共查询到20条相似文献,搜索用时 15 毫秒
1.
F. Gervais N. Petit C. Popon P. Buvat 《The European Physical Journal B - Condensed Matter and Complex Systems》2003,31(1):47-52
The reflectivity spectrum of a polyaniline CSA-doped in presence of m-cresol has been measured over the wide wavenumber range
25-15,000 cm-1 (0.003-1.9 eV) for three different doping levels. Since spectra cannot be fitted correctly with the conventional Drude model,
several extensions are tested. A model derived from the factorized form of the dielectric response and including the effect
of Anderson localization in disordered metals, is proposed and found to yield good fit to data with a satisfactory physical
meaning. Data are reduced to a small number of parameters potentially useful for further comparison with other conducting
polymers or even other non-Drude conducting media like oxides.
Received 6 February 2002 / Received in final form 12 August 2002 Published online 27 January 2003
RID="a"
ID="a"e-mail: gervais@delphi.phys.univ-tours.fr
RID="b"
ID="b"UMR 6157 CNRS/CEA 相似文献
2.
A. La Magna R. Pucci 《The European Physical Journal B - Condensed Matter and Complex Systems》1998,4(4):421-429
In this paper we have introduced a variational approach to investigate the ground state of a model which includes both the
Holstein electron-phonon interaction and the extended Hubbard electron-electron interaction. We have considered a variational
state for the phonon subsystem which generalizes the previous used forms. This state allows to take into account the possibility
of extended phonon mediated correlations. The effective electron Hamiltonian, which we have obtained, includes first and second
neighbor electron-electron interaction terms. We have treated exactly, through a Lanczos method, this effective model in the
one-dimensional case. We have applied our method to two Bechgaard salts and in these cases we have estimated the correlation
parameters. We have shown that the introduction of electron-phonon interaction allows an estimate of the on site U and nearest-neighbor V Coulomb repulsion, which are in agreement with the experimental optical spectra of the above mentioned two compounds.
Received: 30 October 1997 / Revised: 28 January 1998 / Accepted: 10 April 1998 相似文献
3.
Optical properties of an interacting large polaron gas 总被引:1,自引:0,他引:1
V. Cataudella G. De Filippis G. Iadonisi 《The European Physical Journal B - Condensed Matter and Complex Systems》1999,12(1):17-22
The normal state conductivity, , of a system of interacting large polarons is calculated within the Random Phase approximation and some numerical results
are presented. The behaviour of the optical absorption as a function of the charge carrier density and of the temperature
is analyzed for different values of the electron-phonon coupling constant. It is shown that exhibits features similar to those observed in the infrared spectra of the cuprates.
Received 27 January 1999 相似文献
4.
R.T. Senger A. Erçelebi 《The European Physical Journal B - Condensed Matter and Complex Systems》2000,16(3):439-446
In the limit of strong electron-phonon coupling, we provide a unified insight into the stability criterion for bipolaron formation
in low-dimensionally confined media. The model that we use consists of a pair of electrons immersed in a reservoir of bulk
LO phonons and confined within an anisotropic parabolic potential box, whose barrier slopes can be tuned arbitrarily from
zero to infinity. Thus, encompassing the bulk and all low-dimensional geometric configurations of general interest, we obtain
an explicit tracking of the critical ratio of dielectric constants below which bipolarons can exist.
Received 15 September 1999 and Received in final form 20 March 2000 相似文献
5.
6.
Polaronic effects on the energy levels of a double donor impurity in quantum wells in the presence of a magnetic field 总被引:3,自引:0,他引:3
Zi-xin Liu Zhen-jiang Lai Yong-chang Huang Ya Liu Guo-jun Cheng 《The European Physical Journal B - Condensed Matter and Complex Systems》1999,12(3):347-350
In the presence of a magnetic field the Hamiltonian of the single or double polaron bound to a helium-type donor impurity
in semiconductor quantum wells (QWs) are given in the case of positively charged donor center and neutral donor center. The
couplings of an electron and the impurity with various phonon modes are considered. The binding energy of the single and double
bound polaron in AlxlGa 1-xlAs/GaAs/AlxrGa 1-xrAs QWs are calculated. The results show that for a thin well the cumulative effects of the electron-phonon coupling and the
impurity-phonon coupling can contribute appreciably to the binding energy in the case of ionized donor. In the case of neutral
donor the contribution of polaronic effects are not very important, however the magnetic field significantly modifies the
binding energy of the double donor. The comparison between the binding energies in the case of the impurity placed at the
quantum well center and at the quantum well edge is also given.
Received 16 February 1999 相似文献
7.
Qinghu Chen Yuhang Ren Zhengkuan Jiao Kelin Wang 《The European Physical Journal B - Condensed Matter and Complex Systems》1999,11(1):59-63
The Feynman-Haken variational path integral theory is, for the first time, generalized to calculate the ground-state energy
of an electron coupled simultaneously to a Coulomb potential and to a longitudinal-optical (LO) phonon field in parabolic
quantum wires. It is shown that the polaronic correction to the ground-state energy is more sensitive to the electron-phonon
coupling constant than the Coulomb binding parameter and monotonically stronger as the effective wire radius decreases. We
apply our calculations to several semiconductor quantum wires and find that the polaronic correction can be considerably large.
Received 16 November 1998 相似文献
8.
Q.-H Chen Y.-H. Ren Z.-K Jiao 《The European Physical Journal B - Condensed Matter and Complex Systems》1998,3(3):307-313
The general properties of one-dimensional large Fr?hlich polarons in motion are investigated with the previous extended coherent
states where two-phonon correlations are considered. As a result, the polaron energy, velocity, effective mass, and average
number of virtual phonons as a function the polaron total momentum are evaluated in a wide range of the coupling constant.
In addition, rich information about virtual phonons emitted by the electron in motion is obtained. More importantly, some
intrinsic features of 1D moving polarons are presented for the first time, which may also be suited to moving polarons in
more than one dimensions.
Received: 23 October 1997 / Revised and Accepted: 27 January 1998 相似文献
9.
V. D. Lakhno A. N. Korshunova 《The European Physical Journal B - Condensed Matter and Complex Systems》2007,55(1):85-87
This paper presents the results of numerical experiments
simulating Bloch oscillations of solitons in a deformable
molecular chain subject to a constant electric field. By using as an example a
homogeneous polynucleotide chain, it is shown that the system under
consideration can exhibit complicated dynamical behaviour: when
subject to field intensities less than a certain critical value, a
soliton exhibits oscillations as a whole, while at field
intensities exceeding this threshold, the soliton becomes a breather
that oscillates. It is shown that the motion of a charge in a
deformable chain is infinite, which in contrast to that in a rigid
chain. 相似文献
10.
R. Desquiotz M. Hofmann E. Dormann 《The European Physical Journal B - Condensed Matter and Complex Systems》2000,16(3):403-410
Conduction electron properties of the quasi-one-dimensional conductors and (PE = perylene, THF = tetrahydrofurane) were investigated by measuring magnetic susceptibility and microwave conductivity
in the temperature range from 10 K to 300 K. For quantitative analysis of the measurements a microscopic model was developed.
Received 23 November 1999 相似文献
11.
A. Carbone B. K. Kotowska D. Kotowski 《The European Physical Journal B - Condensed Matter and Complex Systems》2006,50(1-2):77-81
The f-γ sloped current noise power spectra, observed
in organic semiconductors, have been interpreted within a variable range hopping mechanism of the fluctuations. The
relative current noise power spectral density
exhibits a maximum
at the trap-filling transition
between the ohmic and the space-charge-limited-current
regime [Phys. Rev. Lett. 95, 236601 (2005)]. Here, we
discuss the electronic conditions determining the crossover from
ohmic to space-charge-limited transport. These arguments shed
light on the need to adopt a percolative fluctuation
picture to account for the competition between insulating and
conductive phases coexisting at the transition, where small
changes in the external bias lead to dramatic effects in the
fluctuations. 相似文献
12.
A bound polaron in a spherical quantum dot 总被引:12,自引:0,他引:12
H.-J. Xie C.-Y. Chen 《The European Physical Journal B - Condensed Matter and Complex Systems》1998,5(2):215-218
The binding energy of a bound polaron in a spherical quantum dot has been investigated by using the variational method. The
influence of LO and SO phonons have taken into consideration. Result shows that the phonon contribution to the binding energy
is dependent on the size of the quantum dot as well as the position of the impurity in the quantum dot. Numerical calculation
on the ZnSe quantum dot shows that such contribution is about 5% to 20% of the total binding energy.
Received: 13 October 1997 / Revised: 4 March 1998 / Accepted: 26 May 1998 相似文献
13.
W. Westerburg F. Martin P.J.M. van Bentum J.A.A.J. Perenboom G. Jakob 《The European Physical Journal B - Condensed Matter and Complex Systems》2000,14(3):509-513
We measured the temperature dependence of the linear high field Hall resistivity of ( K) and ( K) thin films in the temperature range from 4 K up to 360 K in magnetic fields up to 20 T. At low temperatures we find a
charge-carrier density of 1.3 and 1.4 holes per unit cell for the Ca- and Sr-doped compound, respectively. In this temperature
range electron-magnon scattering contributes to the longitudinal resistivity. At the ferromagnetic transition temperature
a dramatic drop in the number of charge-carriers n down to 0.6 holes per unit cell, accompanied by an increase in unit cell volume, is observed. Corrections of the Hall data
due to a non saturated magnetic state will lead a more pronounced charge-carrier density collapse.
Received 22 July 1999 and Received in final form 7 October 1999 相似文献
14.
J. Chatterjee M. Mitra A.N. Das 《The European Physical Journal B - Condensed Matter and Complex Systems》2000,18(4):573-578
A two-site double exchange model with a single polaron is studied using a perturbation expansion based on the modified Lang-Firsov
transformation. The antiferromagnetic to ferromagnetic transition and the crossover from small to large polaron are investigated
for different values of the antiferromagnetic interaction (J) between the core spins and the hopping (t) of the itinerant electron. Effect of the external magnetic field on the small to large polaron crossover and on the polaronic
kinetic energy are studied. When the magnetic transition and the small to large polaron crossover coincide for some suitable
range of J/t, the magnetic field has very pronounced effect on the dynamics of polarons.
Received 1 June 2000 相似文献
15.
P. Paci C. Grimaldi L. Pietronero 《The European Physical Journal B - Condensed Matter and Complex Systems》2000,13(2):235-243
The inclusion of nonadiabatic corrections to the electron-phonon interaction leads to a strong momentum dependence in the
generalized Eliashberg equations beyond Migdal's limit. For a s-wave symmetry of the order parameter, this induced momentum dependence leads to an enhancement of when small momentum transfer is dominant. Here we study how the d-wave symmetry affects the above behavior. We find that the nonadiabatic corrections depend only weakly on the symmetry of
the order parameter provided that only small momentum scatterings are allowed for the electron-phonon interaction. In this
situation, We show that also for a d-wave symmetry of the order parameter, the nonadiabatic corrections enhance . We also discuss the possible interplay and crossover between s- and d-wave depending on the material's parameters.
Received 12 May 2000 相似文献
16.
M. Dumm M. Dressel M. Nicklas P. Lunkenheimer A. Loidl M. Weiden F. Steglich B. Assmann H. Homborg P. Fulde 《The European Physical Journal B - Condensed Matter and Complex Systems》1998,6(3):317-322
The magnetic susceptibility, using dc and electron spin resonance (ESR) methods, the specific heat, and the infrared properties
of the one-dimensional molecular semiconductors lithium phthalocyanine (LiPc) and the iodinated compound LiPcI have been investigated
for temperatures K. LiPc has a half-filled conduction band and is expected to be an organic metal. However, due to the strong Coulomb repulsion
the system is a one-dimensional Mott-Hubbard insulator with a Hubbard gap of 0.75 eV as inferred from optical measurements.
The localized electrons along the molecular stacks behave like a S = 1/2 antiferromagnetic spin chain. The spin susceptibility, as determined by ESR experiments, and the magnetic contribution
to the heat capacity show a Bonner-Fisher type of behavior with an exchange constant K. LiPcI is an intrinsic narrow-gap semiconductor with an optical gap of 0.43 eV. In ESR experiments it is silent, indicating
that all the unpaired electrons have been removed from the macrocycle via doping with iodine.
Received: 16 June 1998 / Accepted: 14 July 1998 相似文献
17.
C. Buschhaus R. Desquiotz K. Eichhorn M. Hofmann K. Hümmer V. Illich M. Kelemen S. Tarragona Auga T. Wokrina A. Zitsch E. Dormann 《The European Physical Journal B - Condensed Matter and Complex Systems》1999,8(1):57-66
Crystal growth and X-ray structural analysis are reported for the new quasi-one-dimensional organic conductor perylene hexafluoroantimonate.
Due to deviation from exact 4:3 stoichiometry and anion-chain disorder the three-dimensional Peierls transition is suppressed
to temperatures below 30 K in spite of a molecular field transition temperature of 330 K. Anisotropy of the microwave conductivity
exceeds 3000:1 at room temperature. Curie paramagnetic defects with comparatively small electron spin resonance line width
predominate at low temperature. Thermally activated paramagnetic defects, giving rise to pronounced Overhauser shift, are
separated in the 30-100 K range. They are explained by neutral Perylene intra-stack defects, whose concentration can be reduced
by both aging and annealing. The angular and temperature dependence of the conduction electron spin resonance line is analysed
in detail, exhibiting the influence of intra-stack dipole interaction growing with temperature. Restricted diffusion of the
conduction electron spins with diffusion coefficient of about 6 cm2/s parallel to the stacking direction is detected by fixed gradient pulsed electron spin resonance at room temperature.
Received 17 July 1998 相似文献
18.
D. Rönnow L.F. Lastras-Martínez M. Cardona 《The European Physical Journal B - Condensed Matter and Complex Systems》1998,5(1):29-35
Within the past years the optical excitations of electrons have been measured for semiconductor samples of different isotope
compositions. The isotope shift observed have been compared with calculations of the effects of electron-phonon interaction
on the electronic band structure. While qualitative agreement has been obtained, some discrepancies remain especially concerning
the E1 and transitions. We have remeasured the effect of isotope mass on the E1 and transitions of germanium with several isotopic compositions. The results, obtained by means of spectroscopic ellipsometry,
confirm that the real part of the gap self-energies induced by electron-phonon interaction is larger than found from band
structure calculations, while the imaginary part agrees with those calculations, which are based on a pseudopotential band
structure and a bond charge model for the lattice dynamics. Our results agree with predictions based on the measured temperature
dependence of the gaps. We compare our data for E1 and with results for the lowest direct (E0) and indirect (Eg) gaps. The measured values of and increase noticeably with increasing isotope mass. Similar effects have been observed in the temperature dependence of in and . A microscopic explanation for this effect is not available.
Received: 6 March 1998 / Revised: 27 April 1998 /
Accepted: 15 May 1998 相似文献
19.
L. Lanotte G. Ausanio V. Iannotti G. Pepe G. Carotenuto L. Nicolais 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,21(4):485-489
A composite material of a polyethylene matrix filled by a fine silver powder was prepared with different Ag contents and physical
behaviours ranging from insulator to conductor. Ac differential magnetic susceptibility χ measurements show the samples are
paramagnetic up to an Ag concentration of ∼65%. At low temperatures the composite is spin-glass type, whereas the transition
from insulator to conductor corresponds to an abatement of χ at zero magnetizing field. Magneto-conductivity effects have
been observed in resistivity measurements at low temperatures. They can be explained in terms of an effective exchange electronic
scattering mechanism between the conduction electrons and the diluted magnetic moments arising from unpaired electron spins
of boundary silver particles. Moreover, the presence of a broad minimum in the resistivity curve at T = ∼ 20 K, observed in samples with an Ag concentration just above the percolation threshold, addresses to possible interference
effects similar to those reported in disordered materials.
Received 17 October 2000 and Received in final form 22 February 2001 相似文献
20.
Interface polarons in a realistic heterojunction potential 总被引:9,自引:0,他引:9
S.L. Ban J.E. Hasbun 《The European Physical Journal B - Condensed Matter and Complex Systems》1999,8(3):453-461
The ground states of interface polarons in a realistic heterojunction potential are investigated by considering the bulk and
the interface optical phonon influence. A self-consistent heterojunction potential is used and an LLP-like method is adopted
to obtain the polaron effect. The numerical computation has been done for the Zn1-xCdxSe/ZnSe system to obtain the polaron ground state energy, self energy and effective mass parallel to the interface. A simplified
coherent potential approximation is developed to obtain the parameters of the ternary mixed crystal and the energy band offset
of the heterojunction. It is found that at small Cd concentration the bulk longitudinal optical phonons give the main contribution
for lower areal electron densities, whereas the interface phonon contribution is dominant for higher areal electron densities.
The interface polaron effect is weaker than the effect obtained by the three dimensional bulk phonon and by the two dimensional
interface phonon models.
Received 17 September 1998 相似文献