Energy levels of 92Nb and 94Tc from 92Zr, 94Mo(p,nγ)92Nb, 94Tc

The γ-decays of the energy levels of ⁹²Nb and ⁹⁴Tc were measured following the ⁹²Zr(p, n)⁹²Nb and ⁹⁴Mo(p, n)⁹⁴Tc reactions. For ⁹²Nb the γ-ray thresholds were measured and a detailed excitation function was obtained near the ⁹³Zr ground-state isobaric analog resonance. Also, γ-γ coincidence measurements with two Ge(Li) detectors were made for both ⁹²Nb and ⁹⁴Tc. The coincidence measurements determined ten energy levels in ⁹²Nb and two levels in ⁹⁴Tc. A comparison with particle transfer reactions is used to elucidate the structure of ⁹²Nb levels observed here but not seen in the transfer reactions.     

Energy levels of92Nb from 92Zr(p,nγ)92Nb

The energy levels of⁹²Nb were studied by means of the⁹²Zr(p, nγ) reaction. The deexcitation γ-rays were observed with a high-resolution Ge(Li) detector in the proton energy range 3.00–4.80 MeV in steps of about 25 keV. Many new excited states of ⁹²Nb were populated by this reaction. Excitation energies up to 1.77 MeV were determined with high precision, and a level scheme of ⁹²Nb is proposed. From a Hauser-Feshbach analysis, the γ-decay scheme and other information, the spin-parities of many levels were assigned.     

A proton stripping study of92Nb

Levels up to energies of 4 MeV have been studied with the⁹¹Zr(³He,d)⁹²Nb reaction with an incident particle energy of 25.5 MeV. The product deuterons were analyzed by a split-pole spectrometer. Angular distributions were obtained for many of the transitions and compared with DWBA calculations. The assigned transferl values and spectroscopic factors were used to assign shell model structures to these levels.     

Cross-section measurement for the ~(93)Nb(n,2n)~(92g)Nb reaction at the neutron energy of 14.6 MeV by the AMS method

The cross-section for the~(93)Nb(n,2n)~(92g)Nb reaction has been measured at the neutron energy of 14.6 Me V using neutron activation and accelerator mass spectrometry(AMS)determination of the long-lived product nuclide~(92g)Nb.The neutron energy was generated from the D+T neutron source at the China Institute of Atomic Energy(CIAE).The neutron flux was monitored by measuring the activity of~(92m)Nb produced in the competing reaction channel of~(93)Nb(n,2n)~(92m)Nb.At the neutron energy of 14.6 MeV,the~(93)Nb(n,2n)~(92g)Nb reaction cross-section of(736±220)mb was obtained for the first time.     

The 93Nb(p,d)92Nb reaction at 26.3 MeV

The ⁹³Nb(p, d)⁹²Nb reaction was studied at a proton energy of 26.3 MeV. Angular distributions were obtained for outgoing deuterons to 37 states in ⁹²Nb up to an excitation energy of 4.2 MeV. The results were compared with DWBA calculations to extract l-values and spectroscopic factors. Fourteen previously unobserved l = 1 transitions were measured.     

Decay scheme of92m Nb

The beta decay of the 2^{+ 92m} Nb was reinvestigated via⁹³Nb(γ, n) reaction. The feeding of the 2⁺ 2,067 keV level of⁹²Zr was determined measuring the intensity of the 1,132 keV gamma-ray transition.     

Gamow-teller strength distribution in the vicinity of A = 90: (I). Schematic calculation of GT strength in 90, 92, 94Nb

The distributions of Gamow-Teller strength in ^{90, 92, 94}Nb have been calculated utilizing the so-called GT force in the random phase approximation. For ⁹⁰Nb the calculated distribution is in striking agreement with that part of the ⁹⁰Zr(p, n) excitation function leading to 1⁺ excitations in ⁹⁰Nb and qualitative agreement is demonstrated for data from the reactions ^{92, 94}Zr(p, n). Some 25 % of the GT strength is found to lie well below the structureless giant resonance proposed by Ikeda et al. The implications of this result to the β-decay properties of neutron rich nuclei near A = 90 are discussed.     

Cumulative fission yield measurements with 14.7 MeV neutrons on 238U

The fission yield data in the 14 MeV energy neutron induced fission of ²³⁸U play an important role in decay heat calculations and generation-IV reactor designs. In order to accurately measure fission product yields (FPYs) of ²³⁸U induced by 14 MeV neutrons, the cumulative yields of fission products ranging from ⁹²Sr to ¹⁴⁷Nd in the ²³⁸U(n, f) reaction with a 14.7 MeV neutron were determined using an off-line γ-ray spectrometric technique. The 14.7 MeV quasi-monoenergetic neutron beam was provided by the K-400 D-T neutron generator at China Academy of Engineering Physics (CAEP). Fission products were measured by a low background high purity germanium gamma spectrometer. The neutron flux was obtained from the ⁹³Nb (n, 2n)^92mNb reaction, and the mean neutron energy was calculated using the cross-section ratios for the ⁹⁰Zr(n, 2n)⁸⁹Zr and ⁹³Nb(n, 2n)^92mNb reactions. With a series of corrections, high precision cumulative yields of 20 fission products were obtained. Our FPYs for the ²³⁸U(n, f) reaction at 14.7 MeV were compared with the existing experimental nuclear reaction data and evaluated nuclear data, respectively. The results will be helpful in the design of a generation-IV reactor and the construction of evaluated fission yield databases.     

The (n, 2n) excitation functions for93Nb and103Rh with special respect to the isomeric states in92Nb and102Rh

By means of the activation technique the excitation functions for the reactions⁹³Nb(n,2n)^92mNb(10.15d),¹⁰³Rh(n,2n)^102mRh(2.9y), and¹⁰³Rh(n,2n)^102gRh(206d) were measured with an average total uncertainty of about ±8% between 10 and 20 MeV neutron energy. In addition the total⁹³Nb(n, 2n) cross-section was compared with the⁵⁹Co(n, 2n) cross-section at 16.8 MeV by direct neutron detection using the time-of-flight technique. The results are compared with statistical theory, especially with theoretical expectations for the isomeric cross-section ratios, which are only in reasonable agreement with the experiment if one assumes a ground state spinI _g=5 for⁹²Nb andI _g=2 for¹⁰²Rh.     

Isomeric ratios in photonuclear reactions of molybdenum isotopes induced by bremsstrahlung in the giant dipole resonance region

We have determined the isomeric ratios of isomeric pairs ^97m,gNb, ^95m,gNb and ^91m,gMo produced in ⁹⁸Mo(γ, p)^97m,gNb, ⁹⁶Mo(γ, p)^95m,gNb and ⁹²Mo(γ, n)^91m,gMo photonuclear reactions in the giant dipole resonance (GDR) region by the activation method. The results were analyzed, discussed and compared with the similar data from literature to examine the role of excitation energy, neutron configuration, channel effect and direct and pre-equilibrium processes in (γ, p) photonuclear reactions. In this work the isomeric ratios for ^97m,gNb from 14 to 19 MeV, for ^195m,gNb from14 to 24 MeV except 20 and 23.5 MeV and for ^91m,gMo at 14 and 15 MeV are the first time measurements.     

Moments of charge distributions in the reaction92Mo+92Mo at 14.7 MeV/u

First and second moments of primary charge distributions were determined as a function of the total kinetic energy loss in the reaction⁹²Mo+⁹²Mo at an incident energy of 14.7 MeV/u. Up to energy losses of 200 MeV no significant drift of the first moments is observed. The second moments are in agreement with predictions of a stochastic model derived at lower bombarding energies.     

Alpha scattering from 92Zr and 94Zr

Scattering of 35.4 MeV α particles from ⁹²Zr and ⁹⁴Zr has been studied with an energy resolution of 25–30 keV. Angular distributions were measured from 10 to 45 degrees for an E_x range of up to 6.1 MeV and 4.4 MeV for ⁹²Zr and ⁹⁴Zr, respectively. Several new spin assignments have been made by comparing angular distributions with collective DWBA calculations. An implicit folding procedure was used to derive isoscalar transition rates, which for E_x > 2.5 MeV were previously unknown. Most of the levels are well described by a vibrational model form factor.     

Low-lying levels of 92Nb from the 92Zr(3He,t) and 92Zr(3He,p2nγ) reactions

The structure of ⁹²Nb has been investigated using the 33.8 MeV ⁹²Zr(³He, t) and (³He, p2nγ) reactions. Several previously unobserved levels, including several belonging to the $\text{π(}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)ν(}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}{}^{\mathrm{?1}}$ multiplet, are reported. The results are discussed in terms of the shell model.     

Gamma-gamma directional correlation study in92Zr

The gamma-gamma directional correlation of the 2⁺′-2⁺-0⁺, 913(Iγ=1.69)-934(Iγ =100)keV cascade in⁹²Nb decay has been investigated with a NaI-Ge(Li) system. Our results yieldδ=?0.013 _?0.024 ^+0.041 . This is one of a very few cases where the second 2⁺ to first 2⁺ transition is not predominatelyE2. This may be related to the closed neutron shell, as earlier suggested. [Radioactivity⁹²Zr; measuredγ-γ(θ), deducedδ]     

Multipolarities of γ-rays from 92, 94Nb and 94,95,96,97,98Tc

^{92, 94}Nb and ^{94, 96, 98}Tc have been produced by the (p, n) reaction at proton energies on and near the $\text{d}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}$ isobaric analog resonance. ^95,97Tc have been produced by the (p, γ) reaction below the (p, n) threshold. Internal conversion electrons due to the decay of their excited states were detected on-line with a mini-orange spectrometer which is optimized for the energy range 50 to 500 keV. Gamma rays from these nuclei were detected with a thin Ge(Li) detector. Isomeric-delayed internal conversion electrons and γ-rays were observed, using a nanosecond-pulsed beam. The internal conversion coefficients for 55 transitions in these nuclei have been determined and their multipolarities deduced. The multipolarity of the transitions in these nuclei is predominantly M1. Negative parities have been assigned through use of the $\text{d}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}$ isobaric analog resonance enhancements of the population of negative-parity final states. The systematic behavior of the 2^?, 3^? doublet and of the $\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{?}\text{d}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}$ multiplet in these nuclei is discussed.     

Energy levels in 93Mo populated by the 93Nb(p,nγ) reaction

Energy levels of ⁹³Mo have been investigated by means of the ⁹³Nb(p, nγ)⁹³Mo reaction. The excitation functions of the level de-excitation γ-rays were measured with a Ge(Li) detector under proton bombardment in the energy range 3.0 to 5.0 Me V. A detailed γ-ray decay scheme which includes 69 levels and 123 γ-ray lines was constructed from the threshold energies for 64 γ-rays and the γ-ray excitation functions around five isobaric analogue resonances in the ⁹³Nb(p, nγ) reaction. Spin-parity values for 59 levels and favourable values for 8 levels were assigned from the analysis of relative neutron yields via the isobaric analogue resonances of the parent odd-odd nucleus ⁹⁴Nb. The results of the present experiment are compared with shell-model calculations.     

Study of low-lying states in 92Tc with the 92Mo(3He,t) reaction

States in ⁹²Tc have been studied by means of the ⁹²Mo(³He, t) reaction at 27.5 MeV. The Q-value for this reaction and the excitation energy of the isobaric ground state analogue of ⁹²Mo were determined to be ?7.882 ± 0.030 MeV and 3.813 ± 0.030 MeV respectively. Strongly populated levels in ⁹²Tc appear to belong to configurations arising from the $\text{(1g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}{}_{\mathrm{\pi }}\text{(1g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}{}_{\mathrm{\nu }}{}^{\mathrm{?1}}$ multiplet.     

Absence of proton weak coupling states in93Nb

The reactions⁹³Nb(p, p)⁹³Nb,⁹³Nb(p, n)⁹³Mo, and⁹³Nb(p, p′) through isobaric analog resonances in⁹⁴Mo have been used to study the structure of low-lying⁹³Nb states, specifically the degree to which these states can be described as single protons coupled to the core states of⁹²Zr. Excitation curves were obtained from 5.8 to 7.6 MeV incident proton energy, for eight states in⁹³Nb. Results of this work are compared to results from Coulomb excitation studies,⁹³Nb(n, n′γ),⁹³Nb(d,p),⁹²Zr(³He,d),⁹⁴Mo(d,³He) and other related work.     

The level structure of92Ru up to high spin values

The level structure of⁹²Ru has been studied by means of γ-ray spectroscopy. The nucleus was produced by the⁵⁸Ni(⁴⁰Ca, α2p)⁹²Ru reaction at beam energies of 147 and 187 MeV. The NORDBALL detector system including particle selection was used. A large number of new levels with excitation energies up to 11.3 MeV and spin values up to 22 or 23 units of angular momentum have been established. The level scheme is compared with recent shell model calculations using¹⁰⁰Sn as a core. Some systematics of the g ₉ ^2/?2 configuration is discussed and a strong correlation between the levels in⁹⁰Mo and⁹²Ru is found.     

First identification and shell model structure of92Rh

Excited states in theN=47 nucleus⁹²Rh were populated via the fusion evaporation reaction⁵⁸Ni(⁴⁰Ca,αpn)⁹²Rh at 180 MeV beam energy. A level scheme reaching up to about 7 MeV and probable spins of (19⁺) and (21^?) was established and interpreted with the shell model in the (p _1/2,g _9/2) model space.