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1.
We deposited amorphous Bi films with a thickness between 3 and 6.5 nm at 4.2 K on top of previously deposited Co clusters having a mean size of ~4.5 nm. The Co cluster layers thickness was between 2.3 and 5 nm. In-situ electrical transport measurements were performed between 2 and 100 K. Measurements on as-prepared samples having a Bi layer thickness of 3.0 nm show hopping (tunneling) conductivity as σ(T) = σ 0 exp[?(T 0/T)1/2] above the superconducting transition temperature T C and re-entrance behavior again with hopping (tunneling) conductivity below T C . Annealing of films having a Bi layer thickness of 5.5 nm results in a decrease of resistivity, with variable-range hopping conduction behavior as σ(T) = σ 0 exp[?(T 0/T)1/3 ]. Quite different are the findings for films having a Bi layer thickness of 6.5 nm: annealing of these films results in a power-law behavior as σ(T) = σ 0 T α with α = 2/3, indicating that these films are close to a quantum critical point separating superconducting and insulating phases. A phase diagram including all experimental observations is proposed.  相似文献   

2.
The ultraviolet bands of mercury bromide have been excited in uncondensed discharge and photographed with a quartz Littrow spectrograph. The class II system, lying betweenλ 2900 å to 2700 å, suggested byWieland as due to the triatomic molecule, has been studied in detail and ascribed to the diatomic molecule. The bands in the regionλ 2900 å to 2770å have been analysed into two systems which may form the two components of a2 II ?2 σ electronic transition with a2 II interval equal to 969·4 cm?1. Another system most probably due to2 σ?2 σ has been observed in the regionλ 2770 to 2720.  相似文献   

3.
We report on measurements of the electrical conductivity on a two-dimensional packing of metallic disks when a stable current of ~1 mA flows through the system. At low applied currents, the conductance σ is found to increase by a pattern σ(t) = σ ? Δσ E α [ ? (t/τ) α ], where E α denotes the Mittag-Leffler function of order α ∈ (0,1). By changing the inclination angle θ of the granular bed from horizontal, we have studied the impact of the effective gravitational acceleration g eff = gsinθ on the relaxation features of the conductance σ(t). The characteristic timescale τ is found to grow when effective gravity g eff decreases. By changing both the distance between the electrodes and the number of grains in the packing, we have shown that the long term resistance decay observed in the experiment is related to local micro-contacts rearrangements at each disk. By focusing on the electro-mechanical processes that allow both creation and breakdown of micro-contacts between two disks, we present an approach to granular conduction based on subordination of stochastic processes. In order to imitate, in a very simplified way, the conduction dynamics of granular material at low currents, we impose that the micro-contacts at the interface switch stochastically between two possible states, “on” and “off”, characterizing the conductivity of the micro-contact. We assume that the time intervals between the consecutive changes of state are governed by a certain waiting-time distribution. It is demonstrated how the microscopic random dynamics regarding the micro-contacts leads to the macroscopic observation of slow conductance growth, described by an exact fractional kinetic equations.  相似文献   

4.
Eliashberg theory is generalized with account of the specific properties of two-band electron-phonon (EP) systems. The superconducting transition temperature T c is examined in two-band materials, one of the representatives of which are pnictides. The strong EP coupling and the pairing within the full width of the electron band and not only in a narrow region near the Fermi surface are taken into account. It is found that the effect of the pairing of electrons belonging to different bands is crucial to the appearance of high T c in these materials. It is shown that the high T c value in the materials, such as pnictides, is displayed with the use of a two-band spectral function of the EP interaction derived from calculations and from tunnel experiments. The existence of specific conditions for the high T c appearance in the two-band materials is established.  相似文献   

5.
The magnetite/maghemite content within iron oxide nanoparticles can be determined using the mean isomer shift (\(\overline {\delta }\)). However, accurate characterisation of the composition is limited by the uncertainty associated with \(\overline {\delta }\). We have identified four independent sources of uncertainty and developed a quantitative expression for the uncertainty budget. Sources of uncertainty are categorised as follows: that from the fitting of the Mössbauer spectrum (σ fit), that of the calibration of the α-Fe reference spectrum (σ cal), thermal corrections to the spectrum due to second order Doppler shift (SODS) (σ Δδ ) and other experimental errors (σ err). Each contribution is discussed in detail using 57Fe Mössbauer spectra obtained from an iron oxide nanoparticle system at temperatures between 16 K and 295 K on different spectrometers in two different laboratories.  相似文献   

6.
For a single-band conductor where two or more scattering mechanisms are present, each giving rise to a characteristic thermoelectric powerS n and a electrical resistivity? n the resultant thermoelectric powerS is given, as a first approximation, by\(S = \sum\limits_n {\varrho _n S_n /\varrho } \). Denoting withS 0 the characteristic thermoelectric power due to the scattering of the conduction electrons by the boundary atoms, and withS i and? i the resultant thermoelectric power and electrical resistivity arising from all other scattering mechanisms, one may writeS=S 0+? i(S i?S 0)/?. The thermoelectric powerS and the electrical resistivity? of thin layers of potassium, evaporated in a vacuum ~5·10?9 Torr on a glass substrate at 90° K temperature, were measured at different thicknesses. The variation ofS as a function of 1/? verifies the above mentioned relation. Thus, the thermoelectric power, characteristic for the scattering by potassium boundary atoms can be determined.  相似文献   

7.
We consider mass-conserving self-similar solutions for Smoluchowski’s coagulation equation with kernel K(ξ,η)=(ξη) λ with λ∈(0,1/2). It is known that such self-similar solutions g(x) satisfy that x ?1+2λ g(x) is bounded above and below as x→0. In this paper we describe in detail via formal asymptotics the qualitative behavior of a suitably rescaled function h(x)=h λ x ?1+2λ g(x) in the limit λ→0. It turns out that \(h \sim 1+ C x^{\lambda/2} \cos(\sqrt{\lambda} \log x)\) as x→0. As x becomes larger h develops peaks of height 1/λ that are separated by large regions where h is small. Finally, h converges to zero exponentially fast as x→∞. Our analysis is based on different approximations of a nonlocal operator, that reduces the original equation in certain regimes to a system of ODE.  相似文献   

8.
State equation P(V/V 0, T) and baric dependences of thermal properties of diamond have been obtained without any fitting parameters from the interatomic pair Mie–Lennard-Jones potential and the Einstein model of a crystal. Calculations have been performed along two isotherms (at T = 300 and 3000 K) up to P = 10000 kbar = 1000 GPa, i.e., to a relative volume of V/V 0 = 0.5. The baric dependences have been obtained for the following characteristics: isothermal elastic modulus B T and B'(P), isochoric heat capacity C v and C v ' (P), isobaric heat capacity C p ; thermal expansion coefficient α p and α p ' (P); and specific surface energy σ, as well as its derivatives σ'(P) and σ'(T). It is shown that for P → ∞, functions B T (P) and σ(P) vary linearly, functions B'(P), α p (P), C v (P), C p (P) and σ'(P) tend to constants, while functions α p '(P), C v '(P), and difference C p (P)–C v (P) tend to zero. Good agreement with experimental data has been demonstrated.  相似文献   

9.
By the method of functional integration the two-point functionS F for the spinor model with the interaction\( - \lambda (\bar \psi \psi )^2 \) is calculated in a two-dimensional space-time. After Fourier-transformationS F (p) results as a power series with respect to 1/√λ. If we change the order of terms, we get a series in powers of γp. Each coefficient is a series in powers of 1/√λ. The first terms of this series are considered as a good approximation for bigλ. By reasons of convergence of the integrals we must displace the expansion centre of the series in powers ofγ p fromp 2=0 top 2=a 2.  相似文献   

10.
We study the asymptotic structure of the first K largest eigenvalues λ k,V and the corresponding eigenfunctions ψ(?;λ k,V ) of a finite-volume Anderson model (discrete Schrödinger operator) \(\mathcal{H}_{V}= \kappa \Delta_{V}+\xi(\cdot)\) on the multidimensional lattice torus V increasing to the whole of lattice ? ν , provided the distribution function F(?) of i.i.d. potential ξ(?) satisfies condition ?log(1?F(t))=o(t 3) and some additional regularity conditions as t→∞. For zV, denote by λ 0(z) the principal eigenvalue of the “single-peak” Hamiltonian κΔ V +ξ(z)δ z in l 2(V), and let \(\lambda^{0}_{k,V}\) be the kth largest value of the sample λ 0(?) in V. We first show that the eigenvalues λ k,V are asymptotically close to \(\lambda^{0}_{k,V}\). We then prove extremal type limit theorems (i.e., Poisson statistics) for the normalized eigenvalues (λ k,V ?B V )a V , where the normalizing constants a V >0 and B V are chosen the same as in the corresponding limit theorems for \(\lambda^{0}_{k,V}\). The eigenfunction ψ(?;λ k,V ) is shown to be asymptotically completely localized (as V↑?) at the sites z k,V V defined by \(\lambda^{0}(z_{k,V})=\lambda^{0}_{k,V}\). Proofs are based on the finite-rank (in particular, rank one) perturbation arguments for discrete Schrödinger operator when potential peaks are sparse.  相似文献   

11.
An analysis is made of the thermoelectric and galvanomagnetic properties of solid solutions based on bismuth and antimony chalcogenides (Bi,Sb)2(Te,Se,S)3 with n-and p-type conductivities and different substitutions in the Bi2Te3 sublattices. It is shown that the thermoelectric efficiency Z is observed to increase in compositions with a low carrier scattering anisotropy in the reflection plane. The relaxation time tensor component τ 33 along the trigonal direction perpendicular to the crystal growth axis is found to decrease as compared to the components along the binary (τ 11) and bisector (τ 22) directions.  相似文献   

12.
An electric Molecular-Beam-Resonance-Spectrometer has been used to measure simultanously the Zeeman- and Starkeffect splitting of the hyperfinestructure of TlF. Electric fourpole lenses served as focusing and refocusing fields of the spectrometer. A homogenous magnetic field (Zeeman-Field) was superimposed to the electric field (Stark-Field) in the transition region of the apparatus. The observedΔm J =±1 -transitions were induced electrically. Completely resolved spectra of Tl205F19 in theJ=1 rotational, andυ=0 vibrational state have been measured. The obtained quantities are: The rotational magnetic momentμ J of Tl205F19 in the stateJ=1,υ=0, and the difference of the magnetic shielding (σ 1,±1?σ 1,0) of both nuclei as well as the difference of the molecular susceptibility (ξ 1,±1?ξ 1,0) in the states (J, m J)=(1,±1) and (J, mJ)=(1, 0). The sign of the rotational magnetic moment could be determined unambigously by the influence of offdiagonal matrix elements. The numerical values for Tl205F19 in the stateJ=1 andυ=0 are:μ J =?29,153(21) · 10?6 μ Bohr (σ 1,±1?σ 1,0)Tl=?0,002291 (33) (σ 1,±1?σ 1,0)F=?0,000206(9) (ξ 1,±1-ξ 1,0)=+3,02(15) · 10?30erg/Gauß2 The quantities in brackets are root-mean-square deviations in units of the last digit. From these data and the known values for the spin-rotational interaction constants a number of expressions are derived which characterise the electronic charge distribution in the molecule.  相似文献   

13.
We have found a possible example of the rare decayσ + →nΜ + Ν, which violatesδS=δQ. The positive decay track of theσ + comes to rest in the hydrogen bubble chamber and decays into ane +. This track has all the characteristics of a stoppingΜ +. The decay neutron fortuitously scatters twice, producing two recoil protons. The only other possible interpretation of the event isσ +nγ(π + →Μ + Ν), where theπ + →Μ + Ν decay produces no deflection (θ<0.1 rad) and no significant change in curvature. Using thep-wave radiative decay predictions ofBarshay et al. we calculate that the integrated branching ratio for such “accidental” events isγ(σ + →nγ(π + →Μ stop + Ν))/γ(σ + →nπ +)=1.6×10?6. Most of the contribution to this “accidental” branching ratio comes from radiative decays where theπ + mesons have ranges less than 1 mm (p π<20 MeV/c). If one excludes thoseΜ's with ranges less than 1.2 cm the above “accidental” branching ratio becomes 5.5×10?7. With this figure we estimate that we should have seen 6.5×10?2 events of this type thusfar in our experiment. The neutron momentum does not help in deciding between the two hypotheses. We therefore assign a confidence level of 7% for the radiative hypothesis. For the leptonic hypothesis we obtain an estimate of the branching ratio,γ(σ + →nΜ + Ν)/γ(σ + →nπ +)=5×10?5. If one further accepts theσ + →nπ + Ν event reported byBarbaro-Galtieri et al. and theσ + →ne + Ν event reported byNauenberg et al., one obtains theδS=?δQ leptonic branching ratio [γ(σ + →nΜ + Ν)+γ(σ + →ne + Ν)]/γ(σ + →nπ +)=(4±3)×10?5.  相似文献   

14.
The dimension D of a polycrystalline film and the optical anisotropy m = εzx of uniaxial crystallites with the principal components εx = εy and εz of the tensor of the dielectric constant have been shown to produce a strong influence on the effective dielectric constant εD* and the effective refractive index nD* = (εD*)1/2 of the film in the optical transparency region, as well as on the boundaries of the intervals BDl ≤ εD*BDu. The intervals Δ2(m) = B2lB2u and Δ3(m) = B3lB3u are separated by a gap for m in the range 1 < m < 2, whereas the theoretical dependence ε2*(m) is separated by a gap from the interval Δ3(m) for m in the range 1 < m < 4. This is confirmed by a comparison of the experimental (noP) and theoretical (nD*) ordinary refractive indices for uniaxial polycrystalline films of the conjugated polymer poly(p-phenylene vinylene) (PPV) with uniaxial crystallites and appropriate values of m. In the visible transparency region of the PPV films with a change in m(λ) in the range 2 < m(λ) < 3 due to the dependence of the components εx,z(λ) on the light wavelength λ, the refractive indices noP2(λ) = εoP(λ) are consistent with the theoretical values of ε2*(λ) and lie outside the interval Δ3(m). For m(λ) > 3 near the electronic absorption band of the crystallites, the values of εoP(λ) lie in the region of the overlap of the intervals Δ2(m) and Δ3(m). The boundaries mc of the range 1 < m < mc are determined, for which the interval Δ2(m) is separated by a gap from the dependences ε3*(m) corresponding to the effective medium theory with spherical crystallites and hierarchical models of a polycrystal, as well as from the proposed new dependence ε3*(m).  相似文献   

15.
Nine experimental isomeric cross-section ratios for the reactions59Co(n, γ)60Co,60Ni(n,p)60Co, and63Cu(n,α)60Co are analysed in terms of statistical theory by means of the method ofHuizenga andVandenbosch. Theγ-cascades are treated by a new model which was recently published. The results confirm the energy dependence of the spin cut-off factor for60Coσ~U1/4 which should not be neglected. As a mean value (σ=4.3±0.3 is obtained forU=B n =7.5 MeV in good agreement with a nuclear moment of inertia for a rigid sphere.  相似文献   

16.
The effects caused by vapor inhomogeneity over liquid helium are considered. Both pure isotopes have surface levels, whose population increases with temperature T. We separated their contribution to the temperature dependence of surface tension σ3(T) and σ4(T) and compared our theoretical results with the results of Japanese experimental works [1–3]. For liquid He3, one has σ3(T)=σ3(0)?σ 3 T2 at 0.2 K<T<1 K and σ3(T)=σ3(0)?α 3 0 T2exp(?Δ3/T) at T<0.2 K, with Δ3≈0.25 K. For liquid He4, σ4(T)=σ4(0)?AT7/3? α 4 0 T2exp(?Δ4/T) at T<2 K, where A is the Atkins constant and Δ4≈4 K. The parameters α 3 0 , α 3 , and α 4 0 depend on the fluid properties.  相似文献   

17.
The imaginary parts of microwave conductivity σ″(T<Tc) and resistivity ρ (T)=1/σ(T>Tc) along (σ ab and ρab) and across and (σ c and ρc the cuprate ab planes of a YBa2Cu3O7?x crystal with the oxygen doping level x varying from 0.07 to 0.47 were measured in the temperature range 5≤ T≤200 K. In the superconducting state, the σ ab (T)/σ ab (0) and σ c (T c (0) curves coincide for an optimally doped (x=0.07) crystal, but, with an increase in x, the slopes of the σ c (T)/σ c (0) curves decrease noticeably at T<Tc/3, on the background of small changes happening to the σ ab (T ab (0) curves. The two-dimensional (2D) transport along the ab planes in the normal state of YBa2Cu3O7?x is always metallic, but there is a crossover (at x=0.07) from the Drude to hopping (at x>0.07) conductivity along the c axis. This is confirmed both by the estimates of the lowest metallic and the highest tunneling conductivities along the c axis and by quantitative comparison of the measured ρc(T) curves with the curves calculated in the polaron model of quasiparticle transport along the c axis.  相似文献   

18.
Liquid Argon was irradiated with bremsstrahlung from 18 to 31 MeV endpoint energy in steps of 2 MeV. The yields of the reactions Ar40(γ, n)+(γ, p) and Ar38(γ, n) were measured by detecting the 269a and the 35d rest activity with a low-level-counter. Cross section curves for the (γ, n)-processes could be found from the yield values, and they allowed together withσ N, σ(γ, p) andσ(γ, np) a determination ofσ(γ, 2n) and σγabs for Ar40. The integrated cross section forσ(γ, n) from threshold to 33 MeV yields (200±40) MeVmb for Ar40 and (210±40) MeVmb for Ar38, the corresponding value for σγabs being (450±60) MeVmb for Ar40.  相似文献   

19.
We numerically study the thermoelectric transport in AB- and AA-stacked bilayer graphene in the presence of a strong magnetic field and disorder. In the AB-stacked case, we find that the thermoelectric conductivities display different asymptotic behaviors, depending on the ratio between the temperature and the width of the disorder-broadened Landau levels (LLs), similar to those of monolayer graphene. In the high temperature regime, the transverse thermoelectric conductivity α xy saturates to a universal value 5.54k B e/h at the center of each LL, and displays a linear temperature dependence at low temperatures. The calculated Nernst signal has a peak with a height of the order of k B /e, and the thermopower changes sign at the central LL. We attribute this unique behavior to the coexistence of particle and hole LLs. In the AA-stacked bilayer case, it is found that the thermoelectric transport properties are consistent with the behavior of a band insulator. The obtained results demonstrate the sensitivity of the thermoelectric conductivity to the band gap near the Dirac point.  相似文献   

20.
The effect of a uniaxial mechanical compression (σm ≤ 100 bar) on the spectral dependences (300–800 nm) of the birefringence Δn i and refractive indices n i of K2SO4 crystals is studied. The electronic polarizabilities, refractions, and parameters (λ0i , B 1i ) of ultraviolet oscillators of mechanically compressed crystals are calculated. It is shown that the dispersions of Δn i(λ) and n i(λ) are normal and sharply increase near the absorption edge. It is found that the uniaxial compression changes the value of the dispersions dΔn i/dλ and dn i/dλ rather than their character. It is ascertained that the simultaneous action of the compressions σx and σz, as well as of σy and σz, leads to the appearance of new isotropic states in the K2SO4 crystal, which manifests itself in the equality of corresponding birefringences. It is shown that the baric dependences n i(σ) are determined by the change in the density of oscillators (~30%), by the shift of the absorption edge and effective band maximum and by the change in the oscillator strength (~70%).  相似文献   

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