Time reversal of ultrafast waveforms by wave mixing of spectrally decomposed waves

Two different realizations of time-reversal experiments of ultrafast waveforms are carried out in real time by use of four-wave mixing arrangements of spectrally decomposed waves. The first, conventional, method is based on phase conjugation of the waveform's spectrum and achieves time reversal of real amplitude waveforms. The second arrangement of the spectrally decomposed waves spatially inverts the waveform's spectrum with respect to the optical axis of the processor and achieves true time reversal for complex-amplitude ultrafast waveforms. We compare and contrast these two real-time techniques.     

Ultrafast optical frequency comb synthesizer and analyzer

We propose an ultrafast optical arbitrary waveform synthesizing/analyzing technique demonstrated with 2 Tbit/s waveforms. An ultrafast waveform was generated by manipulating the amplitude and phase of a 400?GHz optical frequency comb using a newly developed colorless optical synthesizer. The 400?GHz optical frequency comb was generated from a 25?GHz optical frequency comb using a colorless arrayed waveguide grating. This waveform was then analyzed on the frequency axis using a custom heterodyne-detection technique based on the dual-heterodyne mixing method. The phase and amplitude spectra can be observed in parallel using another optical frequency comb as a reference combined with an arrayed waveguide grating. This optical system, named the ultrafast optical frequency comb synthesizer and analyzer, can synthesize and analyze an arbitrary waveform in the THz frequency region.     

Ultrafast on‐Chip Remotely‐Triggered All‐Optical Switching Based on Epsilon‐Near‐Zero Nanocomposites

On‐chip‐triggered all‐optical switching is a key component of ultrahigh‐speed and ultrawide‐band information processing chips. 1 - 4 This switching technique, the operating states of which are triggered by a remote control light, paves the way for the realization of cascaded and complicated logic processing circuits and quantum solid chips. Here, a strategy is reported to realize on‐chip remotely‐triggered, ultralow‐power, ultrafast, and nanoscale all‐optical switching with high switching efficiency in integrated photonic circuits. It is based on control‐light induced dynamic modulation of the coupling properties of two remotely‐coupled silicon photonic crystal nanocavities, and extremely large optical nonlinearity enhancement associated with epsilon‐near‐zero multi‐component nanocomposite achieved through dispersion engineering. Compared with previous reports of on‐chip direct‐triggered all‐optical switching, the threshold control intensity, 560 kW/cm², is reduced by four orders of magnitude, while maintaining ultrafast switching time of 15 ps. This not only provides a strategy to construct photonic materials with ultrafast and large third‐order nonlinearity, but also offers an on‐chip platform for the fundamental study of nonlinear optics.     

Linear and Nonlinear Fiber Propagation of Partially Coherent Fields Exhibiting Temporal Correlations

Using an ultrafast photonic first-order differentiator applied on a partially coherent field, the generation of two correlated temporal waveforms is reported and their correlation properties upon linear and nonlinear propagation along the two orthogonal polarization axes of a dispersive optical fiber are studied. Temporal correlations are maintained in linear propagation whereas Kerr nonlinearity generates anticorrelated temporal intensity patterns for both partially and uncorrelated fields. Experiments are in close agreement with the theoretical analysis.     

Large Kerr effect in bulk Se-based chalcogenide glasses

High-speed optical communication requires ultrafast all-optical processing and switching capabilities. The Kerr nonlinearity, an ultrafast optical nonlinearity, is often used as the basic switching mechanism. A practical, small device that can be switched with ~1-pJ energies requires a large Kerr effect with minimal losses (both linear and nonlinear). We have investigated theoretically and experimentally a number of Se-based chalcogenide glasses. We have found a number of compounds with a Kerr nonlinearity hundreds of times larger than silica, making them excellent candidates for ultrafast all-optical devices.     

Ultrafast optical switching by use of fully phase-matched cascaded second-order nonlinearities in a polarization-gate geometry

We show that cascaded second-order nonlinear-optical processes can occur in a convenient polarization-gate beam geometry. Our arrangement uses type II phase matching, and both individual second-order processes (upconversion and downconversion) are simultaneously phase matched. This geometry can be applied to efficient ultrafast optical switching. With a beta-barium borate crystal and lightly focused 250-fs, 7.3-microJ pulses, we achieve a switching efficiency of 15% and an on-off ratio of 3 x 10(4) on a pulse-length-limited time scale.     

Nonlinear directional coupler in periodically poled lithium niobate

Nonlinear wave propagation was investigated experimentally in coupled waveguides by means of the cascaded nonlinearity in quasi-phase-matched second-harmonic generation. With a specially designed wave-vector-mismatch distribution along the propagation axis, cascading was optimized for low fundamental depletion. High-contrast, ultrafast all-optical switching with switching powers of tens of watts was observed.     

Directionally anisotropic Si nanowires: on-chip nonlinear grating devices in uniform waveguides

Computational studies are used to show that the crystalline structure of Si causes the waveguide Kerr effective nonlinearity, γ, to vary by 10% for in-plane variation of the orientation of a silicon nanowire waveguide (SiNWG) fabricated on a standard silicon-on-insulator wafer. Our analysis shows that this angular dependence of γ can be employed to form a nonlinear Kerr grating in dimensionally uniform SiNWGs based on either ring resonators or cascaded waveguide bends. The magnitude of the nonlinear index variation in these gratings is found to be sufficient for phase matching in four-wave mixing and other optical parametric processes.     

Ultrafast optical power limiting in free-standing Pt–polyvinyl alcohol nanocomposite films synthesized in situ

Free-standing platinum–polyvinyl alcohol nanocomposite films have been prepared by a simple in situ method. By thermal annealing, Pt nanoparticles of different sizes and shapes have been obtained. Their optical nonlinearity is measured using ultrafast (100 fs) laser pulses at 404 nm, in the absorption wing region. A strong optical power limiting is found in the films. The timescale of this limiting action is ultrafast, as it happens within the incident laser pulsewidth. Experimental results and numerical simulation indicate that the sign of the nonlinearity can be controlled by varying the film composition and annealing temperature. Use of ultrashort laser pulses in the free-standing film configuration permits a direct and unambiguous determination of the electronic nonlinearity of the material, since accumulative effects occur at later times lying outside the sharp measurement window.     

Upconversion time microscope demonstrating 103 x magnification of femtosecond waveforms

We present the operational principles and results of a temporal imaging system, configured as a time microscope, that achieves 103 x magnification of waveforms with 300-fs resolution and a 5.7-ps field of view. The quadratic-phase time-lens element is realized by upconversion of the dispersed input waveform with a linearly chirped 5-THz bandwidth pump. The system allows expansion of ultrafast optical waveforms to a time scale that is directly accessible with slower conventional technology, in real time, on a single-shot basis.     

Designing novel chalcone single crystals with ultrafast nonlinear optical responses and large multi-photon absorption coefficients

A chalcone single crystal, 1-(4-chlorophenyl)-3-(4-methoxyphenyl)prop-2-en-1-one that is transparent over the visible to infrared region is introduced as a new potential material to third-order nonlinear optical applications. The crystal exhibits ultrafast optical response (≤90 fs) and large optical nonlinearity in the wavelength range 800–1200 nm. A very large effective two-photon absorption coefficient β_eff exceeding 120 cm/GW can be obtained with this chalcone crystal, at a low intensity threshold of 41 MW/cm². The mechanism of nonlinear absorption at different levels of intensity has been discussed. The crystal shows no damage against the laser pulse intensity as high as 8 GW/cm². We discuss the molecular and crystal designing of chalcones with large and ultrafast optical nonlinearity combined with low optical cut-off (<450 nm).     

Time division vector optical sampling for ultrafast amplitude/phase modulation device characterization

A technique is proposed and demonstrated for measuring the waveforms of optical signals by making use of homodyne in-phase and quadrature detection combined with nonlinear optical sampling. The technique is based on time division sampling of electric field components with a discretely phase-modulated local oscillator light and is applied for the evaluation of the ultrafast response in a semiconductor optical amplifier.     

Ultrahigh-bandwidth, on-chip all-optical pulse erasure using the χ(3) process in a nonlinear chalcogenide waveguide

We demonstrate on-chip all-optical pulse erasure based on four-wave mixing and cross-phase modulation in a dispersion engineered chalcogenide (As(2)S(3)) rib waveguide. We achieve an erasure efficiency of ~15 dB for picosecond pulses in good agreement with numerical simulations using the nonlinear Schr?dinger equation. The combined effect of the high instantaneous optical nonlinearity (γ = 9900 (W km)(-1)) and small group-velocity dispersion (D = 29 ps/nm km), which reduces pulse walk-off, will enable all-optical pulse erasure for ultrafast signal processing.     

Ultrafast nonlinear optical response of a single gold nanorod near its surface plasmon resonance

The ultrafast optical nonlinearity of an optically characterized single gold nanorod is investigated around its surface plasmon resonance, by combining a far-field spatial modulation technique with a high sensitivity pump-probe setup. The spectrally and temporally dependent response is quantitatively interpreted in terms of the bulklike optical nonlinearity enhanced by the plasmonic effect. The plasmon resonance dynamics is shown to be mostly governed by nonequilibrium electron and phonon processes. Their contributions to the nonlinear optical response of a single metal nano-object are elucidated, and the latter is connected to the nonlinearities of ensembles.     

Ultrafast all-optical first- and higher-order differentiators based on interferometers

We demonstrate that a conventional two-arm interferometer can implement first-order temporal differentiation of ultrafast arbitrary optical waveforms. Straightforward extension of this technique to nth-order optical differentiation is also suggested. This approach is experimentally demonstrated by an efficient and accurate first- and second-order temporal differentiation of (sub-)picosecond Gaussian optical pulses.     

Optical Nonlinearity in a Novel Optical Signal Regeneration System Based on Cross-Gain Modulation Using Cascaded Semiconductor Optical Amplifiers

We propose a novel optical signal regeneration system based on wavelength converters by use of cross gain modulationin cascaded semiconductor optical amplifiers. The nonlinearity in optical input/output characteristics and eye opening using NRZ signal were archived.     

Ultrafast nonlinear optical response of carbon nanotubes functionalized with water soluble porphyrin

A new nanocomposite is obtained by functionalizing carbon nanotubes (CNTs) with a water soluble metalloprophyrin using a simple chemical technique and characterized by optical absorption, IR, and Raman spectroscopy. Results from spectroscopic studies indicate the noncovalent nature of interaction between CNTs and porphyrin. The ultrafast nonlinear response is characterized by measuring the nonlinear absorption coefficient and refractive index by z-scan technique in the femtosecond pulse regime. The nanocomposite is found to exhibit two-photon absorption (TPA) with a reasonably large nonlinear optical coefficient, whereas pure CNTs is known to exhibit saturable absorption. Design of such water soluble nanocomposites offers scope for obtaining materials with enhanced ultrafast optical nonlinearity.     

Ultrafast laser fabrication of low-loss waveguides in chalcogenide glass with 0.65 dB/cm loss

This Letter reports on the fabrication of low-loss waveguides in gallium-lanthanum-sulfide chalcogenide glasses using an ultrafast laser. Spatial beam shaping and temporal pulse width tuning were used to optimize the guided mode profiles and optical loss of laser-written waveguides. Highly symmetric single-mode waveguides guiding at 1560 nm with a loss of 0.65 dB/cm were fabricated using 1.5 ps laser pulses. This Letter suggests a pathway to produce high quality optical waveguides in substrates with strong nonlinearity using the ultrafast laser direct writing technique.     

Proposal and analysis of a reconfigurable pulse shaping technique based on multi-arm optical differentiators

We propose and numerically investigate an optical pulse re-shaping method based on multi-arm ultrafast optical differentiators. In this approach, the desired (arbitrary) optical pulse shape is synthesized by coherently overlapping different successive time derivatives of an input optical pulse (not necessarily a Gaussian-shape pulse), including the input pulse itself, with suitable relative weights. Time derivatives of (sub-)picosecond pulses can be obtained using first and higher-order ultrafast optical differentiators practically implemented with integrated waveguide or fiber-based linear filtering technologies. Different output pulse shapes can be generated from the same platform by properly programming the relative weights among the different pulse derivatives. The effective bandwidth of the output waveform is not necessarily limited by the input pulse bandwidth but rather it depends on the highest derivative order used for the pulse synthesis. Our results reveal that interesting transform-limited pulse shapes (including flat-top and parabolic waveforms) can be synthesized from Gaussian-like (e.g. Gaussian, sech) pulses using a simple and practical three-arm ultrafast differentiation system with amplitude-only relative weights.     

Picosecond linear optical pulse shapers based on integrated waveguide Bragg gratings

We demonstrate a general linear pulse-shaping technique based on integrated III-V Bragg gratings (BGs). Such a technique allows for the synthesizing of complex waveforms with picosecond resolution using a compact single-waveguide design. This approach is experimentally demonstrated by fabricating and testing a series of integrated ultrafast optical pulse shapers based on BG geometries acting as time-domain code generators operating at 500 Gbits/s.