Insulating surface layer on single crystal K $\mathsf{_{3}}\mathsf{C}\mathsf{_{60}}$

Using angle-dependent photoemission spectra of core and valence levels we show that metallic, single crystal K³C₆₀ is terminated by an insulating or weakly-conducting surface layer. We attribute this to the effects of strong intermolecular correlations combined with the average surface charge state. Several controversies on the electronic structure are thereby resolved.Received: 16 July 2004, Published online: 5 November 2004PACS: 71.20.Tx Fullerenes and related materials; intercalation compounds - 73.20.-r Electron states at surfaces and interfaces - 79.60.Bm Clean metal, semiconductor, and insulator surfaces     

Magnetic order in RCr\mathsf{_{2}}Si\mathsf{_{2}} intermetallics

The magnetic structure and ordering temperatures of three intermetallic compounds which crystallize in the tetragonal ThCr₂Si₂ structure, TbCr₂Si₂, HoCr₂Si₂ and ErCr₂Si₂, have been determined by neutron diffraction, differential scanning calorimetry and magnetization measurements. The Cr-sublattice orders anti-ferromagnetically with Néel temperatures of 758 K for TbCr₂Si₂, 718 K for HoCr₂Si₂ and 692 K for ErCr₂Si₂. Chromium atoms located at 4d crystallographic sites are aligned anti-parallel along the c-axis, with G_ZCr magnetic modes. In contrast with metallic bcc Cr, the refined room temperature value of the ordered Cr moment is anomalously large for all three compounds. No long range magnetic order of the R sublattice in TbCr₂Si₂ and HoCr₂Si₂ is observed, whilst the Er sublattice in ErCr₂Si₂ orders independently of the Cr sublattice below 2.4 K with moments ferromagnetically aligned in the basal plane.Received: 4 November 2003, Published online: 30 January 2004PACS: 75.25. + z Spin arrangements in magnetically ordered materials (including neutron and spin-polarized electron studies, synchrotron-source X-ray scattering, etc.) - 75.30.Cr Saturation moments and magnetic susceptibilities - 75.50.Ee Antiferromagnetics     

Microwave fluctuational conductivity in YBa\mathsf{_{2}}Cu\mathsf{_{3}}O \mathsf{_{7-\delta}}

We present measurements of the microwave complex conductivity at 23.9 and 48.2 GHz in YBa₂Cu₃O $_{7-\delta}$ films, in the fluctuational region above T _c . With increasing temperature, the fluctuational excess conductivity drops much faster than the well-known calculations within the time-dependent Ginzburg-Landau theory [H. Schmidt, Z. Phys. 216, 336 (1968)]. Approaching the transition temperature, slowing down of the fluctuations is observed. We discuss the results in terms of a modified Gaussian theory for finite-frequency fluctuational conductivity, where renormalization is introduced in order to account for the $T\rightarrow T_{c}$ regime, and a spectral cutoff is inserted in order to discard high-momentum modes. The data are in excellent agreement with the modified theory, when formulated for three-dimensional, anisotropic superconductors, in the whole experimentally accessible temperature range, and for both frequencies.     

Feshbach resonances in $\mathsf{^{23}}$Na- $\mathsf{^{87}}$Rb

We describe s-wave collisions between ultracold ²³Na and ⁸⁷Rb atoms in the presence of a magnetic field. For any collision input channel knowledge of the singlet and triplet intermolecular potentials [1] enables us to predict the variation in scattering lengths as a function of the magnetic field. We employ the Born-Oppenheimer approximation to predict several Feshbach resonances for ²³Na⁸⁷Rb. We also include a discussion of why these resonances are expected to be narrow as observed in the case of ⁸⁷Rb₂.Received: 6 August 2004, Published online: 23 November 2004PACS: 34.90. + q Other topics in atomic collisions - 03.75.Hh Multicomponent condensates