Isospin dependence of the isotopic distributions from 36Ar and 40Ar fragmentation at about 60 MeV/nucleon

Fragments produced in the reactions of 69 MeV/nucleon ³⁶Ar and 55 MeV/nucleon ⁴⁰Ar on a Be target have been measured experimentally. The isotopic distributions from fragmentation reaction for both projectiles are compared with modified statistical abrasion-ablation model calculations. A strong isospin effect exhibits in the fragment distributions produced in ³⁶Ar and ⁴⁰Ar fragmentation. Experimental evidence for the disappearance of the isospin effect in the isotopic distributions produced by projectile fragmentation is observed with the increase of the violence of nuclear reaction. Received: 15 November 2000 / Accepted: 11 April 2001     

Collision-induced fragmentation and neutralization of methanol cluster cations

This contribution addresses the inelastic interaction of positively charged molecular cluster ions with a solid surface at kinetic energies up to 30 eV/molecule. We report experimental results on the scattering of mass-selected, protonated methanol cluster cations (CH₃OH)_nH⁺, n = 4-32, off a diamond-coated silicon surface. In particular we provide fragment size distributions of methanol cluster ions following their impact on the target, as well as surface-induced neutralization probabilities of methanol cluster ions as a function of the size and the kinetic energy of the parent clusters. Received 30 November 2000     

II. The intermediate velocity source in the 40Ca + 40Ca reaction at Elab = 35AMeV

The shape of the velocity distributions of charged particles projected on the beam direction can be explained if emissions from the hot projectile-like fragment and the target-like fragment are supplemented by an emission from an intermediate velocity source located between them. The creation of this source is predicted by a two-stage reaction model where, in the second stage, some of the nucleons identified in the first stage as participants form a group of clusters located in the region between the colliding nuclei. The cluster coalescence process is governed on the average by the maximum value of entropy, although its fluctuations are also significant. The properties of the intermediate velocity source are precisely described, including the isotopic composition of the emitted particles. Received: 12 March 2001 / Accepted: 20 June 2001     

Kinematically complete final state investigations of molecular photodissociation: two- and three-body decay of laser-prepared H 3 3 s ? 2 A 1 '

We have performed kinematically complete investigations of molecular photodissociation of triatomic hydrogen in a fast beam translational spectrometer recently built in Freiburg. The apparatus allows us to investigate laser-induced dissociation of neutral molecules into two, three, or more neutral products. The fragments are detected in coincidence and their vectorial momenta in the center-of-mass frame are determined. We demonstrate the potential of the method at the fragmentation of the 3 s ² A ₁ ^′ ( N = 1, K = 0) state of triatomic hydrogen. In this state, three-body decay into ground state hydrogen atoms H+H+H, two-body predissociation into H+H ₂ (v , J), and photoemission to the H ₃ ground state surface with subsequent two-body decay are competing channels. In the case of two-body predissociation, we determine the rovibrational population in the H ₂ (v , J) fragment. The vibrational distribution of H ₂ is compared with approximate theoretical predictions. For three-body decay, we measure the six-fold differential photodissociation cross-section. To determine accurate final state distributions, the geometric collection efficiency of the apparatus is calculated by a Monte Carlo simulation, and the raw data are corrected for apparatus efficiency. The final state momentum distribution shows pronounced correlation patterns which are characteristic for the dissociation mechanism. For a three-body decay process with a discrete kinetic energy release we have developed a novel data reduction procedure based on the detection of two fragments. The final state distribution determined by this independent method agrees extremely well with that observed in the triple-coincidence data. In addition, this method allows us to fully explore the phase space of the final state and to determine the branching ratios between the two- and three-body decay processes. Received 29 March 2001     

Granular flow from a silo: Discrete-particle simulations in three dimensions

Molecular (or granular) dynamics methods are used to study the gravity-driven flow of granular material through a horizontal aperture in three dimensions. The grains are spherical and modeled using a short-range repulsive interaction, together with normal and tangential frictional damping forces. The material is contained in a rough-walled cylindrical container with a circular hole in its base, and to permit flow measurements under steady-state conditions a continuous feed approach is employed in which exiting grains are replaced at the upper surface of the material. The dependence of flow velocity and discharge rate on aperture diameter is found to agree with experiment; other quantities such as the kinetic energy and pressure distributions are also examined. Received 5 June 2000 and Received in final form 21 September 2000     

I. The properties of hot Ca-like fragments from the 40Ca + 40Ca reaction at 35AMeV

The creation of hot Ca-like fragments was investigated in the ⁴⁰Ca + ⁴⁰Ca reaction at 35 AMeV. Using the AMPHORA 4π detector system, the primary projectile-like fragment was reconstructed and its properties were determined. Both primary and secondary distributions are compared with the predictions of a Monte Carlo code describing a heavy-ion collision as a two-step process. Some of the nucleons which are identified as participants in the first step are transferred in the second step to these final states, which correspond on the average to the maximum value of entropy (thermodynamic probability). The model allows for competition between mean-field effects and nucleon-nucleon interactions in the overlap zone of the interacting nuclei. The analysis presented here suggests a thermalized source picture of the decay of the projectile-like fragment. The validity of the reconstruction procedure for projectile-like fragments is discussed. Received: 12 March 2001 / Accepted: 20 June 2001     

Isotope dependent predissociation in the C 1 Σ + , v =0 and v =1 states of CO

Rotationally resolved spectral lines in the C - X (1, 0) band of carbon monoxide are investigated under high resolution using a coherent vacuum ultraviolet laser source, continuously tunable near 107 nm. Transition frequencies are determined by calibrating against a reference standard of iodine lines, recorded with saturation spectroscopy in the visible range, yielding an absolute accuracy of 0.003 cm^-1 in the vacuum ultraviolet. Improved molecular constants for the excited state are derived and no effects of perturbation are found at the present level of accuracy. Line broadening measurements result in information on the excited state lifetime of the C ¹ Σ ⁺ , v = 1 state for five natural isotopomers of carbon monoxide: τ( ¹² C ¹⁷ O ) = 280 ps, τ( ¹² C ¹⁸ O ) = 210 ps, τ( ¹³ C ¹⁶ O ) = 295 ps, τ( ¹³ C ¹⁷ O ) = 160 ps, and τ( ¹³ C ¹⁸ O ) = 150 ps. Within the accuracy of the present measurements no effects of J-dependent lifetimes were observed, for neither of the isotopomers. In addition direct time domain measurements of the lifetime of the C ¹ Σ ⁺ , v = 0 and v = 1 states of the main isotopomer are performed in a pump-probe experiment using a picosecond VUV-laser, yielding τ( ¹² C ¹⁶ O ) = 1780 ps for v = 0 and τ( ¹² C ¹⁶ O ) = 625 ps for v = 1. For C ¹ Σ ⁺ , v = 0 in ¹²C¹⁶O and ¹³C¹⁶O the same lifetime is found; this lifetime matches experimental values of the oscillator strength and hence supports previous results showing pure radiative decay in this state; the error margins however do not exclude some low level of predissociation. The measurements indicate that the C ¹ Σ ⁺ , v = 0 state of the ¹³C¹⁸O isotopomer is predissociated with an estimated yield of 17% (i.e. above the level of predissociation for ¹²C¹⁶O.) From the combined data predissociation yields upon excitation of the C ¹ Σ ⁺ , v = 1 state are derived, lying in the range 0.84-0.91 for the five less abundant isotopomers; for the main ¹²C¹⁶O isotopomer a strongly deviating predissociation yield of 0.65 is deduced. Received 21 December 2000 and Received in final form 26 March 2001     

General theory of population transfer by adiabatic rapid passage with intense, chirped laser pulses

We present a general theory of adiabatic rapid passage (ARP) with intense, linearly chirped laser pulses. For pulses with a Gaussian profile and a fixed bandwidth, we derive a rigorous formula for the maximum temporal chirp rate that can be sustained by the pulse. A modified Landau-Zener formula displays clearly the relationships among the pulse parameters. This formula is used to derive the optimal conditions for efficient, robust population transfer. As illustrations of the theory, we present results for two- and four-level systems, and selective vibronic excitation in the I₂ molecule. We demonstrate that population transfer with chirped pulses is more robust and more selective than population transfer with transform-limited pulses. Received 6 September 2000 and Received in final form 25 September 2000     

Effect of shell structure on energy dissipation in heavy-ion collisions

The effect of shell structure on the distribution of the excitation energy between fragments of the deep inelastic collisions is analysed in the microscopic approach. It is shown that the density of the single-particle levels of the proton and neutron subsystems near the Fermi surface determines the ratio between the excitation energies of fragments at the initial stage of the collision. It is shown also that the shell structure strongly influences the correlations between the width of the charge distributions and the total kinetic energy losses. Calculations are performed for the ^40,48Ca+²⁴⁸Cm reactions. The results obtained suggest a possible interpretation for the observed concentration of the excitation energy in the light fragment in deep inelastic collisions for a wide range of the total kinetic energy losses. Received: 27 July 1999 / Accepted: 29 March 2000     

Magnetic guiding of cold neutral atoms using a V-shaped current-carrying conductor

A new scheme to magnetically guide cold, neutral atoms using a V-shaped current-carrying conductor is proposed. The spatial distributions of the magnetic fields, potentials and forces generated by the V-shaped current-carrying conductor are calculated, and the relationship between the magnetic field and the parameters of the V-shaped current-carrying conductor are analyzed in detail. Our study shows that the V-shaped current-carrying conductor proposed here can be used to guide cold atoms in the weak-field-seeking state, and to construct various atom-optical elements, such as atomic funnel, atomic beam-splitter and atom interferometer and so on, and even to realize a single-mode atomic waveguiding under certain conditions. Received 17 November 2000 and Received in final form 26 May 2001     

A new test for random events of an exponential distribution

A new statistical test procedure is described to evaluate whether a set of radioactive-decay data is compatible with the assumption that these data originate from the decay of a single radioactive species. Criteria to detect contributions from other radioactive species and from different event sources are given. The test is applicable to samples of exponential distributions with two or more events. Received: 24 March 2000 / Accepted: 13 April 2000     

Size and randomness effects on the temperature-dependent hopping conductivity of nanocrystalline chains

Developing a renormalization group approach, we study the hopping conductivity of nanocrystalline chains with different site energies. Exact calculations show that many parameters including nano-sizes, randomness of grain distributions, lattice distortions, site energies, transition rates, Fermi energy, and temperature influence the conductivity. Some new singular features, for example the frequency shift, the amplitude fluctuations, and the interchange between “peak” and “valley” behavior of the imaginary part of the conductivity can be caused by certain parameters mentioned above, while the interface distortions modulate mainly the overall amplitudes of the conductivity at the whole frequency region. Received 13 January 2000 and Received in final form 12 September 2000     

(<Emphasis Type="Italic">p</Emphasis>,π<Superscript>±</Superscript>) correlations in central heavy-ion collisions at 1 ÷ 2 AGeV

The proton–charged pion correlated emission is studied in the reactions Au (1.06 AGeV) + Au, Ni (1.06 and 1.93 AGeV) + Ni and Ni (1.97 AGeV) + Cu within the BUU approach. The associated invariant mass distributions are shifted to smaller energies with respect to the free Δ(1232) mass distribution due to kinematical reasons. We find that the existing and partly conflicting experimental data do not allow to draw definite conclusions on the in-medium modification of the Δ(1232). Received: 18 October 1999 / Revised version: 4 February 2000     

Sum rule for the optical absorption of an interacting many-polaron gas

A sum rule for the first frequency moment of the optical absorption of a many-polaron system is derived, taking into account many-body effects in the system of constituent charge carriers of the many-polaron system. In our expression for the sum rule, the electron-phonon coupling and the many-body effects in the electron (or hole) system formally decouple, so that the many-body effects can be treated to the desired level of approximation by the choice of the dynamical structure factor of the electron (hole) gas. We calculate correction factors to take into account both low and high experimental cutoff frequencies. Received 26 April 2000 and Received in final form 5 December 2000     

Molecular picture of excited states and fragmentation paths of the Na 5 F 4 cluster

The stability against fragmentation and possible relaxation of the lowest excited states of the Na₅F₄ cluster (representative of cubic non stoechiometric clusters with an excess sodium atom, also called sodium-tail) is investigated by means of one-electron pseudopotential calculations with particular reference to photoabsorption processes from the ground state. Whereas the equilibrium configuration of the ground state has C_3v symmetry, the doubly degenerate 1²E excited state is affected by a conical intersection and a Jahn-Teller effect associated with the rotation of the sodium tail around the C₃-axis. This yields a “Mexican hat" topology for the lowest sheet with three equivalent C_s minima. Alternatively the 2²A₁ state has a minimum retaining the C_3v symmetry. The dissociation paths of the cluster along the C₃-axis into respectively Na₄F_{4 +} Na and Na₄F_{3 +} NaF are also investigated. Among the former paths, the excited states are found adiabatically stable with respect to the products. However in the A₁ symmetry, fragmentation into NaF exhibits an interesting avoided crossing between configurations correlated respectively with Na₄F₃ ^{+ +} NaF^- and Na₄F_{3 +} NaF. Such interaction, similar to the well-known charge exchange processes in elementary molecules might induce non adiabatic predissociation of the 2²A₁ state. This mechanism is invoked to explain the differences between R2PI and depletion spectra, correlated with the dissociation or relaxation of the excited states. Received 24 March 2000 and Received in final form 11 July 2000     

Present and future experiments with stored exotic nuclei at relativistic energies

Pioneering experiments with stored and cooled exotic nuclei at relativistic energies have been performed using the combination of the fragment separator FRS with the storage-cooler ring ESR. Exotic nuclei created in peripheral collisions are spatially separated in-flight and injected into the storage ring for high-precision mass and unique lifetime measurements. Lifetimes of stored bare and few-electron nuclei have been measured to study the influence of the electron density on the β decay. This condition, relevant for stellar plasma, can now be systematically investigated in the laboratory for the first time. Characteristic experiments of the present FRS-ESR system are presented and perspectives for a next-generation facility are briefly outlined. Received: 1 May 2001 / Accepted: 4 December 2001     

Effective resolvent applied to interacting resonances

The wave operator theory of quantum dynamics is applied to characterize coupled metastable states. The theory extends to quasi bound states methods which are standard for dealing with bound levels. It is shown that interacting resonances can be investigated by means of small-dimensional effective Hamiltonians containing all the significant information of intrinsic properties which drive the various dynamical processes taking place. The study of the vibrational predissociation of I₂Ne, mediated by intramolecular energy redistribution, illustrates the power of the method. In addition to its accuracy to determine spectroscopic profiles and survival probabilities, it results more efficient than usual energy or time-domain numerical calculations. Received 25 January 2001 and Received in final form 11 May 2001     

Localization of a macroscopic object induced by the factorization of internal adiabatic motion

To account for the phenomenon of quantum decoherence of a macroscopic object, such as the localization and disappearance of interference, we invoke the adiabatic quantum entanglement between its collective states (such as that of the center-of-mass (CM)) and its inner states based on our recent investigation. Under the adiabatic limit where motion of the CM does not excite the transition of inner states, it is shown that the wave function of the macroscopic object can be written as an entangled state with correlation between adiabatic inner states and quasi-classical motion configurations of the CM. Since the adiabatic inner states are factorized with respect to each component of the macroscopic object, this adiabatic separation can induce the quantum decoherence. This observation thus provides us with a possible solution to the Schr?dinger cat paradox. Received 24 October 2000 and Received in final form 8 March 2001     

Chiral invariant phase space event generator

An event generator based on the CHIPS model is implemented in the GEANT4 simulation toolkit. Nuclear fragment production in the process of pion capture on nuclei is used to tune the parameters of the CHIPS model describing clusterization of nucleons in nuclei. The spectra of nucleons and nuclear fragments in pion capture and in photonuclear reactions at 60 MeV are compared with experimental data. Received: 30 May 2000 / Accepted: 2 November 2000     

Stability and instability of a hot and dilute nuclear droplet

The diabatic approach to dissipative collective nuclear motion is reformulated in the local-density approximation in order to treat the normal modes of a spherical nuclear droplet analytically. In a first application the adiabatic isoscalar modes are studied and results for the eigenvalues of compressional (bulk) and pure surface modes are presented as function of density and temperature inside the droplet, as well as for different mass numbers and for soft and stiff equations of state. We find that the region of bulk instabilities (spinodal regime) is substantially smaller for nuclear droplets than for infinite nuclear matter. For small densities below 30% of normal nuclear matter density and for temperatures below 5 MeV all relevant bulk modes become unstable with similar growth rates. The surface modes have a larger spinodal region, reaching out to densities and temperatures way beyond the spinodal line for bulk instabilities. Essential experimental features of multifragmentation, like fragmentation temperatures and fragment-mass distributions (in particular the power-law behavior) are consistent with the instability properties of an expanding nuclear droplet, and hence with a dynamical fragmentation process within the spinodal regime of bulk and surface modes (spinodal decomposition). Received: 4 September 2000 / Accepted: 14 November 2000