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《Angewandte Chemie (International ed. in English)》2017,56(20):5485-5489
The coordination chemistry of plant polyphenols and metal ions can be used for coating various substrates and for creating modular superstructures. We herein explored this chemistry for the controlled release of guests from mesoporous silica nanoparticles (MSNs). The selective adsorption of tannic acids (TAs) on MSN silica walls opens the MSN mesoporous channels without disturbing mass transport. The channel may be closed by the coordination of TA with CuII ions. Upon exposure to light, photolysis of Trojan horse guests (photoacid generators, PAGs) leads to acid generation, which enables the release of payloads by decomposing the outer coordination shell consisting of TA and CuII. We also fabricated a modular assembly of MSNs on glass substrates. The photoresponsive release characteristics of the resulting film are similar to those of the individual MSNs. This method is a fast and facile strategy for producing photoresponsive nanocontainers by non‐covalent engineering of MSN surfaces that should be suitable for various applications in materials science. 相似文献
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Inside Cover: Coordination Assembly of Discoid Nanoparticles (Angew. Chem. Int. Ed. 31/2015) 下载免费PDF全文
Dr. Kenji Hirai Dr. Bongjun Yeom Dr. Shu‐Hao Chang Dr. Hang Chi Dr. John F. Mansfield Dr. Byeongdu Lee Sungsik Lee Prof. Ctirad Uher Prof. Dr. Nicholas A. Kotov 《Angewandte Chemie (International ed. in English)》2015,54(31):8850-8850
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Dr. Ana Albu‐Yaron Prof. Dr. Moshe Levy Prof. Dr. Reshef Tenne Dr. Ronit Popovitz‐Biro Marc Weidenbach Dr. Maya Bar‐Sadan Dr. Lothar Houben Dr. Andrey N. Enyashin Prof. Dr. Gotthard Seifert Prof. Dr. Daniel Feuermann Dr. Eugene A. Katz Prof. Dr. Jeffrey M. Gordon 《Angewandte Chemie (International ed. in English)》2011,50(8):1728-1728
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Cover Picture: Engineering Multifunctional Capsules through the Assembly of Metal–Phenolic Networks (Angew. Chem. Int. Ed. 22/2014) 下载免费PDF全文
Junling Guo Dr. Yuan Ping Dr. Hirotaka Ejima Dr. Karen Alt Mirko Meissner Joseph J. Richardson Dr. Yan Yan Prof. Karlheinz Peter Prof. Dominik von Elverfeldt Assoc. Prof. Christoph E. Hagemeyer Prof. Frank Caruso 《Angewandte Chemie (International ed. in English)》2014,53(22):5475-5475
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Anat Frydman‐Marom Meirav Rechter Irit Shefler Yaron Bram Deborah E. Shalev Dr. Ehud Gazit Prof. 《Angewandte Chemie (International ed. in English)》2009,48(11):1868-1868
The accumulation of amyloid‐β (Aβ) as amyloid fibril deposits may play a central role in the pathogenesis of Alzheimer's disease, which is among the most common diseases of the 21st century. E. Gazit and co‐workers describe in their Communication on page 1981 ff. a novel Aβ fibrilization inhibitor, whose mechanism of action is based on targeting aromatic recognition modules together with a unique Cα‐methylation β‐breakage strategy. We thank Tal Mazor for the graphical assistance with the cover.