Plasmonic emission and plasma lattice structures induced by pulsed laser in Purcell cavity on silicon

The lattice structure image of a plasma standing wave in a Purcell cavity of silicon is observed. The plasma wave produced by the pulsed laser could be used to fabricate the micro-nanostructure of silicon. The plasma lattice structures induced by the nanosecond pulsed laser in the cavity may be similar to the Wigner crystal structure. It is interesting that the beautiful diffraction pattern could be observed in the plasma lattice structure. The radiation lifetime could be shortened to the nanosecond range throughout the entire spectral range and the relaxation time could be lengthened for higher emission efficiency in the Purcell cavity, which results in the fact that the plasmonic emission is stronger and its threshold is lower.     

光子晶体垂直腔面发射850nm波长激光器研究

文章报道了国内首次研制成功的光子晶体垂直腔面发射850nm波长激光器, 实现了连续电注入激射.发现器件能否激射直接依赖于光子晶体结构参数,而激光器的阈值、输出功率、输出模式等与光子晶体的晶格常数、占空比、腔的大小等因素有关.     

Laser systems specialized for laser spectroscopy at storage rings

Laser spectroscopy at storage rings often suffers from a limited resolution due to Doppler-broadened resonances. Broadening is caused by the velocity spread of the ions stored in the beam. In the following, the present status of our work on laser systems specialized on the specific needs of laser spectroscopy at storage rings is reported. Two pulsed laser systems were developed. One is a dye laser whose spectral bandwidth can be switched by inserting different Littrow-prisms into the resonator. An increase in bandwidth up to a factor of 45 was achieved. This laser was used for fast qualitative scans and high resolution measurements. The other laser system is a Nd : YAG laser pumped optical parametric oscillator. It is a tunable laser system covering the spectral range from 410 to 4000 nm. Furthermore, a continuous wave laser with a frequency shifted feedback cavity is described. It shows broadband emission with an adjustable bandwidth of up to 4.5 GHz. This laser can be advantageous for laser cooling of ion beams. This revised version was published online in August 2006 with corrections to the Cover Date.     

Improving the emission efficiency of periodic plasmonic structures for lasing applications

We report on a two dimensional plasmonic structure that utilizes an Ag film for the generation of surface plasmons and a layer of the organic semiconductor tri(8-hydroxyquinoline) aluminum (Alq₃) doped with the laser dye 4-dicyanmethylene-2-methyl-6-(p-dimethylaminostyryl)-4 H-pyran (DCM) as an active medium. The dispersion diagram of this structure exhibits a plasmonic bandgap in the dye emission wavelength range. At the flat band-edge, the group velocity tends to zero, so that the density of surface plasmon modes is high. This may yield a lasing action. However, the device suffers from the energy dissipation due to metal absorption and unwanted radiation. We examine how some of them may be overcome. Firstly, we propose the use of long range surface plasmons (LRSPs) characterized by a low loss coefficient. To this end, we investigate theoretically and experimentally the best conditions for the excitation of these modes. A strong emission is observed compared to that from a planar structure. These modes provide a high performance-an enhancement factor of 3-when the dye thickness is about 100 nm, a value consistent with the numerical findings. We further demonstrate that the use of a spacer layer significantly increases the emission efficiency. Finally, we suggest a specific design for the laser structure for minimal radiation loss.     

UV-Laser Ablation Spectroscopy in Element Analysis of Solid Surface

Laser ablation for the atomic emission spectroscopy of a glass sample is studied using pulsed UV laser systems and the effect of the laser wavelength is investigated. The threshold fluence for ablation is decreased and the detection sensitivity is improved for shorter wavelengths. Furthermore, very thin (less than 1 nm/shot) surface slicing is possible at a wavelength as short as 193 nm. Polymers also show good ablation characteristics. Improvement of sensitivity and spatial resolution by using shorter wavelength laser ablation is discussed for Na detection in a glass sample.     

TiO2∶Mo体系的光子雪崩上转换

在978nm激光二极管的激发下，Mo掺杂的TiO₂材料表现出很强的宽带上转换发光 ，该发光来源于［MoO₄］^2-基团的激发态³T₁, ³T₂能级到基态¹A₁能级的电子跃迁.通过研究发光强度与抽运功率的关系及上转换发光的上升时间曲线，发现TiO₂∶Mo体系的上转换发光中存在着雪崩机制，应用转 关键词： 上转换 光子雪崩 转移函数理论     

Role of nitrogen and oxygen in emission of Si quantum dots formed by pulse laser

Silicon quantum dots fabricated by nanosecond pulsed laser in nitrogen, oxygen or air atmosphere have enhanced photoluminescence (PL) emission with the stimulated emission observed at about 700 nm. It is difficult to distinguish between the photoluminescence peaks emitted from samples prepared in different atmospheres. The reason for the appearance of similar peaks may be the similar distribution of the localised states in the gap for different samples when silicon dangling bonds of quantum dots are passivated by nitrogen or oxygen. It is revealed that both the kind and the density of passivated bonds on quantum dot surface prepared in oxygen or nitrogen have a strong influence on the enhancement of PL emission.     

Experimental investigation of the impact on nearby solid boundary during laser-generated bubble collapse

Cavitation damage has been considered as being responsible for many effects in hydraulic machinery and biological medicine. In order to better understand the cavity interaction with nearby solid surfaces, the impact loading induced by the high-speed liquid-jet and subsequent jet flow during the final stage of the bubble collapse in a static fluid is investigated by focusing a Q-switched pulsed laser into water. By means of a new method based on a fibre-coupling optical beam deflection technique, a detailed experimental study has been made to clarify the relationship of the impact pressure against a solid boundary as a function of the dimensionless γ that is generally used to describe the bubble dynamics with its definition γ= s/R_{max}(R_{max} being the maximum bubble radius and s denoting the distance of the cavity inception from the boundary). The experimental results are shown that for γ in the range of about 0.67 to 0.95 with a pulsed laser energy 230mJ, the transient pressure applied on the solid surface is maximum; while for γ>1 or γ<0.67, it is gradually decreased. By combination of our experimental results with the other work that detected the acoustic emission during the bubble collapse at different γ, it is concluded that in this range of 0.67－0.95, the destructive effect due to a liquid-jet and the following jet flow impact actually outweighs the well-known effect of shock wave emission and plays a vital role during the cavitation bubble collapse.     

带有多孔二氧化硅间隔层的导模共振光栅实现染料激光器发射增强

导模共振光栅是一种典型的平面波导共振结构,可在光栅表面或波导层内形成较强的局域电场,能增强光与物质的相互作用.本文在导模共振结构的光栅层和基底层之间,引入低折射率的多孔二氧化硅间隔层,显著增强了局域电场与增益介质的接触度.结果表明,引入多孔二氧化硅后,共振产生的电场增强区域上移至激光染料层,增加了激光染料与电场的相互作用,实现了激光出射增强.本文基于时域有限差分法,对结构参数进行分析优化,研究了820 nm共振波长激发下的出射激光特性,得到了连续的激光出射,其能量阈值约为2.5 mJ/cm^2,线宽约为0.3 nm.本文提出的结构实现了对表面局域电场的有效调控,增强了激发光与增益介质的相互作用,不但可应用于激光器,还为其它发光器件的设计提供了参考.     

不同气体氛围下硅量子点的结构及其发光机理

纳秒脉冲激光在氮气、氧气和空气等不同氛围中加工出的硅量子点都有光致荧光(PL)的发光增强效应,并且在700 nm波长附近观察到了受激辐射.在不同氛围下生成的样品有几乎相同的PL光谱分布,其原因是不同氛围下加工出的样品带隙中有相同的电子态分布.计算结果显示:当硅量子点表面被氮或氧钝化后,在带隙中能够形成几乎相同的局域电子态,这种局域电子态可以俘获来自导带的电子,从而形成亚稳态,这是PL发光增强乃至产生受激辐射的关键因素. 关键词： 硅量子点 PL光谱 发光增强 电子局域态     

基于多形貌银纳米颗粒的多波长相干随机激光研究

采用溶剂热法分别制备了球形银纳米颗粒和多形貌银纳米颗粒,其中球形银纳米颗粒具有400 nm的窄带等离激元共振峰,而多形貌银纳米颗粒的共振区间在400～700 nm之间,将它们分别掺入R6G与PVP的混合溶液中,利用旋涂法在玻璃基板上制备银纳米颗粒嵌入染料掺杂聚合物薄膜随机激光器。采用纳秒脉冲激光进行随机激光泵浦实验,实验结果表明球形银纳米颗粒染料掺杂聚合物薄膜只有自发辐射峰,而多形貌银纳米颗粒染料掺杂聚合物薄膜具有线宽<0.8 nm的相干随机激光发射光谱,其阈值为1.9 mJ·cm-2, 这可能是由于银纳米颗粒的等离激元共振区间与R6G的发射光谱重叠,支持局域等离激元效应的形成,明显的局域场增强有效地改善了与附近分子的相互作用,从而激发了更多的辐射光子,促进了高增益的形成。进一步,利用多形貌银纳米颗粒在银纳米颗粒染料掺杂聚合物薄膜中随机分布的特性,通过改变泵浦位置,实现了20 nm范围内的随机激光输出波长的调控,具体输出范围为590.1～610.4 nm。认为这是由于多形貌银纳米颗粒在不同位置的组成和分布不同,改变了表面等离激元的相互作用和光子的散射能力,从而形成不同的增益效应和不同的封闭光振荡路径。此外,考虑到多形貌银纳米颗粒的共振波长较宽,探究了其用于输出其他颜色光的可能性。以与上述银纳米颗粒R6G染料掺杂聚合物薄膜相似的制备方法,制备了多形貌银纳米颗粒掺杂DCJTB染料聚合物薄膜,并且进行随机激光泵浦实验。结果表明,可以有效的产生波长为675 nm,半高宽<0.8 nm的相干红光随机激光,并且阈值仅为0.98 mJ·cm-2。研究结果在宽带可调谐随机激光器研究以及多色随机激光器研究领域具有重要的参考价值。     

多孔硅量子点的受激辐射：陷阱态的作用

 经激光辐照和高温退火后能够在硅基上生成氧化多孔硅结构。用514 nm的激光泵浦,观测到该多孔硅的受激辐射。当激励强度超过阈值时,在650～750 nm区域有很强的受激发光峰。这些受激发光峰的半高宽小于0.5 nm。激光辐照和高温退火后,在样品上能形成某些特殊的氧化结构。在傅里叶红外光谱分析中,显示有硅氧双键或硅氧桥键在硅表面形成。计算结果表明：当硅氧双键或硅氧桥键形成时,电子的陷阱态出现在纳晶硅的带隙中。价带顶和陷阱态之间的粒子数反转是解释这种受激辐射的关键。     

多孔硅量子点的受激辐射：陷阱态的作用

经激光辐照和高温退火后能够在硅基上生成氧化多孔硅结构。用514 nm的激光泵浦,观测到该多孔硅的受激辐射。当激励强度超过阈值时,在650～750 nm区域有很强的受激发光峰。这些受激发光峰的半高宽小于0.5 nm。激光辐照和高温退火后,在样品上能形成某些特殊的氧化结构。在傅里叶红外光谱分析中,显示有硅氧双键或硅氧桥键在硅表面形成。计算结果表明：当硅氧双键或硅氧桥键形成时,电子的陷阱态出现在纳晶硅的带隙中。价带顶和陷阱态之间的粒子数反转是解释这种受激辐射的关键。     

Formation of silver nanoparticles with dielectric shell on the silver-containing glass during laser evaporation and ablation

We demonstrate a new method of silver nanoparticles formation on a silver-containing glass surface due to its irradiation by a pulsed CO₂ and YAG:Nd lasers. The particles are formed as a result of reduction of silver ions from the glass at the edges of a laser torch emerging during evaporation and ablation. The settled particles are then fixed on sample surface by a shell of glass dielectric components. The method allows creating plasmonic nanostructures on the glass surface for sensing applications.     

Critical role of laser wavelength on carbon films grown by PLD of graphite

The structure of thin films deposited by pulsed laser ablation (PLD) is strongly dependent on experimental conditions, like laser wavelength and fluence, substrate temperature and pressure. Depending on these parameters we obtained various kinds of carbon materials varying from dense, mainly tetrahedral amorphous carbon (ta-C), to less compact vertically oriented graphene nano-particles. Thin carbon films were grown by PLD on n-Si 〈100〉 substrates, at temperatures ranging from RT to 800°C, from a rotating graphite target operating in vacuum. The laser ablation of the graphite target was performed by a UV pulsed ArF excimer laser (λ=193 nm) and a pulsed Nd:YAG laser, operating in the near IR (λ=1064 nm). The film structure and texturing, characterised by X-ray diffraction analysis, performed at grazing incidence (GI-XRD), and the film density, evaluated by X-ray reflectivity measurements, are strongly affected both by laser wavelength and fluence and by substrate temperature. Micro-Raman and GI-XRD analysis established the progressive formation of aromatic clusters and cluster condensation into vertically oriented nano-sized graphene structures as a direct function of increasing laser wavelength and deposition temperature. The film density, negatively affected by substrate temperature and laser wavelength and fluence, in turn, results in a porous bulk configuration and a high macroscopic surface roughness as shown by SEM characterisation. These structural property modifications induce a relevant variation also on the emission properties of carbon nano-structures, as evidenced by field emission measurements. This work is dedicated to our friend Giorgio who passed away 20th August.     

Short‐wavelength infrared defect emission as a probe of degradation processes in 980 nm single‐mode diode lasers

Infrared emission from 980‐nm single‐mode high power diode lasers is recorded and analyzed in the wavelength range from 0.8 to 8.0 μm. A pronounced short‐wavelength infrared (SWIR) emission band with a maximum at 1.3 μm originates from defect states located in the waveguide of the devices. The SWIR intensity is a measure of the non‐equilibrium carrier concentration in the waveguide, allowing for a non‐destructive waveguide mapping in spatially resolved detection schemes. The potential of this approach is demonstrated by measuring spatially resolved profiles of SWIR emission and correlating them with mid‐wavelength infrared (MWIR) thermal emission along the cavity of devices undergoing repeated catastrophic optical damage. The enhancement of SWIR emission in the damaged parts of the cavity is due to a locally enhanced carrier density in the waveguide and allows for an analysis of the spatial damage patterns. The figure shows a side view of a diode laser during catastrophic degradation as recorded by a thermocamera within 5 successive current pulses. The geometry of the device is given in grayscale. The position of the laser chip is indicated by the dotted line. The thermal signatures of the internal degradation of the diode laser are overlaid in color. The bi‐directional spread of the damage along the laser cavity is clearly visible.     

光子晶体垂直腔面发射850nm波长激光器研究

文章报道了国内首次研制成功的光子晶体垂直腔面发射850nm波长激光器，实现了连续电注入激射．发现器件能否激射直接依赖于光子晶体结构参数，而激光器的阈值、输出功率、输出模式等与光子晶体的晶格常数、占空比、腔的大小等因素有关．     

基于增益光纤长度优化的双波长运转掺铒光纤锁模激光器

构建了可自启动的双波长运转掺铒光纤锁模激光器.通过优化增益光纤长度,利用掺铒光纤在1530nm附近的再吸收效应调节激光器的增益谱,使激光器在1530nm和1560nm附近具有相同的增益强度.实验中采用31cm掺铒光纤作为增益光纤,以透射式半导体可饱和吸收体作为锁模器件,实现了自启动双波长锁模运转.激光器锁模输出重复频率为58.01MHz,信噪比为58.2dB,最高输出功率为4.8mW.锁模输出的光谱在1532.4nm和1552.3nm处具有两个强度接近的谱峰,谱峰间距约为20nm.该激光器无需手动调节即可实现双波长运转,更便于实际使用.     

激光二极管端面抽运Nd:YVO4实现1386 nm连续波激光输出

在Nd:YVO4晶体的4F3/2-4I13/2跃迁带内,除了1342 nm激光辐射之外,其它的跃迁谱线由于小的受激发射截面和强的寄生振荡,很难形成激光振荡.通过调整谐振腔损耗,获得了光纤耦合激光二极管端面抽运1386 nmNd:YVO4激光器激光连续输出.在抽运功率达到4.24 W时,得到了305 mW的1386 nm激光连续输出,最高输出功率下的斜效率为13.9%.实验中还观察到了1342 nm和1386 nm的双波长运转.根据抽运阈值能量和实验数据,计算得到了Nd:YVO4晶体中1386 nm激光辐射处的受激发射截面大约为(3±1)×10-19cm2.     

环形定子的激光致表面波机理及可视化探测研究

开展了用于新型激光驱动马达的环形定子的激光致表面波机理及实验研究. 提出一种带有凹槽阵列结构的环形定子新设计, 建立了激光在环形定子表面激发表面波的物理模型, 揭示了影响表面波幅值的关键因素; 采用一种新颖的激光致表面波可视化探测方法, 在波长1053 nm, 脉宽30 ns, 单脉冲能量1 mJ的激光激发下, 对表面波在铜质环形定子表面的传播特性进行了可视化探测实验. 理论与实验研究表明: 当激发光斑的位置紧邻凹槽阵列时, 沿着圆环向凹槽方向传播的表面波会被齿状凹槽阵列迅速衰减和吸收, 而沿着圆环向远离凹槽方向传播的表面波能够持续传递, 从而首次实现了激光致表面波在环形定子上的单向传播; 而对没有凹槽阵列结构的圆环进行的对比实验表明, 激光致表面波在圆环表面双向传播, 最终因相互混叠和串扰等而处于混乱状态. 由激光在该种环形定子表面激发出的单向表面波, 可望在光致表面波马达及驱动机构中获得应用. 关键词： 激光致表面波 环形定子 表面波可视化 激光驱动