引入量子干涉的双光子共振非简并四波混频

研究了级联四能级系统中双光子共振非简并四波混频(NFWM)由于加入耦合光场而产生的量子干涉效应，发现在强耦合场作用下NFWM频谱呈现AT劈裂，它反映的是两个缀饰态的能级.量子干涉还使NFWM信号被抑制或增强.此方法牵涉到三光子共振，因此可以成为研究原子或分子高激发态的有效光谱学工具. 关键词： 四波混频 量子干涉     

缀饰态理论在碰撞能量转移过程中的应用

利用缀饰态理论研究了由分子和原子组成的混合共振系统中分子和原子之间的碰撞能量转移过程.结果发现:在单模强激光场作用下,该混合共振系统由于发生了碰撞能量转移,而使得粒子在相应能级上产生重新布居,并在一定条件下呈现出量子干涉增强效应,导致了不同缀饰态能级之间出现交叠区.这一结果与现有实验报导相符,为研究多能级系统的量子干涉效应提供了一种新的理论途径.     

在缀饰场中四能级“Ladder”系统的布局数转移

利用"反直觉"频率啁啾激光脉冲分析了偶能级ladder系统的布局数迁移,其中在缀饰激光场作用下N-2个中间态进行耦合.作为偶能级ladder系统的代表,我们着重分析了四能级ladder系统.研究发现如果缀饰激光场足够强且发生共振,则在能级1和能级4之间发生完全布局数迁移必须要求有一个恰当的脉冲叠加面积,调谐pump激光和stokes激光,使其中一个缀饰中间态发生共振,则可以使这个四能级系统简化为三能级系统.     

Y型四能级中的双电磁感应透明和超窄吸收

采用密度矩阵方程．对双光场耦合的分子Y型四能级系统的粒子数分布和吸收特性进行了计算和分析,在此能级系统中得到了双暗态共振和双电磁感应透明．并讨论了相应的物理机制。同时,我们讨论了Y型四能级两个上能级的自发辐射产生的量子干涉效应对电磁感应透明的影响,发现自发辐射干涉相消可以产生超窄线宽和导致探测光的吸收增强,自发辐射干涉相长可以展宽谱线和减弱探测光的吸收,并运用缀饰态理论对以上计算结果进行分析,与采用密度矩阵方程的计算结果一致。     

倒Y型四能级原子系统中电磁诱导透明的相干控制

研究了倒Y型四能级原子系统中相干控制电磁诱导透明.应用微扰理论给出一阶近似条件下,不同控制场原子系统对探测光场响应的解析式及电磁诱导透明窗宽度的解析式.在探测场为弱场时,分析了系统中控制光场强度、耦合光场强度及其失谐量对电磁诱导透明窗的影响.研究发现电磁诱导透明窗随控制光场强度的增强变宽,而随耦合光场强度的增强变窄,当探测光场与耦合光场偏离双光子共振时,透明窗外的吸收增加,透明窗变宽.在弱探测场、弱控制场条件下,分析了初始时刻原子处在相干叠加态时的相对相位、相对强度与探测场和控制场的相对相位等对系统吸收特性及透明窗的影响.结果表明探测场与控制场的相对相位对吸收的影响与相干叠加态中两能级之间几率幅的相对相位对吸收的影响作用相反,系统在两下能级干涉极大时,存在一个很宽的透明带.应用缀饰态理论和量子相干理论对所得结果进行了解释.     

缀饰原子系统中双光子共振非简并四波混频

本文研究了缀饰原子系统中的双光子共振非简并四波混频.理论上我们研究了多普勒增宽的四能级系统中耦合光场对双光子共振非简并四波混频的影响,发现加入强耦合场后,非简并四波混频频谱出现Autler-Townes分裂;在不同双光子共振失谐时,由于量子干涉双光子共振非简并四波混频的信号能够被抑制或增强.实验上我们在Ba原子蒸汽中,通过引入基态6s2和自电离里德堡态6pnd之间的原子相干证实了该现象.本方法提供了一种不仅可以测得共振频率和横向弛豫,而且可以测得两个高激发原子态之间的跃迁的偶极矩阵元的新的光谱学工具.     

光学外差法测量Ba原子的自电离态

提出了把三光子共振非简并六波混频(NSWM)和双光子共振非简并四波混频(NFWM)应用于研究Ba原子自电离态的光学外差探测方法。采用该方法测量了Ba原子的6P_３／２19d自电离态,并观察到了三光子共振 NSWM和双光子共振NFWM信号干涉引起的信号增强。该方法是一种纯非线性光学方法,具有优秀的空间分辨率和简单的光路。其中双光子共振非简并四波混频信号作为本地振荡光束,三光子共振非简并六波混频信号作为信号光束,通过 改变信号光束的频率来达到用光学外差探测法研究Ba原子自电离态的目的。该方法中,实现相位匹配所要求的条件不是很严格,可以在很宽的频率范围内实现相位匹配,而一般的六波混频很难做到相位匹配, 并且所测量的信号是相干光, 当用窄带宽的激光时,可以获得消多普勒的分辨率。     

微波驱动下超导量子比特与磁振子的相干耦合

实验上展示了钇铁石榴石(YIG)晶体小球中磁振子与超导量子比特的驱动缀饰态之间的相干强耦合,磁振子的加入使得在超导量子比特中形成了双重缀饰态.实验中一个钇铁石榴石晶体小球与一个超导量子比特同时放置在三维谐振腔中,分别通过磁偶极相互作用和电偶极相互作用与谐振腔中的本征场(TE102模式)耦合,并通过腔模作为媒介实现两者之间的有效相干强耦合.给超导量子比特施加一个共振的微波驱动并改变驱动强度,测得耦合系统能级劈裂随驱动强度的变化,并理论上利用粒子-空穴对与玻色场耦合的模型做了计算.在大部分的驱动强度范围内实验结果都与理论计算结果符合得较好,表明驱动下的比特-磁振子耦合系统可以用来模拟粒子-空穴对称对与玻色场的耦合系统.本文使用的混合量子系统为模拟玻色子与费米子的混合系统提供了一个新途径.     

基于简并四波混频的双信道双频段增益谱

基于大规模光通信中频分复用的需求,本文以热原子的简并四波混频为模型,研究了具有双频段特性的双信道增益光谱.一束缀饰场诱导激发态能级发生分裂,由于量子干涉效应,四波混频信号的增益在双光子共振处被抑制,从而使增益谱线的包络由单频段转变为"M"型的双频段结构.同时,缀饰场还提高了相干基态的原子布居,进一步增强了四波混频信号的强度.最终实验上在铯原子气室内获得了一对具备双频段的双信道高增益光谱,并通过调节缀饰场的强度和频率失谐,实现了对双增益峰频率间隔的有效操控.     

四能级系统中ac-Stark分裂研究

提出一双光场作用下的四能级系统,并对四能级模型的共振荧光谱作了详尽的研究.原子的共振荧光谱随Rabi频率的变化展示出能级的acStark分裂,且在很大参量范围内光谱具有这一特性.但当只有一个激发通道时不产生acStark分裂.在一定的条件下原子的共振荧光谱出现了两条黑线(darkline).可以认为acStark分裂的产生是多通道量子干涉的结果.利用缀饰态理论对acStark分裂给出很好的解释 关键词： 四能级系统模型 ac-Stark分裂 黑线(darkline) 多通道量子干涉     

Three-Photon Resonant Nondegenerate Six-Wave Mixing in a Dressed Atomic System

We report a three-photon resonant nondegenerate six-wave mixing （NSWM） in a dressed cascade five-level system. It has advantages that phase match condition is not stringent and NSWM signal is enhanced tremendously due to the multiple resonance with the atomic transition frequencies. In the presence of a strong coupling field, the threephoton resonant NSWM spectrum exhibits＂ Autler-Townes splitting. This technique provides a spectroscopic tool for measuring not only the resonant frequency and dephasing rate but also the transition dipole moment between two highly excited atomic states.     

Electromagnetically induced transparency based six-wave mixing in a Doppler-broadened folded four-level system

We study phase-conjugate six-wave mixing spectroscopy based on electromagnetically-induced-transparency in a Doppler-broadened folded four-level system.It is found that the six-wave mixing spectrum can be either Doppler-free or very broad,depending on whether the interference between the polarisations of atoms with different velocities is constructive or destructive.To obtain the Doppler-free six-wave mixing spectrum in the folded four-level system,the conditions are more stringent in comparison with those in the cascade and N-type four-level systems.This polarisation interference can be controlled in the presence of a strong coupling field.     

Dressed multi-wave mixing in a V-type four-level atomic system

The dressed four- and six-wave mixings in a V-type four-level system are considered. Under two different dressed conditions, two- and three-photon resonant Autler--Townes splittings, accompanied by enhancement and suppression of wave mixing signal, are obtained analytically. Meanwhile, an electromagnetic induced transparency of multi-wave mixing is presented, which shows multiple peaks and asymmetric effects caused by one-photon, two-photon and three-photon resonances, separately. The slow light propagation multiple region of multi-wave mixing signal is also obtained.     

消多普勒三光子共振六波混频

研究多普勒系统中的位相共轭三光子共振六波混频(SWM).得到当入射激光为窄带线宽时，SWM频谱是消多普勒的，因此可成为一种研究原子或分子高激发态和高角动量态的高分辨相干非线性光谱学.本方法还具有位相匹配条件不严格，有良好的空间分辨率，光路配置简单等优点. 关键词： 六波混频 多普勒效应     

Polarization interference of multi-wave mixing in a confined five-level system

We investigated the coexisting four-wave mixing, six-wave mixing and eight-wave mixing in ultra-thin, micrometer and long cells. Such multi-wave mixing (MWM) processes can be modified by the polarization interference. The degree of destructive interference of atomic polarizations can be controlled by the wave vector, dressing field and cell length. Specifically, the oscillation behavior of intensity and linewidth of MWM signal results from the destructive interference in ultra-thin cell. For a doubly-dressed four-wave mixing, the inner dressing field suppresses the destructive polarization interference in micrometer and long cells, induces resonance enhancement. However, the outer dressing field only enhances destructive interference.     

Competition between Dispersion and Absorption of Doubly-Dressed Four-Wave Mixing and Dressed Six-Wave Mixing

We study the competition between dispersion and absorption of doubly-dressed four-wave mixing （DDFWM） and dressed six-wave mixing. In the case of weak coupling fields limit, we find DDFWM signal is affected by destructive interference between four-wave mixing（FWM） and six-wave mixing as wen as constructive interference between FWM and eight-wave mixing. By analysing the difference between two kinds of doubly dressing mechanisms （parallel cascade and nested cascade） in this opening five-level system, we can further understand the generated high-order nonlinear optical signal dressed by multi-fields.     

Cross-molecular coupling in combined photoassociation and Feshbach resonances

We model combined photoassociation and Feshbach resonances in a Bose-Einstein condensate. When the magnetic field is far-off resonance, cross coupling between the two target molecules--enabled by the shared dissociation continuum--leads to an anomalous dispersive shift in the position of laser resonance, as well as unprecedented elimination and enhancement of resonant photoassociation via quantum interference. For off-resonant lasers, a dispersive shift and quantum interference appear similarly in resonant three-body Feshbach losses, except that the Feshbach node is tunable with intensity.     

Two-photon resonant third-harmonic generation in La2CuO4

Combining linear absorption and nonlinear third harmonic generation (THG) experiments, we investigate details of the electronic structure of the highly correlated electronic system in La2CuO4. We demonstrate strong THG mainly due to the charge transfer excitation from O (2p(sigma)) to Cu (3d(x2-y2)). The THG spectrum shows pronounced features due to three-photon and two-photon resonance enhancement as well as quantum interference effects. We obtain excellent agreement with a THG spectrum calculated in terms of the excitonic cluster model and can identify both odd and even symmetry excitation modes.