共查询到20条相似文献,搜索用时 15 毫秒
1.
S. Kawasaki T. Oka X.F. Wang Guo-qing Zheng 《Journal of Physics and Chemistry of Solids》2011,72(5):501-504
75As-zero-field nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) measurements are performed on CaFe2As2 under pressure. At P=4.7 and 10.8 kbar, the temperature dependence of nuclear-spin-lattice relaxation rate (1/T1) measured at tetragonal phase show no coherence peak just below Tc and decrease with decreasing temperature. The superconductivity is of gapless at P=4.7 kbar but evolves to multiple gaps at P=10.8 kbar. We find that the superconductivity appears near a quantum critical point. Both electron correlation and superconductivity disappear in the collapsed tetragonal phase. A systematic study under pressure indicates that electron correlations play a vital role in forming Cooper pairs in this compound. 相似文献
2.
Kosuke KakuyanagiKen-ichi Kumagai Yuji Matsuda 《Journal of Physics and Chemistry of Solids》2002,63(12):2305-2308
We report a site-selective 17O spin-lattice relaxation rate T1−1 in the vortex state of YBa2Cu4O8. We found that T1−1 at the planar sites exhibits an unusual nonmonotonic NMR frequency dependence. Based on T1−1 in the vortex core region, we establish strong evidence that the local density of states within the vortex core is strongly reduced. 相似文献
3.
Neutron scattering has been used to measure the charge and spin structure in the YBa2Cu3O6+x superconductors. Incommensurate static charge ordering is found at low doping levels while only charge fluctuations are found at higher doping. The spin structure is complex with both a commensurate resonance and incommensurate structure observed at low temperatures. The scattering results are used to construct a phase diagram for stripes in the YBa2Cu3O6+x system. 相似文献
4.
CeCoIn5 is an unconventional heavy fermion superconductor with a relatively large transition temperature . NMR measurements of the spin lattice relaxation rate at the In(1) site reveal a significant anisotropy of the fluctuating hyperfine fields, which reverses below 30 K. These results suggest that two-dimensional fluctuations of the Ce 4f moments are relevant for the superconducting pairing. 相似文献
5.
We examine the possible electron-phonon spectra that produce both Tc=39 K and an isotope coefficient β=0.32±0.01, with Eliashberg theory. We assess the viability of the conventional electron-phonon mechanism in light of these results, compared with ab initio calculations of the electron-phonon spectrum. Comparisons are made with similar considerations for low Tc materials. 相似文献
6.
R.S. Gonnelli A. CalzolariD. Daghero G.A. UmmarinoV.A. Stepanov P. FinoG. Giunchi S. CeresaraG. Ripamonti 《Journal of Physics and Chemistry of Solids》2002,63(12):2319-2323
We studied the voltage and temperature dependency of the dynamic conductance of normal metal-MgB2 junctions obtained either with the point-contact technique (with Au and Pt tips) or by making Ag-paint spots on the surface of MgB2 samples. The fit of the conductance curves with the generalized BTK model gives evidence of pure s-wave gap symmetry. The temperature dependency of the gap, measured in Ag-paint junctions (dirty limit), follows the standard BCS curve with 2Δ/kBTc=3.3. In out-of-plane, high-pressure point-contacts we obtained almost ideal Andreev reflection characteristics showing a single small s-wave gap Δ=2.6±0.2 meV (clean limit). 相似文献
7.
Measurements of the a.c.susceptibility (χ=χ′+iχ″) have been made on the Mg substituted high TC superconducting system, CuBa2(MgxCa1−x)3Cu4O12−y (Cu-1234) with x=0, 0.10 & 0.20, at different values of the a.c.field amplitude. Estimates of the intergranular critical current density(JC) made from the field dependent χ″-T curves show an improvement in the Mg-substituted Cu-1234 system. Results have been analysed in the light of the crystal structure and the superconducting anisotropy factor (γ=ξab/ξc) of the Cu-1234 system. Lower superconducting anisotropy emanating from Mg substitution has been found to be significant, resulting in better superconducting properties. 相似文献
8.
The magnetic excitation spectrum of electron-doped copper oxide superconductors is calculated using the Hubbard model on a square lattice. First, the on-site repulsion is treated with the random phase approximation. The spectrum of electron-doped systems in the superconducting state is compared with that of hole-doped systems, and the relationship between the frequency at which a peak grows in the spectrum and the superconducting energy gap at a hot spot (an intersection of the Fermi surface and the magnetic Brillouin zone boundary) is investigated. As compared with the hole-doped systems, the resonance condition is difficult to be satisfied in the electron-doped systems because of the small density of states around the hot spot. Moreover, the correlation effect in the Hubbard model is treated by the fluctuation-exchange approximation (FLEX), and the spin fluctuation spectra in the superconducting state in a wide region of the wave vector and frequency are calculated. We have found that the intensity of the magnetic spectrum at incommensurate wave vectors obtained with the FLEX is considerably weaker than that obtained with the RPA. The validity of the Fermi-liquid approach is also discussed. 相似文献
9.
The well known phenomenon of the increase of Tc of YBCO after slow cooling or low temperature annealing without change of the oxygen content, was found also for the YBCO like tetragonal superconductors of (CaxLa1−x)(LauBa1−u)2Cu3Oy (this compound has been previously denoted as CLBLCO, CLBCO or CaLaBaCuO). It has been observed at 150 and 100 °C for oxygen underdoped, optimally- and overdoped ceramics. The products retain their tetragonal unit cells. The possible reasons of this phenomenon are discussed. 相似文献
10.
We investigate the possibility of a novel kind of optical pump probe spectroscopy where the two laser pulses are focused on different areas of the sample. The response to the destruction of the superconducting state in a large part of a mesoscopic ring is studied numerically. We use the time dependent Ginzburg-Landau equations with periodic boundary conditions and external magnetic field. We evaluate the relaxation rates of the superconducting order parameter as well as the voltage induced by the charge imbalance. Computer simulations confirm that the perturbation of superconductivity on one part of the ring induces a voltage which decelerates the superconducting electrons on the other part of the ring. This deceleration results in the decrease of the superconducting current and the superfluid density. The relaxation times are of the order of the picosecond, the induced voltage of few millivolts and the variation of the superconducting gap of 10% which we believe to be suitable for time resolved femtosecond optical spectroscopy. 相似文献
11.
J.W Quilty S TajimaS Adachi A Yamanaka 《Journal of Physics and Chemistry of Solids》2002,63(12):2361-2364
We report plane-polarised Raman spectra from YBa2Cu4O8 single crystals between 300 and 10 K. In the normal state we observe a gap-like depletion of intensity from the electronic continuum extending to around 1200 cm−1 with an onset temperature of around 225 K. We remove the phonons and pseudogap depletion from the spectra using a simple model and recover a characteristic high-Tc superconductor continuum. In the superconducting state, intensity returns to the continuum in the form of a very broad pair-breaking peak. 相似文献
12.
Bond covalency and valence of elements in HgBa2Can−1CunO2n+2+δ (n=1, 2, 3, 4) were calculated and their relationship with Tc was discussed. For both oxygen and argon annealed samples, the results indicated that with the increase of n, the trend of bond covalency of Hg-O and Cu-O was the same or opposite compared with that of superconducting temperature. This may suggest that the magnitudes of Cu-O and Hg-O bond covalency are important in governing the superconducting temperature. For the highest Tc sample, Hg had the lowest valence, implying that lower valence of Hg was preferred in order to produce higher Tc. For fixed n, the valence of Cu in oxygen annealed samples was larger than that in argon annealed samples, indicating that oxygen annealed samples produced more carriers than argon annealed samples. 相似文献
13.
Y.J. Cui C.H. Cheng Y.Z. Wang Y. Zhao 《Journal of Physics and Chemistry of Solids》2011,72(5):449-452
A series of the SmFeAsO1−xFx and GdFeAsO1−xFx (x=0.05, 0.1, 0.15, 0.2, 0.25) samples have been prepared using nano-scaled ReF3 as the fluorine resource at a relatively low temperature. The samples have been sintered at 1100 and 1120 °C for SmFeAsO1−xFx and GdFeAsO1−xFx, respectively. These temperatures are at least 50-60° lower than other previous reports. All of the so-prepared samples possess a tetragonal ZrCuSiAs-type structure. Dramatically supression of the lattice parameters and increase in Tc proved that this low temperature process was more effective to introduce fluorine into REFeAsO. Superconducting transition appeared at 39.5 K for SmFeAsO1−xFx with x=0.05 and at 22 K for GdFeAsO1−xFx with x=0.1. The highest Tc was detected to be 54 K in SmFeAsO0.8F0.2 and 40.2 K in GdFeAsO0.75F0.25. The use of the nano-scaled ReF3 compounds has improved the efficiency of the present low temperature method in synthesizing the fluorine-doped iron-based superconductors. 相似文献
14.
The effects of mercury doping on the superconductivity, crystal structure, and electronic structure have been investigated in Hg-doped BaPb0.75Bi0.25O3 (BaPb0.75−xHgxBi0.25O3, BPHBO) by magnetic measurement, powder X-ray diffraction (XRD), and X-ray photoemission spectroscopy (XPS). At lower doping levels, the system is metallic and superconducting. However, the superconductivity is fully suppressed by Hg doping at x>0.25 and recovered with further increase in Hg content at x>0.3, showing a superconductivity reentrant phenomenon. XPS analysis reveals that BPHBO experiences dual metal-insulator transitions (MITs) at these two superconductivity points, which are accompanied by lattice distortions, suggesting that they may be driven by Peierls transitions. The first MIT may be a Mott-transition, while the second may be due to competition between the band filling effect and modification of the charge-disproportionate state. 相似文献
15.
Takahiro Iijima Keigo Hamada Kazunaka Endo 《Journal of Physics and Chemistry of Solids》2005,66(6):1101-1106
The temperature dependences of 2H NMR spectra and spin-lattice relaxation time T1 have been measured for paramagnetic [Mn(H2O)6][SiF6]. The obtained 2H NMR spectra were simulated by considering the quadrupole interaction and paramagnetic shift. The variation of the spectra measured in phase III was explained by the 180° flip of water molecules. The activation energy Ea and the jumping rate at infinite temperature k0 for the 180° flip of H2O were obtained as 35 kJ mol−1 and 4×1014 s−1, respectively. The spectral change in phases I and II was ascribed to the reorientation of [Mn(H2O)6]2+ around the C3 axis where the Ea and k0 values were estimated as 45 kJ mol−1 and 1×1013 s−1, respectively. From the almost temperature independent and short T1 value, the correlation time for electron-spin flip-flops, τe, and the exchange coupling constant J were obtained as 3.0×10−10 s and 2.9×10−3 cm−1, respectively. The II-III phase transition can be caused by the onset of the jumping motion of [Mn(H2O)6]2+ around the C3 axis. 相似文献
16.
D. Reznik T. Fukuda A.Q.R. Baron S. Tsutsui K. Yamada 《Journal of Physics and Chemistry of Solids》2008,69(12):3103-3107
Inelastic X-ray scattering (IXS) was used to study the Cu-O bond-stretching vibrations in the static stripe phase compound La1.48Nd0.4Sr0.12CuO4. It was found that the intrinsic width in Q-space of the previously reported huge anomalous phonon softening and broadening is approximately 0.08 r.l.u. HWHM. A detailed comparison was also made to inelastic neutron scattering (INS) studies, which indicate a two-peak lineshape (with superimposed broad and narrow peaks) in the vicinity of the anomaly. The high resolution IXS data show that the narrow peak is mostly an artifact of the poor transverse Q-resolution of INS. Otherwise, the agreement between the INS and IXS was excellent. 相似文献
17.
R.S. Gonnelli A. CalzolariD. Daghero L. NataleG.A. Ummarino V.A. StepanovM. Ferretti 《Journal of Physics and Chemistry of Solids》2002,63(12):2369-2373
We studied the doping dependence of the superconducting gap in La2−xSrxCuO4 (LSCO) by means of Andreev reflection measurements in Au/LSCO point-contact junctions. The Andreev reflection features were found to disappear at TcA close to the bulk Tc. The fit of the conductance curves with the BTK-Tanaka-Kashiwaya model gives good results if a (s+d)-wave gap symmetry is used. The low-temperature dominant isotropic gap component Δs follows very well the Tc vs. x curve, while the gap-like features observed by angle-resolved photoemission spectroscopy and tunneling scale with T∗. This confirms the different origin of these two energy scales at T<Tc. 相似文献
18.
N.J. Curro 《Journal of Physics and Chemistry of Solids》2002,63(12):2181-2185
We discuss the crossover of the form of the Cu Nuclear magnetic resonance (NMR) spin echo decay at the onset of Cu wipeout in lanthanum cuprates. Experimentally, the echo decay undergoes a crossover from Gaussian to exponential form below the temperature where the Cu NMR intensity drops. The wipeout and the change in behavior both arise because the nuclei experience spatially inhomogeneous spin fluctuations at low temperatures. We argue that regions where the spin fluctuations remain fast are localized on length scales of order 1-2 lattice spacings. The inhomogeneity is characterized by the local activation energy Ea(r); we estimate the functional form of Ea(r) for points where Ea>(r)∼0. 相似文献
19.
We report experimental results of nuclear magnetic resonance (NMR) at the La site and nuclear quadrupole resonance (NQR) at the As site in the normal state of the superconducting compound LaOs4As12. Measurements have been performed on powder sample obtained from high quality single crystals. The temperature dependences of the nuclear spin-lattice relaxation rates, 1/T1, of 75As and 139La nuclei were measured. No scaling between them was found indicating a local character of relaxation processes. The relaxation of 75As nuclei can consistently be understood in terms of antiferromagnetic spin fluctuations, as deduced from the T-dependence of (1/T1T)=C/(T−θ)1/2. 相似文献
20.
R. Okazaki H. Shishido M. Konczykowski Y. ōnuki 《Journal of Physics and Chemistry of Solids》2008,69(12):3208-3210
We report local magnetization measurements on the heavy fermion superconductor CeCoIn5 using a micro-Hall probe. Below a critical point T0 (), the local magnetization shows a clear jump at the superconducting transition temperatures for both H∥a and H∥c, indicating that the phase transition at the upper critical field Hc2 becomes a first-order phase transition. In addition, we observed an undershoot behavior of magnetization jump above (H∥c), which suggests a rapid change of textured superconducting structure with vortices and the nodal planes expected in the Fulde-Ferrell-Larkin-Ovchinnikov state. 相似文献