 480D dye solution doped with TiO₂ nanoparticles. Onset of laser action was observed at a pump laser pulse energy below 500 μJ. The nanosecond laser pumping experiment was performed with 7 ns laser pulses at 1064 nm, and the gain media was a Rhodamine 640 dye solution doped with TiO₂ nanoparticles. Onset of laser action was observed at a pump laser energy ∼18 mJ. Our results suggest that there exists an optimal pulse duration of the pumping laser in two-photon pumped random lasing that leads to minimum photodamage of the gain media and still keeps a high pumping efficiency. PACS 33.50.Dq; 42.55.Mv; 42.55.Zz     

一维随机介质中准态模式的局域化程度对其阈值的影响

基于将Maxweil方程与四能级原子系统速率方程相结合而建立起的随机激光时域理论,并利用有限时域差分法,研究了一维随机激活介质中激光模式的输出强度与抽运速率之间的关系.结果表明,与传统激光模式相似,随机激光模式的强度随抽运速率的变化不仅具有阈值特性,而且具有饱和特性.用模式的空间区域来表征模式的局域化程度,发现局域化程度越强的模式,阈值越低.不过,这种关系不是一一对应的.这表明模式的局域化程度是决定阈值大小的重要因素,但不是唯一的因素.     

Two-Time Intensity Correlations and Multiple Interference Mechanisms in a Driven Cascade Atom

We examine the intensity correlation functions of the two fluorescent fields that are emitted from the top and middle states of a doubly driven three-level atom in the cascade configuration. Novel interference effects are shown. （i） Both of the fluorescent fields have anticorrelations which can exist for long times when the applied fields are on the two-photon resonance and far off one.photon resonances. （ii） Both of the fluorescent fields have strong correlations when the applied fields are far off one- and two-photon resonances. In particular, the extremely strong correlation occurs for the photons emitted from the top state. The above phenomena are traced to the multiple interference mechanisms.     

599.2 nm diffuse band radiation generated by two-photon exciting molecular and atomic potassium

Diffuse band radiation around 599. 2 nm in K_2 was generated by the two photon pumping potassium dimers or by the two-photon resonant pumping atomic potassium with following atoms-molecules collision energy transfer. The pumping wavelengths are in a wide range of 697-745 nm. The relevant mechanisms were discussed.     

基于光放大的长脉冲抽运太赫兹激光

为了获得较窄增益带宽、较大光强的太赫兹辐射,尝试了利用TEA CO₂激光器对6 W可调谐连续波CO₂种子激光实行双程光放大实验,以期望获得长脉冲、高峰值功率的抽运光.通过实验,获得了大约30倍的放大系数,放大光输出功率随种子光注入功率的增加而增加,其中10 P （20）支线表现更加突出,并且被放大的激光支线半峰全宽在14 μs左右.基于这种长脉冲抽运源,建立了一种产生脉冲太赫兹的动力学模型,给出了产生太赫兹辐射的饱和抽运光强表达式,确定了抽运光的光强范围.另外, 关键词： 激光物理 长脉冲 动力学模型 太赫兹激光     

Theoretical investigation on temporal properties of random lasers pumped by femtosecond-lasing pulses

Pulsing random lasing property has been investigated in both one- and two-dimensional random medium by numerically solving Maxwell’s equations and rate equations in which the pumping rate is described by a time function with duration of 10s or 100s of femtoseconds. The peak intensity, width and delay time of a random lasing pulse are traced with the variation of the peak intensity, duration, shape and numbers of a pumping pulse. Results show that the behavior of random lasing depends strongly on the pumping process, some of which are in agreement with previously reported experiments pumped by femtosecond-lasing pulses. The present work enriches the knowledge about random lasers, especially in temporal regime, and could offer more guidance for relevant experiments.     

飞秒抽运随机激光输出波形的可控性研究

本文基于随机激光的时域理论,研究了飞秒脉冲抽运下二维随机激光的辐射特性,并着重讨论了抽运脉冲的峰值强度、脉宽和脉冲波形对辐射光时域波形的影响.结果表明, 辐射光的时域波形强烈依赖于抽运光脉冲的参数,通过调整抽运方式可以控制辐射光的输出波形.数值模拟结果为研究随机激光输出波形的可控性技术提供了理论依据. 关键词： 激光物理 随机激光器 飞秒抽运 脉冲波形     

Light amplification in CdTe and InSe under two-photon pumping

Photoluminescence measurements in CdTe and InSe under high intensity two-photon pumping are reported. The relative non-linear absorption coefficients of both materials have been measured. Stimulated emission spectra of both CdTe and InSe show an amplification effect due to excitonic recombination involving a cooperative process; the related optical gain coefficients have been measured.     

Two-photon hybrid resonance laser and photodissociation laser by two-photon pumping covering a wide wavelength region in the potassium vapor

This paper reports the results about the laser generation based on the two-photon hybrid resonance and on the photodissociation by two-photon pumping covering a wide wavelength region respectively. In the former, 3.66, 3.64, 3.16, 3.14, and 2.71 μm laser lines were obtained by collision energy transfer from a potassium dimer in an excited state to the potassium atom in the ground state, and then followed by the resonance excitation of the potassium atom from the 4P to 6S state. In the latter, 2.71, 3.14, and 3.16 μm dissociation laser lines were obtained by two-photon pumping of the potassium dimer covering a wide pumping range about 650 Å at the red wavelength region.     

The features of nonlinear absorption during resonance one- and two-photon excitation of the basic exciton transition in colloidal CdSe/ZnS quantum dots

The features of the nonlinear absorption of CdSe/ZnS quantum dots (colloidal solution) in the case of resonant one- and two-photon excitation of the basic exciton transition by powerful ultra-short laser pulses were determined. In one-photon excitation, with an increasing intensity of impulses, a decrease in absorption (bleaching) is relayed by an increase in absorption, which is associated with the process of the filling of the states (saturation) of a two-level system with the lifetime of the excited state depending on the light intensity. The arising Fresnel or Fraunhofer diffraction of the laser ray that pass through a colloidal solution with a high concentration of quantum dots is associated with the formation of the transparency channel and self-diffraction of laser ray on an induced diaphragm. In two-photon excitation, the features of the nonlinear absorption and luminescence tracks (the dependence of luminescence intensity on distance) were explained by the influence, in addition to the two-photon absorption, of the processes that are responsible for the slower growth of nonlinear absorption and luminescence quenching at high intensities of laser pulses.     

Bound-bound saturation effect on nuclear spin polarization in two-photon ionization

Optical saturation within the discrete state space of the atom is shown to affect destructively the nuclear spin polarization of the ion formed in a two-photon process. An optimal laser intensity is found to exist ensuring the highest quality of the nuclear spin-polarized ion source.     

Spatially correlated light emission from a resonant-cavity light-emitting diode

We present the angular-resolved intensity noise characteristics of a resonant-cavity light-emitting diode under quiet pumping conditions. Measurements by a sensitivity-enhanced lock-in amplifier detection scheme yielded a spatial anticorrelation between the intensity noise of the central and peripheral parts of the emitted far field. Proposals for possible explanations of this anticorrelation from a semiconductor emitter point of view and its consequences for applications in quantum optical imaging are discussed.     

Resonant two-photon single ionization of two identical atoms

Resonant two-photon single ionization in a system consisting of two spatially well-separated identical atoms is studied. Because of two-center electron-electron correlations, the ionization may also proceed through photoexcitation of both atoms with subsequent interatomic Coulombic decay. We show that this channel may qualitatively change the dependence of the photoionization on the field intensity as well as the spectra of emitted electrons.     

CS_2分子激发态的紫外多光子电离——双色激光单共振离化的功率密度关系

本文报道气相CS_2紫外双色激光单共振离化的功率密度关系和对高激发态(1~Ⅱg),共振离化特性的研究结果,实验指出通过中间共振态(1~Ⅱ_g)的双光子共振激发三光子离化具有比通过中间共振态((?)A_2)的单光子共振激发三光子离子为高的总离化率,在10~7W/cm~2的功率密度下,观察到饱和效应.实验显示了双色激光单共振离化功率密度关系的研究提供了一种新的光谱学分析方法.这对研究分子高激发态的结构是很重要的.