Anomalous conversion of 127 keV (E3) transition in134Cs

The total conversion coefficient of the 127.49 keV E3 isomeric transition in the decay of^134mCs was measured using the gamma intensity balance method with the help of a high resolution low energy photon detector. Theα _Tvalue was found to be 5.84±0.47 as against the theoretical value of 6.96, thus showing an anomaly of (16.1±6.7)%. TheK-conversion coefficient,α _kwas also measured using the X-ray peak to gamma ray intensity method and found to be 2.24±0.04 as against the theoretical value of 2.72, which shows an anomaly of (17.6±1.4)% consistent with the experimental anomaly inα _T. TheE3 hindrance factor of the isomeric transition was estimated to be (3.44±0.23) ·10⁴.     

A Si(Li) detector system for conversion coefficient measurements and application to the decays of51Cr and87Y

An electron detector system with a 3 mm × 100 mm² Si(Li) detector with a cooled FET and vacuum air lock for changing sources was constructed. The absolute efficiency was measured as a function of energy for use in the measurement ofK conversion coefficients. With the Si(Li) and a Ge(Li) detector, theK conversion coefficient of the 320 keV transition in⁵¹V was measured to be 0.00156 ± 0.00008 where theK conversion coefficients of the 661 and 279 keV transitions in¹³⁷Ba and²⁰³Tl were used as standards. From absolute detection efficiency measurements, theK conversion coefficients of the 388 and 483 keV transitions in⁸⁷Sr were measured to be 0.16 ± 0.02 and 0.0024 ± 0.0003, respectively.     

AnomalousK-conversion coefficient of the 124keV transition in131Cs

The absoluteK-conversion coefficients of the 496 keV-124 keV cascadeγ-rays in¹³¹Cs have been determined from angular correlation experiments using a new approach. The value ofα _K =0.0100±0.0007 obtained for the 496 keV transition is in excellent agreement with the theory whereas a strong case is presented for the existence of an anomalous nuclear-structure-dependent conversion coefficient for the 124 keV transition. TheK-conversion coefficient for this transition has been measured to be 0.742±0.077 giving a value of 1.25±0.13 for the ratioα _K ^(expet) /α _K ^(theory) . The result is interpreted as being due to the presence of electric monopole,E0, electron transition. A value of 0.26±0.14 has been obtained for theE0/E2 electron conversion ratio and the absolute value of the electric monopole matrix element has been determined to be 0.07±0.02.     

Vibrational band structure in 184W populated in the decay of 184Re

The decay of ^184mRe has been investigated through γ-ray and conversion electron studies. The band head of the K^π = 2^? octupole band has been established at 1130.0 keV. The E2/M1 mixing ratios of three transitions from the γ-vibrational band to the ground state band have been determined by angular correlation measurements. A mixing of El, M2 and E3 multipolarity has been derived for the 921 keV transition combining angular correlation and conversion electron data. A value B(E3, 0⁺ → 3^? = (25 ± 5) × 10⁴e² · fm⁶ was obtained from the measured E2/M1 mixing of the 91 keV 3^? → → 2^? transition and γ-branchings. The data are discussed in terms of the collective model taking into account band mixing.     

Total conversion coefficient and γ-line of the 13.34 keV level in73Ge

The total conversion coefficient of the lowest excited state in⁷³Ge has been measured to be α_tot=1310±60, which is close to the theoretically predicted value 1080 of Hager and Seltzer for a pureE2 transition. The energy of the γ-line is (13.34±0.04) keV. A calculation, based on the experimental data, shows that the Mössbauer effect on this level is measurable.     

Verzweigungsverhältnisse und Konversionskoeffizienten von angeregten Zuständen des208Tl

The branching ratios of theγ rays of the second and fourth excited states of²⁰⁸Tl have been investigated by coincidence measurements between the α rays of²¹²Bi and subsequent 40keVγ ray. The detectors employed were a silicon surface barrier counter for α particles, and a 1.5 in ×2 mm NaJ (Tl) crystal forγ rays. It has been found that (75.6±3.7)% of all transitions of the 328 keV state and (94±7)% of all transitions of the (492 keV+473 keV) states populate the first excited state of²⁰⁸Tl. The 40 keV state is excited to (3.4±0.3)% by transitions of higher excited states relative to the direct excitation by α particles. The number of α particles with energyE _α = 6.047 MeV and the number of subsequent 40keVγ rays resulted in a conversion coefficient α(40keV)=22.55± 0.46. Similarly coincidence measurements between Tl-x rays and α particles have been used to determine theK- conversion coefficients α_K(328 keV)=0.31±0.03 and α_K(492 keV+ 473keV)=0.100±0.015. The experimental results are in good agreement with the theoretical values ofSliv.     

Coulomb excitation in 180Hf

Coulomb excitation studies have been performed to measure transition probabilities of collective quadrupole vibrational states in ¹⁸⁰Hf. The I = 2 level of the K^π = 2⁺ collective γ-band is established at 1200.5 keV with B(E2)_exc = (11.0 ± 1.1) × 10^?50e² · cm⁴ (3.6 ± 0.4 s.p.u.). The angular distribution of the de-exciting γ-rays from this level yields δ = 9.6⁺²²_?5.8 or, less likely, 0.7 ± 0.2 for the 1107.2 keV 2_γ⁺ → 2_g⁺ transition. The B(E2)_exc for any K^πI = 0⁺2 stateorother 2⁺ states up to 1500 keV is less than 5 × 10^?51e² · cm⁴ (< 0.2. s.p.u.).     

The investigation of the reaction22Na(n,p)22Ne for a neutron energy to 1,000 eV

TheK-internal conversion coefficient of the 205 keV (7/2⁺→5/2⁺) transition in¹⁰⁷Cd was determined. From the measured value α _K =0.0552±0.0009 and the known value of theE2/M1 mixing ratio δ² a value of 6.3±1.5 was deduced for the penetration parameterλ. Information derived on effective gyromagnetic ratios in the frame of an extreme single particle model is briefly discussed.     

Measurement of the parity non-conservation in nuclear forces in 75As, 171Tm,and 175Lu and of the polarized bremsstrahlung from 51Cr, 170Tm, 177Lu,and 198Au

The circular polarization P of γ-rays from unpolarized sources of ⁷⁵Se, ¹⁷¹Er, and ¹⁷⁵Yb of strengths ? 500 Ci has been measured with a Compton polarimeter of the radial transmission type. Eight NaI crystals and a four-fold current integration system were used to simultaneously record the data in four independent channels. The results are: P = ?(1.8 ± 6.0) × 10^?5 for the 401 keV transition in ⁷⁵As (the experimental error is ± 1.5 × 10^?5, the remaining part is due to the uncertainty in the decay scheme of ⁷⁵Se), P = (0.8 ± 1.5) × 10^?4 for the 296 keV and 308 keV transition in ¹⁷¹Tm, and P = (5.7 ± 0.8) × 10^?5 for the 396 keV transition in ¹⁷⁵Lu. The last value confirms the parity non-conservation in nuclear forces. The polarimeter was calibrated with bremsstrahlung from ¹⁷⁰Tm. The correction for polarized bremsstrahlung was given special attention. Correction factors are derived for ⁵¹Cr, ¹⁷⁷Lu, and ¹⁹⁸Au from a comparison of the measured and calculated bremsstrahlung yields.     

Der Zerfall von Er171 und Er165

Theγ-spectrum of a neutronactivated probe of natural Er₂O₃ revealed an additional peak at 55 keV, which was attributed to the characteristicK-Röntgenstrahlung from the decay of Er¹⁶⁵ by measurement of its half-life in a NaJ-wellcrystal. The activation cross section for thermal reactor neutrons for Er¹⁶⁴ (n, γ) Er¹⁶⁵ has been determined to σ _A =20±7 barn. The averaged conversion coefficient of the 111, 116 and 124 keV γ-rays from Er¹⁷¹→Tm¹⁷¹ have been remeasured with scintillation counter equipment.     

Measurement of the 15N(α, γ)19F resonances at Ec.m. = 536 keV and 542 keV

The E_c.m. = 536 keV and E_c.m. = 542 keV resonances in the ¹⁵N(α, γ)¹⁹F reaction have been studied using a thick Ti¹⁵N target, determining ωγ = (9.7 ± 2.0) × 10⁻⁵ eV and ωγ < 1 × 10⁻⁵ eV for these two resonances, respectively. For the 542 keV resonance this value is substantially smaller than had been assumed in earlier model calculations, and this reduces the rate of the analog ¹⁵O(α, γ)¹⁹Ne reaction (connecting the Hot CNO cycle and the rp-process) by a factor of ≈ 3 for temperatures in the region of T₉ = 1.     

Decay of the first excited state at 13.3 keV in73Ge

Singles and coincidence measurements of the 13.3 keV transition of⁷³Ge are reported. The total andK conversion coefficients of this gamma-ray and the half-life of this level have been determined. The results are: α _T =1095±55; α _K =312±30;T _1/2=2.98±0.05 μs.     

The decay of141Ce

The decay of¹⁴¹Ce has been reinvestigated using different experimental methods. The efficiency extrapolation technique applied to 4πβ —γ coincidence measurements has been employed for the determination of the disintegration rate of the sources and of the total internal conversion coefficient. TheK X-ray andγ-ray emisssion rates have been measured with a calibrated Si(Li) and an intrinsic germanium detector. Additionally the photon intensities have been determined from the internal conversion coefficients. Electron experiments with a magneticβ-spectrometer yielded the relative intensities, the shape factors and the maximum energies of the two β^?-transitions and the internal conversion ratiosK/L andK/(L + M+...). TheK-shell internal conversion probability has been determined with an electronK X-ray coincidence technique using the magneticβ-spectrometer together with a high energy resolution Si(Li) detector. New values for the following decay properties have been deduced:β ^?-intensities (p ₁ =0.306 + 0.006,p ₂= 0.694±0.006), shape factorsC = const (1+Aε) (A ₁ = ?(0.24±0.03),A ₂=?(0.22±0.04)), maximumβ ^?-energies (E ₀₁ = (582.2±2.6) keV,E ₀₂= (436.7±4.6) keV),K- shell internal conversion coefficient (α _K = 0.376±0.008), total internal conversion coefficient (α = 0.438±0.010), internal conversion ratios (K/L = 7.29±0.24, K/(L + M + ...) = 5.78±0.18),γ-ray intensity (I _γ = 0.482±0.003),K X-ray intensity (I_{K X} = 0.168±0.002) and the photon intensity ratio (I _{K X} /I _γ = 0.349±0.005). The procedure of uncertainty quotation is presented in some detail. The results are discussed with respect to existing experimental data.     

Der Zerfall von Nb94 m

Using scintillation spectrometers and coincidence techniques the decay of Nb^{94 m} has been investigated. TheK-shell conversion coefficient of the 41.5 keV isomeric transition was found to be 570±100 indicating aM 3 transition. The maximum energy of theβ-decay to the 0.87 MeV level of Mo⁹⁴ is (1.15±0.03) MeV occurring (4·5±0·7)×10^?3 per disintegration, anotherβ-decay to the 1.57 MeV level was found to be (4·0±1·3)×10^?5. From this the parities and spins of the levels involved in the decay of Nb^{94 m} are determined.     

Measurements of someK-internal conversion coefficients near threshold

TheK-internal conversion coefficients have been measured by the XPG technique for a number of low energyγ-ray transitions whose energies do not exceed theK-binding energies by more than 4 keV. Using Si(Li) detectors in singles and coincidence arrangements, the following results were obtained: 63.1 keV El in¹⁶⁹Tm(α_K=1.02±0.15), 72.0 keV E1 in¹⁸⁷Re (0.75±0.05), 57.8 keV M1 in¹⁶²Ho (11.42±0.67), 56.6 keV M1 in¹⁶⁴Ho (12.04±0.70), and 67.1 keV M1 in¹⁷⁴Lu(10.25±0.58). The experimental results are compared with the theoretical calculations which include transition energies down to 1 keV above threshold.     

Internal conversion coefficient of the 113.8 keV transition in175Lu

The work contains the α _K internal conversion coefficient measurement by XPG method of 113.8 keV transition in¹⁷⁵Lu. We obtained α _K =1.82±0.15. The 113.8 keV transition in¹⁷⁵Lu supports a large penetration effect, as it can seen from computedλ parameter values.     

Multipole mixing ratios of transitions in168Er

Time-integral and time-differentialγ-γ directional correlation measurements were performed for cascades in¹⁶⁸Er populated from the electron-capture decay of¹⁶⁸Tm(87d). The¹⁶⁸Tm source was dissolved in HF acid to minimize extranuclear perturbations. The results of the time-differential experiment for the 448-99.3 keV and 448-198 keV cascades showed agreement with time dependent interaction and gaveλ ₂(1094)=(0.79±0.09) ×10⁷ sec^?1. The attenuation factors for the 80 keV level were determined asG ₂₂ (80)=0.90±0.01 and G₄₄(80)=0.94±0.01. OnlyI=4 spin value for the 1094 keV level is consistent with our measurements. The 632, 731, 741, and 816 keV transitions connecting theK=2⁺ andK = 0⁺ rotational bands were found to be of almost pureE2 character. The 99.3, 198, 547, 720, 830, and 1277 keV transitions are of practically pureE1 multipolarity. The 448 keVMl transition has (0.8 _?0.4 ^+2.0 )%E2 admixture. The results for the 1014?80keV cascade give (23±4)%E3 component in the 1014 keV transition.     

Reevaluation of the conversion coefficient of the 14.4 keV transition in57Fe

Existing values of the conversion coefficient of the 14.4 keV transition in⁵⁷Fe have been reevaluated using newK-shell fluorescence yields and recent decay scheme information. Previous disagreements are removed and the mean values found are α _T =8.26±0.19, α _K =7.37±0.17.     

Gamma branching and total conversion coefficients of intraband transitions in the groundstate rotational band of245Cm

With calibrated Ge(Li) detectors, γ-γ coincidences have been observed in the decay of²⁴⁹Cf. The total conversion coefficient of the 54.7 and 66.7 keV transitions in the first rotational band have been determined to be 237±30 and 69±15, respectively. The branching ratio of the 121.5keV crossover transition is (22±7)%. The errors are the 2σ statistical uncertainties, linearily added to the errors in the detector efficiencies.     

Conversion electron measurements in the decay of156Tb

The conversion electron spectrum from the decay of¹⁵⁶Tb to¹⁵⁶Gd was measured with an iron, double-focusing spectrometer. TheK conversion coefficient of the 1222.4 keV transition was measured relative to theK conversion coefficient of the 661.6 keV transition in¹³⁷Cs and found to be 0.00174±0.00013. This result was used to normalize electron and gamma-ray data to obtain theK conversion coefficients of 33 transitions in¹⁵⁶Gd. The 1009.6 and 1040.6 keV transitions have largeE0 components.