Nonlinear Absorption and Dispersion Response in Optically Dense Media Driven by a Single-Mode Laser

Taking the density-dependent near dipole-dipole （NDD） interaction into consideration, we theoretically investigate the response of nonlinear absorption and dispersion in optically dense media of three-level atoms driven by a single-mode probe laser. The influence of the NDD effects on the absorption and dispersion spectra of the probe field is predicted via numerical calculations. It is shown that the NDD effects reduce gradually to transient absorption and amplification with the increase of the strengths of the NDD interaction, but do not change the steady-state behavior. Due to the presence of the NDD effects, steady-state absorption spectra exhibit asymmetric double-peak structure and overall shifts when a continuous-wave （cw） probe field is applied. However, frequency dispersion spectra are insensitive to them near the zero detuning.     

Nonlinear Absorption-Gain Response and Population Dynamics in a Laser-Driven Four-Level Dense Atomic System

We theoretically investigate the response of nonlinear absorption and population dynamics in optically dense media of four-level atoms driven by a single-mode probe laser, via taking the density-dependent near dipole-dipole (NDD) interactions into consideration. The influence of the NDD effects on the absorption of the probe field and population dynamics is predicted via numerical calculations. It is shown that the NDD effects can reduce gradually to transient absorption with the increase of the strengths of the NDD interactions, and transient amplification can be achieved. In the steady-state limit, the probe field exhibits transparency for strong NDD interactions. Alternatively, the population entirely remains at the ground state due to the NDD effects.     

少周期脉冲在稠密V型三能级介质中传播时的粒子布居演化

利用由预估计校正-时域有限差分(PC-FDTD)法求解Maxwell-Bloch方程得到的数值解,研究少周期激光脉冲在稠密V型三能级原子介质中传播时各能级粒子数布居的演化特性.结果表明,两跃迁偶极矩的比值(γ)对稠密介质中粒子数布居反转出现的时间和振荡的次数具有显著的影响,γ=1时,考虑洛仑兹局域场修正(LFC)时,粒子数反转出现的较晚,近偶极-偶极(NDD)相互作用延缓了粒子数的反转;γ>1时,考虑LFC时,粒子数反转出现的较早,NDD相互作用加快了粒子数的反转;电偶极矩不同时,粒子数布居振荡的次数比相同时多.粒子数布居在稠密介质中的演化特性与稀疏介质中显著不同,在入界处,稀疏介质中粒子数布居可以实现长时间的反转;随着介质密度的增大,粒子数布居产生准周期性的振荡,但考虑LFC时,振荡的次数比不考虑LFC时少.     

Dispersion Theory of Liquids Containing Optically Linear and Nonlinear Maxwell Garnett Nanoparticles

Kramers-Kronig relations and sum rules for effective linear permittivity of the Maxwell Garnett liquid-nanosphere system were obtained using complex analysis and general expression of the effective permittivity. When reflectance from optically linear and nonlinear Maxwell Garnett nanoparticles was calculated it was observed that the reflectance, in the case of attenuated total reflection, depends on the fill fraction of the nanospheres and their nonlinear susceptibility. According to simulations a good sensitivity of the nonlinear contribution on the reflectance can be obtained by using a probe wavelength corresponding to the resonance frequency of the nanosphere system. In Kretchmann#x0027;s configuration it was observed that the surface-plasmon-resonance angle depends on the fill fraction and on the intensity of the incident light. By using reflectance, it is possible to detect optically nonlinear nanospheres in liquids.     

可见光在酞菁钴薄膜介质中吸收和色散的研究

对可见光在酞菁钴（ＣｏＰｃ）薄膜中的折射率、吸收率和吸收系数作了理论计算。理论结果和文献［１］的实验测量值符合得很好。并对光在介质中吸收、色散随频率变化的理论公式作了深入的分析。     

Dynamical Properties of a Single-Mode Laser Driven by Quadratic Pump Noise

We propose a single-mode laser model driven by quadratic pump noise with cross correlation between the real and imaginary parts of the pump noise. The effect of the cross-correlation coefficient λp between the real and imaginary parts of the pump noise on dynamical properties is studied by using of the linear approximation. The theoretical expressions of intensity correlation function λ（t）, normalized intensity fluctuation λ（0） are calculated. It is found that the most conspicuous effects of λp on both the intensity correlation function and the normalized intensity fluctuation appear at ｜λP｜ = /0.5, but not at ｜λP｜ = 1.     

相对论电子的逆韧致吸收

在激光强度大于１０＾１８Ｗ／ｃｍ＾２的条件下，利用强激光场中完全相对论的电子运动轨迹，得到了稀薄等离子体中的韧致吸收系数计算公式，并与原有的逆韧致吸收系数的计算公式进行了比较。     

Controllable Absorption and Dispersion Properties of an RF-drivenFive-Level Atom in a Double-Band Photonic-Band-Gap Material

The probe absorption-dispersion spectra of a radio-frequency (RF)-driven five-level atom embedded in a photonic crystal are investigated by considering the isotropic double-band photonic-band-gap (PBG) reservoir. In the model used, the two transitions are, respectively, coupled by the upper and lower bandsin such a PBG material, thus leading to some curious phenomena. Numerical simulations are performed for the optical spectra. It is found that when one transition frequency is inside the band gap and the other is outside the gap, there emerge three peaks in the absorption spectra. However, for the case that two transition frequencies lie inside or outside the band gap, the spectra display four absorption profiles. Especially, there appear two sharp peaksin the spectra when both transition frequencies exist inside the band gap. The influences of the intensity and frequency of the RF-driven field on the absorptive and dispersive response are analyzed under different band-edge positions. It is found that a transparency window appears in the absorption spectra and is accompanied by a very steep variation of the dispersion profile by adjusting system parameters. These results show that the absorption-dispersion properties of the system depend strongly on the RF-induced quantum interference and the density of states (DOS) of the PBG reservoir.     

三能级级联型介质的正常色散与反常色散

建议利用三能级级联型介质实现从正常色散到反常色散的变换.在级联型介质中,两个偶极跃迁分别与两个不同的相干场耦合.探测场或者与上跃迁耦合,或者与下跃迁耦合.利用谐振展开方法把介质密度矩阵元方程组转换成在定态条件下系数不依赖时间的方程组,然后用逆矩阵求解,并用此解求得介质的吸收与色散谱.结果表明,对于每一种情形,在同一频率区域系统既能呈现正常色散,也能呈现反常色散.通过改变耦合到探测跃迁的驱动场强度,可以实现从正常色散到反常色散的转换.级联系统与Λ和V系统之间呈现两个差别.第一,如果利用Λ和V系统的两个跃迁同时与探测场耦合获得色散转换,则需要利用近简并能级,而本方案利用缀饰态获得等价的近简并能级,其间距由相应驱动场强度进行控制.第二,如果利用Λ和V系统的单个跃迁耦合探测场建立色散转换,当退耦合态起主要作用时,系统不能产生色散转换,而级联系统不涉及退耦合态.     

非线性吸收诱导掺镱光纤激光器中的光学双稳

研究了在掺镱光纤激光器中观察到的光学双稳态现象.激光信号光和驻留泵浦光的双稳特性来源于激光器在小信号和增益饱和两种情况下,掺镱光纤对信号的非线性吸收导致的激光器内腔非线性损耗.同时分析了把泵浦光中的光学双稳行为通过分叉的腔结构扩展到切换式双波长光纤激光器的可行性.     

负折射介质中三阶非线性色散项对超短脉冲传输的影响

采用分步傅里叶法研究了三阶非线性色散项对超短脉冲传输的影响.通过模拟数值计算得出,在德鲁德模型频率选取的一定范围内,三阶非线性色散项对超短脉冲传输所造成的影响是不可忽略的.结果表明:三阶非线性色散项系数取负值时,在正常色散区超短脉冲不对称展宽,脉冲中心向前沿偏移;在零色散点超短脉冲不对称展宽程度加剧并在脉冲前沿形成振荡,脉冲中心向前沿偏移;在反常色散区超短脉冲不对称变窄,脉冲中心仍向前沿偏移.     

有机分子激发态非线性吸收的瞬态特性研究

提出了一种通过测量单脉冲光的输入与输出波形来研究激发态非线性吸收的新方法，用这种方法研究了纳秒脉作用下类卟啉镉溶液与甲基橙溶液的三重激发态的非线性吸收特性，前者为反饱和吸收现象，后者是由饱和吸收转化为反饱和吸收的新现象，实验结果验证了理论模拟和正确性。     

Intensity Correlation Function of a Single-Mode Laser Driven by Two Colored Noises with Colored Cross-Correlation

By using the linear approximation method, the intensity correlation function and the intensity correlation time are calculated in a gain-noise model of a single-mode laser driven by colored cross-correlated pump noise and quantum noise, each of which is colored. We detect that, when the cross-correlation between both noises is negative, the behavior of the intensity correlation function C(t) versus time t, in addition to decreasing monotonously, also exhibits several other cases, such as one maximum, one minimum, and two extrema (one maximum and one minimum), i.e., some parameters of the noises can greatly change the dependence of the intensity correlation function upon time. T3.     

可调谐激光器腔内色散棱镜及其组合

分析了色散棱镜的特性及其顶角设计问题。讨论了色散棱镜和扩束棱镜在布鲁斯特角入射状态下，可组合使用的形式及单程角色散。提出将色散棱镜与扩束棱镜组合使用，可减少色散棱镜个数而获得更大角色散的方法。并据此设计了两个色散棱镜组，在Ｔｉ∶Ｓ激光器中得到实际使用。     

受驱动光学系统腔场噪声的内腔多光子吸收减低

在受驱动光学系统中增设内腔多光子吸收元件是抑制腔场噪声的有效手段，为在好腔条件（ｋ＜＜ｒ／／，ｒ⊥）下获得低噪声强光场，应选用高吸收非线性元件，若所需场强较弱，在主动腔状态应选用非线性吸收最低的双光子吸收体，在被动腔状态则应让系统工作在无吸收状态。     

Intensity Correlation Function of a Single-Mode Laser Driven by Two Colored Noises with Colored Cross-Correlation

By using the linear approximation method, the intensity correlation function and the intensity correlation time are calculated in a gain-noise model of a single-mode laser driven by colored cross-correlated pump noise and quantum noise, each of which is colored. We detect that, when the cross-correlation between both noises is negative, the behavior of the intensity correlation function C(t) versus time t, in addition to decreasing monotonously, also exhibits several other cases, such as one maximum, one minimum, and two extrema (one maximum and one minimum), i.e., some parameters of the noises can greatly change the dependence of the intensity correlation function upon time. Moreover, we find that there is a minimum Tmin in the curve of the intensity correlation time versus the pump noise intensity, and the depth and position of Train strongly depend on the quantum noise self-correlation time T2 and cross-correlation time T3.     

Negative Nonlinear Absorption Effect for 1.5 μm Laser in an Erbium Chloride Solution

The dependence of the negative nonlinear absorption effect on both modulation degree and frequency of the incident laser was investigated in an erbium chloride solution using a 1.5μm laser diode. The reversed-phase waveform was observed at modulation degrees smaller than 71%. As modulation frequency increased, the transmitted waveforms became asymmetrical and the effect was suppressed. The effect was obtained at wavelengths of 1510.3 to 1510.8 nm. The negative nonlinear absorption effect for 1.5 μm. can be explained by considering an enhanced absorption model for a four-level system of the Er³⁺ ion.     

周期量级激光脉冲在不同密度的原子介质中传播行为的比较(英文)

利用不含慢变包络近似和旋波近似的全波Maxwell-Bloch方程组的数值解,研究了周期量级超短激光脉冲在Ladder型三能级原子介质中的传播行为并与在相应的稀疏介质中的情况进行了比较.我们发现,在传播过程中,超短脉冲在稠密介质中的时间演化规律与在稀疏介质中明显不同,而且这种差别将随初始脉冲面积的增大而加大.当初始脉冲面积较小时,在传播过程中,脉冲形状在稀疏介质中只有小的改变而在稠密介质中却有显著的变化.当初始脉冲面积足够大时,在稠密介质中在不同的传播距离处脉冲分裂为不同数量和形状的亚脉冲;在稀疏介质中脉冲形状在传播过程中仍然只有小的改变。产生以上差别的原因在于稠密原子介质中近偶极-偶极(NDD)相互作用导致的局域场修正(LFC)及比稀疏原子介质更强的极化电场的影响.其中,更强的极化电场的影响起着主要的作用,但局域场修正的作用也不能忽略,而极化电场的增强是由于原子密度的增加.     

周期量级激光脉冲在不同密度的原子介质中传播行为的比较

利用不含慢变包络近似和旋波近似的全波Maxwell-Bloch方程组的数值解,研究了周期量级超短激光脉冲在Ladder型三能级原子介质中的传播行为并与在相应的稀疏介质中的情况进行了比较.我们发现,在传播过程中,超短脉冲在稠密介质中的时间演化规律与在稀疏介质中明显不同,而且这种差别将随初始脉冲面积的增大而加大.当初始脉冲面积较小时,在传播过程中,脉冲形状在稀疏介质中只有小的改变而在稠密介质中却有显著的变化.当初始脉冲面积足够大时,在稠密介质中在不同的传播距离处脉冲分裂为不同数量和形状的亚脉冲|在稀疏介质中脉冲形状在传播过程中仍然只有小的改变。产生以上差别的原因在于稠密原子介质中近偶极-偶极(NDD)相互作用导致的局域场修正(LFC) 及比稀疏原子介质更强的极化电场的影响.其中,更强的极化电场的影响起着主要的作用,但局域场修正的作用也不能忽略,而极化电场的增强是由于原子密度的增加.