Atomic Coherent Trapping and Properties of Trapped Atom

Based on the theory of velocity-selective coherent population trapping, we investigate an atom-laser system where a pair of counterpropagating laser fields interact with a three-level atom. The influence of the parametric condition on the properties of the system such as velocity at which the atom is selected to be trapped, time needed for finishing the coherent trapping process, and possible electromagnetically induced transparency of an altrocold atomic medium,etc., is studied.     

Properties of Coherent State for Hydrogen Atom

We construct the coherent state for the two-dimensional hydrogen atom, for which the averaged motion ofposition describes a Kepler ellipse. The coherent state can be expanded with respect to the eigenstates of 2D hydrogenatom, from which we evaluate the binding energy of the wave packet for this state.     

双模量子光场驱动的拉曼型光致离化系统中原子的相干俘获

研究了由双模量子光场驱动的拉曼型光致离化系统中原子的相干俘获性质，分析了反映原子－光场耦合性质的参量对系统相干俘获的影响，论证了在定的条件下，双模ＳＵ（２）相干光场可以将原子完全俘获。     

级联型三能级原子与单模光场耦合系统中的场量子特性

利用J-C模型,采用数值计算方法研究了相干态光场与级联型三能级原子相互作用过程中场的压缩效应和反聚束效应。讨论了选择原子测量对相干态光场与级联型三能级原子相互作用过程中场压缩效应和反聚束效应的影响。     

被驱动的V型三能级原子在压缩真空中的稳态行为

研究了相干驱动的Ｖ型三能级在原子在压缩真空入射的劣质腔中的稳态行为,分析了原子的稳态粒子布居数与库场平均光予数、压缩关联强度和相位及相干激光场的强度的关系。对相干捕获现象的发生作了讨论。     

三能级原子与少周期脉冲串作用中的相干布居捕获

研究了少周期脉冲串作用下三能级原子中的布居转移和相干布居捕获现象.在非旋波近似的情况下求解了密度矩阵方程.研究结果表明在等时间间隔的锁相脉冲作用下,系统能级的布居逐步转移并积累,系统基态相干也逐步积累.在满足脉冲重复频率为基态能级频差的整数分之一倍时,三能级系统和频率梳中两梳齿频率成分作用形成相干布居捕获现象,原子暗态布居值达到最大,介质对脉冲透明.在适当选取少周期脉冲参量的情况下,在0.5个ns的时间内三能级系统相干性演化到最大后到达稳态,相干布居捕获发生.与脉宽为100个fs的多周期脉冲相比,少周期脉冲串在介质中建立相干布居捕获的时间缩短两个数量级.由于频率梳中与三能级系统发生作用的梳频成份有相同的频移,相干布居捕获的条件双光子共振仍然满足.因而,当两基态能级频率差较大时,如果选取少周期脉冲载波频率为系统能级1至2和1至3的传输频率之和的一半ω=(ω₁+ω₂)/2,室温下原子热运动的引起的多普勒频移并不会破坏相干布居捕获.     

Tunable Phase-Coherent Source of the Bichromatic Light Field for the Spectroscopy of Resonances of the Coherent Population Trapping in Rare-Earth Atoms

A technique for creating the source of a bichromatic laser field with a stable mean value of the difference frequency is realized. The spectral characteristics of a femtosecond passive mode-locked laser are used in this technique. Such a source operating in the region of 780 nm is created. The possibility of using the phenomenon of coherent population trapping (CPT) in three-level systems of the rare-earth atoms for the development of secondary frequency standards in the optical range is considered. The contributions of the processes affecting the width and contrast of the CPT resonances and defining their attainable Q factors are studied. The prospects of using the experimental technique developed for the spectroscopy of the CPT resonances in samarium and thulium vapors are discussed.     

利用V型原子与单模光场的非共振相互作用制备四光子相干态

提出了一种利用简并V型三能级原子与振幅很大的单模相干光场的远离共振相互作用,制备四光子相干态的有效新方案.同时证明了在相同的条件下,按照相同的方法不能制备出四成分以上的相干态的叠加态, 即当在腔中注入的第三个原子的速度与第二个原子的速度相等时,腔场将保持这种四光子相干态不变.     

Coherent effects in a three-photon CPT process of Ca+

Linewidth narrowing and other quantum coherent effects based on three-photon coherent population trapping (CPT) in Ca⁺ ions are investigated. If the propagation directions of the three lasers obey the phase matching condition, the dark linewidth resulting from the CPT can be very narrow, and it can be controlled by adjusting the parameters of the lasers.     

对相干态与级联三能级原子相互作用过程中原子与场的动力学特性

研究对相干态与级联三能原子相互作用的动力学特性。结果表明，无论场模与原子的中间能级是否失谐，拉比振荡和互关联函数的时间演化都呈现崩溃与回复现象，但崩溃的持续时间随失谐量的增加而迅速延长，且两模之间随时间的演化即出现关联也出现反关联。     

一个特殊模型中的相干布居俘获

外场作用下,对称双势阱中将发生相干布居俘获现象. 在氨分子模型中,当分子初始处在较低的本征态时,在一定的条件下激发态上将没有粒子数布居,外加光场强烈地使较低的双重态耦合在一起,且粒子数布居总保持为1,尽管此时外场与|2〉→|3〉接近共振. 这是一般模型所不能得到的结论. 关键词： 相干布居俘获 Ξ型三能级系统 双势阱     

相干布居数囚禁原子频标的实现及相关实验参数研究

原子频标要求高信噪比和窄线宽的鉴频信号,但对于被动型相干囚禁态原子频标(CPT频标), 改善鉴频信号信噪比以增加线宽为代价,因此选择合适的信噪比和线宽组合是研制CPT原子频标频标的重要环节。文章介绍了用桌面CPT频标系统地研究了鉴频信号与温度、光强等参数的关系所获得的研究结果,由此获得了合适选取的信噪比与线宽组合的依据。文章还给出了关于光源非理想偏振导致的消相干效应对CPT频标的影响所开展的实验结果。文章所提供的研究结果不仅帮助我们研制成功了CPT频标,而且对于CPT物理现象研究和其他CPT频标的研制也有参考价值。     

原子捕集-火焰原子吸收光谱法测定中草药中痕量镉

考察了火焰条件、捕集管与燃烧器和光束的距离、冷却水流量、捕集时间等实验条件对原子捕集 火焰原子吸收光谱法测定镉的灵敏度的影响 ,实验优选出的最佳实验条件为 :乙炔流量 90L·h- 1 ,捕集管距离燃烧器缝口 5mm ,捕集管距离光束 2mm ,冷却水流量 1 5L·min- 1 ;采用 5 0ng·mL- 1 的镉标准溶液对吸光度与捕集时间的关系进行了考察 ,结果发现 ,在 0～ 6min的捕集时间内二者呈良好的线性关系。在最佳实验条件下 ,捕集时间为 2min时 ,镉的特征浓度为 1 8ng·mL- 1 ,检出限为 0 4 2ng·mL- 1 ,分别较常规火焰原子吸收光谱法的特征浓度和检出限改善了 16倍和 5倍 ,方法的精密度 (RSD)为 1 8%。利用所建立的原子捕集 火焰原子吸收光谱法 ,在最佳实验条件下 ,对人参、丹参、苦参和党参及其水煎液中的痕量镉进行了测定 ,样品的测定回收率在 89 5 %～ 10 4 %之间 ,结果令人满意。     

Improved Performance of On-line Atom Trapping in Flame Furnace Atomic Absorption Spectrometry by Chemical Vapor Generation: Determination of Cadmium in High-Salinity Water Samples

ABSTRACT

On-line atom trapping inside a nickel flame furnace using chemical vapor generation for sample introduction was proposed for the determination of trace cadmium by flame atomic absorption spectrometry (AAS). Cadmium volatile species was generated upon reaction with potassium borohydride and then flushed into a flame furnace for on-line trapping by a flow of nitrogen carrier gas. The middle part of the flame furnace, where the carrier gas impacts, is cooled by the gas flow, and this provides a fine strategy for on-line atom trapping for the purpose of preconcentration. A stainless steel plate is put on the top of the flame burner in the middle to form a flame-free zone, which also greatly lowers the temperature of the flame furnace and facilitates the atom-trapping process. Due to the introduction of chemical vapor generation, matrix effect was greatly alleviated compared with direct pneumatic nebulization for on-line atom trapping in flame furnace AAS. With trapping time of 35 s, the current approach achieved an excellent limit of detection of 20 ng L^?1. The proposed method was successfully applied for the quantification of cadmium in high-salinity samples.     

Enhanced Deflection of Light Ray by Atomic Ensemble on Coherent Population Oscillation

In recent experiments [e.g., Nature Physics 2 (2006) 332], the enhancedlight deflection in an atomic ensemble due to inhomogeneous fields is demonstrated by the electromagnetically induced transparency (EIT) based mechanism. In this paper, we explore a different mechanism for the similar phenomenon of the enhanced light deflection. This mechanism is based on the coherent population oscillation, which leads to the hole burning in the absorption spectrum. The medium causing the deflection of probe light is an ensemble of two-level atoms manipulated by a strong controlled field on the two photon resonances. In the large detuning condition, the response of the medium to the pump field and signal field is obtained with steady state approximation. And it is found that after the probe field travels across the medium, the signal ray bends due to the spatial-dependent profile of thecontrol beam.     

Λ型原子与单模光场的非共振作用制备四光子相干态

根据简并Λ型三能级原子与单模光场的改进型有效哈密顿量 ,通过矩阵形式法推导出原子光场系统的波函数 ,提出利用简并Λ型三能级原子与单模光场的远离共振相互作用制备四光子相干态的有效方案。并且证明按照同样的方法不能制备出四成分以上的相干叠加态 ,即当在腔中注入的第三个原子的速度与第二个原子的速度相等时 ,腔场将保持这种四光子相干叠加态不变     

Coherent population trapping magnetometer by differential detecting magneto–optic rotation effect

A pocket coherent population trapping(CPT) atomic magnetometer scheme that uses a vertical cavity surface emitting laser as a light source is proposed and experimentally investigated.Using the differential detecting magneto–optic rotation effect,a CPT spectrum with the background canceled and a high signal-to-noise ratio is obtained.The experimental results reveal that the sensitivity of the proposed scheme can be improved by half an order,and the ability to detect weak magnetic fields is extended one-fold.Therefore,the proposed scheme is suited to realize a pocket-size CPT magnetometer.     

Transient responses of transparency in a far-off resonant atomic system

Transient coherent oscillations in a closed Λ system under far-off resonant Raman fields were investigated theoretically. It has been found that the coherent superposition of the ground states can be formed due to the absorption even for initial maximal mixed ground states. The absorption oscillates with a period depending on the two-photon detuning when the system is initially in a transparent state and the two-photon Raman detuning is suddenly changed. The amplitude of the absorption decays with the decay rate of the ground states, which is different from the case when the lasers are applied resonantly. These transient coherent oscillations can be used to measure the relaxation rate of the ground states.     

铯原子气室中相干布居俘获的参数依赖关系研究

基于铯原子基态6S_1/2的两个超精细能级（F=3与F=4）与激发态6P_3/2的超精细能级（F′=4）构成的Λ型三能级系统,采用室温下的未充缓冲气体和充有分压为266.6 Pa的氖气作为缓冲气体的铯原子气室对于相干布居俘获（CPT）的参数依赖关系进行了实验研究和理论分析.主要研究了CPT信号的半高全宽和幅度对于频率差为铯原子基态6S_1/2的超精细分裂（9.19263177 GHz）且位相锁定的两激光束的功率、光强比值、光斑直径、磁屏蔽之后的剩余磁场以及是否充缓冲气体等实验参数的依赖关系.在优化的实验参数条件下获得了约340 Hz的CPT信号半高全宽.