Optical resonant processes in thin excited films

It is shown that coherent processes of elastic scattering of resonant radiation form a “buffer” electromagnetic field near the boundary of excited media. This part of radiation is not governed by the standard refractive index, but precisely this part of radiation forms the beams reflected and refracted by the excited medium. The presence of the “buffer” field causes the suppression of stimulated emission near the boundary and leads to the appearance of a frequency angular broadening of the beam transmitted through a thin film of excited atoms at an oblique angle.     

Incoherent properties of induced radiation

The evolution of a quantized electromagnetic field in a thermally excited dispersion medium is determined by two scattering channels. The coherent channel is formed exclusively by the elastic scattering of quanta. The incoherent channel, along with elastic scattering processes, necessarily contains inelastic scattering processes, including induced radiation. Interference between the channels is absent because of the orthogonality of the wave functions of the medium in its final states, which correspond to different scattering channels. Therefore, in an excited medium, interference processes that are not described by its refractive index may arise. An interference pattern of this kind can be formed, in particular, as a result of the superposition of the resonance radiation incident on an excited medium and the radiation reflected from this medium. In this case, the conventional perturbation theory proves to be inadequate.     

Laser diagnostics of ultrasonic outgassing of an insulating liquid

The efficiency of hydrogen evolution from transformer oil into a vacuum and into air under normal pressure is studied for the case when the oil is exposed to focused ultrasonic radiation. The study is performed by the method of spectroscopy of biharmonic-pumping coherent anti-Stokes Raman scattering (CARS) based on stimulated Raman scattering (SRS). Ultrasonic radiation at a frequency of 1.76 MHz is excited by a spherical piezoceramic transducer mounted on the bottom of the vessel and is focused on the surface of the oil. This causes the intense stirring of the oil with the formation of a fountain. The room-temperature diffusion coefficient of hydrogen in the transformer oil, 10⁻⁷ m²/s, is found by approximating experimental data by a theoretical relationship for hydrogen evolution into air. It is shown that ultrasonic radiation with a power density of 2.2 kW/m² accelerates diffusion processes ten-to fifteen-fold.     

Detection of frequency red shifts and blue shifts for single-mode IR laser radiation in Rydberg matter

Stimulated emission and laser gain were recently reported for the excited condensed matter Rydberg matter (RM). This shows that RM is in an excited and inverted state. A low-intensity single-mode IR laser beam is here red shifted in reflection from a layer of RM, and blue shifted when it passes through a cloud of RM. The shifts of approximately 0.02 cm^-1 are observed with a temperature-stable Fabry–Pérot interferometer. The process giving the wavelength shifts is proposed to be stimulated Raman scattering. RM is here formed from Rydberg states of both K atoms and nitrogen molecules inside a vacuum chamber, and it may be in liquid or solid form. PACS 78.30.-j; 42.65.Dr; 42.55.Ye     

Coherent effects in the incoherent channel of resonant radiation scattering from excited atoms

Scattering of a resonance electromagnetic field from excited atoms cannot be described by the semiclassical theory of radiation operating with nonquantized electromagnetic fields. Field quantization effects are manifested in this case on the macroscopic level and lead to evolution of statistical properties of radiation in the course of scattering. It is found that a combined process coupling elastic scattering from an atom and induced emission from the same atom, which cannot be studied by the methods of the standard perturbation theory, plays a significant role in this effect. The process of combined scattering in extended media exhibits coherent properties that cannot be described by the standard refractive index.     

A reciprocal phase-perturbation theory for rough-surface scattering

Abstract

We study the scattering of a scalar plane wave from a two-dimensional, randomly rough surface, on which the Dirichlet boundary condition is satisfied. The scattering amplitude is obtained in the form of the Fourier transform of an exponential, in which the exponent is written as an expansion in powers of the surface profile function. It is shown that the latter expansion can be written in such a way that the corresponding scattering matrix is manifestly reciprocal. Numerical results for the reflectivity, and for the contribution to the mean differential reflection coefficient from the incoherent component of the scattered field, are obtained and compared with the predictions of small-amplitude perturbation theory and the Kirchhoff approximation. As the wavelength of the incident wave is varied continuously the results of the phase-perturbation theory change continuously from those of the small-amplitude perturbation theory to those of the Kirchhoff approximation.     

X-ray scattering from a randomly rough surface

Abstract

On the basis of the method of reduced Rayleigh equations we present a simple and reciprocal theory of the coherent and incoherent scattering of x-rays from one- and two-dimensional randomly rough surfaces, that appears to be free from the limitations of earlier theories of such scattering based on the Born and distorted-wave Born approximations. In our approach, the reduced Rayleigh equation for the scattering amplitude(s) is solved perturbatively, with the small parameter of the theory η(ω) = 1 - ε(ω), where ε(ω) is the dielectric function of the scattering medium. The magnitude of η(ω) for x-rays is in the range from 10^?6 to 10^?3, depending on the wavelength of the x-rays. The contributions to the mean differential reflection coefficient from the coherent and incoherent components of the scattered x-rays are calculated through terms of second order in η(ω). The resulting expressions are valid to all orders in the surface profile function. The results for the incoherent scattering display a Yoneda peak when the scattering angle equals the critical angle for total internal reflection from the vacuum-scattering medium interface for a fixed angle of incidence, and when the angle of incidence equals the critical angle for total internal reflection for a fixed scattering angle. The approach used here may also be useful in theoretical studies of the scattering of electromagnetic waves from randomly rough dielectric-dielectric interfaces, when the difference between the dielectric constants on the two sides of the interface is small.     

Strongly Beamed,Polarized Radio Emission from CU Virginis

We propose the plasma mechanism of generation of the strongly beamed, fully polarized radio emission from a chemically peculiar star CU Vir observed with VLA at 1.4 GHz in June 2, 6, and 9, 1998. The radio emission arises from the Rayleigh scattering of longitudinal waves excited near the upper-hybrid resonance due to the loss-cone instability on suprathermal electrons in the magnetosphere of CU Vir. It is shown that the nonlinear stimulated scattering of upper-hybrid waves and the regular refraction of radiowaves in the stellar corona are the main factors forming the angular pattern of the radio emission. As the result, the angular pattern of the radiation of CU Vir narrows to 3^°-10^°.     

Intraband coherence of Bloch oscillations after momentum scattering

Resonantly excited secondary emission of light (RSE) in GaAs/AlGaAs superlattices gives a direct proof for the stability of coherent Bloch dynamics beyond the optical coherent regime. The polarization analysis of the RSE signal confirms its nonlinear origin resulting from coherent intraband density dynamics. It is shown that the intraband coherence of Bloch oscillations (BO) persists after momentum scattering of the photoexcited states. A variation of emission angle and excitation density allows to distinguish two momentum scattering processes contributing to the RSE. A static disorder mediated contribution is restricted to directions near the reflection direction. A further contribution of carrier induced momentum scattering is resolved in directions well separated from diffraction directions. The dependence of the RSE as a function of an external electric field demonstrates an enhancement of momentum scattering with increasing field. PACS 78.47.+p; 63.20Kr; 71.35.-y.     

Thermally stimulated emission of electrons and photons in nonlinear LiB3O5 crystals

The results of an investigation of the thermally stimulated emission of electrons and photons in lithium triborate single crystals are presented. The investigation is performed mainly by simultaneously measuring the thermally stimulated emission of electrons and photons after various radiation treatments. In particular, the thermally stimulated exoelectron emission of LiB₃O₅ crystals is discovered for the first time and studied in detail. An analysis of the experimental results reveals two new trapping centers. It is established that the thermal annealing of these centers at 450 and 515 K makes a contribution only to the exoelectron emission. It is postulated that a field fluctuation process, which lowers the potential barriers of the trapping centers, takes place in LiB₃O₅ at 100–140 K. This process is attributed to thermally stimulated relaxation of the radiation-induced charge. A significant dependence of the parameters of the thermally stimulated processes in LiB₃O₅ on the parameters of the radiation treatment is discovered. Zh. Tekh. Fiz. 67, 121–125 (July 1997)     

Generation of a continuum and stimulated Raman scattering harmonics during scattering of electromagnetic radiation of relativistic intensity

A theory of the propagation instability of plane, monochromatic, circularly polarized electromagnetic waves of relativistic intensity in matter is developed for a spatially three-dimensional geometry including arbitrary polarization of the scattered radiation. Harmonic generation owing to striction and relativistic nonlinearity is examined, as well as scattering owing to electron recoil, the decay instability of the harmonics with formation of scattered electromagnetic waves (Stokes components of the stimulated Raman scattering and plasmons), the interaction of electromagnetic waves in the plasma (antistokes stimulated Raman scattering), and the generation of a radiative continuum. The transition of the three-dimensional theory to a one-dimensional problem in the nonrelativistic limit is discussed. Zh. éksp. Teor. Fiz. 113, 2034–2046 (June 1998)     

Collinear and noncollinear emission of anti-stokes and second order stokes Raman radiation

Generating higher order stimulated Raman scattering in benzene, apart from phase-matched anti-Stokes radiation a collinear anti-Stokes emission is observed, which is explained by parametric four-photon processes under mismatch condition.     

Nuclear resonant scattering using synchrotron radiation

A one-dimensional quantum model for nuclear resonant scattering using synchrotron radiation has been developed. This model gives a clear physical interpretation of the most prominent features of the coherent forward scattering process namely, the “speed-up” and “dynamical beat” effects. The form of the solution, for the time-dependent forward scattered intensity of the resonant radiation from the resonant medium after synchrotron radiation excitation, is a finite series. This unique solution can be interpreted in terms of a summation over all multiple forward scattering paths the radiation takes in reaching the detector. The resonant medium is represented by a linear chain of N effective resonant nuclei. The analysis starts from a coupled set of quantum mechanical equations for the relevant amplitudes in frequency space. Transformation to the time domain gives an analytical expression for the forward scattered intensity. The contribution of every order of the multiple scattering processes from the N effective nuclei appears naturally. The expression gives a clear physical understanding of all relevant aspects of resonant forward nuclear scattering. Furthermore, the present formalism allows the consideration of incoherent processes. This permits the study of processes in which there is gamma emission with recoil or emission of internal-conversion electrons. This revised version was published online in August 2006 with corrections to the Cover Date.     

Origin of temporally stable continuous-wave stokes emission in stimulated Brillouin scattering: evidence of spectral self-phase conjugation

We report results on the appearance of temporally stable Stokes emission in stimulated Brillouin scattering (SBS) excited by continuous-wave pump radiation in optical fiber. With increasing pump strength the stable component emerges from stochastic emission slightly above the SBS threshold to become the dominant contribution, independent of fiber characteristics. These findings are shown to be a manifestation of spectral self-phase conjugation, providing what is to our knowledge the first experimental evidence of this phenomenon in optics.     

Stimulated photoluminescence emission and trap states in Si/SiO2 interface formed by irradiation of laser

Stimulated photoluminescence （PL） emission has been observed from an oxide structure of silicon when optically excited by a radiation of 514nm laser. Sharp twin peaks at 694 and 692nm are dominated by stimulated emission, which can be demonstrated by its threshold behaviour and linear transition of emission intensity as a function of pump power. The oxide structure is formed by laser irradiation on silicon and its annealing treatment. A model for explaining the stimulated emission is proposed, in which the trap states of the interface between an oxide of silicon and porous nanocrystal play an important role.     

Optical and luminescent VUV spectroscopy of La2Be2O5 crystals

Electronic excitations and the processes of their radiative relaxation are studied in pure and Ce³⁺ ion-doped crystals of lanthanum beryllate excited by synchrotron radiation in the x-ray and VUV ranges by methods of optical and luminescent vacuum ultraviolet time-resolved spectroscopy. Manifestations of excitons of the valence band are absent in the reflection spectra. However, a fast (τ=1.7 ns) and a slow (microsecond range) channel corresponding to two possible types of self-trapped excitons (STE) are found in radiative relaxation of intrinsic electronic excitations at T=10 K. The slow channel corresponds to emission of STE formed through recombination, the fast channel corresponds to emission of relaxed metastable excitons from the STE state. In the energy region higher than 14 eV (E>2E _g), the effect of multiplication of electronic excitations due to generation of secondary electron-hole pairs resulting from inelastic scattering of both hot photoelectrons and hot photoholes is exhibited.     

Phase of reflection of very low energy electrons at crystal surfaces

The amplitude coefficients of electron reflection at crystal surfaces are complex numbers, each of which may be characterized by a reflection intensity (the squared modulus of the coefficient) and a phase. The phase of reflection of very low energy (? 10 eV) electron reflection is described on the basis of existing theory, and experimental approaches to phase determination are reviewed. Theoretical properties of the phase are described on the basis of the two-beam dynamical theory of diffraction. The model considered is an idealized substrate crystal with an attached selvedge (surface region). The indirect effect of inelastic scattering (absorption) is included by going to complex values of the electron energy or of the surface-normal component K of the propagation vector. In the absence of a selvedge the phase is determined solely by the band structure of the substrate crystal. If a selvedge is present there are large additional effects on the phase associated with zeros of the amplitude coefficient of reflection on the complex K plane. The experimental approaches considered are: (1) measurement of the kinetic energy distributions of ions produced in the field ion microscope, and (2) measurement of the periodic deviations from the Schottky line in field-assisted thermionic emission and photo-emission. Recent results of phase determination for W (011) surface by method (1) are summarized and compared with theoretical expectations.