Transport through artificial single-molecule magnets: Spin-pair state sequential tunneling and Kondo effects

The transport properties of an artificial single-molecule magnet based on a CdTe quantum dot doped with a single Mn+2 ion(S=5/2) are investigated by the non-equilibrium Green function method.We consider a minimal model where the Mn-hole exchange coupling is strongly anisotropic so that spin-flip is suppressed and the impurity spin S and a hole spin s entering the quantum dot are coupled into spin pair states with(2S+1) sublevels.In the sequential tunneling regime,the differential conductance exhibits(2S+1) possible peaks,corresponding to resonance tunneling via(2S+1) sublevels.At low temperature,Kondo physics dominates transport and(2S+1) Kondo peaks occur in the local density of states and conductance.These peaks originate from the spin-singlet state formed by the holes in the leads and on the dot via higher-order processes and are related to the parallel and antiparallel spin pair states.     

Nonequilibrium spintronic transport through an artificial Kondo impurity: conductance,magnetoresistance, and shot noise

We investigate the nonequilibrium transport properties of a quantum dot when spin flip processes compete with the formation of a Kondo resonance in the presence of ferromagnetic leads. Based upon the Anderson Hamiltonian in the strongly interacting limit, we predict a splitting of the differential conductance when the spin flip scattering amplitude is of the order of the Kondo temperature. We discuss how the relative orientation of the lead magnetizations strongly influences the electronic current and the shot noise in a nontrivial way. Furthermore, we find that the zero-bias tunneling magnetoresistance becomes negative with increasing spin flip scattering amplitude.     

Nonequilibrium Keldysh formalism for interacting leads—Application to quantum dot transport driven by spin bias

The conductance through a mesoscopic system of interacting electrons coupled to two adjacent leads is conventionally derived via the Keldysh nonequilibrium Green’s function technique, in the limit of noninteracting leads [Y. Meir, N.S. Wingreen, Phys. Rev. Lett. 68 (1992) 2512]. We extend the standard formalism to cater for a quantum dot system with Coulombic interactions between the quantum dot and the leads. The general current expression is obtained by considering the equation of motion of the time-ordered Green’s function of the system. The nonequilibrium effects of the interacting leads are then incorporated by determining the contour-ordered Green’s function over the Keldysh loop and applying Langreth’s theorem. The dot–lead interactions significantly increase the height of the Kondo peaks in density of states of the quantum dot. This translates into two Kondo peaks in the spin differential conductance when the magnitude of the spin bias equals that of the Zeeman splitting. There also exists a plateau in the charge differential conductance due to the combined effect of spin bias and the Zeeman splitting. The low-bias conductance plateau with sharp edges is also a characteristic of the Kondo effect. The conductance plateau disappears for the case of asymmetric dot–lead interaction.     

Spin-Polarized Transport Through a Quantum Dot Coupled to Ferromagnetic Leads:Kondo Correlation Effect

We investigate the linear and nonlinear transport through a single level quantum dot connected to two ferromagnetic leads in Kondo regime, using the slave-boson mean-field approach for finite on-site Coulomb repulsion. We find that for antiparallel alignment of the spin orientations in the leads, a single zero-bias Kondo peak always appears in the voltage-dependent differential conductance with peak height going down to zero as the polarization grows to P=1. For parallel configuration, with increasing polarization from zero, the Kondo peak descends and greatly widens with the appearance of shoulders, and finally splits into two peaks on both sides of the bias voltage around P～0.7 until disappearing at even larger polarization strength. At any spin orientation angle θ, the linear conductance generally drops with growing polarization strength. For a given finite polarization, the minimum linear conductance always appears at θ=π.     

Interaction-driven spin precession in quantum-dot spin valves

We analyze spin-dependent transport through spin valves composed of an interacting quantum dot coupled to two ferromagnetic leads. The spin on the quantum dot and the linear conductance as a function of the relative angle theta of the leads' magnetization directions is derived to lowest order in the dot-lead coupling strength. Because of the applied bias voltage spin accumulates on the quantum dot, which for finite charging energy experiences a torque, resulting in spin precession. The latter leads to a nontrivial, interaction-dependent, theta dependence of the conductance. In particular, we find that the spin-valve effect is reduced for all theta not equal pi.     

Kondo effect in quantum dots coupled to ferromagnetic leads

We study the Kondo effect in a quantum dot coupled to ferromagnetic leads and analyze its properties as a function of the spin polarization of the leads. Based on a scaling approach, we predict that for parallel alignment of the magnetizations in the leads the strong-coupling limit of the Kondo effect is reached at a finite value of the magnetic field. Using an equation of motion technique, we study nonlinear transport through the dot. For parallel alignment, the zero-bias anomaly may be split even in the absence of an external magnetic field. For antiparallel spin alignment and symmetric coupling, the peak is split only in the presence of a magnetic field, but shows a characteristic asymmetry in amplitude and position.     

Quantum Phase Transition and Ferromagnetic Spin Correlation in Parallel Double Quantum Dots

We investigate electronic transport through a parallel double quantum dot （DQD） system with strong on-site Coulomb interaction, as well as the interdot tunnelling. By applying numerical renormalization group method, the ground state of the system and the transmission probability at zero temperature are obtained. For a system of quantum dots with degenerate energy levels and small interdot tunnel coupling, the spin correlations between the DQDs is ferromagnetic, and the ground state of the system is a spin-1 triplet state. The linear conductance will reach the unitary limit （2e^2/h） due to the Kondo effect at low temperature. As the interdot tunnel coupling increases, there is a quantum phase transition from ferromagnetic to anti-ferromagnetic spin correlation in DQDs and the linear conductance is strongly suppressed.     

Multipeak Kondo effect in one- and two-electron quantum dots

We have fabricated a few-electron quantum dot that can be tuned down to zero electrons while maintaining strong coupling to the leads. Using a nearby quantum point contact as a charge sensor, we can determine the absolute number of electrons in the quantum dot. We find several sharp peaks in the differential conductance, occurring at both zero and finite source-drain bias, for the one- and two-electron quantum dot. We attribute the peaks at finite bias to a Kondo effect through excited states of the quantum dot and investigate the magnetic field dependence of these Kondo resonances.     

Kondo effect in the presence of itinerant-electron ferromagnetism studied with the numerical renormalization group method

The Kondo effect in quantum dots (QDs)-artificial magnetic impurities-attached to ferromagnetic leads is studied with the numerical renormalization group method. It is shown that the QD level is spin split due to the presence of ferromagnetic electrodes, leading to a suppression of the Kondo effect. We find that the Kondo effect can be restored by compensating this splitting with a magnetic field. Although the resulting Kondo resonance then has an unusual spin asymmetry with a reduced Kondo temperature, the ground state is still a locally screened state, describable by Fermi liquid theory and a generalized Friedel sum rule, and transport at zero temperature is spin independent.     

Kondo effect in the presence of magnetic impurities

We measure transport through gold grain quantum dots fabricated using electromigration, with magnetic impurities in the leads. A Kondo interaction is observed between dot and leads, but the presence of magnetic impurities results in a gate-dependent zero-bias conductance peak that is split due to a RKKY interaction between the spin of the dot and the static spins of the impurities. A magnetic field restores the single Kondo peak in the case of an antiferromagnetic RKKY interaction. This system provides a new platform to study Kondo and RKKY interactions in metals at the level of a single spin.     

Reprint of : Kondo effect in a carbon nanotube with spin–orbit interaction and valley mixing: A DM-NRG study

We investigate the effects of spin–orbit interaction (SOI) and valley mixing on the transport and dynamical properties of a carbon nanotube (CNT) quantum dot in the Kondo regime. As these perturbations break the pseudo-spin symmetry in the CNT spectrum but preserve time-reversal symmetry, they induce a finite splitting $\Delta$ between formerly degenerate Kramers pairs. Correspondingly, a crossover from the SU(4) to the SU(2)-Kondo effect occurs as the strength of these symmetry breaking parameters is varied. Clear signatures of the crossover are discussed both at the level of the spectral function as well as of the conductance. In particular, we demonstrate numerically and support with scaling arguments that the Kondo temperature scales inversely with the splitting $\Delta$ in the crossover regime. In presence of a finite magnetic field, time reversal symmetry is also broken. We investigate the effects of both parallel and perpendicular fields (with respect to the tube's axis) and discuss the conditions under which Kondo revivals may be achieved.     

Spin filters with Fano dots

We compute the zero bias conductance of electrons through a single ballistic channel weakly coupled to a side quantum dot with Coulomb interaction. In contrast to the standard setup which is designed to measure the transport through the dot, the channel conductance reveals Coulomb blockade dips rather then peaks due to the Fano-like backscattering. At zero temperature the Kondo effect leads to the formation of broad valleys of small conductance corresponding to an odd number of electrons on the dot. By applying a magnetic field in the dot region we find two dips corresponding to a total suppression in the conductance of spins up and down separated by an energy of the order of the Coulomb interaction. This provides a possibility of a perfect spin filter.Received: 6 November 2003, Published online: 2 April 2004PACS: 72.15.Qm Scattering mechanisms and Kondo effect - 73.23.Ad Ballistic transport - 72.25.-b Spin polarized transport     

Transport through quantum dots in mesoscopic circuits

We study the transport through a quantum dot, in the Kondo Coulomb blockade valley, embedded in a mesoscopic device with finite wires. The quantization of states in the circuit that hosts the quantum dot gives rise to finite size effects. These effects make the conductance sensitive to the ratio of the Kondo screening length to the wires length and provide a way of measuring the Kondo cloud. We present results obtained with the numerical renormalization group for a wide range of physically accessible parameters.     

Transport through a quantum dot subject to spin and charge bias

Spin and charge transport through a quantum dot coupled to external nonmagnetic leads is analyzed theoretically in terms of the non-equilibrium Green function formalism based on the equation of motion method. The dot is assumed to be subject to spin and charge bias, and the considerations are focused on the Kondo effect in spin and charge transport. It is shown that the differential spin conductance as a function of spin bias reveals a typical zero-bias Kondo anomaly which becomes split when either magnetic field or charge bias are applied. Significantly different behavior is found for mixed charge/spin conductance. The influence of electron-phonon coupling in the dot on tunneling current as well as on both spin and charge conductance is also analyzed.     

Ferromagnetically coupled magnetic impurities in a quantum point contact

We investigate the ground and excited states of interacting electrons in a quantum point contact using an exact diagonalization method. We find that strongly localized states in the point contact appear when a new transverse conductance channel opens and longitudinal resonant level is formed due to momentum mismatch. These localized states form magnetic impurity states which are stable in a finite regime of chemical potential and excitation energy. Interestingly, these magnetic impurities have ferromagnetic coupling, which sheds light on the experimentally observed puzzling coexistence of Kondo correlation and spin filtering in a quantum point contact.     

Tunable Kondo effect in a double quantum dot coupled to ferromagnetic contacts

We investigate the effects induced by ferromagnetic contacts attached to a serial double quantum dot. Spin polarization generates effective magnetic fields and suppresses the Kondo effect in each dot. The superexchange interaction J(AFM), tuned by the interdot tunneling rate t, can be used to compensate the effective fields and restore the Kondo resonance when the contact polarizations are aligned. As a consequence, the direction of the spin conductance can be controlled and even reversed using electrostatic gates alone. Our results demonstrate a new approach for controlling spin-dependent transport in carbon nanotube double dot devices.     

Observation of the Kondo effect in a spin-3/2 hole quantum dot

We report the observation of Kondo physics in a spin-3/2 hole quantum dot. The dot is formed close to pinch-off in a hole quantum wire defined in an undoped AlGaAs/GaAs heterostructure. We clearly observe two distinctive hallmarks of quantum dot Kondo physics. First, the Zeeman spin splitting of the zero-bias peak in the differential conductance is independent of the gate voltage. Second, this splitting is twice as large as the splitting for the lowest one-dimensional subband. We show that the Zeeman splitting of the zero-bias peak is highly anisotropic and attribute this to the strong spin-orbit interaction for holes in GaAs.     

Inelastic Cotunneling Current and Shot Noise of an Interacting Quantum Dot with Ferromagnetic Correlations

We explore inelastic cotunneling through a strongly Coulomb-blockaded quantum dot attached to two ferromagnetic leads in the weak coupling limit using a generic quantum Langevin equation approach. We first develop a Bloch-type equation microscopically to describe the cotunneling-induced spin relaxation dynamics, and then develop explicit analytical expressions for the local magnetization, current, and its fluctuations. On this basis, we predict a novel zero-bias anomaly of the differential conductance in the absence of a magnetic field for the anti-parallel configuration, and asymmetric peak splitting in a magnetic field. Also, for the same system with large polarization, we find a negative zero-frequency differential shot noise in the low positive bias-voltage region. All these effects are ascribed to rapid spin-reversal due to underlying spin-flip cotunneling.     

Influence of intradot Coulomb correlations on the Andreev reflection in a ferromagnetic metal/quantum dot/superconductor hybrid junction

Spin-dependent tunneling through a quantum dot coupled to one ferromagnetic and onesuperconducting electrodes is studied in the Andreev reflection (AR) regime. Electricalconductance is calculated within the nonequilibrium Green function technique. Features ofthe AR current involved by the intradot Coulomb correlations (or the dot’s chargingenergy U) and in the presence of the Zeeman splitting of the dotdiscrete level are analyzed in both linear and nonlinear transport regimes. A newinterference effect due to AR is predicted to appear in the case of a weak on-dotrepulsion. Strong Coulomb correlations studied in nonequilibrium situation revealedsignificant modifications of the AR differential conductance occurring only in case ofspin-polarized transmission. Origin of a variety of the multipeak structure of theconductance for the system with the interacting quantum dot, as well as the conditions forthe perfect U-dependent AR transmission are also discussed.