The field of radiative forces and the acoustic streaming in a liquid layer on a solid half-space

The acoustic field and the field of radiative forces that are formed in a liquid layer on a solid substrate are calculated for the case of wave propagation along the interface. The calculations take into account the effects produced by surface tension, viscous stresses at the boundary, and attenuation in the liquid volume on the field characteristics. The dispersion equations and the velocities of wave propagation are determined. The radiative forces acting on a liquid volume element in a standing wave are calculated. The structure of streaming is studied. The effect of streaming on small-size particles is considered, and the possibilities of ordered structure formation from them are discussed.     

Localization of the electromagnetic field in the vicinity of gold nanoparticles: Surface modification of different substrates

Theoretical predictions and experimental results for nanosized modification of metal (Au), semiconductor (Si), or dielectric (soda lime glass) substrates using near-electromagnetic field enhancement in the vicinity of gold nanoparticles are presented. The near field properties for the system consisting of an isolated gold nanoparticle or nanoparticle aggregate deposited on the substrates, which is irradiated by electromagnetic wave, are investigated using Finite Difference Time Domain Simulation technique. The influence of the substrate material on the near field distribution characteristics is predicted. The results reveal that the field on the substrate surface is enhanced in the three investigated cases, but its spatial distribution and magnitude depend on the substrate material. In the case of the metal and semiconductor substrate the enhanced near field is strongly localized in the vicinity of the contact point with the particle, in an area with diameter smaller than the particle's one. The intensity of the enhanced field on the glass is more than an order of magnitude lower than the case of using silicon substrate. The properties of the near field on the substrate surface also depend on the particle arrangement. For a two-dimensional gold nanoparticle array, when the particles are closely arrayed, the intensity of the enhanced field on the substrate surface is minimal. With the increase of the interparticle distance the near field intensity increases. The validity of the obtained theoretical results is confirmed experimentally.     

Physical forces exerted by microbubbles on a surface in a traveling wave field

The effect of a wave with a varying traveling component on the bubble activity as well as the physical force generated by microbubbles on a surface has been studied. The acoustic emission from a collection of bubbles is measured in a 928 kHz sound field. Particle removal tests on a surface, which actually measures the applied physical force by the bubbles on that surface, indicate a very strong dependence on the angle of incidence. In other words, when the traveling wave component is maximized, the average physical force applied by microbubbles reaches a maximum. Almost complete particle removal for 78 nm silica particles was obtained for a traveling wave, while particle removal efficiency was reduced to only a few percent when a standing wave was applied. This increase in particle removal for a traveling wave is probably caused by a decrease in bubble trapping at nodes and antinodes in a standing wave field.     

Simple and high efficient optical trapping using a cylindrical lens and a single plane wave of incidence

We suggest a simple and high efficient method for trapping particles in the evanescent field. In this method, a single plane wave is normally incident on the cylindrical surface of a cylindrical lens and then incident on the plane surface of the lens at an angle larger than the critical angle. Multiple reflections of light within the cylindrical lens create two evanescent waves with different directions in the transmitted field. Interference of two evanescent waves comes into being a standing wave which can stably trap particles close to the top of the cylindrical lens. Based on the Rayleigh approximation, we obtain analytical expressions of optical force acting on a Rayleigh particle placed in the vicinity of the lens. We find that the trap stiffness and trap depth is dependent on the radius of the cylindrical lens, wavelength and polarization of light, and incident angle at the lens–liquid interface.     

On nonlinear periodic capillary-fluctuation wave flow in a thin liquid film on a solid substrate

Analytical calculation of a nonlinear periodic wave flow on the free surface of a charged layer of an ideal incompressible conducting liquid resting on a solid substrate is carried out for the case when fluctuation-induced forces (the dispersion component of the wedging pressure) have a decisive effect on the system. It is shown that wave flows emerge in the liquid in calculations of the second order of smallness in the wave amplitude, which is assumed to be small compared with the thickness of the liquid layer. These flows result from nonlinear interaction as nonlinear corrections to the waves set at the zero time. The field of fluctuation-induced forces displaces these flows toward the periphery of the area of influence of these forces. This effect takes place both in the presence of an external electric field near the free surface and in its absence. The sign and value of the nonlinear corrections depend on whether an electric field is present near the free surface of the liquid. In the presence of an electric field, the curvature of the crest of the nonlinear waves increases; in its absence, the curvature decreases.     

Numerical simulation of laser-generated surface acoustic waves in the transparent coating on a substrate by the finite element method

The optimum finite element model in the system consisting of a transparent coating and an opaque substrate is established based on the analysis of two important parameters: meshing size and time step, and the stability of solution. Taking into account the temperature dependence of material properties, the transient temperature and temperature gradient field are obtained. According to the thermoelastic theory, this temperature gradient field can be taken as a buried bulk source to generate ultrasonic wave. The surface acoustic waves (SAWs) are obtained. The influence of the coating thickness on the SAWs is analyzed. The model provides a useful tool for the determination of modes which are generated by a laser source in transparent coating on opaque substrate. The surface skimming longitudinal wave exists for the multiple oscillations and it charges from unipolar waveforms to dipolar.     

Conditions for laser-induced plasma to effectively remove nano-particles on silicon surfaces

Particles can be removed from a silicon surface by means of irradiation and a laser plasma shock wave.The particles and silicon are heated by the irradiation and they will expand differently due to their different expansion coefficients,making the particles easier to be removed.Laser plasma can ionize and even vaporize particles more significantly than an incident laser and,therefore,it can remove the particles more efficiently.The laser plasma shock wave plays a dominant role in removing particles,which is attributed to its strong burst force.The pressure of the laser plasma shock wave is determined by the laser pulse energy and the gap between the focus of laser and substrate surface.In order to obtain the working conditions for particle removal,the removal mechanism,as well as the temporal and spatial characteristics of velocity,propagation distance and pressure of shock wave have been researched.On the basis of our results,the conditions for nano-particle removal are achieved.     

Removal mechanisms of micro-scale particles by surface wave in laser cleaning

This paper is to investigate the mechanisms of micro-scale particle removal by surface wave, which was induced by a short pulse laser in a cleaning process. The authors analyzed the adhesive forces of particles on substrate surface and the clearance force produced by surface wave in laser cleaning. The physical model of particle removal by laser-induced surface wave was established to predict the removal area and the processing conditions of laser cleaning. In this research, a KrF excimer laser was applied to irradiate 304 stainless steel specimen distributed with copper particles to generate surface wave for copper particle removal. Considering that a time-varying and uniformly distributed heat source irradiates on material surface with thermao-elastic behavior, the displacement and acceleration of substrate induced by a pulsed laser were solved by an uncoupled thermal–mechanical analysis based on the finite element method. The processing parameters such as laser energy, laser spot size are discussed, respectively. A series of laser cleaning experiments were designed to compare with computation results. The results show that the removal area by surface wave beyond the laser spot increases with the laser energy and that, the surface acceleration decreases with the increase of the laser spot size.     

The transmission enhancement of a THz pulse through an Ag/Ag2O layer detected by terahertz time-domain spectroscopy

This paper reports a new way to detect the enhanced transmission of a THz electromagnetic wave through an Ag/Ag2O layer by THz-TDS （time-domain spectroscopy）. As the THz beam illuminates the sub-wavelength Ag particles gained by Ag2O thermal decomposition, the evanescent wave is generated. The evanescent wave is coupled by a 500μm-GaAs substrate, which attaches behind the Ag/Ag2O layer, and then it transmits to the far field to be detected. The experimental results indicate that the transmitting amplitude is enhanced, as well as the frequent shifting and spectra broadening.     

Mechanical stresses in an irradiated target with a disturbed surface

Mechanical stresses generated in a disturbed-surface solid target irradiated by intense fluxes of accelerated charged particles are studied numerically and analytically. The disturbed surface is needed to analyze the influence of microirregularities present on real surfaces on the stress pattern. Three basic components of the stress field are revealed: a shock wave; stresses localized in the energy liberation region; and disturbed stresses, which are due to the disturbed surface. The disturbed stresses are localized in a surface layer of width comparable to the disturbance wavelength and account for about 30% of the field stress energy. It is concluded that the disturbance of the surface and disturbance-induced stresses should be taken into account in analysis of structural transformations under irradiation.     

驻波声场中单分散细颗粒的相互作用特性

利用外加声场促进悬浮在气相中的细颗粒发生相互作用,进而引起颗粒的碰撞和凝并,使得颗粒平均粒径增大、数目浓度降低,是控制细颗粒排放的重要技术途径.为探究驻波声场中单分散细颗粒的相互作用,建立包含曳力、重力、声尾流效应的颗粒相互作用模型,采用四阶经典龙格-库塔算法和二阶隐式亚当斯插值算法对模型进行求解.将数值模拟得到的颗粒声波夹带速度和相互作用过程与相应的解析解和实验结果进行对比,验证模型的准确性.进而研究颗粒初始条件和直径对相互作用特性的影响.结果表明,初始时刻颗粒中心连线越接近声波波动方向、颗粒位置越接近波腹点,颗粒间的声尾流效应就越强,颗粒发生碰撞所需要的时间就越短.研究还发现,颗粒直径对颗粒相互作用的影响取决于初始时刻颗粒中心连线偏离声波波动方向的程度.当偏离较小时,颗粒直径越大,颗粒发生碰撞所需要的时间越短;当偏离很大时,直径较小的颗粒能够发生碰撞,而直径较大的颗粒则无法发生碰撞.     

Uniform plasmonic near-field nanopatterning by backward irradiation of femtosecond laser

We present localized optical field distribution properties in the vicinity of gold particles on a silicon substrate by backward and forward irradiation. It is technically difficult to fabricate nanostructures on the surface by a conventional forward laser incident to the substrate because gold nanoparticles easily aggregate to form double-layered particle arrays. We calculated enhanced optical field properties in order to pattern the substrate surface only with a template of the bottom-layered particle arrays in the case that the backward irradiation of a femtosecond laser is used in the system of aggregated double-layered gold nanoparticle arrays. With the backward irradiation, the optical field intensity in the substrate for the double-layered hexagonal arrays is found to be only 30% lower than the mono-layered system. Moreover, a near field cannot be generated with the forward irradiation. As a result, only the backward irradiation scheme is found to be effective for uniform surface nanopatterning at enhanced plasmonic near-field zones.     

激光等离子体去除微纳颗粒的热力学研究

微杂质污染一直是影响精密器件制造质量和使用寿命的关键因素之一.对于微纳米杂质颗粒用传统的清洗方式(超声清洗等)难以去除,而激光等离子体冲击波具有高压特性,可以实现纳米量级杂质颗粒的去除,具有很大的应用潜力.本文主要研究了激光等离子体去除微纳米颗粒过程中的热力学效应:实验研究了激光等离子体在不同脉冲数下对Si基底上Al颗粒去除后的颗粒形貌变化,发现大颗粒会发生破碎而转变成小颗粒,一些颗粒达到熔点后发生相变形成光滑球体,这源于等离子体的热力学效应共同作用的结果.为了研究微粒物态转化过程,基于冲击波传播理论研究,得到冲击波压强与温度特性的演化规律;同时,利用有限元模拟方式研究激光等离子冲击波压强和温度对微粒作用规律,得到了颗粒内随时间变化的应力分布和温度分布,并在此基础上得到等离子体对颗粒的热力学作用机制.     

Retarded treatment of substrate-related effects on granular films I. Polarizability of a single sphere

A multipolar treatment of the retarded fields radiated by a metal sphere on a dielectric substrate under the influence of an incident plane wave described. Unlike previous treatments, the present one allows boundary conditions, both on the spherical surface and on the substrate interface, to be matched by simply solving an adequate number of linear equations. The problem is thus reduced to inverting three complex matrices, whose sizes depend on the number of multipoles included in the field forms. The solutions, which represent the object and image multipoles (both in the incidence and in the transmission media) associated with the polarized sphere, are given the form of linear combinations of the multipoles associated with the unperturbed field (incident and reflected waves).     

Capture into resonance: a method for efficient control

To achieve large changes in adiabatic invariants using small control input, a conservative dynamical system must possess an internal resonance. Capture into resonance is an inherently probabilistic process. We propose a control method to make it more structured. We study the motion of charged particles in an electromagnetic field as an example of such a system. When the nominal dynamics brings particles close to a resonance surface, a short control pulse forces the capture of a particle into the resonance with the wave. A captured particle is transported by the wave across the energy levels. The second pulse releases a particle from the resonance when the desired energy level is achieved. We discuss the distribution of energy achieved by the method.     

Influence of laser-ablation plume dynamics on the room-temperature epitaxial growth of CeO2 on silicon

High-quality epitaxial CeO₂ thin films were obtained on Si(001) buffered with a yttria-stabilised zirconia layer by pulsed laser deposition. Although the best structural properties were achieved at high substrate temperature, high-quality epitaxy was obtained even at room temperature. Epitaxial growth at low temperature is promoted by the high kinetic energy of particles reaching the substrate. The oxygen pressure and target-substrate distance had a strong influence on the crystallographic structure and surface morphology in low-temperature deposition. This behaviour is attributed to a change in the kinetic energy of the particles, which was evaluated from the plasma expansion velocity determined by an intensified CCD camera. If a shock wave forms, a minimum substrate temperature of 550 °C is necessary for epitaxial growth.     

Enhancement of the Local Electromagnetic Field over Planar “Particles” Formed on the Surface of a Polar Crystal

Small “particles” of an open surface were formed on a SiC polar crystal with openings in the opaque metal mask covering the sample. The dimensions of the holes were about surface phonon polariton wavelength. Such a sample was irradiated with an electromagnetic wave ( λ = 10.68μm) at a frequency close to the lattice resonance of SiC. A significant enhancement in the field amplitude of surface phonon polariton waves was detected over such “particles” compared to the amplitude over an infinite open surface of SiC. Such a phenomenon, observed by us in the IR band, is similar to plasmon resonance on small metal particles in the visible band, but the lateral resolution of the ASNOM used (no worse than 30 nm at 10 μm) makes the obtained field distribution more detailed. The maps of the local field amplitude and phase obtained on SiC surface with ASNOM are in a good quantitative agreement with simulations using the Green’s function.     

Radiation of a charge moving over the diffraction grating

The states of a charged particle with a finite free path are determined in the field of a resonant electromagnetic wave. The exact resonance conditions, the modulation and beam instability mechanisms, the charge and current densities (Ohm's law) are obtained for the collisionless beam of resonance particles. Quantum theory of radiation is developed for the resonant adiabatic interaction between a particle and a wave taking into account the interaction with a constant magnetic field induced at the grating surface by the charge and nonresonant waves. The radiation power, the spectrum, and the range of generated frequencies are determined. The results obtained can be used in the plasma and solid-state theories and in electronics.     

Particle transport by standing waves on an electric curtain

Discrete-element simulations are performed to study particle transport by standing waves on an electric curtain. An electric curtain consists of a series of parallel electrodes with oscillating potential field embedded in a dielectric surface. The study shows that particles can be transported in two different modes under excitation by standing waves. In the first mode, particles roll along the surface in a constant direction with average velocity equal to the wave speed. In the second mode, particles hop along the surface in a manner akin to a Brownian motion. Effect of particle collisions on these transport modes is evaluated.     

Positioning of small particles by an ultrasound field excited by surface waves

A method for the controlled positioning of small particles in one or two dimensions by an ultrasound field excited by a surface wave is presented. Particles of a diameter between 10 and 100 microm placed on a surface can be concentrated at certain locations and moved over the surface. In other approaches it is possible to let the particle levitate freely in the fluid. However for the use of ultrasonic positioning in for example microassembling it is necessary to move particles over a surface as well as to let them levitate over the surface. Physical principle: A two- or three-dimensional ultrasound field is excited in a fluid filled gap between a rigid surface at the bottom and a vibrating surface of a solid at the top. The height of the gap varies between 0.1 and 2 mm. A one-dimensional sinusoidal vibration of the upper surface excites a two-dimensional ultrasound field in the fluid. Particles that are arbitrarily distributed on the lower surface will be concentrated in lines by the ultrasound field. First the calculation of the field of forces on particles in the fluid layer is presented. Then the dispersion relation of a vibrating plate which is in contact with a fluid on one side is derived. The technical setup will be introduced. Finally the experiments are shown and compared to the theoretical results.