穿孔率和穿孔直径耦合下微穿孔板吸声体整体吸声性能

微穿孔板几何参数的耦合性及其对整体吸声性能的影响,对于设计微穿孔板吸声体和优化其工作性能具有指导作用。根据微穿孔板吸声体基本理论,研究了穿孔率和穿孔直径双参数耦合作用下微穿孔板吸声体的整体吸声性能。穿孔率和穿孔直径之间的耦合性与其本身取值密切相关,而与板厚和板后腔深无明显关系;在穿孔率-穿孔直径参数域上,吸声体存在吸声系数为1.0的吸收峰,整体吸声性能随穿孔率或穿孔直径从小到大变化,呈现出先增强后减弱的变化趋势。该结论能够准确解释微穿孔板受粉尘污染后吸声性能的变化规律和演变路径。论文的工作为设计微穿孔板吸声体提供了一种新的理论依据和实施方法。     

Improving low-frequency sound absorption of micro-perforated panel absorbers by using mechanical impedance plate combined with Helmholtz resonators

The traditional Micro-perforated plate (MPP) is a kind of clean and non-polluting absorption structure in the middle and high frequency and has been widely used in the field of noise control. However, the sound absorption performance is dissatisfied at low frequencies when the air-cavity depth is restricted. In this paper, a mechanical impedance plate (MIP) is introduced into the traditional MPP structure and a Helmholtz resonator is attached to the MIP. Mechanical impedance plate (MIP) provides a good absorption at low frequency by using mechanism of mechanical resonance and the acoustic energy is dissipated in the form of heat with viscoelastic material. Helmholtz resonator can fill in the defect of the poor absorption effect between the Micro-perforated plate (MPP) and the mechanical impedance plate (MIP). The acoustic impedance of the proposed sound absorber is investigated by using acoustic electric analogy method and impedance transfer method. The influence of the tube’s length of Helmholtz resonator and the number of Helmholtz resonator on the sound absorption is studied. The corresponding results are in agreement with the theoretical calculation and prove that the composite structure has the characteristics of improving the low frequency sound absorption property.     

Enhancing the low frequency sound absorption of a perforated panel by parallel-arranged extended tubes

This paper is concerned with the use of a perforated panel with extended tubes (PPET) to improve the sound absorption confined to low frequencies. In comparison with a micro-perforated panel (MPP), the sound absorption can be significantly improved by using the PPET at the expense of the bandwidth of the sound absorption. A particular configuration combining four parallel-arranged PPETs with different cavities is introduced to achieve a wider bandwidth of the sound absorption at low frequencies. The analysis is extended to the combination of three parallel-arranged PPETs and a MPP to further increase the bandwidth of the sound absorption. A theoretical model is described to predict the sound absorption coefficient and the simulated annealing method is introduced to the proposed absorbers, allowing optimization of the overall performance. The theory with experimental validations demonstrates that the proposed configurations offer a potential improvement of more than one octave in the bandwidth of the sound absorption at low frequencies.     

Sound absorption of a double-leaf micro-perforated panel with an air-back cavity and a rigid-back wall: Detailed analysis with a Helmholtz-Kirchhoff integral formulation

So far the electro-acoustical equivalent circuit analysis has been widely used to analyse micro-perforated panel (MPP) absorbers, however, as for the double-leaf MPP the equivalent circuit analysis inevitably includes an approximation. In this paper, the sound absorption characteristics of a double-leaf MPP absorber backed by a rigid wall are analysed by wave theory using Helmholtz-Kirchhoff integral formulation to obtain a strict solution. The present wave theory is experimentally validated with existing measured results. The theory is also compared with the equivalent circuit solutions so that the differences between the two theories appear and the effect of the approximation is clarified. The comparison shows that the difference mainly appears in the vicinity of the resonance peaks: the differences occur in the resonance frequencies and the absorption coefficient at frequencies between the two resonance peaks.     

多层微穿孔板结构声学性能计算方法对比分析

计算多层微穿孔板结构声学特性方法传统主要用声电类比法,目前出现阻抗转移法和传递矩阵法,对比分析这三种计算方法,同时进行相应的实验验证。结果表明:阻抗转移法和传递矩阵法实质上是相同的,这两种方法计算结果与实验结果吻合良好。声电类比法在空腔较大时计算结果偏离实验值,原因是声电类比法采用集总参数分析,计算多层结构时,空腔单元只考虑声顺,忽略声质量,导致误差。阻抗转移法和传递矩阵法不存在这一误差,计算准确。     

Synthesis and field emission of diamond-like carbon nanorods on TiO2/Ti nanotube arrays

Highly ordered TiO₂/Ti nanotube arrays were fabricated by anodic oxidation method in 0.5 wt% HF. Using prepared TiO₂/Ti nanotube arrays deposited Ni nanoparticles as substrate, high quality diamond-like carbon nanorods (DLCNRs) were synthesized by a conventional method of chemical vapor deposition at 750 °C in nitrogen atmosphere. DLCNRs were analyzed by filed emission scanning electron microscopy and Raman spectrometer. It is very interesting that DLCNRs possess pagoda shape with the length of 3–10 μm. Raman spectra show two strong peaks about 1332 cm⁻¹ and 1598 cm⁻¹, indicating the formation of diamond-like carbon. The field emission measurements suggest that DLCNRs/TiO₂/Ti has excellent field emission properties, a low turn-on field about 3.0 V/μm, no evident decay at 3.4 mA/cm² in 480 min.     

Growth of aligned carbon nanotube arrays on metallic substrate and its application to supercapacitors

Aligned carbon nanotube arrays (ACNTAs) with lengths up to 150 μm were fabricated on metallic alloy (Inconel 600) substrates by pyrolysis of iron (II) phthalocyanine (FePc) in the presence of ethylene (C₂H₄). The as-grown ACNTAs, formed by aligned multi-walled carbon nanotubes with high purity, were characterized by scanning electron microscopy (SEM), high resolution transmission electron microscopy (HRTEM), and Raman spectroscopy techniques. The ACNTAs were used directly as electrode materials in supercapacitors with (Et)₄NBF₄ + propylene carbonate (PC) as electrolyte, and their electrochemical properties were investigated. A rectangular-shaped cyclic voltammetry (CV) curve was observed even at a sweep rate of 1000 mV s⁻¹. The specific capacitance measured at 1000 mV s⁻¹ was about 57 % (47 F g⁻¹) of that obtained at 1 mV s⁻¹ (83 F g⁻¹), and an equivalent series resistance (ESR) of 0.55 Ω was measured for the ACNTA and activated carbon pair electrodes embedded in a coin cell. The results indicated that the ACNTAs could be a promising candidate as electrode materials in supercapacitors.     

Field emission of carbon nanotube array with normal-gate cold cathode

A hexagon pitch carbon nanotube (CNT) array vertical to the normal gate of cold cathode field emission displayer (FED) is simulated by solving the Laplace equation. The calculated results show that the normal gate causes the electric field around the CNT tops to be concentrated and emission electron beam become a column. The field enhancement factor and the emission current intensity step up greatly compared with those of diode structure. Emission current density increases rapidly with the decrease of normal-gate aperture. The gate voltage exerts a critical influence on the emission current.     

Molecular dynamic investigation of mechanical properties of armchair and zigzag double-walled carbon nanotubes under various loading conditions

Using molecular dynamic simulation (MDS), effects of chirality and Van der Waals interaction on Young's modulus, elastic compressive modulus, bending, tensile, and compressive stiffness, and critical axial force of double-walled carbon nanotube (DWCNT) and its inner and outer tubes are considered. Achieving the highest safety factor, mechanical properties have been investigated under applied load on both inner and outer tubes simultaneously and on each one of them separately. Results indicate that as a compressive element, DWCNT is more beneficial than single-walled carbon nanotube (SWCNT) since it carries two times higher compression before buckling. Except critical axial pressure and tensile stiffness, in other parameters zigzag DWCNT shows higher amounts than armchair type. Outer tube has lower strength than inner tube; therefore, most reliable design of nanostructures can be attained if the mechanical properties of outer tube taken as the properties of DWCNT.     

Characterisation of carbonaceous materials using Raman spectroscopy: a comparison of carbon nanotube filters,single‐ and multi‐walled nanotubes,graphitised porous carbon and graphite

Multi‐walled carbon nanotube (MWCNT) filters have been recently synthesised which have specific molecular filtering capabilities and good mechanical strength. Optical and scanning electron microscopy (SEM) reveals the formation of highly aligned arrays of bundles of carbon nanotubes having lengths up to 500 µm. The Raman spectra of this material along with four other carbonaceous materials, commercially available single‐walled carbon nanotubes (SWCNTs) and MWCNTs, graphitised porous carbon (Carbotrap) and graphite have been recorded using two‐excitation wavelengths, 532 and 785 nm, and analysed for band positions and shape with special emphasis paid to the D‐, G‐ and G′‐bands. A major difference between the different MWCNT varieties analysed is that G‐bands in the MWCNT filters exhibit almost no dispersion, whereas the other MWCNTs show a noticeable dispersive behaviour with a change in the excitation wavelength. Spectral features similar to those of the MWCNT filter varieties were observed for the Carbotrap material. From the line shape analysis, the intensity ratio, I_D/I_G, of the more ordered MWCNT filter material using the integral G‐band turns out to be two times lower than that of the less ordered MWCNT filter product at both excitation wavelengths. This parameter can, therefore, be used as a measure of the degree of MWCNT alignment in filter varieties, which is well supported also by our SEM study. Copyright © 2008 John Wiley & Sons, Ltd.     

Improvement on the wave absorbing property of a lossy frequency selective surface absorber using a magnetic substrate

An equivalent-circuit model is used to analyse the improvement of the wave absorbing performance of the lossy frequency selective surface(FSS) absorber by using a magnetic substrate,showing that it is possible to widen the wave absorbing bandwidth.Three pieces of magnetic substrates are prepared.According to the complex permittivity and permeability,the reflectivity of the corresponding absorber is calculated by the finite difference time-domain(FDTD) method,and the bandwidth of the reflectivity below 10 dB is optimized by genetic algorithm.The calculated results indicate that the wave absorbing performance is significantly improved by increasing the complex permeability of the substrate;the reflectivity bandwidth below 10 dB of the single layer FSS absorber can reach 3.6-18 GHz with a thickness of 5 mm,which is wider than that with a dielectric substrate.The density of the FSS absorber is only 0.92 g/cm 3.Additionally,the absorption band can be further widened by inserting a second lossy FSS.Finally,a double layer lossy FSS absorber with a magnetic substrate is fabricated based on the design result.The experimental result is consistent with the design one.     

Instability threshold of rippled carbon nanotube nanotweezers in the low vacuum gas flow incorporating Dirichlet and Neumann modes of Casimir energy

The aim of this research work is to address the influences of dispersion forces and rippled configuration on the instability threshold of carbon nanotube (CNT) based nanotweezers. To this end, the Dirichlet and Neumann modes of Casimir force arisen from the electric and magnetic energies is developed for cylinder–cylinder geometry. Moreover, the CNTs rippling deformation which experimentally revealed is included in the Euler-Bernoulli beam model to modify the governing equations. The differential quadrature method (DQM) in conjunction with the 4th-order Runge-Kutta algorithm is employed to numerically simulate the non-linear partial differential equations. It is interestingly demonstrated that these phenomena remarkably affect the electromechanical behavior of nanotweezers fabricated from CNTs. By taking the rippling configuration and Casimir attraction between tubes into account, the pull-in voltage decreases. On the other hand, when the gas damping effect due to low vacuum environment is taken into consideration, the pull-in value increases. The accuracy of the present modeling is compared with those experimentally published in the literature, giving excellent results.     

Abrasive wear under multiscratching of polystyrene + single-walled carbon nanotube nanocomposites. Effect of sliding direction and modification by ionic liquid

Single-walled carbon nanotubes (NTs) and single-walled carbon nanotubes modified (NTms) by the room-temperature ionic liquid (IL) 1-octyl, 3-methylimidazolium tetrafluoroborate ([OMIM]BF₄) were added in a 1 wt.% to polystyrene (PS) and processed by compression or injection moulding to obtain PS + NT and PS + NTm, respectively. Friction coefficients and abrasive wear from penetration depth, residual depth and viscoelastic recovery were determined under multiple scratching. The effect of the moulding process, the additives and the sliding direction was studied. Compression moulded PS shows a transition to more severe damage after a critical number of successive passes. Addition of NTs or NTms to compression moulded PS induces a strain hardening effect and reduces friction, residual depth and viscoelastic recovery. Strain hardening is also observed in injection moulded PS with sliding in the longitudinal and random directions, but not in the transverse direction. The scratch resistance of PS + NTm depends on sliding direction. The lowest friction coefficient and residual depth values, and the highest viscoelastic recovery were found for injection moulded PS + NTm, in the sliding direction parallel to injection flow. Mechanisms of surface damage are discussed upon scanning electron microscopy (SEM), focused ion beam-field emission scanning electron microscopy (FIB-FESEM), 3D surface topography, surface roughness and profilometry observations.     

Comparison of Activated Carbon,Multiwalled Carbon Nanotubes,and Cadmium Hydroxide Nanowire Loaded on Activated Carbon as Adsorbents for Kinetic and Equilibrium Study of Removal of Safranine O

Activated carbon (AC), multiwalled carbon nanotube (MWCNT), and cadmium hydroxide nanowire loaded on activated carbon (Cd(OH)₂-NW-AC) have been used for the removal of safranine O (SO) from wastewater. The effects of various parameters including pH, temperature, concentration of the dye, amount of adsorbents, and contact time on the SO adsorption efficiency for all adsorbents has been investigated. Graphical correlation of fitting experimental data to various adsorption isotherm models like those of Langmuir, Freundlich, Tempkin, and Dubinin–Radushkevich for all adsorbents have been calculated. It was found that safranine O adsorption on all adsorbents was endothermic and feasible in nature. Fitting the experimental data to different kinetic models suggests that the adsorption process follows pseudo-second-order kinetics with involvement of the particle diffusion mechanism.