Beta-decay properties of strongly neutron-rich nuclei

Experimental β-strength functions for about 50 neutron-rich mass-separated fission products with half-lives between 0.8 s and 30 s have been obtained at the OSIRIS facility. The β-strength to excited states depopulating by delayed-neutron emission is evaluated separately. The β^? strength functions are found to increase strongly with excitation energy, which is in contrast to the approximately energy-independent β-strength found for EC decay. By using semiempirical values for the level density, the average transition rate per energy level was evaluated under the assumption that only allowed transitions contribute to the decay. This alternative way of analyzing the data gives a more uniform picture of the β-decay to highly excited states since the transition rates are found to be roughly independent of excitation energy (above the pairing energy). A model of constant transition rate to each final level is introduced and its systematic behaviour is studied. Its use for estimating half-lives of unmeasured nuclides is of value for calculations on nucleosynthesis by the “r-process”. (A listing of β-feed and β-strength functions is available on request.)     

Beta-decay properties of exotic nuclei and the astrophysical r-process

The r-process abundances are evaluated with the use of three different β-decay models, i.e., the second version of the Gross Theory, the semi-Gross Theory and a QRPA approach. The necessary Q_β-values, as well as the neutron separation energies, are obtained from the TUYY, ETFSI and FRDM mass predictions. A comparison is made among the β-decay half-lives predicted by these β-decay models for the nuclei on a typical r-process path, as well as among the resulting r-process abundances.     

Beta-decay study of Tz = - 2 proton-rich nucleus 24Si

$ \beta$ -decay spectroscopy on a T _z = - 2 proton-rich nucleus ²⁴Si was performed. The decay scheme of ²⁴Si was reconstructed by the $ \beta$ -delayed $ \gamma$ -ray and proton measurements. Two $ \beta$ branches to the bound 1₁ ⁺ and 1₂ ⁺ states in ²⁴Al were observed for the first time. The observation of the allowed transition firmly established the spin-parity assignment for the 1₂ ⁺ states. The branching ratios to the 1₁ ⁺ and 1₂ ⁺ states were determined to be 31(4)% and 23.9(15)%, respectively. The branching ratios to three unbound states in ²⁴Al including a new level at 6.735MeV were also determined for the first time. The level structure of ²⁴Al was compared with its mirror nucleus ²⁴Na . The Thomas-Ehrman shift on the 1₂ ⁺ state indicates s -wave dominance in the state as well as a characteristic behavior of the weakly bound s -wave proton in ²⁴Al .     

Beta-decay of 71Co and 73Co

A decay spectroscopy study of the neutron-rich cobalt isotopes has been performed using fragmentation of a ⁸⁶Kr³⁶⁺ beam and the new LISE2000 spectrometer at GANIL. For ⁷¹Co and ⁷³Co, the -delayed radiation has been observed for the first time, and the half-lives were found to be 79(5) ms and 41(4) ms, respectively. Features of the decay are discussed qualitatively in terms of nuclear models.     

Beta-decay of even-A neutron-deficient Pr isotopes

Even-A praseodymium activities have been produced and identified in the⁴⁰Ca +^92–96Mo reactions at 5.8 MeV/u:¹²⁶Pr[T_1/2=(3.0 ±0.4)s]¹²⁸Pr[T_1/2=(3.1 ±0.3)s],¹³⁰Pr[T_1/2 =(40.0 ±0.4)s]¹³²Pr[T_1/2=1.6 min]. Several new low-energy levels have been populated in even-even cerium nuclei.     

25Mg (α, n)28Si and 26Mg(α, n)29Si as neutron sources in explosive neon burning

The yields of neutrons from the reaction ²⁵Mg(α, n)²⁸Si and of γ-rays from the reaction ²⁵Mg(α, nγ)²⁸Si have been measured as a function of bombarding energy over the range 1.8–6.3 MeV, and the yield of neutrons from ²⁶Mg(α, n)²⁹Si has been measured over the range 1.8–6.0 MeV. Cross sections for ^{25, 26}Mg(α, n)^{28, 29}Si were extracted from the data and compared with global statistical-model calculations. The agreement is very good. Thermonuclear reaction rates under stellar conditions appropriate for explosive neon burning are calculated and their significance for the nucleosynthesis of rare neutron-rich nuclei is discussed.     

Beta-decay energy and nuclear mass of100Nb

Radiofrequency measurements of the zero-field hyperfine intervals in low levels of¹⁶⁷Er and^161,163Dy have been made as part of a systematic study of the second half of the 4f^N6s² configuration of the neutral rare-earth atoms. Almost no precise hfs data exist for this region, and a preliminary analysis indicates systematic differences between ab initio theory and experiment.     

Beta-decay branching ratios of 62Ga

Beta-decay branching ratios of ⁶²Ga have been measured at the IGISOL facility of the Accelerator Laboratory of the University of Jyv?skyl?. ⁶²Ga is one of the heavier T _z = 0 , 0⁺ → 0⁺ β -emitting nuclides used to determine the vector coupling constant of the weak interaction and the V_ud quark-mixing matrix element. For part of the experimental studies presented here, the JYFLTRAP facility has been employed to prepare isotopically pure beams of ⁶²Ga . The branching ratio obtained, BR = 99.893(24) %, for the super-allowed branch is in agreement with previous measurements and allows to determine the ft value and the universal Ft value for the super-allowed β -decay of ⁶²Ga .     

Beta-decay studies of neutron-rich Sc- Cr nuclei

The neutron-rich nuclei ₂₁^{57, 58}Sc, ₂₂^58-60Ti, ₂₃^60-63V, ₂₄^62-66Cr have been produced at Ganil via interactions of a 61.8A MeV ⁷⁶Ge beam with a ⁵⁸Ni target. Beta-decay studies have been performed using combined - and -ray spectroscopy. Half-lives have been determined and -decay schemes are proposed for ⁵⁸Ti, ⁶¹V and ⁶²Cr. From these studies, new hints for the existence of -decaying isomers in ⁶⁰V and in ⁶²Mn are provided. These results are compared to shell model calculations. The role of the f_7/2- f_5/2 proton-neutron interaction is examined through its influence on the lifetime values.     

Precise half-life measurement of the 26Si ground state

The β-decay half-life of ²⁶Si was measured with a relative precision of 1.4·10^?3. The measurement yields a value of 2.2283(27) s which is in good agreement with previous measurements but has a precision that is better by a factor of 4. In the same experiment, we have also measured the non-analogue branching ratios and could determine the super-allowed one with a precision of 3%. The experiment was done at the Accelerator Laboratory of the University of Jyväskylä where we used the IGISOL technique with the JYFLTRAP facility to separate pure samples of ²⁶Si.     

Structural properties of Si and GaP

Total energies are calculated for crystalline Si and GaP within the local-density functional formalism using first principles non-local pseudopotentials. Ground state structural properties (total energy, bulk modulus and lattice constant) are obtained for Si and GaP and are in good agreement with experimental values (differences < 6%). Si is used as a test and compared with other theoretical calculations.     

Temperature-dependent 29Si NMR resonance shifts in lightly- and heavily-doped Si:P

Careful NMR measurements on a very lightly-doped reference silicon sample provide a convenient highly precise and accurate secondary chemical shift reference standard for ²⁹Si MAS-NMR applicable over a wide temperature range. The linear temperature-dependence of the ²⁹Si chemical shift measured in this sample is used to refine an earlier presentation of the paramagnetic (high-frequency) ²⁹Si resonance shifts in heavily-doped n-type silicon samples near the metal–nonmetal transition. The data show systematic decreases of the local magnetic fields with increasing temperature in the range 100–470 K for all samples in the carrier concentration range from 2×10¹⁸ cm⁻³ to 8×10¹⁹ cm⁻³. This trend is qualitatively similar to that previously observed for the two-orders of magnitude larger ³¹P impurity NMR resonance shifts in the same temperature and concentration ranges. The ²⁹Si and ³¹P resonance shifts are not related by a simple scaling factor, however, indicating that impurity and host nuclei are affected by different subsets of partially-localized extrinsic electrons at all temperatures.     

Beta-decay energies and nuclear masses of very neutron-rich Rb and Cs isotopes

Theβ-endpoint energies of very neutron-rich Rb and Cs isotopes with mass numbers 94≦A≦98 and 142≦A≦146, respectively, have been measured with a plastic scintillatorβ-telescope at the on-line mass separator OSTIS. From these,Q _β-values and mass excesses are calculated and compared with the results obtained in direct mass determinations.     

Beta-decay experiments of neutral atoms in a magneto-optical trap

Magneto optical traps (MOT) allow the cooling and storing of neutral atoms in a volume of a few cubic millimeters by use of laser beams and a magnetic field. Such devices offer new and exciting opportunities for precision measurements of radioactive isotopes. Here we present experiments performed with a double-MOT system coupled to the on-line separator TISOL at TRIUMF/Vancouver, Canada. For the first time, the Β-decay of free atoms stored in such a device could be observed. We report on coincidence measurements between beta-particles and the argon recoils in the decay of ³⁷K and ³⁸rm{m}}K. The charge state ratios of the recoil-ions were deduced by Time-Of-Flight separation in an acceleration field. The final goal of those investigations is a precision test of the Standard Model by measuring the –nu-correlation parameter a. This revised version was published online in July 2006 with corrections to the Cover Date.     

Beta-decay of the N = Z nucleus 72Kr

The beta-decay of the N = Z, even-even nucleus ⁷²Kr has been studied at the ISOLDE PSB facility at CERN. Measurements of βγ and βγγ coincidences have enriched the decay scheme of the daughter nucleus ⁷²Br with 27 new low spin levels. A more precise half-life of T _1/2 = 17.1(2) s has been determined. Strong feeding to the ⁷²Br ground state is established yielding an unambiguous J ^π = 1⁺ assignment for this state. Candidates for the ⁷²Br g.s. wave function are discussed in the framework of a self-consistent deformed mean-field calculation with SG2 Skyrme force and pairing correlations. A search for beta-delayed particle emission was made and an upper limit of 10^-6 for this decay branch obtained. The cumulated experimental level density of 1⁺ states has been fitted with the constant temperature formula. The comparison indicates that most likely all 1⁺ levels up to 1.2 MeV have been observed in this investigation. The corresponding nearest-neighbour level spacing does not follow a Poisson distribution. The Gamow-Teller strength distribution is compared, in terms of nuclear deformation, with different calculations made in the framework of the quasiparticle random phase approximation. Received: 7 February 2002 / Accepted: 31 October 2002 / Published online: 6 March 2003 RID="a" ID="a"e-mail: borge@pinar2.csic.es RID="b" ID="b"Present address: Centre d' Etudes Nucléaires de Bordeaux-Gradignan, Le Haut Vigneau, F-33175 Gradignan Cedex, France. RID="c" ID="c"Present address: University Mentouri, 25000 Constantine, Algeria. Communicated by J. ?yst?     

Experimental and theoretical studies of Si/P substituted orthorhombic Fe2P

A Mössbauer spectroscopic study of orthorhombic Fe₂P_1–x Si _x withx 0.35 was performed. A large spread in magnetic hyperfine fields was found at the six Fe positions ranging from 10–26 T at 4.2 K. Small rearrangements in the crystal positions as compared to the hexagonal phase cause large changes in the magnetic field. Large changes in Fe magnetic moments have also been obtained in a spin-polarized LMTO band calculation performed on orthorhombic Fe₂P as compared to a similar calculation of hexagonal Fe₂P.     

Beta-decay of148,150,152Pr into levels of148,150,152Nd

Theβ ^?-decay of^148,150,152Pr into levels of^148,150,152Nd has been studied byγ-singles,γγ-coincidence and for¹⁴⁸Pr also byγγ-angular correlation measurements. The praseodymium activities have been obtained by thermal neutron-induced fission of²³⁵U followed by on-line mass separation with the helium-jet coupled mass separator HELIOS. Decay schemes for these heaviest praseodymium nuclides are proposed. From the angular correlation measurements spin values for the seven lowest levels of¹⁴⁸Nd are deduced. Spin and parity assignments for the lower levels in^150,152Nd have been extrapolated from level systematics.