Excitation of the dynamical dipole in the charge asymmetric reaction O + Sn

The γ-ray emission from the dynamical dipole formed in heavy-ion collisions during the process leading to fusion was measured for the N/Z asymmetric reaction ¹⁶O + ¹¹⁶Sn at beam energies of 8.1 and 15.6 MeV/nucleon. High-energy γ-rays and charged particles were measured in coincidence with the heavy recoiling residual nuclei. The data are compared with those from the N/Z symmetric reaction ⁶⁴Ni + ⁶⁸Zn at bombarding energies of 4.7 and 7.8 MeV/nucleon, leading to the same CN with the same excitation energies as calculated from kinematics. The measured yield of the high-energy γ-rays from the ¹⁶O-induced reaction is found to exceed that of the thermalized CN and the excess yield increases with bombarding energy. The data are in rather good agreement with the predictions for the dynamical dipole emission based on the Boltzmann–Nordheim–Vlasov model. In addition, a comparison with existing data in the same mass region is performed to extract information on the dipole moment dependence.     

35MeV/u 36Ar+112,124Sn反应中中等质量碎片关联函数的入射道依赖

³⁶Ar+^112,124Sn反应中小角关联出射的中等质量碎片(IMF)约化速度关联函数. 结果表明³⁶Ar+¹²⁴Sn反应系统中的约化速度关联函数在小约化速度处的反关联程度比³⁶Ar+¹¹²Sn反应系统中的强, 表现出明显的入射道依赖性. 考察出射粒子对的单核子总动量时, 发现这种差异主要来自于高动量粒子对的贡献. 用三体弹道理论模型MENEKA分别计算了两个系统的IMF发射时标, 在³⁶Ar+¹¹²Sn反应系统中约为150fm/c, 而在³⁶Ar+¹²⁴Sn反应系统中, 约为120fm/c. 同位旋相关的量子分子动力学计算表明, ³⁶Ar+¹²⁴Sn系统中IMF的发射时间谱比³⁶Ar+¹¹²Sn系统略有前移, 相应地, 其中心密度从最高点随时间的下降亦比³⁶Ar+¹¹²Sn系统略快.     

Surface reaction mechanism of Y2O3 atomic layer deposition on the hydroxylated Si(1 0 0)-2 × 1: A density functional theory study

The surface reaction mechanism of Y₂O₃ atomic layer deposition (ALD) on the hydroxylated silicon surface is investigated by using density functional theory. The ALD process is designed into two half-reactions, i.e., Cp₃Y (Cp = cyclopentadienyl) and H₂O half-reactions. For the Cp₃Y half-reaction, the chemisorbed complex is formed along with the change of metal-Cp bonding from Y-C(π) to Y-C₁(σ). For the H₂O half-reactions, the chemisorbed energies are increased with the relief of steric congestion around yttrium metal center. In addition, Gibbs free energy calculations show that it is thermodynamically favorable for the Cp₃Y half-reactions. By comparing with the reaction of H₂O with {Si}-(O₂)YCp, it is thermodynamically more favorable and kinetically less favorable for the reactions of H₂O with {Si}-OYCp₂ as well as with {Si}-OYCp(OH).     

Nuclear temperature measurements with the double isotope ratio technique: Influence of the experimental conditions

The dependence of the nuclear temperatures of highly excited systems, extracted by means of the double ratios of the emitted isotopes, on the experimental conditions is investigated. Experimental data obtained in the Xe+Cu 30 MeV/nucleon reaction are used to study the sensitivity of the method and the effects of the energy thresholds on the obtained temperature values. We find that the temperatures extracted using the He/Li ratios can be strongly influenced by the experimental energy thresholds which are different for different elements. These distortions depend on the velocity of the emitting system and on the detection angle and therefore particular care is needed in the choice of the detectors in those experiments in which velocities are low and angles are large. The use of four isotopes of the same element make negligible such effects. Received: 6 October 1999 / Accepted: 28 May 2000     

Instabilities in nuclear matter and finite nuclei

Spinodal instability in nuclear matter and finite nuclei is investigated. This instability occurs in the low-density region of the phase diagram. The thermodynamical and dynamical analysis is based on Landau theory of Fermi liquids. It is shown that asymmetric nuclear matter can be characterized by a unique spinodal region, defined by the instability against isoscalar-like fluctuation, as in symmetric nuclear matter. Everywhere in this density region the system is stable against isovector-like fluctuations related to the species separation tendency. Nevertheless, this instability in asymmetric nuclear matter induces isospin distillation leading to a more symmetric liquid phase and a more neutron-rich gas phase.     

Fragmentation Cross Sections of 12C on Different Targets at Beam Energies from 50 to 100MeV/Nucleon

The fragmentation cross sections of reactions ^12C＋^2H, ^12C, ^14N, ^16O at beam energies from 50 to 100 MeV/nucleon are investigated using the isospin-dependent Boltzmann-Langevin equation model. It is found that fragment species increase approximately with the increasing target mass. The fragment species and some fragments production cross sections in reactions of ^12C＋^12C, ^14N, ^16O show an obvious variation at the beam energies from 50 to 80 MeV/nucleon. However the calculated fragment production cross sections do not change much when the incident energy increases from 80 to 100 MeV/nucleon.     

Rate coefficients measurement for the energy-pooling collisions Cs(5D) + Cs(5D) → Cs(6S) + Cs(nl = 9D, 11S, 7F)

We report experimental rate coefficients for the energy-pooling collisions Cs(5D) + Cs(5D) → Cs(6S) + Cs(nl = 9D, 11S, 7F). In the experiment the Cs(5D) state was populated via photodissociation of Cs₂ molecules using an argon-ion laser at wavelength 488.0 nm. We also consider the competing process 6P_1/2 + 7S → 6S + (nl = 9D, 11S, 7F) that might also populate 9D, 11S and 7F. An intermodulation technique was used to select the fluorescence contributions due only to the process 6P_1/2 + 7S → 6S + (nl = 9D, 11S, 7F). The excited atom (nl_J) density and spatial distribution were mapped by monitoring the absorption of a counterpropagating probe laser beam tuned to various transitions. The measured excited atom densities are combined with measured fluorescence ratios to yield rate coefficients for the energy-pooling collisions Cs(5D) + Cs(5D) → Cs(6S) + Cs(nl = 9D, 11S, 7F). The rate coefficients for nl = 9D, 11S, 7F are (4.1 ± 2.0) × 10⁻¹⁰ cm³ s⁻¹, (1.6 ± 0.8) × 10⁻¹⁰ cm³ s⁻¹ and (3.6 ± 1.8) × 10⁻¹⁰ cm³ s⁻¹, respectively. The contributions to the rate coefficients from other energy transfer processes are also discussed.     

Structural, optical properties and band gap alignments of ZrOxNy thin films on Si (1 0 0) by radio frequency sputtering at different deposition temperatures

ZrO_xN_y thin films have been prepared by radio frequency magnetron sputtering at various substrate temperatures. The effect of substrate temperature on structural, optical properties and energy-band alignments of as-deposited ZrO_xN_y thin films are investigated. Atomic force microscopy results indicate the decreased root-mean-square (rms) values with substrate temperature. Fourier transform infrared spectroscopy spectra indicate that an interfacial layer has been formed between Si substrate and ZrO_xN_y thin films during deposition. X-ray photoelectron spectroscopy and spectroscopy ellipsometry (SE) results indicate the increased nitrogen incorporation in ZrO_xN_y thin films and therefore, the decreased optical band gap (E_g) values as a result of the increased valence-band maximum and lowered conduction-band minimum.     

Isospin and symmetry energy effects on nuclear fragment production in liquid-gas-type phase transition region

We have shown that the isospin of nuclei influences the fragment production during the nuclear liquid-gas phase transition. Calculations for Au¹⁹⁷, Sn¹²⁴, La¹²⁴ and Kr⁷⁸ at various excitation energies were carried out on the basis of the statistical multifragmentation model (SMM). We analyzed the behavior of the critical exponent τ with the excitation energy and its dependence on the critical temperature. Relative yields of fragments were classified with respect to the mass number of the fragments in the transition region. In this way, we have shown that nuclear multifragmentation exhibits a “bimodality” behavior. We have also shown that the symmetry energy has a small influence on fragment mass distribution; however, its effect is more pronounced in the isotope distributions of produced fragments.     

Inhomogeneities in 130 MeV Au ion irradiated Au/n-Si (1 0 0) Schottky structure

The electrical characteristics of Au/n-Si (1 0 0) Schottky rectifier have been studied in a wide irradiation fluence range using conventional current-voltage (I-V) and capacitance-voltage (C-V) measurements. The I-V characteristics showed an abnormal increase in forward current at low voltage. The device shows a bend in forward I-V and reverses bias C-V characteristics due to extra current, suggesting that there are two independent contributions to thermionic current, corresponding to two levels of the Schottky barrier. It is shown that the excess current at low voltage can be explained by taking into account the role of heavy ion irradiation induced defects at the metal semiconductor interface.     

K0 Condensation in Hyperonic Neutron Star Matter

In the framework of the relativistic mean field theory, we investigate K^0 condensation along with K^- condensation in neutron star matter including the baryon octet. The results show that both K^0 and K^- condensations can occur well in the core of the maximum mass stars for relatively shallow optical potentials of K^- in the range of-100 MeV～ -160 MeV. With the increasing optical potential of K^-, the critical densities of K^- decrease and the species of baryons appearing in neutron stars become fewer. The main role of K^0 condensation is to make the abundances of particles become identical leading to isospin saturated symmetric matter including antikaons, nucleons and hyperons. K^- condensation is chiefly responsible for the softening of the corresponding equation of state, which leads to a large reduction in the maximum masses of neutron stars. In the core of massive neutron stars, neutron star matter including rich particle species, such as antikaons, nucleons and hyperons, may exist.     

Renormalization group dependence of the QCD coupling

The general relation between the standard expansion coefficients and the beta function for the QCD coupling is exactly derived in a mathematically strict way. It is accordingly found that an infinite number of logarithmic terms are lost in the standard expansion with a finite order, and these lost terms can be given in a closed form. Numerical calculations, by a new matching-invariant coupling with the corresponding beta function to four-loop level, show that the new expansion converges much faster.     

The influence of Isospin Dependence of In-Medium NN Cross Sections on the Ratio of Emitted Neutrons to Protons in HICs

The influence of isospin dependence of in-medium nucleon-nucleon cross sections on the nip ratios for emitted nucleons in reactions 96Zr-j-96Zr and 96Ru-j-96RH at Eb z 400 AMeV is investigated by means of an improved quantum molecular dynamics model. Our results show that the high energy part of the spectra of the n//p ratios for emitted nucleons is sensitive to the isospin dependence of in-medium nucleon-nucleon cross sections for neutron-rich reaction systems. Therefore, we propose that the nip ratio of emitted high energy nucleons in a very neutron-rich reaction system at several hundreds of AMeV can be taken as sensitive observables to constrain the isospindependence of in-medium nucleon-nucleon cross sections.     

Temperature dependence of the current-voltage characteristics of the Al/Rhodamine-101/p-Si(1 0 0) contacts

The current-voltage (I-V) characteristics of Al/Rhodamine-101/p-Si/Al contacts have been measured at temperatures ranging from 280 to 400 K at 20 K intervals. A barrier height (BH) value of 0.817 eV for the Al/Rh101/p-Si/Al contact was obtained at the room temperature that is significantly larger than the value of 0.58 eV of the conventional Al/p-Si Schottky diode. While the barrier height Φ_b0 decreases the ideality factors (n) become larger with lowering temperature. The high values of n depending on the sample temperature may be ascribed to decrease of the exponentially increase rate in current due to space-charge injection into Rh101 thin film at higher voltage. Therefore, at all temperatures, it has been seen that the I-V characteristics show three different regions, the ohmic behavior at low voltages, and the space charge limited current with an exponential distribution of traps at high voltages.     

Mass flows and angular momentum density for px + ipy paired fermions in a harmonic trap

We present a simple two-dimensional model of a p_x + ip_y superfluid in which the mass flow that gives rise to the intrinsic angular momentum is easily calculated by numerical diagonalization of the Bogoliubov-de Gennes operator. We find that, at zero temperature and for constant director l, the mass flow closely follows the Ishikawa-Mermin-Muzikar formula .     

Adsorption of gold on hydrogen terminated Si(0 0 1): Formation of chain structure

Possible formation of stable Au atomic wire on the hydrogen terminated Si(0 0 1): 3×1 surface is investigated under the density functional formalism. The hydrogen terminated Si(0 0 1): 3×1 surface is patterned in two different ways by removing selective hydrogen atoms from the surface. The adsorption of Au on such surfaces is studied at different sub-monolayer coverages. At 4/9 monolayer (ML) coverage, zigzag continuous Au chains are found to be stable on the patterned hydrogen terminated Si(0 0 1): 3×1 surface. The reason for the stability of the wire structures at 4/9 ML coverage is explained. It is to be noted that beyond 4/9 ML coverage, the additional Au atoms may introduce clusters on the surface. The continuous atomic gold chains on the substrate may be useful for the fabrication of atomic scale devices.     

Study of the early stages of Cr/6H-SiC(0 0 0 1) interface formation

The early stages of the Cr/6H-SiC(0 0 0 1) interface formation at room temperature were investigated using XPS, LEED and work function (WF) measurements. Upon stepwise Cr evaporation in UHV up to a thickness of 5-10 monolayers (ML) at RT, the binding energy of the XPS Cr 2p_3/2 core level peak shifted from 576.1 eV, at submonolayer coverage, to 574.7 eV (corresponding to metallic Cr) for the final Cr deposit, while the binding energies of the substrate XPS core level peaks remained stable. The WF exhibited a steep decrease of about 0.5 eV from the initial SiC substrate value, upon submonolayer coverage, but then increased gradually to saturation at a value of about 4.8 eV (polycrystalline Cr film with some chemisorbed oxygen). The growth of the ultrathin film was via 3D-cluster formation. The height of the Schottky barrier for the Cr/6H-SiC(0 0 0 1) contact was found by XPS to be 0.5 ± 0.1 eV. The results, generally, indicate the absence of any extended interfacial silicide-like interaction at RT.     

High-temperature measurements of the rates of the reactions CH2O + Ar → Products and CH2O + O2 → Products

The two-channel thermal decomposition of formaldehyde [CH₂O], (1a) CH₂O + Ar → HCO + H + Ar, and (1b) CH₂O + Ar → H₂ + CO + Ar, was studied in shock tube experiments in the 2258-2687 K temperature range, at an average total pressure of 1.6 atm. OH radicals, generated on shock heating trioxane-O₂-Ar mixtures, were monitored behind the reflected shock front using narrow-linewidth laser absorption. 1,3,5 trioxane [C₃H₆O₃] was used as the CH₂O precursor in the current experiments. H-atoms formed upon CH₂O and HCO decomposition rapidly react with O₂ to produce OH via H + O₂ → O + OH. The recorded OH time-histories show dominant sensitivity to the formaldehyde decomposition pathways. The second-order reaction rate coefficients were inferred by matching measured and modeled OH profiles behind the reflected shock. Two-parameter fits for k_1a and k_1b, applicable in this temperature range, are:

     

Single-Proton Pickup Reaction of the Halo Nucleus ^6He on a ^9Be Target at 25 MeV/nucleon

The inclusive differential cross sections of the ^7 Li nucleus in a reaction induced by ^6He on a ^9Be target are measured at an incident energy of 25 MeV/nucleon. Finite-range distorted-wave Born approximation calculations suggest that these ^7 Li particles are formed in a direct single-proton pickup reaction ^9Be（^6He,^7 Li）^8Li. The experimental data can be well reproduced by taking into account of the contributions of both the ground states and the first excited states of ^7Li and ^8Li.