Intrinsic states,high-spin rotational bands and rotation alignment in 177Os and 179Os

Low-lying intrinsic states and their associated rotational bands have been identified in ¹⁷⁷Os and ¹⁷⁹Os. They are the mixed i_{$\text{13}\text{2}$} neutron states and the $\text{1}\text{2}$^?[521] states in ¹⁷⁷Os and ¹⁷⁹Os, as well as the $\text{5}\text{2}$^?[512] state in ¹⁷⁷Os and the $\text{7}\text{2}$^?[514] state in ¹⁷⁹Os. The $\text{1}\text{2}$^? sta is assumed to be the ground state, the other intrinsic states giving rise to isomers. The in-band decay properties of the $\text{7}\text{2}$^?[514] band, and the i_{$\text{13}\text{2}$} bands show the effect of mixing. In the rotational bands in ¹⁷⁷Os a low frequency backbending anomaly is observed but no anomaly is observed in the i_{$\text{13}\text{2}$}. band. In ¹⁷⁹Os the i_{$\text{13}\text{2}$} band does backbend but at a higher frequency than in the yrast bands of the even neighbours. The systematics of the backbending frequencies, and the effects of blocking, are discussed. The rotation aligned angular momentum is deduced, and a comparison made between the i_{$\text{13}\text{2}$} bands and the s-bands in the even neighbours. The results broadly support the identification of the s-bands with the aligned (i_{$\text{13}\text{2}$})² configuration.     

Intrinsic and rotational excitations in 175Lu

The γ-ray cascades following the ¹⁷⁶Yb(p, 2n)¹⁷⁵Lu reaction are studied with Ge(Li) detectors and interpreted within the level scheme of ¹⁷⁵Lu. According to this interpretation the $\text{1}\text{2}$⁺[411], $\text{1}\text{2}$^?[541], $\text{5}\text{2}$⁺[402], $\text{7}\text{2}$⁺[404] and $\text{9}\text{2}$^?[514] rotat $\text{15}\text{2}$⁺, $\text{21}\text{2}$^?, $\text{13}\text{2}$⁺, $\text{19}\text{2}$⁺ and $\text{19}\text{2}$^? members, respectively. Fu band head is determined to be 626.6 keV. The data for the rotational bands are discussed within the particle-rotor model and compared with the available information on the corresponding bands in the adjacent Lu isotopes.     

High spin rotational states in 154Dy, 164Er And 162Yb

High spin rotational states in ¹⁵⁴Dy, ¹⁶⁴Er and ¹⁶²Yb have been investigated with (α, 4nγ) and (α, 6nγ) reactions. The ground state rotational bands have been identified up to spin 14 for ¹⁵⁴Dy and ¹⁶²Yb and spin 16 for ¹⁶⁴Er. Anomalous behaviour of the moment of inertia has been observed in ¹⁶⁴Er.     

Ground-state rotational band in 181Ta

The ground-state rotational band in ¹⁸¹Ta has been observed up to a spin of $\text{21}\text{2}{}^{\mathrm{+}}$ using Coulomb excitation with ⁸⁴Kr ions. The nuclear lifetimes of the band members have been determined from the Doppler-broadened lineshapes of the de-excitation γ-rays, and the angular distributions of the γ-rays have been measured. It is found that the E2 transition rates from higher spin states $\text{(≧}\text{17}\text{2}{}^{\mathrm{+}}\text{)}$ are retarded relative to the rotational model predictions. A suggestion is made that this retardation may be due to the Coriolis antipairing effect.     

Transition probabilities in the doubly odd nuclei 176Lu and 182Ta

The depopulation of isomeric states in ¹⁷⁶Lu and ¹⁸²Ta was studied in the (n, γ) reaction by means of delayed γ-γ coincidence measurements with NaI(Tl) and Ge(Li) detectors. The following half-lives, unknown so far, have been obtained for ¹⁷⁶Lu: $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{(198.0}\text{keV}\text{) = 35.0 ± 1.0}\text{ns}$, $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{(638.8}\text{keV}\text{) = 8.0±1.0}\text{ns}$ and $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{(662.1}\text{keV}\text{) = 6.3±0.5}\text{ns}$; and for ¹⁸²Ta: $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{(270.4}\text{keV}\text{) = 1.2 ± 0.2}\text{ns}$, $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{(402.6}\text{keV}\text{) = 1.00 ± 0.05}\text{ns}$ and $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{(443.6}\text{keV}\text{) = 2.2 ± 0.2}\text{ns}$. The existence of the isomeric level at 443.6 keV in ¹⁸²Ta was confirmed. Weisskopf hindrance factors have been deduced for the K- and Ω-forbidden transitions. The K-allowed transitions are considered in terms of the Nilsson model taking into account pairing correlations. The experimental results for the transitions de-exciting the 270.4 keV level in ¹⁸²Ta agree with earlier model predictions including band mixing effects. The influence of the pairing effect on K-allowed E1 transitions in doubly odd nuclei is demonstrated.     

The 181Ta(γ, π+)181Hf reaction

Yields for the reaction ¹⁸¹Ta(γ, π⁺)¹⁸¹Hf have been measured by an activation method using bremsstrahlung radiation with end-point energies in the range 150–360 MeV. The data have been unfolded to give cross section results corresponding to bombarding with monoenergetic photons. A comparison is made with respect to previous results and a semiclassical cascade-model calculation.     

Magnetic moments of high-spin states above the rotational band of 168Hf and 172Hf

The transient magnetic field IMPAC technique was used to measure the magnetic moments of high-spin states above the rotational band of ¹⁶⁸Hf and ¹⁷²Hf, populated in the reactions ^{156, 160}Gd(¹⁶O, 4n). The average g-factors of these prerotational feeding states were deduced to be 0.07 ± 0.04 and 0.14 ± 0.04 for ¹⁶⁸Hf and ¹⁷²Hf, respectively. These results are in agreement with a reduction of the collective g-factors due to a neutron phase transition.     

One- and three-quasiparticle states in 171Hf and high spin rotational bands

The $\text{1}\text{2}{}^{\mathrm{?}}\text{[521]}\text{and}\text{7}\text{2}{}^{\mathrm{+}}\text{[633]}$ one-quasiparticle bands in the N = 99 nucleus ¹⁷¹Hf have been identified to spins of about $\text{45}\text{2}$ using (heavy ion, xn) reactions. The moments of inertia of these bands are consistent with the absence of backbending in the N = 98 core nucleus. The half-life of the $\text{5}\text{2}{}^{\mathrm{?}}\text{[512]}$ intrinsic state was measured as 63.6 ns. The strength of the $\text{5}\text{2}{}^{\mathrm{?}}\text{[512] →}\text{7}\text{2}{}^{\mathrm{+}}\text{[633]}\text{E}\text{1}$ transition is discussed. Two three-quasiparticle isomers with spins and parities $\text{19}\text{2}{}^{\mathrm{+}}\text{and}\text{23}\text{2}{}^{\mathrm{?}}$ have been identified and their suggested configurations are a $\text{7}\text{2}{}^{\mathrm{+}}\text{[633]}$ neutron added to the 6⁺ and 8^? two-quasiproton states of the core. The moment of inertia of a rotational band based on the $\text{23}\text{2}{}^{\mathrm{?}}$ isomer supports this suggestion, and shows the effect of partial rotation alignment of the $\text{i}{}_{\mathrm{<mtext>13</mtext><mtext>2</mtext>}}$ neutron.     

Elastic and Raman scattering of 8.5–11.4 MeV photons from 175Lu and 181Ta

Differential cross sections for elastic and inelastic Raman scattering from ¹⁷⁵Lu and ¹⁸¹Ta were measured. Five photon energies between 8.5 and 11.4 MeV were used and were obtained from the (n, γ) reaction on Ni and Cr using thermal neutrons. The results are compared with calculations using a modified simple rotator model (SRM) of the giant dipole resonance (GDR) in which the effect of Delbrück scattering was incorporated. In general, fair agreement between theory and experiment is obtained. A new set of GDR parameters is extracted, based on photon scattering data and, as expected, yield better agreement between experimental and predicted cross sections.     

Reactions of 40Ar with 159Tb, 142Nd and 144Sm; New α-activities from 189Bi, 173Pt and 177Au

Reactions of ⁴⁰Ar ions with targets of ¹⁵⁹Tb, ¹⁴²Nd, and ¹⁴⁴Sm have been studied at energies below 300 MeV with a helium gas-jet system. Excitation functions for (Ar, xn) reactions, where x = 5–10, were obtained for the radioactive products that decay by α-emission. Based on the characteristics of these excitation functions and on the systematics of α-decay, evidence is presented for the existence of the nuclides ¹⁸⁹Bi with α-particle energy E_α = 6.67±0.01 MeV and half-life < 1.5 sec, and ¹⁷³Pt with E_α = 6.19±0.01 MeV; and for the emission from ¹⁷⁷Au of an α-particle with E_α = 6.15±0.01 MeV.     

High-spin states in 107Sn and 107In isotopes

The isotopes ¹⁰⁷Sn and ¹⁰⁷In were produced through the ¹⁰⁶Cd(³He, 2n)¹⁰⁷Sn and ¹⁰⁶Cd(³He, pn)¹⁰⁷In reactions. They were studied by means of γ-spectroscopy, excitation functions, γγ coincidences and angular distributions of γ-rays. A level scheme is proposed for the newly discovered ¹⁰⁷Sn, and new states belonging to ¹⁰⁷In are given. Microscopic calculations have been performed in a three-quasiparticle approximation for a large number of tin isotopes in order to get a wide view of the systematic evolution of the various states.     

Neutron hole states in 138La and 140Pr

Protons accelerated to 30 MeV were used to investigate low-lying states in the odd-odd nuclei ¹³⁸La and ¹⁴⁰Pr with (p, d) reactions. The elastic scattering of 30 MeV protons and 23 MeV deuterons was also studied to determine optical potentials. Experimental angular distributions are compared with distorted-wave Born approximation calculations to extract spin, parity, and spectroscopic factors for levels up to 432 keV of excitation in ¹⁴⁰Pr and 530 keV in ¹³⁸La. Comparisons with the simple shell-model predictions and extended shell-model calculations are presented. The ¹⁴⁰Pr levels appear experimentally to have an almost pure particle-hole structure whereas the ¹³⁸La levels exhibit substantial mixing.     

High-spin states of 39K and 42Ca

High-spin states of ³⁹K and ⁴²Ca have been investigated with the ²⁸Si(¹⁶O, αpγ)³⁹K and ²⁸Si(¹⁶O, 2pγ)⁴²Ca reactions at a beam energy of 45 MeV. Gamma-gamma coincidence, γ-ray angular distribution and linear polarization measurements were performed with a Ge(Li)-NaI(Tl) Compton suppression spectrometer and a three-crystal Ge(Li) Compton polarimeter. High-spin states of ³⁹K at E_x = 7.14,7.78and8.03 and of ⁴²Ca at E_x = 7.75MeV are established. Unambiguous spin-parity assignments of $\text{J}{}^{\mathrm{\pi }}\text{=}\text{11}\text{2}{}^{\mathrm{?}}\text{,}\text{13}\text{2}{}^{\mathrm{?}}\text{,}\text{15}\text{2}{}^{\mathrm{+}}\text{,}\text{15}\text{2}{}^{\mathrm{?}}\text{,}\text{17}\text{2}{}^{\mathrm{+}}\text{and}\text{19}\text{2}{}^{\mathrm{?}}$ to the ³⁹K levels at E_x = 5.35, 5.72, 6.48, 7.14, 7.78 and 8.03 MeV and of 6^?, 7^?, 8^?, 9^? and(8, 10)^? to the ⁴²Ca levels at E_x = 5.49, 6.15, 6.41, 6.55 and 7.37 MeV, respectively, have been obtained. Further spin-parity restrictions, lifetime limits, excitation energies, branching ratios and multipole mixing ratios are reported. Discrepancies with previous J^π assignments are discussed in detail.     

High-spin states in 58Ni

High-spin states of ⁵⁸Ni were investigated via the study of in-beam γ-ray induced by the compound reaction ⁴⁸Ti(¹²C, 2n)⁵⁸Ni between 26 and 48 MeV. The energies and decay modes of these levels were determined from the analysis of γ-γ coincidence measurements at 35 MeV. The most intense lines in the ⁵⁸Ni γ-ray spectrum correspond to a cascade to the ground state, through levels at 1.454, 2.459, 3.619 and 4.381 MeV, also fed in other reactions, and by two previously unknown levels at 5.125 and 5.662 MeV; the spin assignments based on the present study are (apart from the ground state) 2, 4, 4, 5, 6 and 7 respectively for these levels. The first three were already known and the last three are new. The mixing ratios for the transitions between these levels are also determined. We observe also the same cascade in the reaction ⁵⁶Fe(α, 2n)⁵⁸Ni at an incident energy 18–24 MeV. Comparisons with other reactions, previous studies and recent shell-model calculations are presented.     

High-spin states in 38K

High-spin states in ³⁸K are investigated with the ²⁴Mg(¹⁶O, pnγ)³⁸K reaction at $\text{E(}{}^{16}\text{O}\text{) = 36–44}\text{MeV}$. A recently developed Compton-suppression spectrometer with 120 msr solid angle and a pulsed beam are employed to study their γ-decay. For the E4 transition from the isomeric level at E_x = 3458 keV to the ground state a branching ratio of (0.15 ± 0.02)% is found. On the basis of angular distribution and polarization measurements, in which the delayed feeding component is eliminated, spin-parity assignments are obtained of J^π(2646 keV) = (2, 4)^?, J^π(3420 keV) = (4, 6)^? and J^π(3458 keV) = (5, 7)⁺. Prompt-delayed and prompt γγ coincidence experiments are performed to locate high-spin levels above the isomer. Hitherto unobserved levels of high spin are found at E_x = 5254, 7397, 8693, 8747 and 10980 keV and assignments of J^π = (9⁺), (10^?), (12^?), (11^?) and (13^?) respectively, are suggested by weak-coupling considerations. The experimental results are compared with a large-scale shell-model calculation performed in a configuration space with a ²⁸Si core and ten active particles distributed over the ($\text{2}\text{s}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{, 1}\text{d}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}\text{, 1}\text{f}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}\text{, 2}\text{p}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}\text{)}$ shells. The high-spin states appear to have a rather simple shell-model structure.     

High-spin states in 208Rn

The yrast decay scheme of ²⁰⁸Rn has been investigated up to spin $\text{≈ 20}\text{h}\text{?}$ and an excitation energy of ≈ 6 MeV. Several different γ-ray spectroscopic techniques were used to determine the properties of excited states and transitions in the nucleus. Significant changes to the previously established level scheme are proposed, based on the existence of an unobserved 3.1 keV transition. Simple empirical shell-model calculations of level energies aided in the assignment of shell-model configurations to excited states and the decay scheme is discussed in terms of these configurations. The energy level systematics for the even radon isotopes, from A = 206 to 212 are discussed, as are core polarization effects in the even radon isotopes (A = 204 to 210) and polonium isotopes (A = 202–208).     

Excited states in 216Ra

Excited states in ²¹⁶Ra have been studied using in-beam spectroscopic techniques. The reactions used were ²⁰⁸Pb(¹²C, 4n)²¹⁶Ra and ²⁰⁸Pb(¹³C, 5n)²¹⁶Ra at 80 and 95 MeV, respectively. The level scheme of ²¹⁶Ra was extended up to the (28^?) state at 6266 keV. Two new isomers, whose mean lives are 8.7 ± 0.6 ns and 9.7 ± 0.9 ns, were found to be the 19^? state at 3763 keV and the (25^?) state at 5170 keV. Levels up to the (25 ^?) state in ²¹⁶Ra are interpreted as arising from the weak coupling of two neutrons to the excited states in ²¹⁴Ra.     

Single-proton states in 151Pm

The ${}^{152}\text{Sm}\text{(}\text{t}\text{, α)}{}^{151}\text{Pm}$ reaction was studied using 17 MeV polarized tritons from the tandem Van de Graaff accelerator at the Los Alamos Scientific Laboratory. The α-particles were analyzed using a Q3D magnetic spectrometer and detected with a helical-cathode position-sensitive counter. The overall resolution was ～ 18 keV FWHM. Measurements of the ¹⁵⁰Nd(³He, d)¹⁵¹Pm reaction were made using 24 MeV ³He beams from the McMaster University tandem accelerator. The deuteron spectra were analyzed with a magnetic spectrograph using photographic emulsions for detectors, yielding a resolution of ～ 13 keV FWHM. By comparing the measured angular distributions of ($\text{t}\text{, α}$) and (³He, d) cross sections and ($\text{t}\text{, α}$) analyzing powers with DWBA predictions it was possible to assign spins and parities to many levels. The present results confirm earlier assignments of rotational bands based on the low-lying $\text{5}\text{2}{}^{\mathrm{+}}\text{[413],}\text{5}\text{2}{}^{\mathrm{?}}\text{[532],}\text{3}\text{2}{}^{\mathrm{+}}\text{[411]}\text{and}\text{1}\text{2}{}^{\mathrm{+}}\text{[420]}$ orbitals. In addition, states at higher excitation have now been assigned to the $\text{1}\text{2}{}^{\mathrm{+}}\text{[411]}\text{and}\text{7}\text{2}{}^{\mathrm{+}}\text{[404]}$ orbitals, and members of the $\text{3}\text{2}{}^{\mathrm{+}}\text{[422],}\text{5}\text{2}{}^{\mathrm{+}}\text{[402],}\text{3}\text{2}{}^{\mathrm{?}}\text{[541]}\text{and}\text{7}\text{2}{}^{\mathrm{?}}\text{[523]}$ bands are tentatively proposed. The spectroscopic strengths can be explained reasonably well by the Nilsson model when pairing and Coriolis mixing effects are included.     

High-spin states in 34CI

High-spin yrast states in ³⁴Cl have been studied with the reactions ³¹P(α, nγ)³⁴Cl at E_α = 11.7?16.3 MeV and ²⁴Mg(¹²C, pnγ)³⁴Cl at E(¹²C) = 32–35 MeV. Ambiguities in the ³⁴Cl level scheme for levels at E_x = 4.82 and 5.32 MeV have been resolved through combination of threshold measurements with the ³¹P + α reaction and gamma-gamma coincidence and E_γ-measurements with the ²⁴Mg + ¹²C reaction. Gamma-gamma coincidence and in-beam γ-γ angular correlation experiments have been performed employing a Compton-suppression spectrometer with a solid angle of 120 msr.Unambiguous spin-parity assignments of J^π = 6^?, 5⁺ and 7⁺ to the ³⁴Cl levels at E_x = 4.74, 4.82 and 5.32 MeV, respectively, are obtained.Previously unreported levels of high spin are found at E_x = 7.25 and 7.80 MeV with J^π = (9⁺) and (8⁺); τ_m = 200 ± 70 fs and 100 ± 70 fs, respectively. Excitation energies, mean lives, branching ratios and multipole mixing ratios are reported. The experimental results are compared with large-scale shell-model calculations. The high-spin yrast levels can be characterized by a rather simple shell-model structure.     

High-spin states in 90Nb

The high-spin states in ⁹⁰Nb have been studied by in-beam γ-ray spectroscopy using the 35 MeV ⁸⁹Y(α, 3nγ)⁹⁰Nb and 33 MeV ⁹⁰Zr(³He, p2nγ)⁹⁰Nb reactions. A new isomeric state with half-life 0.44±0.02 σs and J^π = 11^? has been located in this nucleus. The level scheme derived from these measurements is compared with shell-model calculations.