Kondo effect in a deformed molecule coupled asymmetrically to ferromagnetic electrodes

The nonequilibrium Kondo effect is studied in a molecule quantum dot coupled asymmetrically to two ferromagnetic electrodes by employing the nonequilibrium Green function technique. The current-induced deformation of the molecule is taken into account, modeled as interactions with a phonon system, and phonon-assisted Kondo satellites arise on both sides of the usual main Kondo peak. In the antiparallel electrode configuration, the Kondo satellites can be split only for the asymmetric dot-lead couplings, distinguished from the parallel configuration where splitting also exists, even though it is for symmetric case. We also analyze how to compensate the splitting and restore the suppressed zero-bias Kondo resonance. It is shown that one can change the TMR ratio significantly from a negative dip to a positive peak only by slightly modulating a local external magnetic field, whose value is greatly dependent on the electron--phonon coupling strength.     

Kondo Effect Versus Magnetic Coupling in Indirectly Coupled Double Quantum Dots

We theoretically investigate a device consisting of two quantum dots(QDs) side-coupled to a quantum wire which has many physicalingredients of an artificial heavy fermion system. An extra parameter, the distance L between the two QDs, is introduced and it plays an important role on the competition of the Kondo temperature and magnetic coupling. Three different phases are found: antiferromagnetic phase, Kondo phase with spin S=1/2, and Kondo phase with S=1, depending on the distance L, the magnetic coupling, and the Kondo temperature. Quantum transport properties are qualitatively different for different phases: for the S=1 Kondo and the antiferromagnetic phases, the conductance tends to the unitary value 2e²/h; for the S=1/2 Kondo phase the conductance is strongly dependent on the distance.     

Tunability of the Kondo effect in an asymmetrically tunnel coupled quantum dot

The transport properties of a single quantum dot were measured at low temperature in a regime of strong asymmetric tunnel coupling to leads. By tuning this asymmetry, the two parameters of the Kondo effect in a quantum dot, the Kondo temperature and the zero-bias zero-temperature conductance, were independently controlled. A careful analysis of the Coulomb energies and of the tunnel couplings was performed. It allowed an estimate of the Kondo temperature independently of its value obtained via the temperature dependence of the conductance. Both are in good agreement. We finally compared our experimental data with an exact solution of the Kondo problem which provides the dependence of the differential conductance on temperature and source-drain voltage. Theoretical expectations fit quite well our experimental data in the equilibrium and out-of-equilibrium regimes.     

Phonon-assisted Kondo effect in single-molecule quantum dots coupled to ferromagnetic leads

Based on the infinite-U Anderson model spin-polarized transport through the tunnel magnetoresistance (TMR) system of single-molecule quantum dot is investigated under the interplay of strong electron correlation and electron-phonon (e-ph) coupling. The spectral density and the nonlinear differential conductance are studied using the extended non-equilibrium Green's function method through calculating the dot-level splitting self-consistently. The results exhibit that a serial of peaks emerge on the two sides of the main Kondo peak for the antiparallel magnetic configuration of electrodes, while for the parallel case both the main and phonon-assisted satellite Kondo peaks all split up into two asymmetric peaks even at zero-bias. Correspondingly, the nonlinear differential conductance displays a set of satellite-peaks around the Kondo-peak in the presence of the e-ph interaction. Furthermore, extra maxima and minima appear in the TMR curve. The TMR alternates between the positive and the negative values along with the variation of bias voltage.     

Localization length in anderson insulator with Kondo impurities

The localization length, xi, in a two-dimensional Anderson insulator depends on the electron spin scattering rate by magnetic impurities, tau(-1)(s). For antiferromagnetic sign of the exchange, the time tau(s) is itself a function of xi, due to the Kondo correlations. We demonstrate that the unitary regime of localization is impossible when the concentration of magnetic impurities, n(M), is smaller than a critical value, n(c). For n(M)>n(c), the dependence of xi on the dimensionless conductance, g, is reentrant, crossing over to unitary, and back to orthogonal behavior upon increasing g. Sensitivity of Kondo correlations to a weak parallel magnetic field results in a giant parallel magnetoresistance.     

Heat and spin transport in magnetic nanowires

Transport measurements are carried out in which temperature oscillation is applied to magnetic nanostructures. Using spin valves, this measurement reveals aspects of the spin transport in non-collinear configurations. In one implementation, an AC voltage is detected when a DC current is driven through the nanostructure under test and its temperature is made to oscillate by illuminating it with a laser diode. A simpler approach is presented that relies on Joule heating to generate the temperature oscillation, thus eliminating the need for any optical component.     

The Bilinear and Intrinsic Biquadratic Coupling in Magnetic Metallic Trilayers

We find the exact Green's functions of the Anderson s-d mixing model for magnetic trilayers with arbitrary spin canting angle between two ferromagnetic layers within the rneanfield theory of the on-site Coulomb repulsion. A bilinear exchange coupling and an intrinsic biquadratic coupling which does not vanish in the limit of flat interfaces is obtained by those Green's functions. It is shown that both of these couplings oscillate in the experimental range of the spacer thickness only when the s-d mixing is strong enough. When the mixing strength is large enough one finds that the oscillation period of the intrinsic biquadratic term is equal to half of the corresponding one for the bilinear term. We also find that the temperature dependence of those interlayer couplings is considerably enhanced with the decrease of the Hubbard coupling. It is also shown that the biquadratic coupling falls off much more rapidly with increasing temperature than the bilinear one.     

AC Conductance Through a Vibrating Molecular Dot in Kondo Regime

In the present paper, by applying the Lang-Firsov canonical transformation and the so-called non-crossing approximation technique, we investigate the joint effects of the electron-phonon interaction and an external alternating gate voltage on the transport of a quantum dot system in the Kondo regime. We find that, while the satellite Kondo resonant peaks appear in both the averaged local density of states and the differential conductance, the main Kondo peak at the Fermi energy is greatly suppressed. These results confirm the previous ones derived by other methods, such as the equation of motion solution. Furthermore, based on the picture of virtual transition between quasi-eigenstates in the system, we also give a slightly different explanation on these phenomena.     

Kondo effect of an adsorbed cobalt phthalocyanine (CoPc) molecule: the role of quantum interference

It has been shown that by distorting a CoPc molecule adsorbed on a Au(111) surface a Kondo effect is induced with a temperature higher than 200 K. We examine a model in which an atom with strong Coulomb repulsion (Co) is surrounded by four atoms on a square (molecule lobes), with two atoms above and below it representing the apex of the STM tip and an atom on the gold surface (all with a single atomic orbital). The Hamiltonian is solved exactly for the isolated cluster, and, after connecting the leads, the conductance is calculated by standard techniques. Quantum interference prevents the existence of the Kondo effect when the orbitals on the square do not interact (undistorted molecule); the Kondo resonance shows up after switching on that interaction. The weight of the Kondo resonance is controlled by the interplay of couplings to the STM tip and the gold surface and between the molecule lobes.     

Is the quantum dot at large bias a weak-coupling problem?

We examine the two-lead Kondo model for a dc-biased quantum dot in the Coulomb blockade regime. From perturbative calculations of the magnetic susceptibility, we show that the problem retains its strong-coupling nature, even at bias voltages larger than the equilibrium Kondo temperature. We give a speculative discussion of the nature of the renormalization group flows and the strong-coupling state that emerges at large voltage bias.     

Conductance oscillations and transport spectroscopy of a quantum dot

Results are reported for low temperature measurements of the conductance through small regions of a two-dimensional electron gas (2 DEG). An unconventional GaAs heterostructure is used to form a 2 DEG whose density can be tuned by the gate voltage applied to its conductive substrate. Electron beam lithography is used to pattern a narrow channel in the 2 DEG interrupted by two constrictions, defining a small 2 DEG island between them. The conductance is found to oscillate periodically with the gate voltage, namely with electron density. Calculations of the capacitance between the substrate and the island show that the period of oscillation corresponds to adding one electron to the island. The oscillatory behavior results primarily from the discreteness of charge and the Coulomb interaction between electrons. However, the observed temperature dependence of these oscillations requires a more sophisticated treatment which includes the quantized electron energy levels as well. The magnetic field dependence of the oscillations allows us to extract the discrete energy spectrum of the quantum dot in the quantum-Hall regime.     

Identification of Radial Distance of Plasma Dispersionless Injection Boundary from the Injection Source

Measurements of energetic particles obtained by the two geosynchronous satellites （1991-080 and LANL-97A） are performed to investigate the plasma injection boundary and source region during the magnetospheric substorms. The measurement method is developed to allow remote sensing of the plasma injection time and the radial distance of injection boundaries by using measured energy dispersion and modelling particle drifts within the Volland-Stern electric field and the dipole magnetic field model. The radial distance of the injection boundary deduced from a dispersion event observed by the LANL-97A satellite on 14 June 1998 is 7.1RE, and the injection time agrees well with the substorm onset time identified by the Polar Ultraviolet Imager. The method has been applied to an event happened at 22.9 UT on 11 March 1998, when both the satellites （1991-080 and LANL-97A） observed the dispersionless character. The results indicate that the radial distance of injection source locates at 8.1RE at magnetotail, and particles move earthward from magnetotail into inner magnetosphere at 22.5 UT.     

Anomalous curie response of impurities in quantum-critical spin-1/2 Heisenberg antiferromagnets

We consider a magnetic impurity in two different S=1/2 Heisenberg bilayer antiferromagnets at their respective critical interlayer couplings separating Néel and disordered ground states. We calculate the impurity susceptibility using a quantum Monte Carlo method. With intralayer couplings in only one of the layers (Kondo lattice), we observe an anomalous Curie constant C*, as predicted on the basis of field-theoretical work [S. Sachdev, Science 286, 2479 (1999)10.1126/science.286.5449.2479]. The value C* = 0.262 +/- 0.002 is larger than the normal Curie constant C=S(S+1)/3. Our low-temperature results for a symmetric bilayer are consistent with a universal C*.     

Effects of interactions in transport through Aharonov-Bohm-Casher interferometers

We study the conductance through a ring described by the Hubbard model (such as an array of quantum dots), threaded by a magnetic flux and subject to Rashba spin-orbit coupling (SOC). We develop a formalism that is able to describe the interference effects as well as the Kondo effect when the number of electrons in the ring is odd. In the Kondo regime, the SOC reduces the conductance from the unitary limit, and, in combination with the magnetic flux, the device acts as a spin polarizer.     

Coherent quantum transport in two-dimensional electron gas/superconductor double junctions with Rashba spin-orbit coupling

Based on the extended Blonder-Tinkham-Klapwijk (BTK) approach, we have investigated the coherent quantum transport in two-dimensional electron gas/superconductor (2DEG/SC) double tunneling junctions in the presence of the Rashba spin-orbit coupling (RSOC). It is found that all the reflection coefficients in BTK theory as well as conductance spectra oscillate with the external voltage and energy. The oscillation feature of conductance can be tuned largely by the RSOC for low insulating barriers, while for high insulating barriers it is almost independent of the RSOC. These phenomena are essentially different from those found in ferromagnet/superconductor double tunneling junctions.     

Kondo tunneling through real and artificial molecules

When an asymmetric double dot is hybridized with itinerant electrons, its singlet ground state and lowly excited triplet state cross, leading to a competition between the Zhang-Rice mechanism of singlet-triplet splitting in a confined cluster and the Kondo effect (which accompanies the tunneling through quantum dot under a Coulomb blockade restriction). The rich physics of an underscreened S = 1 Kondo impurity in the presence of low-lying triplet-singlet excitations is exposed and estimates of the magnetic susceptibility and the electric conductance are presented, together with applications for molecule chemisorption on metallic substrates.     

嵌入单量子点Aharonov-Bohm环中的近藤效应

使用单杂质的Ansderson模型, 从理论上研究了一个嵌入单量子点Aharonov-Bohm环系统处在 近藤区时的基态性质, 并用slave-boson平均场方法求解了该模型.结果表明：在零温, 当介 观环内电子平均能级间隔大于近藤关联能时, 系统内仍然存在一个被减弱了的近藤效应；系 统的基态性质依赖于系统的宇称和环的大小；而尺寸效应和近藤屏蔽效应的共存导致了系统 丰富的物理性质.同时, 可以通过测量介观环中的持续电流和杂质磁化率, 达到探测近藤屏 蔽云的目的. 关键词： 持续电流 杂质磁化率 宇称效应 近藤效应 近藤屏蔽云     

Observation of microwave-induced zero-conductance state in Corbino rings of a two-dimensional electron system

Using Corbino samples we have observed oscillatory dc conductance in a high-mobility two-dimensional electron system when it is subjected to crossed microwave and magnetic fields. At the strongest of the oscillation minima the conductance is found to be vanishingly small, indicating a macroscopic insulating state associated with this minimum. With increasing voltage bias, a crossover from Ohmic to electron-heating regime is observed.     

Universal scaling and a novel quantum critical behavior of CeRhSb1-xSnx

We observe and explain a universal scaling rhochi = const for the electrical resistivity rho with the inverse magnetic susceptibility chi(-1) for the Kondo insulator CeRhSb(1-x)Snx. In the regime where the Kondo gap disappears (x > 0.12), the system forms a non-Fermi liquid (NFL), which transforms into a Fermi liquid at higher temperature. The NFL behavior is associated with the presence of a novel quantum critical point (QCP) at the Kondo insulator-correlated metal boundary. The divergent behavior of the resistivity, the susceptibility, and the specific heat has been observed when approaching the QCP from the metallic side and is interpreted as due to the competition between the Kondo and the intersite magnetic correlations.     

Kondo model for the "0.7 anomaly" in transport through a quantum point contact

Experiments on quantum point contacts have highlighted an anomalous conductance plateau around 0.7(2e(2)/h), with features suggestive of the Kondo effect. Here, an Anderson model for transport through a point contact analyzed in the Kondo limit. Hybridization to the band increases abruptly with energy but decreases with valence, so that the background conductance and the Kondo temperature T(K) are dominated by different valence transitions. This accounts for the high residual conductance above T(K). The model explains the observed gate-voltage, temperature, magnetic field, and bias-voltage dependences. A spin-polarized current is predicted even for low magnetic fields.