Nuclear resonance fluorescence in94Mo,95Mo and96Mo

Using gaseous sources of Tc₂O₇ containing the radioactive isotopes⁹⁴Tc,⁹⁵Tc and⁹⁶Tc, levels at 871.0keV (⁹⁴Mo), 765.8, 820.6, 947.8, 1074.0keV (⁹⁵Mo) and 778.3keV (⁹⁶Mo) have been excited. From the effective cross sections for nuclear resonance scattering and from the lifetimes of the 947.8, 1074.0 and 778.3keV levels known from Coulomb excitation experiments the profiles of theγ-lines have been determined. A broadening of theγ-lines due to Coulomb explosion of the molecules has been observed. Making use of the line profiles, lifetimes ofΤ=(6.4±1.0) ps andΤ=(0.90 ± 0.20) ps have been determined for the 765.8 and 820.6keV levels, respectively. The angular distribution of the resonantly scattered radiation yields an amplitude ratioδ for the mixed M1 E2 765.8keV transition ofδ=0.14 _?0.009 ^+0.08 . TheB(E2) from a Coulomb excitation experiment and the lifetimeΤ from the present experiment yield ¦δ¦=0.07±0.01 for the 820.6keV transition.     

Parity violation in the 17/2− isomer of93Tc

The parity-violating mixing of the 17/2^? and 17/2⁺ levels in⁹³Tc nuclei, polarized by the tilted multifoil interaction, was measured by the observation of the forwardbackwardγ-ray asymmetry. The asymmetry was determined to beA _γ=1.18(48)×10^?3. The nuclear polarization was determined in a measurement of the quadrupole interaction in a⁹²Mo isomer and the parity violation matrix element 〈H _PV〉 is found to be ¦〈H _PV〉¦ =0.8(4) meV.     

Stark-Effekt-Untersuchungen in der Hyperfeinstruktur der 3s 2 3d 2 D 5/2- und2 D 3/2-Terme des Al I-Spektrums

The resonance fluorescence of the transitions 3d ² D _5/2,3/2 3p ² P _3/2,1/2 in the Al I-spectrum was observed as a function of a magnetic field. Adding an electric field parallel to the magnetic field the shifts of level crossing signals caused by the Stark effect of the electric field were used to separate overlapping signals of the 3d ² D _5/2- and 3d ² D _3/2-states. The following values of the Stark parametersβ of both states and the hyperfine structure constantsA andB of the 3d ² D _3/2-states were deduced: 3d ² D _3/2∶ ¦A¦=99(1) Me/sec · g_J/0,8,B/A=?0,22(12), ¦β¦=0.45 (8) Mc/sec/(kV/cm)² · g_J,/0.8, A/β< 0 3d²D_5/2∶ ¦β¦=0.16 (4) Mc/sec/(kV/cm)² · g_J/1.2, A/β>0. Some qualitative aspects of interconfiguration mixing in the 3d²D-states are discussed.     

Detection and dosimetry of gamma ray emitted from thallium-201 and technetium-99m based on chemiluminescence technique

This report describes the detection and dosimetry of gamma ray emitted from Thallium-201 (²⁰¹Tl) and Technetium-99m (^99mTc) based on chemiluminescence technique. H₂O₂ produced by two gamma emitter radioisotopes of ²⁰¹Tl and ^99mTc were quantitatively measured by chemiluminescence method. Upon producing H₂O₂ in a luminol alkaline solution, in the presence of diperiodatocuprate, as catalyst a chemical reaction was accrued and consequently the emitted light was measured. The determined H₂O₂ concentration was correlated with the gamma ray detection and dosimetry. The sensitivity of chemiluminescence technique for ²⁰¹Tl and ^99mTc dosimetry was determined to be 0.20 and 0.08 MBq/l (Mega Becquerel per liter) respectively (R.S.D. = %5, N = 3). The plotted calibration curves showed detection limits of 3.24 and 1.76 MBq/l for ²⁰¹Tl and ^99mTc, respectively.     

Spin des 921 keV-Zustandes in99Tc

The angular correlation of the⁹⁹Tc 739-181 keV gamma-gamma cascade has been measured in a liquid molybdenium source. The result was:A ₂=0.0930 ± 0.0028,A ₄=?0.0095 ± 0.0042. The spin of the 921 keV level was determined to 3/2⁺. The mixing ratio of the 739 keV gamma-transition was measured to δ (E2/M1)=5.9 _?0.3 ^+0.4 .     

Local magnetic fields in the Mo layer of Mo/Fe multilayer

Using time-differential perturbed-angular-correlation technique, hyperfine fields at ⁹⁹Tc (←⁹⁹Mo) in the Mo layers in polyimide/Fe (10 nm)/[Mo (t _Mo)/Fe (2.0 nm)]₁₂₀, where t _Mo is in the range between 0.4 and 1.5 nm, were measured at room temperature. The values of the magnetic hyperfine field at the Mo/Fe interface were extracted. Its dependence on the Mo layer thickness suggests that the oscillatory interlayer exchange coupling is due to conduction electron spin polarization in the Mo layer, which in turn is produced via an RKKY-type mechanism.     

L ∞ estimates for the space-homogeneous Boltzmann equation

This paper studies the boundedness of solutionsf of the initial-value problem for the space-homogeneous Boltzmann equation for inverse kth power forces, whenk>5, and under angular cutoff. The main result is that if the initial value isf ₀ ? 0 with (1 + ¦υ¦²)φ₀ εL ¹ and (1 + ¦υ¦)^s f ₀ε L^∞ for somes > 2, then (1 + ¦υ¦^s'f _tεL ^∞ fort>0 and ess_υ,t sup(1 + ¦υ¦)^s'f(υ, t,) < ∞ for anys′ ? s whens ? 5, and anys′ ? s ifs > 5.     

Static electric quadrupole interaction of Ta- and Hf-ions in barium and lead titanate

The static electric quadrupole interaction of¹⁸¹Ta and¹⁷⁸Hf in polycrystalline barium and lead titanate at the site of titanium has been measured using time differential PAC and the Mössbauer effect. The electric field gradients (EFG) at room temperature at the¹⁸¹Ta nucleus are ¦V _zz¦=(3.6±0.2)·10¹⁷V/cm² in BaTiO₃ and ¦V _zz¦=(14.6±0.6)·10¹⁷ V/cm² in PbTiO₃. The temperature dependence of the quadrupole interaction has been studied giving the following EFG values: ¦V _zz¦=(2.4±0.2)·10¹⁷ V/cm² in the monoclinic and ¦V _zz¦=(1.1±0.3)·10¹⁷ V/cm² in the rhomboedral phase of BaTiO₃, and ¦V _zz¦=(15.7±0.6)·10¹⁷ V/cm² for¹⁸¹Ta/PbTiO ₃ at 77 °K. The EFG of¹⁷⁸Hf in PbTiO₃ has been derived from a Mössbauer effect experiment to beV _zz=+(10.7±0.5)·10¹⁷ V/cm². The results are compared with EFG's calculated in a point charge model and with experimental EFG's measured at⁴⁴Sc and⁵⁷Fe in the same titanates by other authors. Contributions of covalent bonds to the effective EFG's in perovskit crystals are discussed.     

Study of the Elution Profile of the 99mTc Gel Generator

The generator with gel matrix is considered a perspective type for obtaining ^99mTc. The elution yield of a generator and the course of the elution profile A_Vn = f(V_n) are affected by the properties and conditions of preparation of zirconium molybdate (generator matrix). Furthermore, it is influended by neutron flux density as well as irradiation time and temperature of cooling water during the irradiation. Zirconium molybdate, Mo: Zr = 1.72, in the form of a monodispersion (mean particle size x = 0.175 mm), was irradiated under the neutron flux density ?_n = (0.7 … 2.2) × 10¹³ cm^?2 s^?1. The elution profile and the elution yield of ^99mTc were examined in dependence on the temperature of drying the Zr–Mo matrix (40–100 °C). The kinetics of the passage of ^99mTc into the solution, in dependence on the temperature of drying the hydrogel, was investigated. Some predetermined substitutional functions were tested and the mechanism of the ^99mTc passage into solution was explained.     

High-spin states in99Tc

The level scheme of⁹⁹Tc was studied byγ-ray spectroscopy with the⁹⁶Zr(⁶Li, 3n γ)⁹⁹Tc reaction. New levels were established and spins and parities assigned.⁹⁹Tc is compared with^{93, 95, 97}Tc, with the neighbouring even-even Mo-isotopes and with the results of an IBFM calculation.     

Study of the level structure of239U using the thermal neutron capture reaction

For the investigation of vibrational states in odd A nuclei we have studied the level structure of²³⁹U by the²³⁸U (n _thermal,γ) reaction. Various complementary measurement techniques as curved-crystal-, anti-Compton-,γ-γ coincidence- and conversion electron spectroscopy have been applied. The resulting data have been used to establish the deexcitation scheme of²³⁹U up to ～1.3 MeV and to make spin assignments. Most of the levels are interpreted in terms of the Nilsson model. The data also indicate the presence of the Nilsson states ¦501?¦ and ¦750¦. Three members of theΒ-vibrational band built on the ¦631?¦ state and one member of theΒ-vibration built on the ¦622↑¦ ground state have been identified through transitions with strongE0 admixtures. The octupole vibrational state built on the ¦631?¦ band is proposed at 815 keV.     

Theβ-decay of88Tc

Decay scheme, half life andQ _EC value of⁸⁸Tc were deduced from aβ-decay study. The neutron deficient nucleus⁸⁸Tc was produced by the⁵⁸Ni(³²S,pn)⁸⁸Tc reaction using beam energies of 100, 101 and 105 MeV. The ground- and isomeric states of⁸⁸Tc were found to decay to⁸⁸Mo with similar half lives of 5.8±0.2 and 6.4±0.8 sec. The most probable spins and parities of these states are 3⁺ and 6⁺, respectively, though the order in energy could not be determined. TheQ _EC value was deduced to be 8.6±1.3 MeV.     

A study of the 99Tc(p,d)98Tc reaction

The energy levels of ⁹⁸Tc were studied with the ⁹⁹Tc(p, d)⁹⁸Tc reaction at a bombarding energy of 22.9 MeV and 15 keV resolution (FWHM). The Q-value for this reaction was found to be ?6.755 ± 0.009 MeV and the ⁹⁸Tc mass excess was calculated to be ?86.421 ± 0.011 MeV. This reaction provided the excitation energies for 49 neutron hole states below 1.5 MeV excitation. Comparison of experimental angular distributions with DWBA calculations permitted assignment of lf-values and the extraction of spectroscopic factors for 44 of these levels. Extensive configuration mixing is observed except in the low-lying multiplet. Effective proton-particle, neutron-hole interaction matrix elements were obtained from the low-lying positive-parity multiplet of ⁹⁸Tc.     

99mTc Generator — The Maintenance of High Elution Efficiency

Several protecting procedures were applied to ensure good operating performances of the universal ^99mTc generators based on fission produced ⁹⁹Mo. These procedures include the modifications of the adsorbent. Instead of 1 g of pure Al₂O₃ the adsorption of ⁹⁹Mo is carried out on the multicomponent adsorbent containing the mixture of either Al₂O₃ + SiO₂ or Al₂O₃ · Cu²⁺ + SiO₂. The protection by drying should ensure that the columns contain minimum of moisture during the growth period of ^99mTc. It was found experimentally that the best results are obtained when the ratio of alumina in the mixture was 15 ± 5 (wt.%) and content of copper 365 μg Cu²⁺/column. The comparison of efficiency and applicability of the used protecting procedures is also given.     

Level structure of 99Tc by inelastic scattering and proton stripping

The ⁹⁸Mo(³He, d)⁹⁹Tc and ⁹⁹Tc(d, d') reactions have been used to study the levels of of ⁹⁹Tc. Spin-parity assignments are made for nearly all states below 1.5 MeV excitation. Strong j-dependence is noted for l = 1 transitions in the proton stripping reaction, making possible several new spin assignments. The inelastic scattering data on ⁹⁹Tc are compared to similar data on ⁹⁸Mo, and are found to be in agreement with a coupling scheme based on a shell model with good seniority.     

Quadrupole interaction of8Li and9Li in LiNbO3 and the quadrupole moment of9Li

The quadrupole interaction of nuclear spin polarized⁸Li (I=2) and⁹Li (I=3/2) in LiNbO₃ has been studied at room temperature. The polarization was achieved by optical pumping of a fast atomic beam with circularly polarized laser light. The atoms were implanted into a hexagonal LiNbO₃ single crystal and the quadrupole splitting ofβ-NMR spectra was measured. A ratio of ¦Q(⁹Li)/Q(⁸Li)¦=0.88(4) for the nuclear quadrupole moments was deduced, yielding a new value of ¦Q(⁹Li)¦=25.3 (9) mb for the quadrupole moment of⁹Li.     

Level-Crossing-Experimente zur Untersuchung der Hyperfeinstruktur des 5d 2 D 5/2-Terms im Indium I-Spektrum

The resonance fluorescence of the transition 5d ² D _5/2?5p ² P _3/2 (λ=3256Å) in the In I-spectrum was observed as a function of an external magnetic field. From the level crossing signals the following values of the hyperfine constantsA andB of the 5d ² D _5/2-state were deduced: ¦A¦=148(8) Mc/sec·g _J/1.2 and ¦B/A¦≦0.3. The widths of the signals yielded the mean lifetimet=7.1 (6)·10^?9 sec · 1.2/g _J . From the shifts of the signals caused by a constant electric field parallel to the magnetic field the value of the Stark parameter ¦β¦=0.19(4) Mc/sec/(kV/cm)² ·g _J /1.2 and the sign of the ratioA/β<0 were determined. Calculations with Coulomb wave functions show that the Stark shifts of the electric field are mainly due to admixtures of the 6p ² P _3/2-state.     

Hyperfine structure investigations of some odd levels of Co I by level crossing and optical methods

Using the level crossing technique the ratios and absolute values of the hyperfine structure (hfs) constants of the levelsz ⁴F_9/2 andz ⁴F_7/2 of the configuration 3d ⁷4s4p of Co I were measured:z ⁴ F _9/2: ¦A¦=(811±12)MHz; ¦B¦=(48±93) MHz;B/A=?0.06±0.11 A>0; B<0z ⁴ F _7/2: ¦A¦ = (659 ±11)MHz; ¦B¦=(33±84)MHz;B/A=?0.05±0.13 A>0; B<0. In addition the hfs constants of three other excited levels of Co I could be determined by optical methods:z ⁴ F _9/2:A=525±26 MHz;B=200 MHzy ⁴ F _9/2:A=300±30 MHz;B=?500 MHzy ⁴ G _11/2:A=315±20 MHz;B=400 MHz. The experimental results are compared with known experimental and also with theoretical values which where calculated using the parametric potential method.     

Investigation of224Ra in the226Ra(α, α′ 2n) reaction

Positive and negative parity bands have been followed up to 10⁺ (possibly 12⁺) and 11^? in²²⁴Ra and are compared to the corresponding bands in the isotone²²⁶Th. If a constant value of the intrinsic quadrupole moment is assumed for allE2 transitions in²²⁴Ra theE1/E2 branching ratios are consistent with an intrinsic dipole moment of ¦Q₁¦=0.032(3)e·fm. This small value, as compared to ¦Q₁¦=0.30(2)e·fm for²²⁶Th, can be explained by an almost complete cancellation of large positive liquid-drop and negative shell-model contributions.     

Predictions for anomalous τ+τ−γ production at LEP 1

We calculate distributions for τ⁺τ^?γ production at LEP 1 taking into account a potentially existing anomalous magnetic moment a _τ of the τ lepton. The existing upper limits for ¦a _τ¦ are known from the dependence of the decay Z ⁰ → τ⁺τ^?γ on a _τ ² and are of the order of (1–5)%. We show that such limits are also sensitive to linear terms in a _τ, which are of equal importance at ¦a _τ¦ ～ (1–2)% and dominate below this value. Contributions from an electric dipole moment dτ do not interfere with the electromagnetic vertex or with the anomalous magnetic moment. Appropriate formulae are derived.