PAMELA spectrum of electrons and positrons of cosmic rays in the energy range of 0.05–1.2 TeV

A proprietary method is used to process measurement data from a high-energy particle (protons, electrons, and positrons with Е ≥ 50 GeV) spectrometer in a near-Earth orbit. The data from three detector systems are used: a tracker in a constant magnetic field (TRK), a calorimeter (CAL), and a neutron detector (ND). A relatively simple and efficient way of isolating electrons and positrons from the total charged particle flux entering the PAMELA spectrometer is proposed. A technique for determining the energy of isolated primary particles and retrieving their energy spectra is described. The composite electron and positron spectrum (below, the total electron and positron flux is referred to simply as the electron flux) for energies up to 1.5 TeV is presented.     

Measurement of 10–100 TeV cosmic ray anisotropy at upgraded Carpet-2 installation

The first results obtained during one year of measurements at the upgraded shower Carpet-2 installation at the Baksan Neutrino Observatory of the Institute for Nuclear Research, Russian Academy of Sciences, are presented. The results of calculation of the energy response of the installation are given. The results of data analysis using the standard method and the East-West method are compared. The constraints on amplitudes of harmonics of solar anisotropy for three values of primary energy: E > 12 TeV, E > 40 TeV, and E > 70 TeV, are obtained.     

The absorption spectrum of 12C2H2 IV. The regions 7600–9200 cm−1 and 10600–11500 cm−1

The absorption spectrum of ¹²C₂H₂ has been recorded by intracavity laser absorption spectroscopy (ICLAS) in the 10600–11 500 cm^?1 spectral region, where no absorption bands were previously reported. Fifteen bands starting from the vibrational ground state are observed and rotationally analysed. All corresponding excited vibrational levels were assigned using the polyad model, the so-called cluster model (El Idrissi, M.I., Liévin, J., Campargue, A., and Herman, M., 1999, J. chem. Phys., 110, 2074) which allows vibrational energies, rotational B_v constants and, to some respect, relative band intensities to be predicted. Additional data and constants are also provided in the range 7600–9200cm^?1, whenever improving the literature results, from spectra recorded previously at ULB using Fourier transform spectroscopy. The assignment procedure in the range recorded by ICLAS is detailed, leading to a deeper understanding of vibration-rotation and intensity features of the absorption bands within the frame of the cluster model.     

The infrared spectrum of isoxazole in the range 600–1400 cm−l,including a high-resolution study of the v 7(A′) band at 1370.9 cm−1 and the v 16(A″) band at 764.9 cm−l,together with ab initio studies of the full spectrum

Abstract

The high resolution infrared gas phase spectrum of isoxazole in the range 600–1400 cm^?1 has been recorded and more precise centres obtained for a number of bands; analyses of the v ₇(A′) band at 1370.9cm^?1 and the v ₁₆(A″) band at 764.9cm^?1 have been performed. Use of the Watson Hamiltonian, A-reduction, III^r-representation and simultaneous analysis of the present IR and previous microwave data, has led to rotation constants and quartic centrifugal distortion constants Δ _J , Δ _JK , ΔK, δ _J and δ _K for the ground state and for the v ₁₆ vibrationally excited states. The equilibrium structures and the derived harmonic frequencies have been calculated by ab initio methods using triple zeta+polarization (TZVP) and cc-pVTZ basis sets, with MP2, MP4 and CCSD(T) methods. At each methodology, for closest numerical agreement between the calculated and observed rotation constants, the optimum basis set seems to be TZVP rather than cc-pVTZ basis sets. However, the order of the highest A″ and lowest A′ symmetry vibrations is only resolved by the cc-pVTZ basis set with the MP4 methodology, which does generate the experimental sequence (v ₁₄>v ₁₃) The CCSD(T) methodology does not lead to significant difference over either MP2 or MP4 with the TZVP basis set.     

The infrared spectrum of isothiazole in the range 600–1500 cm−1, including a high-resolution study of the v 11(A′) band at 818 cm−1 and the v 16(A″) band at 727 cm−1, together with ab initio studies of the full spectrum

Abstract

The gas-phase high-resolution infrared spectrum of isothiazole in the range 600–1500 cm^?1 has been recorded, and revised band centres obtained for a number of vibrations. An analysis of the v ₁₁(A′) band at 818 cm^?1 and the v ₁₆(A″) band at 727 cm^?1 has been performed, using the Watson Hamiltonian, A-reduction, III^r representation. These were combined with previous microwave spectral data to provide combined analyses for rotational constants and quartic centrifugal distortion constants Δ _J , Δ _JK , Δ _K , δ _j and δ _K . These extend the knowledge derived from previous microwave and IR spectral studies. The equilibrium structures and the derived harmonic frequencies were calculated by ab initio methods, using a variety of basis sets with MP2, MP4 and CCSD(T) methods, and a comparison of these with experimental data is discussed. At a pragmatic level, the closest correlation of the rotational constants with experiment is not obtained with the most sophisticated methodology. Similarly, the vibration frequencies and intensities also vary strongly with the procedure. In particular, we found that the cc-pVTZ+MP2 results probably provide the best numerical comparison with experimental IR data for this molecule.     

The absorption spectrum of 12C2D2 in the 10000–12500 cm−1 spectral region

The absorption spectrum of dideuteroacetylene has been recorded by intracavity laser absorption spectroscopy (ICLAS) in the 10 200–12 500cm^?1 spectral region. Among 25 absorption bands of ¹²C₂D₂ rotationally analysed in this spectral region, 17 are newly observed. They include one II_u-Σ⁺ _g and thirteen Σ⁺ _u-Σ⁺ _g bands starting from the vibrational ground state and eleven hot bands from the V ₄ = 1 and V ₅ = 1 lower states. The rotational structure of two excited levels is affected by a strongly J-dependent interaction with a perturber which induces intensity transfer to extra lines. The coupling is identified as a I-resonance interaction with δ_u dark states and the vibrational assignment of the perturbers is discussed. Two Σ-Σ bands of the ¹²C¹³ CD₂ species, present in natural abundance in the sample, could also be identified and rotationally analysed. Most of the corresponding excited vibrational levels of ¹²C₂D₂ were unambiguously assigned using the polyad model [Herman, M., el idrissi, M. I., Pisarchik, A., Campargue, A., Gaillot, A.-C., Biennier, L., di lonardo, G. and Fusina, L., 1998, J. chem. Phys., 108, 1377] which allows vibrational energies and B _V rotational constants to be predicted. In particular the previously highlighted 1/244 anharmonic resonance is confirmed by energy and intensity features in several {(V ₁, V ₂, V ₃, V ₄ = 0, V ₅ = 0),(V ₁ ?1, V ₂ + 1, V ₃ V ₄ = 2, V ₅ = 0)} dyads. Significant deviations between predicted and experimental energy levels are observed for a few levels and discussed.     

Infrared spectrum of the Ar-CO complex: observation of the v co = 2 ← 0 band at 4260 cm −1

The spectrum of the weakly-bound van der Waals complex Ar-CO has been observed for the first time in the region of the CO vibrational overtone, using a long-path (180 m) low-temperature (64 K) absorption cell and a Fourier transform infrared spectrometer. The appearance of the spectrum was very similar to that studied previously in the v _co = 1 ← 0 region. However, it was very much weaker, so a detailed analysis was only possible for the relatively uncongested K = 1 ← 0 and 0 ← 1 subbands. The parameters determined here for these sub-bands should help to constrain the C-O bond length dependence of the Ar-CO intermolecular potential in future theoretical models.     

Parameters of the energy spectrum of semiconductive solid solutions of the tetradic system (AlSb)x(HgTe)1−x

From the analysis of the spectra of photoluminescence and transparency in the temperature interval (2–77) K there are determined in the paper, the gap-width and its temperature coefficient as a function of the composition of the melt of (AlSb)_x(HgTe)_1–x. It is shown that for compositions (0.8 x 1) with a lowering of the temperature, the edge of the fundamental absorption is shifted into the domain of large energies, and for compositions (0.05 , x 0.20) with a lowering of temperature, the edge of the fundamental absorption is shifted into the long-wave domain of the spectrum. The dependence of E_g(x, T) has a nonlinear character.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 4, pp. 67–70, April, 1991.     

About the character of the “Knee” at E⋍3×1015 eV in the energy spectrum and the mass composition of primary cosmic rays in the energy range 1015–1017 eV

The method of rescaling from the muon-multiplicity spectrum to the extensive-air-shower spectrum as a function of the total muon number n _μ is presented. The method allows a direct comparison of data obtained in different experiments with muon groups. A direct comparison of data at n _μ>1800 and n _μ=76–660 has been performed. The data in the region n _μ=75–3500 agree better with the assumption that the slope change in the energy spectrum of primary cosmic rays occurs approximately at the same energy per nucleus, E _c=3×10¹⁵ eV, and the mass composition in the energy range 10¹⁵–10¹⁷ eV is close to that observed at 10¹⁴ eV.     

The high-resolution infrared spectrum of ethylene in the 1800–2350 cm−1 spectral region

Fourier transform spectra of ethylene (C₂H₄) have been recorded in the 1800–2350?cm^?1 (4.3–5.6?µm) spectral region using a Bruker IFS125HR spectrometer at a resolution of 0.004?cm^?1 leading to the observation of six vibrational bands, ν ₇?+?ν ₈, ν ₄?+?ν ₈, ν ₆?+?ν ₁₀, ν ₆?+?ν ₇, ν ₄?+?ν ₆ and ν ₃?+?ν ₁₀. The corresponding upper state ro-vibrational levels were fit using a Hamiltonian matrix accounting for numerous interactions. A satisfactory fit could be obtained using a polyad of nine interacting states {8¹10¹,?7¹8¹,?4¹8¹,?8¹12¹,?6¹10¹,?6¹7¹,?4¹6¹,?3¹10¹,?3¹7¹} of which three (8¹10¹, 8¹12¹ and 3¹7¹) are unobserved dark states. As a result a much more accurate and extended set of Hamiltonian constants were obtained than previously derived. The following band centers were determined: ν ₀(ν ₇?+?ν ₈)?=?1888.9783(20)?cm^?1, ν ₀(ν ₄?+?ν ₈)?=?1958.2850(20)?cm^?1, ν ₀(ν ₆?+?ν ₁₀)?=?2047.7589(20)?cm^?1, ν ₀(ν ₆?+?ν ₇)?=?2178.011(60)?cm^?1, ν ₀(ν ₄?+?ν ₆)?=?2252.8026(24)?cm^?1 and ν ₀(ν ₃?+?ν ₁₀)?=?2171.2397(20)?cm^?1. Finally, a synthetic spectrum that could be useful for ethylene detection in planetary atmospheres was generated.     

The infrared spectrum of 12C2HD: the stretching–bending combination bands in the 1800–4700 cm−1 region

The infrared spectrum of ¹²C₂HD has been observed between 1800 and 4700?cm^?1 by Fourier transform spectroscopy. The ν₁, ν₂ and ν₃ absorption bands and the associated hot and combination bands involving the bending modes up to υ_t?=?υ₄?+?υ₅?=?2 have been investigated. Altogether, 60 vibrational bands were analysed, leading to the spectroscopic characterization of 31 vibrationally excited states. Several perturbations have been observed, but the transitions involving the perturbing states have not been detected. As a consequence, an appropriate treatment of the vibrational or ro-vibrational interactions has not been possible. A tentative assignment of the perturbing states has been proposed. Eventually, global fits for each fundamental vibration and its associated cold and hot bands have been performed.     

Influence of silver on the galvanomagnetic properties and energy spectrum of mixed (Bi1− x Sbx)2Te3 crystals

An investigation is made of the temperature dependences of the resistivity in the range 4.2–300 K, the Hall effect, and the Shubnikov-de Haas effect in magnetic fields up to 40 T in (Bi_{1? x} Sb_x)₂Te₃Ag_y single crystals (0 ≤ x ≤ 0.75). Doping (Bi_{1? x} Sb_x)₂Te₃ crystals with silver showed that in Sb₂Te₃ and (Bi_{1? x} Sb_x)₂Te₃ crystals unlike Bi₂Te₃ silver exhibits acceptor properties. The angular and concentration dependences of the Shubnikov-de Haas effect were studied in (Bi_{1? x} Sb_x)₂Te₃Ag_y. It was established that the anisotropy of the ellipsoids of the upper valence band in Bi_0.5Sb_1.5Te₃ remains unchanged as a result of silver doping.     

Assignment of a perturbation in the FT-ICLAS spectrum of 12C2H2 around 12 709.5 cm−1

The vibrational state perturbing the J = 17 and 18 rotational states of the zero-order v ₁ + 3v ₃ state of ¹²C₂H₂ is assigned to the state with vibrational energy predicted at G _ν = 12 685.1 cm^?1 using the cluster model (El Idrissi, M. I., Liévin, J., Campargue, A. and Herman, M., 1999, J. chem. Phys., 110, 2074). The assignment is discussed also in terms of the very special pressure shift behaviour demonstrated previously for absorption lines reaching these levels (Herregodts, F., Hepp, M., Hurtmans, D., Vander Auwera, J. and Herman, M., 1999, J. chem. Phys., 111, 7961). The experimental information arising from a set-up newly running at ULB, called FT-ICLAS brings decisive information in the assignment process. This set-up is described briefly.     

Reconstruction of an energy spectrum of fast neutrons (20–60 MeV) of the radex channel (INR) by the inverse problem method

A procedure for and the results from reconstruction of the energy spectrum of a beam of fast neutrons irradiating a plastic scintillator by solving the inverse problem are described. Good agreement between the reconstructed and initial spectra with different shapes of the neutron beam’s energy dependence is obtained. A similar approach can be used to determine the neutron distributions over energies in the beam of the RADEX channel (INR).     

The absorption spectrum of 12C2H2 between 12800 and 18500cm−1 II. Rotational analysis

The rotational structure of the vibrational bands of ¹²C₂H₂ is investigated in three spectral energy regions not previously systematically explored at high resolution, 12800–13500 cm^?1, 14000–15200 cm^?1 and 16500–18360 cm^?1, on the basis of new spectral data recorded by intracavity laser absorption spectroscopy. The rotational analysis of 17 new absorption bands arising from the ground state is reported (11 Σ_u ⁺ ? Σ_g ⁺ bands and 6Π_u ? Σ_g ⁺ bands). Four bands in the range studied show strong perturbations affecting both the line positions and intensities. Their detailed analysis is performed in order to determine the nature of the coupling schemes, the vibrational species and the rotational constants of the perturber states. Altogether, the vibration-rotation parameters of 21 newly observed vibrational states are derived.     

2p4n) 126Ba at the beam energy of 73 MeV. Lifetimes of the states around the

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The pentad of 12CD4: Line parameter analysis of the IR spectrum in the range 1775–2350 cm−1

In a previous paper (J.-E. Lolck, G. Poussigue, E. Pascaud, and G. Guelachvili, J. Mol. Spectrosc. 111, 235–274 (1985)), we presented the first comprehensive assignment and wavenumber analysis of high-resolution (nearly Doppler limited) rotation-vibrational spectra of the interacting upper states of the ν₁, ν₃, 2ν₂, ν₂ + ν₄, and 2ν₄ bands of the ¹²CD₄ pentad. The present paper continues this work by describing the determination and quality estimation of experimental infrared line strengths from the Fourier transform spectra. These line strengths are interpreted in terms of a theoretical model which contains, as parameters, the dipole moment derivatives and the main Hermann-Wallis coefficients of the infrared-allowed bands: ν₃(F₂), ν₂ + ν₄(F₂), and 2ν₄(F₂). This model also explains the appearance of infrared transitions to upper states, forbidden in infrared in an isolated state approach, through the mixing of states caused by the intervibrational interactions. The intensity analysis leads to the determination of all six parameters in the model and to a reproduction of the experimental intensities with a precision comparable to the experimental accuracy of 10 to 15%.