Helicoidal distributed-feedback cavity action in a ferroelectric liquid crystal

Second-Harmonic (SH) generation was observed in homeotropically aligned ferroelectric liquid-crystal cells using fundamental light propagating along the helicoidal axis. Relatively strong SH light was observed in the helicoidal structure when the optical pitch was nearly the same as the SH-light wavelength, though, otherwise, the cancellation of the generated SH light by the helicoid results in negligibly weak SH intensity. Because the observed SH light is independent of the cell thickness, the SH light is attributed to the one generated from the surface region and the SH light generated inside the cell is confined and lost by the helicoid. This phenomenon indicates the helicoidal Distributed-FeedBack (DFB) cavity action and suggests the possibility of the helicoidal DFB laser using dye-doped ferroelectric liquid-crystal cells.     

Direct observation of localized second-harmonic enhancement in random metal nanostructures

Second harmonic (SH) scanning optical microscopy in reflection is used to image the gold film surface covered with randomly placed scatterers. SH images obtained with a tightly focused tunable (750-830 nm) laser beam show small (approximately 0.7 microm) and very bright (approximately 10(3) times the background) spots, whose locations depend on the wavelength and polarization of light. Comparing SH and fundamental harmonic (FH) images, we conclude that the localized SH enhancement occurs due to the overlap of FH and SH eigenmodes. The probability density function of the SH signal is found to follow the power-law dependence.     

Phase-coherent optical frequency division by 3 of 532-nm laser light with a continuous-wave optical parametric oscillator

Phase-locked 3:1 division of an optical frequency was achieved with a continuous-wave monolithic optical parametric oscillator (OPO) pumped by a 532-nm Nd:YAG laser, by use of 5% MgO-doped LiNbO(3) as a nonlinear optical crystal. The OPO generated signal light (798 nm) with 4-mW power and idler light (1596 nm) with 3-mW power for a pump power of 68 mW. Approximately 2microW of second harmonics (SH's) of the idler light was produced by external-cavity-enhanced SH generation by use of a periodically poled LiNbO(3) crystal. The beat signal between the signal light and the SH of the idler light was observed with a signal-to-noise ratio of 40 dB at a 10-kHz bandwidth and was successfully phase locked to a signal from a synthesizer through the electro-optic effect of the crystal.     

Nanoscale nonlinear optical process: theoretical modeling of second-harmonic generation for both forbidden and allowed light

Based on a combination of the multiple-multipole method and nonlinear coupled-wave equations, a rigorous three-dimensional numerical simulation of nonlinear optical interactions between an optical near field and a nonlinear medium is performed, allowing us to study the dependence of second-harmonic (SH) near-field intensity on tip-sample distance and the polarization state of the incident fundamental wave. It is demonstrated that allowed and forbidden light make different contributions to the SH near-field intensity.     

A simple monitoring system for single subpicosecond laser pulses using an SH spatial autocorrelation method and a CCD image sensor

A simple noncollinear SHG autocorrelator for monitoring the time behavior of single subpicosecond laser pulses is described. A new CCD image-line sensor with high sensitivity in the UV range is used to measure the second-harmonic (SH) spatial distribution which gives information on the duration of the fundamental light pulses. An input energy of only 10 μJ is enough to obtain the SH spatial beam patterns in this highly sensitive autocorrelation system.     

Second harmonic generation in Ga nanoparticle monolayers

Ga nanoparticle monolayers formed by evaporation-condensation in ultrahigh vacuum and embedded in a transparent SiO_x matrix generate second harmonic (SH) signals in transmission and reflection when illuminated by a 150 fs, 800 nm laser pulses. The observed SH light exhibits a critical dependence on input and output polarizations, angle of incidence and azimuthal orientation of the samples. The results lead to a consistent picture of shape and orientation of the nanoparticles. Linear transmittance spectra in the visible range support these findings and the observed size dependence of the SH signal. Received 29 November 2000     

Spectral domain second-harmonic optical coherence tomography

Optical coherence tomography (OCT) provides micrometer-scale structural imaging by coherent detection of backscattered light. Molecular contrast in OCT has been demonstrated using transient absorption, coherent anti-Stokes Raman scattering, and second-harmonic (SH) generation. The sensitivity of molecular contrast signals can be enhanced by use of Fourier domain techniques. We have constructed a spectrometer-based Fourier domain SH-OCT system for simultaneous acquisition of the fundamental and SH signals. We report a >30 dB increase in SH sensitivity over a similar time domain SH-OCT system and demonstrate contrast between cartilage and bone using collagen as the contrast agent.     

Generation of reflected second-harmonic light beam with inhomogeneous transversal distribution of polarization from the surface of chiral medium by normally incident Gaussian beam

A principle possibility of second harmonic generation (SHG) from the surface of a chiral medium by normally incident focused fundamental beam has been shown earlier, and the key features of this phenomenon (forbidden in a planewave approximation) have been outlined in [N.I. Koroteev, V.A. Makarov, S.N. Volkov, Laser Phys. 8 (1998) 532-535]. In our work we have obtained analytical expressions, which describe the distributions of intensity and polarization in the cross-section of a second-harmonic (SH) light beam. It is found that the polarization state drastically changes along the cross-section of the signal light beam. The polarization effects concerning the transversal inhomogeneous polarization distribution were studied in detail. It is shown that the measurement of the polarization state in certain areas of the SH beam cross-section gives us quantitative information directly about the medium material constants.     

Second-Harmonic Generation by a Monolayer of Spherical Two-Layer Nanoparticles

Optics and Spectroscopy - A model for calculating the second-harmonic (SH) intensity at reflection of light from a monolayer of spherical nanoparticles consisting of a dielectric core and a...     

Rotational anisotropy in second harmonic intensity from Cu nanowire arrays on the NaCl (1 1 0) substrates

We have measured the azimuthal angle dependence of the second harmonic (SH) intensity from Cu nanowires on the faceted NaCl (1 1 0) substrates in air at the fundamental photon energy of 1.17 eV. The SH intensity patterns showed two main lobes for p-in/p-out, s-in/p-out, and s-in/s-out polarization configurations. From the results of the experiment and the pattern analysis we have found that the observed SH light is enhanced by the electric field components along the substrate normal.     

Effects of high intensity unltrasound on structural and physicochemical properties of myosin from silver carp

Myosin from silver carp was sonicated with varying power output (100, 150, 200 and 250 W) for 3, 6, 9, and 12 min. The changes in the structure and physicochemical properties of myosin were evaluated by dynamic light scattering, SDS-PAGE and some physicochemical indexes. The ultrasound treatments induced a significant conversion of myosin aggregates to smaller ones with a more uniform distribution, and obvious enhancement in solubility. The structure of myosin was also notably changed by sonication, with a decrease in Ca²⁺-ATPase activity and SH content, and an increase in surface hydrophobicity. Furthermore, SH groups were oxidized, leading to a decrease in reactive SH and total SH contents. SDS-PAGE analysis revealed that ultrasound could induce the degradation of myosin heavy chain and change the protein fraction of myosin. Collectively, the ultrasonic treatment of 100 W for 3 min showed slight influence on the SH content, S₀-ANS, and electrophoretic patterns, and the extent of changes in myosin structure and physicochemical properties tended to increase with ultrasonic power and time. The integrated data indicate that ultrasonic treatment can facilitate the improvement of the solubility and dispersion of myosin, but the choice of a suitable ultrasonic condition to avoid oxidation and degradation of myosin is very important.     

Simultaneous optical second harmonic and sum frequency intensity image observation of hydrogen deficiency on a H-Si(1 1 1) 1 × 1 surface after IR light pulse irradiation

In this study, we developed a microscope for the simultaneous acquisition of optical sum frequency (SF) and second harmonic (SH) intensity images in UHV conditions, and observed resonant electronic and vibrational images of the H-Si(1 1 1) surface after IR light irradiation of pulse width ∼6 μs. The SH intensity images showed a spatial distribution of resonant electronic states, associated with the dangling bonds formed after hydrogen desorption induced by the IR light pulses. This result indicates that the hydrogen coverage decreased to less than ∼0.6 ML in the irradiated area. The SF intensity images before the IR light pulse irradiation showed signals attributed to Si-H stretching vibration on the H-Si(1 1 1) surface. After the IR light pulse irradiation, non-resonant SF signals appeared in the irradiated area. The non-resonant SF signals may originate from a nonlinear optical transition involving the surface electronic levels in the dangling bonds. We also found an unidentified bonding state on the edges of the irradiated area in some light conditions. Both the resonant and non-resonant signals were very weak in this area.     

Intensity modulation on polarization coupling and frequency conversion in periodically poled lithium niobate

Based on cascaded polarization coupling and frequency doubling, we present a scheme to modulate the polarization and intensity of light in periodically poled lithium niobate. In the coupled processes, the introduction of another pump (control light) results in energy redistribution among the optical waves. Numerical results indicate that polarization of the fundamental wave and magnitude of the second harmonic (SH) can be both modulated by adjusting the intensity of control light. This result would be useful when simultaneous signal tuning and frequency conversion are desired.     

Theoretical Study on Intra-Cavity Distributed-Bragg-Reflection Quasi-Phase-Matched Second-Harmonic Lasers

The characteristics of intra-cavity distributed Bragg reflector (DBR) quasi-phase-matched (IDQPM) second-harmonic-generation (SHG) lasers are theoretically studied. In the IDQPM-SHG laser, a QPM device and a DBR for feedback are separately fabricated on the same substrate with the QPM device placed between the DBR and a semiconductor laser. The threshold current of the IDQPM-SHG laser depends on the coupling efficiency between the laser diode and the QPM waveguide and the reflectivity of the DBR. The SH output of the IDQPM-SHG laser is strongly dependent on the generalized SHG conversion efficiency, x. This laser has the potential to attain an SH output over a 30-mW using a currently available 50-mW semiconductor laser for the fundamental light source, when highly efficient QPM device (x=2.2 W⁻¹) is used. Its tolerance for various deviations from the initial design and the problems to develop a commercially available IDQPM-SHG laser are also discussed.     

High-power,blue-light generation in a dual-structure,periodically poled,stoichiometric LiTaO<Subscript>3</Subscript> crystal

High-power blue light was generated from a diode-side-pumped Q-switched 1319 nm Nd:YAG laser with a periodically poled, stoichiometric LiTaO₃ (PPSLT) crystal. The PPSLT sample used in this experiment consists of two segments in series: the first segment has a period of 14.08 μm for the second harmonic generation (SHG) and the second segment has periods of around 4.6 μm for the generation of blue light by mixing fundamental and SH. An average power of 466 mW of a 440 nm blue light was obtained at the fundamental power of ∼5.4 W with a conversion efficiency of 8.6%. The output power fluctuated by 3% over a half-hour period. This result indicates that our scheme is a practical method to construct a reliable compact blue laser. PACS 42.70.Mp; 42.79.Nv; 42.55.Xi     

Single SH guided wave mode generation method for PPM EMATs

Using periodic permanent magnet(PPM) electromagnetic acoustic transducers(EMATs), different shear horizontal(SH) guided wave modes can form simultaneously in some situations, which can interfere with the inspection. The main cause of this phenomenon(typically named multiple modes) is related to the frequency bandwidth of excitation signals and the transducer spatial bandwidth. Simply narrowing the frequency bandwidth cannot effectively limit the number of different SH modes. Previous researches showed that unnecessary SH wave modes can be eliminated by using dual EMATs.However, in practical applications, it is more convenient to change the excitation frequency than to use dual EMATs. In this paper, the stress boundary conditions of the PPM-EMAT are analyzed, the analytical expression of SH guided wave is established, and the magnitude of SH guided wave mode under continuous tone and tone-burst input is obtained. A method to generate a single SH mode by re-selecting an operating point is proposed. Furthermore, the influence of the frequency bandwidth of the tone-burst signal is analyzed. Finally, a single SH mode excitation is achieved with tone-burst input.     

Second-harmonic interferometric spectroscopy of buried interfaces of column IV semiconductors

The technique of combined optical second-harmonic (SH) intensity and phase spectroscopy, which is the spectroscopic modification of SH phase measurements, is proposed to study the nonlinear optical response of semiconductor interfaces with spectrally close resonant contributions. The spectral dependences of SH intensity and phase from oxidised Si (111) and Ge (111) surfaces are studied in the range of 3.5- to 5-eV SH photon energy. The resonant behaviour of combined SH spectra is associated with a superposition of contributions from direct interband transitions at several critical points of Si and Ge band structures. Received: 16 October 2001 / Revised version: 16 April 2002 / Published online: 6 June 2002     

固体板中SH板波非线性效应的实验观察

采用微扰近似和导波的模式展开分析方法,从理论上简要分析了SH板波的二次谐波发生效应;尽管在无限大固体介质中单个切变波的二次谐波发生效应非常微弱,但在一定条件下由两个切变波构成的SH板波可具有强烈的非线性效应;本文的主要工作就是对此结论加以实验验证。试制了激发SH板波的切变波斜劈换能器和接收二次谐波信号的液体斜劈换能器,建立了非线性SH板波的实验研究系统;通过详细的理论分析和对比实验研究,阐明了在一定条件下实验观察到的显著二次谐波信号来源于SH板波传播过程中的强烈非线性效应。此外,针对不同的SH板波传播距离,在远场条件下分别测量了相应的二次谐波幅频曲线;在基频SH板波与二倍频对称兰姆波相速度相等所对应的频率值附近,分析了二次谐波的振幅随传播距离的变化关系,结果证明在一定条件下SH板波的二次谐波振幅可随传播距离积累增长,即SH板波可具有强烈的非线性效应。     

Shear horizontal surface waves on piezoelectric ceramic with layered structure

This paper presents theoretical and experimental results describing the propagation of SH (shear, horizontal) surface waves on a piezoelectric ceramic with a surface layer of different polarization than that in the substrate. An analytical formula for the group velocity of the SH surface waves is developed. The velocity of impulses of the SH surface waves is determined experimentally. Further, the theoretical results are compared to the experimental values.     

Propagation of second-harmonic wave in quasi-phase-matching nonlinear medium

We studied the propagation of the second-harmonic (SH) wave in a quasi-phase-matching (QPM) medium with a slanted nonlinear grating. By solving the electromagnetic boundary value problem for the SH wave, we derived the propagation law for the SH wave, which can be interpreted as a diffraction phenomenon. Such interpretation was supported by a series of SH generation experiments with a periodically-poled lithium niobate crystal with a slanted QPM grating.