核对称轴不同相对取向对熔合动力学的影响

计算了核对称轴不同相对取向时的熔合位垒.基于双核模型观念，考虑了熔合与准裂变的竞争，通过数值法求解主方程，计算了⁷⁶Ge+²⁰⁸Pb，⁴⁸Ca+²⁴⁴Pu核对称轴不同相对取向对熔合概率的影响，探索了最有利于超重元素合成的弹靶相对取向.取向不同时，对熔合反应的影响较大，计算结果表明弹靶碰撞为腰对腰时，更有利于发生熔合反应. 关键词： 超重元素 熔合概率 变形核 方向角度     

基于双核模型对超重元素合成机制的研究

在双核模型基础上，考虑了熔合与准裂变的竞争，通过数值法求解主方程，计算了⁵⁰Ti，⁵⁸Fe+²⁰⁸Pb，²⁰⁹Bi这4个反应系统通过冷熔合反应合成超重元素的激发函数，得到了与实验比较符合的结果.计算了不同入射能量时各角动量分波对熔合概率和超重核存活概率的影响以及对蒸发剩余截面的贡献.这些结果对进一步理解超重核的合成机制有重要意义. 关键词： 超重元素 双核模型 熔合反应 蒸发剩余截面     

中子诱发232Th裂变初始碎片质量及动能分布Monte-Carlo研究

随着第四代反应堆以及先进核能利用系统的发展,对中子核数据提出了高精度、多核素、宽能区的新要求.目前,中国核数据评价库(CENDL库)中相关核裂变的数据较缺失,不足以满足当前核能发展的需求.因此,建立面向中子核数据需求的可靠计算方法和工具变得极为重要.本文基于Monte-Carlo方法建立了裂变碎片质量动能计算模型,研究了中低能中子诱发²³²Th(n,f)反应发射中子前裂变碎片的分布特性.对于裂变碎片质量分布,本模型计算结果与实验值最大偏差约1%,与GEF, TALYS程序计算结果 (与实验值最大偏差约2%)相比具有一定优势.对于发射中子前裂变碎片动能分布,本模型计算结果与实验数据一致.结果表明,所发展的计算模型能够较好地预测²³²Th(n,f)反应发射中子前裂变碎片数据,为中子诱发锕系核裂变反应计算提供一种新思路.     

原子核壳模型单体密度矩阵的数值计算

提出平均场壳模型下原子核单体密度矩阵的一种计算方法,验证该方法的可靠性.计算双幻核⁴⁰Ca,⁹⁰Zr的单体密度矩阵,利用单体密度矩阵计算核子密度分布和动量分布,并分别与Hartree-Fock-Bogolubov理论结果、定域费米气体模型结果以及实验数据进行比较.     

核子-核子碰撞截面对同位素标度参数α的介质效应

核子能量在40—60MeV能区范围,对在两对重离子中心碰撞系统⁴⁰Ca+⁴⁸Ca和⁶⁰Ca+⁴⁸Ca以及¹¹²Sn+¹¹²Sn和¹²⁴Sn+¹²⁴Sn 的反应中就同位素标度参数α对于核子-核子碰撞截面σ^med_NN(α_m)的介质 关键词： 同位素标度行为 介质效应 核子-核子碰撞截面 重离子碰撞     

16O+232Th垒下全熔合裂变

利用裂变碎片的折叠角分布,从实验上实现了全熔合裂变和转移跟随裂变两种成份的区分.在此基础上测量了质心系能量72.61至80.11MeV ¹⁶O+²³²Th全熔合裂变截面和碎片角分布.包含靶核静态形变效应的耦合道模型计算与实验激发曲线一致.然而,裂变统计理论无法解释实验上观察到的全熔合裂变碎片角分布.而鞍点模型与断点模型的理论预言有较明显的差别.     

核子-核子碰撞截面对同位素标度参数α的同位旋效应

对两对重离子中心碰撞系统⁴⁰C+⁴⁰Ca 和⁶⁰Ca+⁴⁰Ca以及¹¹²Sn+¹¹²Sn和¹²⁴Sn+¹²⁴Sn反应中就同位素标度参数α对于核子-核子碰撞截面的同位旋效应进行了研究.计算结果表明α对同位旋相关核子-核子碰撞截面σ^med_{NN关键词： 同位旋效应 核子-核子截面 机理 同位素标度}     

预平衡裂变

实验证明,重离子熔合裂变与入射道的质量不对称有关,说明对于某些反应体系,熔合形成的复合体系,裂变时未忘记其形成的历史.在实验观察的基础上,我们提出了预平衡裂变模型,解释了重离子垒下熔合裂变碎片角分布各向异性异常.     

30MeV/u40Ar+159Tb反应中中等质量碎片的发射时标与发射机制

报道30MeV/u⁴⁰Ar+¹⁵⁹Tb反应中碎片-碎片关联函数的实验结果．利用三体弹道模型从关联函数提取了中等质量碎片发射时间．中等质量碎片的平均发射时间随碎片能量而变化，从低能时的约500fm/c下降至高能时的约100fm/c．中等质量碎片发射时间随束流能量的升高而下降，表明随着束流能量的升高中等质量碎片发射机制逐渐从相继两体衰变向多重碎裂发射过渡．对于⁴⁰Ar+¹⁵⁹Tb反应，此过渡能区在35—45MeV/u之间 关键词：     

重核大集团发射半衰期的计算

重核大集团（¹⁴C-³⁴Si）发射的半衰期在理论上用Wentzel-Kramers-Brillouin近似进行了计算.利用双折叠模型计算大集团和剩余子核间的核相互作用,在折叠积分中选取了密度依赖的、零力程交换项的核子-核子相互作用.计算得到的半衰期和液滴模型结果、系统公式的结果以及实验数据进行了比较,表明目前的计算能够很好地给出重核大集团（¹⁴C-³⁴Si）发射的寿命.这可为重核其他大集团（¹⁵N, ⁴⁶Ar,⁴⁸Ca等）的发射提供可靠的预测. 关键词： 半衰期 双折叠模型 集团发射     

基于双核模型对Z = 116~ 121 超重核产生截面的研究(英文)

在双核模型的理论框架下系统研究了超重元素Z = 116 ~121 的蒸发剩余截面,计算过程中核子扩散由主方程描述,同时考虑了全熔合与准裂变的竞争。计算基本再现了利用热熔合反应48Ca+245Cm,48Ca+249Cf 和48Ca+249Bk 产生116~118 号同位素的合成截面。同样,分别以249Bk,249Cf 和243Am 为靶,以48Ca,50Ti 和58Fe 为炮弹,计算了Z = 119~ 121 号同位素的生成截面。结果表明,这些超重核的生成截面随着质子数的增大进一步变小。例如,利用58Fe+243Am 反应合成121 号同位素的最大蒸发剩余截面仅在fb 量级。基于对选择的几个反应系统的系统分析,发现双核系统在熔合蒸发过程中偶Z 奇N 和奇Z 偶N 复合核分别有强的3n 和4n 蒸发道。The production cross sections of superheavy elements with Z = 116~121 have been investigated systematically within the dinuclear system (DNS) concept, where the master equation is solved numerically to obtain the fusion probability. The competition between complete fusion and quasifission, which can strongly affect the cross section of the compound nucleus formation, is taken into account. The evaporation residue cross sections ER calculated for the hot fusion actinide-based reactions (48Ca+245Cm, 48Ca+249Cf and 48Ca+249Bk) are basically in agreement with the known experimental data within one order of magnitude. Similar calculations for the synthesis of superheavy elements up to Z = 121 are performed using the available 249Bk, 249Cf and 243Am as targets and 48Ca, 50Ti and 58Fe as projectiles. Their production cross sections are relatively small,especially for the 58Fe+243Am→301121 reaction. A systematic analysis indicates that the 3n and 4n channelsare respectively the most favorable fusion-evaporation channels in the synthesis of even- and odd-Z superheavy elements.     

Dynamics of capture and fusion in heavy ion collisions

The effect of entrance channel on decrease of the complete fusion cross sections and on the yield of reaction products are associated with the quasifission which depends on the mass asymmetry and shell structure of colliding nuclei. In reactions of massive projectile and target nuclei, the competition between complete fusion and quasifission appears at the stage of compound nucleus formation, in addition to the increase of the fission probability. It is shown that the yield of quasifission products may be symmetric or asymmetric in dependence on peculiarities of shell structure of reaction fragments. Marima of mass or charge distributions are connected with the peculiarities of shell structure of reaction fragments.     

Entrance-channel dynamics in the reaction ~(40)Ca+~(208)Pb

The entrance-channel dynamics including capture, fusion, and quasifission processes for the reaction ~(40)Ca+~(208)Pb is investigated in the fully microscopic time-dependent Hartree-Fock(TDHF) theory. The calculations are performed in three-dimensional Cartesian coordinate without any symmetry restrictions, in which the full Skyrme energy functional SLy4d and SLy5 are adopted.We study the energy dependence of capture cross sections, and find that the experimental data are well reproduced by the TDHF calculations. Both fusion and quasifission events are observed in the reaction ~(40)Ca+~(208)Pb. The contact time, mass and charge of quasifission fragments show a wide distribution in SLy4d compared with SLy5, implying that more nucleons are transferred in the SLy4d calculations. We find that the total kinetic energy of quasifission fragments in the TDHF calculations is distributed around Viola systematics, indicating that most of the relative kinetic energy is dissipated in quasifission dynamics.     

Synthesis of superheavy elements and the process of complete fusion of massive nuclei

The development of various approaches to describing the complete fusion of nuclei and their connections with experimental studies is discussed. A brief account of the dinuclear-system concept (DNSC), the approach proposed at Dubna, is given. The DNSC revealed two important features of the complete fusion of massive nuclei: the existence of the inner fusion barrier B _fus ^* and the competition between complete fusion and quasifission channels in a dinuclear system formed at the capture stage. The DNSC was applied to the analysis of reactions used to synthesize superheavy elements (SHE). The DNSC provided a basis for the models of competition between complete-fusion and quasifission channels. Using these models, one can describe the cross section for SHE production in cold-and warm-fusion reactions.     

Angular momentum dependence of quasifission dynamics in the reaction <Superscript>48</Superscript>Ca+<Superscript>244</Superscript>Pu

The quasifission dynamics in the reaction ⁴⁸Ca+²⁴⁴Pu is investigated in the framework of time-dependent Hartree-Fock (TDHF) theory. The calculations are performed in three-dimensional Cartesian coordinate without any symmetry restrictions. The full Skyrme energy functional is incorporated in our TDHF implementation. The quasifission dynamics is quite sensitive to the angular momentum of colliding system. The contact time of quasifission decreases as a function of angular momentum and then forms a plateau with small oscillations. The quasifission process is accompanied by an important multi-nucleon transfer. The quantum shell effect plays a crucial role in the mass and charge of quasifission fragments. The mass-angle distribution of the fragments is calculated, which can be compared directly with future experiments.     

Angular momentum dependence of quasifission dynamics in the reaction ~(48)Ca+~(244)Pu

The quasifission dynamics in the reaction ~(48)Ca+~(244)Pu is investigated in the framework of time-dependent Hartree-Fock(TDHF)theory. The calculations are performed in three-dimensional Cartesian coordinate without any symmetry restrictions. The full Skyrme energy functional is incorporated in our TDHF implementation. The quasifission dynamics is quite sensitive to the angular momentum of colliding system. The contact time of quasifission decreases as a function of angular momentum and then forms a plateau with small oscillations. The quasifission process is accompanied by an important multi-nucleon transfer. The quantum shell effect plays a crucial role in the mass and charge of quasifission fragments. The mass-angle distribution of the fragments is calculated, which can be compared directly with future experiments.     

Description of quasifission reactions in the dinuclear system model

The formation and evolution of dinuclear systems in quasifission reactions are investigated. The process of formation of reaction products is analyzed based on the concept of a dinuclear system. Isotopic trends of cross sections of production of superheavy nuclei in quasifission reactions are discussed. The yields of new neutron-rich isotopes of nuclei with Z = 64–80 in quasifission reactions are predicted. The mechanism of production of complex fragments in complete fusion and quasifission reactions is analyzed.     

The effect of the entrance channel on the fission of 216Ra

We have studied mass-energy distributions (MED) of fission fragments using two projectile-target combinations, ¹²C + ²⁰⁴Pb and ⁴⁸Ca + ¹⁶⁸Er, leading to the same compound nucleus ²¹⁶Ra at the excitation energy E*～40 MeV. It has been found that the contribution of the asymmetric mode in the case of the former reaction is 1.5%, and it is 30% in the case of the latter one. We connect such a sharp increase in the yield of asymmetric products in the ⁴⁸Ca + ¹⁶⁸Er reaction with the quasifission process, the MED of which have a clearly expressed shell structure. The characteristics of the fission fragment MED are of such a kind that they can be interpreted by analogy with the low-energy fission of heavy nuclei as a manifestation of an independent mode of nuclear decay which competes with the classical fusion-fission process.     

Comparison of the characteristics of the fusion-fission and quasifission products in reactions with heavy ions

Overlap of quasifission and fusion-fission product mass distributions measured for the ⁴⁸Ca + ¹⁵⁴Sm reaction at near-barrier energies is analyzed. As the incident ion energy increases, the angular distribution of quasifission fragments becomes narrower and they are concentrated near the forward and backward angles. The observed decrease in the yield of quasifission products with increasing collision energy is caused by noncoincidence of the product emission and detector position directions (the latter direction lags behind the beam direction by more than 15°) rather than by a decrease in the number of quasifission events. Our evaluations show that the excitation functions of evaporation residues in the ⁵⁴Cr + ²⁴⁸Cm reaction are several orders of magnitude larger than the excitation functions for the other reactions, ⁵⁸Fe + ²⁴⁴Pu and ⁶⁴Ni + ²³⁸U, used to synthesize a new superheavy element with Z = 120 (A = 302).