Photonuclear reactions from correlated nucleon pairs (II)

A derivation of an expression for the cross section of the photoexcitation of correlated nucleon pairs in a nucleus is given. The final-state wave functions which are obtained from a solution of the Brueckner reaction matrix can be related to the scattering of free nucleons in a vacuum. Some results are presented and include the energy distribution and cross sections of the excited nucleons. An expression for the cross section of the giant dipole resonance is derived purely from the presence of the microscopic two-body forces in nuclei. These cross sections agree with experiment for a particular choice of the final-state single-particle spectrum.     

Study of S11 resonance in nuclei through (γ, η) reactions

In order to study the S₁₁(1535) resonance in the nuclear medium, total cross sections of the (γ, η) reactions on C, Al and Cu have been measured for photon energies between 680 and 1000 MeV. A broad resonance due to the excitation and decay of the S₁₁ resonance in the nucleus has been clearly observed for the first time. The apparent energy and width of the resonance are 900 and 300 MeV, respectively. Model calculations based on the quantum molecular dynamics have been performed. A comparison of the calculations with the data indicates that the S₁₁ resonance in nuclei should have a larger width; the width of about 250 MeV is required while the elementary one is about 150 MeV.     

The quark-meson coupling model for Λ, Σ and Ξ hypernuclei

The quark-meson coupling (QMC) model, which has been successfully used to describe the properties of both infinite nuclear matter and finite nuclei, is applied to a systematic study of Λ, Σ and Ξ hypernuclei. Assumptions made in the present study are, (i) the (self-consistent) exchanged scalar, and vector, mesons couple only to the u and d quarks, and (ii) an SU(6) valence quark model for the bound nucleons and hyperon. The model automatically leads to a very weak spin-orbit interaction for the Λ in a hypernucleus. Effects of the Pauli blocking at the quark level, particularly in the open, coupled, ΣN-ΛN chanel (strong conversion), is also taken into account in a phenomenological way.     

Cross section measurements of the Pd(p, γ)Ag, Sn(p, γ)Sb, and Sn(α, γ)Te reactions relevant to the astrophysical rp- and γ-processes

Total cross section measurements for the ¹⁰²Pd(p, γ)¹⁰³Ag and ¹¹⁶Sn(p, γ)¹¹⁷Sb reactions have been performed in the proton energy range 2.6 to 4.25 MeV, and for the ¹¹²Sn(α, γ)¹¹⁶Te reaction over the alpha beam energy range 7.0 to 10.5 MeV. An activation technique was used in which gamma rays from decays of the reaction products were detected off-line by two hyper-pure germanium detectors in a low background environment. Where possible, reaction rates are derived and the results compared to those of calculations generated by the NON-SMOKER and the MOST statistical model codes so as to judge their applicability for describing the cross sections needed for network calculations of nucleosynthesis in explosive astrophysical environments via the γ- and rp-processes.     

Modeling of a microscopic optical pion-nucleon potential at energies in the (3, 3)-resonance region and nuclear-matter effect on the pion-nucleon amplitude

Differential cross sections for elastic pion scattering on a number of nuclei at energies between 130 and 290 MeV are calculated. For this purpose, use is made of a microscopic optical pion-nucleus potential that was obtained on the basis of the Glauber theory of high-energy scattering and which is determined by the density distribution of pointlike target nucleons and by the pion-nucleon scattering amplitude. The calculation of the cross sections in question is based on solving the respective relativistic wave equation. Three parameters of the pion-nucleon amplitude are fitted in performing a comparison with experimental data. These are the total cross section for pion-nucleon scattering, the ratio of the real to the imaginary part of the forward pion-nucleon scattering amplitude, and the slope parameter. The resulting values of these parameters are then compared with their counterparts for scattering on free nucleons. The character of nuclear-matter-induced changes in these parameters is studied.     

η in the nuclear medium within a chiral unitary approach

The s-wave η self-energy in the nuclear medium is calculated in a chiral unitary approach. A coupled channel Bethe–Salpeter equation is solved to obtain the effective ηN interaction in the medium. The base model reproduces well the free space πN elastic and inelastic scattering at the ηN threshold or N^*(1535) region. The Pauli blocking on the nucleons, binding potentials for the baryons and self-energies of the mesons are incorporated, including the η self-energy in a self-consistent way. Our calculation predicts about −54−i29 MeV for the optical potential at normal nuclear matter for an η at threshold but also shows a strong energy dependence of the potential.     

Spectroscopic and structural investigations of α‐, β‐, and γ‐AlH3 phases

With its reputation as a high‐energy density fuel, aluminum hydride (AlH₃) has received renewed attention as a material that is particularly suitable, not only for hydrogen storage but also for rocket propulsion. While the various phases of AlH₃ have been investigated theoretically, there is a shortage of experimental studies corroborating the theoretical findings. In response to this, we present here an investigation of these compounds based primarily on two research areas in which there is the greatest scarcity of information in the literature, namely Raman and infrared (IR) absorption analysis. To the authors' knowledge, this is the first report of experimental far‐IR absorption results on these compounds. Two different samples prepared by broadly similar ethereal reactions of AlCl₃ with LiAlH₄ were analyzed. Both Raman and IR absorption measurements indicate that one sample is purely γ‐AlH₃ and that the other is a mixture of α‐, β‐, and γ‐AlH₃ phases. X‐ray diffraction confirms the spectroscopic findings, most notably for the β‐AlH₃ phase, for which optical spectroscopic data are reported here for the first time. Copyright © 2010 John Wiley & Sons, Ltd.     

The Fe(α, γ)Ni reaction at excitation energies in the region of the giant dipole resonance

Excitation functions for the ⁵⁶Fe(α, γ₀)⁶⁰Ni and ⁵⁶Fe(α, γ₁)⁶⁰Ni reactions have been measured at 90° to the beam direction over the bombarding energy range 8.0–17.6 MeV. Gamma-ray angular distributions were measured at ten bombarding energies. Excitation functions for the ⁵⁹Co(p, γ₀)⁶⁰Ni and ⁵⁹Co(p, γ₁)⁶⁰Ni reactions were measured over the range E_x = 16.58–16.92 MeV and compared with the (α, γ) data. The angular distribution data indicate that the (α, γ₀) and (α,γ₁) reactions proceed through 1⁻, and 1⁻ and 3⁻ states, respectively. The (α, γ) excitation functions are discussed with respect to isospin splitting of the ⁶⁰Ni giant dipole resonance. The fine structure observed in the excitation functions is shown to be most probably due to Ericson fluctuations. The gross (α, γ) cross sections are shown to be in reasonable agreement with the results of calculations made using the theory of Hauser and Feshbach assuming excitation of the giant dipole resonance.     

Four-nucleon transfer with the 32S(16O, 12C)36Ar reaction

Angular distributions have been measured for the ³²S(¹⁶O,¹²C)³⁶Ar reaction at 45.5 MeV leading to excited states between E_x, = 0 and 8 MeV. Experimental cross sections are compared with exact finite-range DWBA calculations in combination with extensive shell-model calculations, which include sd- and fp-shell configurations. Transitions to low-energy positive-parity states and bound negative-parity states are well reproduced. The calculations, however, fail to describe some high-energy positive-parity states. Calculations with a complete cluster expansion for the four transferred nucleons give about 50% larger cross sections, but can not explain the observed discrepancies. Possible interference of reaction processes other than direct α-transfer and special structure effects are discussed.     

Isomeric ratios of the cross sections for Sn(p, xpyn)X reactions

In proton-nucleus reactions, the ratios of the cross sections for 18 isomeric pairs were measured by the induced-activity method as functions of the initial-proton energy and of the number of emitted nucleons. The isotopic effect and the cross sections for charge-exchange reactions are discussed. The experimental values of the cross sections for disintegration reactions like (p, xpyn) are compared with the theoretical values calculated on the basis of the cascade-evaporation model.     

Lifetime measurement in the α system (C3Δ3-X3Δ3) of TiO

The radiative lifetimes of two rotational levels of the v′ = 2 level of the C³Δ₃ state of TiO have been measured using laser-induced fluorescence and delayed coincidence counting. Individual rotational levels are excited and observed. The measured lifetimes are τ_{J = 17} = 28.21 + 0.15 nsec and τ_{J = 87} = 29.74 ± 0.86 nsec. Argon-TiO collision cross sections have been determined for the two rotational levels and are found to differ by 30%.     

J/Ψ suppression in relativistic heavy ion collisions through final state interactions with excited nucleons

TheJ/Ψ suppression in relativistic heavy ion collisions through final state interactions with excited state nucleons is estimated in a manner analogous to that of Gerschel and Hüfner for ground state nucleons. If excited state nucleons are larger in size than nucleons in their ground state, theJ/Ψ absorption cross section is increased. Because of relativistic time dilation this effect does not significantly alter theJ/Ψ suppression previously found.     

Final-state interactions in the reaction H (p, 2p) n

The cross sections for the reaction ²H(p, 2p)n are calculated by taking into account final state interactions including S, P and D waves for all pairs of outgoing nucleons. The D-state wave functions of the deuteron are also included in the calculation. The angular correlation distributions of the cross sections are compared with data at 156 MeV incident protons.     

Some lifetimes and transition probabilities in Cu(I)

Radiative lifetimes of 7 levels in the Cu(I) 3d⁹ 4s4p configuration have been measured using a delayed coincidence technique; copper vapor was excited in an argon buffer gas and cross sections for collisional destruction of copper levels by argon were also obtained. Transition probabilities of the lines originating from these levels have been determined using the measured lifetimes and branching ratios.     

Effects of non-standard tri-linear couplings in photon-photon collisions (I) γγ → WW

The effect of anomalous couplings in γγ → W⁺W^t- is studied for different energies of the γγ mode of the next linear collider. The analysis based on the maximum likelihood method exploits the variables in the four-fermion semi-leptonic final state. Polarized differential cross sections based on the complete set of diagrams for these channels with the inclusion of anomalous couplings are used and compared to an approximation based on γγ → W⁺W^t- with full spin correlations. To critically compare these results with those obtained in e⁺e^t- we perform an analysis based on the complete calculation of the four-fermion semi-leptonic final state. The anomalous couplings that we consider are derived from the next-to-leading order operators in the non-linear realization of symmetry breaking.     

Electronic transitions in α, θ and γ polymorphs of ultraporous monolithic alumina

Spectroscopy of α, θ, and γ phases of high‐purity ultraporous alumina has been studied at cryogenic temperatures of 7 K in the near‐IR–VUV range of spectra with synchrotron radiation excitation. The UV photoluminescence (PL) spectra are dominated by optical transitions of self‐trapped excitons, while the PL excitation spectra are assigned to free excitons and interband transitions. The analysis of PL excitation spectra indicates a tendency to fundamental bandgap narrowing in order of 9.36 eV (α) to 7.60 eV (θ) and 6.85 eV (γ). Structural defects related to oxygen vacancies are responsible for the visible F⁺/F transitions decrease in order γ > θ > α. (© 2013 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)     

A new method for functionalizing α,γ‐dinitro compounds at the β‐position: application to the cyclization of β‐alkoxy‐α,γ‐dinitro compounds

Treatment of 2,4‐dinitropentane with bromine and sodium methoxide in methanol, affords formation of an ether product, 2,4‐dibromo‐3‐methoxy‐2,4‐dinitropentane, in 59% yield as a mixture of three diastereomers. This observation has led to a general synthesis of 3‐alkoxy‐2,4‐dibromo‐2,4‐dinitropentanes, obtained in 75‐86% yield from 2,4‐dibromo‐2,4‐dinitropentane as the preferred reactant. 4‐Bromo‐2,4‐dinitro‐2‐pentene has been identified as an intermediate in these reactions. The nitroalkene has been isolated and undergoes conjugate addition with alkoxides to afford the same ether products after brominative work‐up. The nitroalkene undergoes conjugate addition with sodium azide to give 3‐azido‐2,4‐dibromo‐2,4‐dinitropentane in 38% yield as a mixture of two isomers in which the (R*,R*) isomer predominates. Sequential treatment of 2,4‐dibromo‐2,4‐dinitropentane with sodium methoxide followed by sodium iodide and acetic acid gives 3‐methoxy‐2,4‐dinitropentane in 63% yield, the overall product of simple methoxylation of 2,4‐dinitropentane. However, attempted complete debromination of 2,4‐dibromo‐3‐methoxy‐2,4‐dinitropentane with excess sodium iodide and acetic acid results only in monodebromination to give 2‐bromo‐3‐methoxy‐2,4‐dinitropentane in 86% yield. Likewise, 2‐bromo‐3‐ethoxy‐2,4‐dinitropentane is formed in 93% yield from the ethoxy analog. A mechanistic rationale is offered for condition‐specific removal of the second Br atom in these reactions. Treatment of 3‐methoxy‐2,4‐dinitropentane with potassium acetate/iodine in dimethyl sulfoxide affords formation of 4,5‐dihydro‐3,4‐dimethyl‐3‐methoxy‐4‐nitroisoxazole 2‐oxide in 30% yield as a single diastereomer. Conversion of 2‐bromo‐3‐methoxy‐2,4‐dinitropentane in 15% yield to 4,5‐dihydro‐3,4‐dimethyl‐3‐methoxy‐4‐nitroisoxazole 2‐oxide is also possible by using potassium acetate in dimethyl sulfoxide. The mechanistic pathways for formation of 4,5‐dihydro‐3,4‐dimethyl‐3‐methoxy‐4‐nitroisoxazole 2‐oxide apparently involve unstable 3‐methoxy‐1,2‐dimethyl‐1,2‐dinitrocyclopropane as the common intermediate. Similarly, 2‐bromo‐3‐ethoxy‐2,4‐dinitropentane affords 4,5‐dihydro‐3‐ethoxy‐3,4‐dimethyl‐4‐nitroisoxazole 2‐oxide in 13% yield. Copyright © 2013 John Wiley & Sons, Ltd.     

Near threshold photoproduction of η mesons from 4 He

Photoproduction of - mesons from ⁴He has been measured for the first time. The experiment was performed at the Mainz Microtron (MAMI) using the TAPS photon spectrometer and the Glasgow/Mainz tagged photon facility. - mesons were identified in coincidence with recoil nucleons. Total and differential cross sections are presented in the photon energy range between threshold and 818 MeV. The exclusive data are used to determine the ratio of the elementary production cross sections on bound neutrons and protons, C_n/C_p = 0.68 - 0.02 - 0.09. In addition, upper limits for the total coherent cross section have been derived.     

Al production cross sections from the Na(α, n)Al reaction

Cross sections have been determined for the production of ^{26g, m}Al from the ²³Na(α, n) reaction. Total ²⁶Al production cross sections were obtained from measurements of the thick-target neutron yield. ^26mAl cross sections were measured using an activation technique. ^26gAl cross sections were deduced by subtracting the ^26mAl cross sections from the total (α, n) cross sections. The principle of detailed balance has been applied to the low-energy data to obtain cross sections for the astrophysically interesting ^26gAl(n, α₀)²³Na reaction. These results are compared with the results of Hauser-Feshbach calculations.