Muon attachment in prompt fission of237Np

The probabilities of muon attachment to fission fragments in the prompt fission of²³⁷Np have been determined as a function of fragment mass and total kinetic energy release in a ( ^–,f ₁ f ₂ e ^–)-coincidence measurement. A strong dependence of the attachment probability on the fragment mass is observed. The experimental results are compared with theoretical predictions.It is a pleasure to thank Professor T. Mayer-Kuckuk for his co-operation in performing the project. We gratefully acknowledge the permanent support of Professor J.P. Blaser and his staff at PSI. We thank Professor R. Engfer, Dr. A.v.d. Schaaf, and Dr. H.C. Walter for their support in using the electron spectrometer SIN-DRUM I. We are thankful to Professor S. Polikanov (GSI) and to Dr. T. Krogulski (University of Warsaw, Bialystok) for intensive and fruitful discussions. We appreciate the collaboration of Professor W. Müller and Dr. J. Pauwels (CBNM-Mol) in the target preparation. This work has been funded by the German Federal Minister for Research and Technology (BMFT) under the contract number 06BN271 (PD, HH, FR, ChR, WS). We thank the following institutions and organisations for financial support: Foundation for Fundamental Research on Matter (FOM), the Netherlands Organisation of the Advancement of Pure Research (NWO) (JK, CdL, AT), and the Swiss National Foundation (SNF) (WB, EH; HP, DV). One of the authors is grateful for a fellowship granted by the Studienstiftung des deutschen Volkes (FR).     

Delayed muon induced fission of209Bi and the role of meson-exchange currents

The probability for delayed muon induced fission of²⁰⁹Bi has been determined from a ( ^–,f ₁ f ₂) measurement. The measured fission probability P _f =(4.2±0.7)×10^–5 is compared with theoretical predictions. The high fission threshold reaction seems well suited for studying the influence of two-body meson-exchange currents in nuclear muon capture.We are indebted to the following institutes or organizations for financial support: Bundesministerium für Forschung und Technologie der Bundesrepublik Deutschland contract number 06 BN 271 (HP, PD, HH, FR, CR), Foundation for Fundamental Research on Matter (FOM) and the Netherlands Organization of the Advancement of Pure Research (NWO) (JK, CTAMdL, WL, AT) and the Schweizer Nationalfonds (LS).     

The decay of the isotopes179Ir and180Ir

The probability for non-radiative (n.r.) excitations in muonic²⁰⁹Bi was determined from a ( ^–,)-measurement by comparing the intensities of muonic X-ray transitions in single and coincidence spectra. The values of P_n.r(3p1s)=(17.9±2.0)% and P_n.r.(3d1s)=(3.0±2.2)% were measured for the first time. The strength of the n.r. decay of the 2p-level was found to be (4.2±2.2)%. The n.r. transition probabilities of two subcomplexes of the (2p1s)-transition leading to different mean excitation energies are (3.2±1.8)% and (5.0±2.0)%, respectively.We are indebted to the following institutes or organizations for financial support: Bundesministerium ffir Forschung und Technologic der Bundesrepubfik Deutschland contract number 06 BN 271 (HP, PD, HH, FR, CR), Foundation for Fundamental Research on Matter (FOM) and the Netherlands Organization of the Advancement of Pure Research (NWO) (JK, CTAMdL, WL, AT) and the Schweizer Nationalfonds (LS).     

AnomalousE1 conversion in octupole-deformed nuclei and muon shake-off in prompt fission

It has been shown that the coexistence of octupole and quadrupole deformation in nuclei gives rise to strong penetration effects in internal conversion for theE1 transitions. This idea has been applied for evaluating the muon shake-off probabilityW _sh. The value obtained,W _sh/–0.5% per prompt fission, is in good agreement with the experimental result. Possibilities for further experimental studies of this effect are discussed.The author would like to acknowledge fruitful discussions of the problem together with Prof. Yu.P. Gangrsky, Dr. V. Yu. Denisov and Prof. D.F. Zaretsky. He is also grateful to Prof. G.Ye. Belovitsky, Prof. P. David and Dr. Ch. Rösel for discussions of the experimental situation. This work was completed at the University of Bonn in the frame of a fellowship from the Heinrich Hertz Foundation.     

The half-life of the 1437 keV 11/2− state in97Mo

Using the (,n) reaction, the half-life of the first 11/2^– level in⁹⁷Mo has been determined as T_1/2(1437.0 keV)=2.5±0.3 ns by means of the pulsed beam method. The experimentally obtainedB(M2) value between theh _11/2 andg _7/2 configurations in⁹⁷Mo has been satisfactorily described within the quasiparticle-phonon model usingg _s ^eff =0.6g _s ^free . Similar calculations and comparisons with experminental data have been performed also for^95,99Mo as well as for⁹⁹Ru and¹⁰¹Pd.This work is partly supported by the Bulgarian National Research Foundation     

Investigation of new neutron-rich gold isotopes203Au and205Au

Using a²⁰⁸Pb beam of the UNILAC accelerator at GSI we produced the new isotopes²⁰³Au and²⁰⁵Au and identified them by measuring their-decay properties. Their half-lives were found to be 60(6)s and 31(2)s, respectively, and theQ-value of²⁰³Au was determined to beQ =2040(60)keV. Nuclear structure information of^203,205Hg was derived from this measurement. Furthermore, production cross-sections of^203,205Au are given and compared to those obtained in other experiments.This work has been supported by the Federal Ministry for Research and Technology (BMFT) under contract number 06 Gö 451-1/2     

The proton g9/2 isomer in theN=50 nucleus87Rb and M2 transition rates in85,87Rb

Low-lying states of theN=50 nucleus⁸⁷Rb have been investigated in the (, ') reaction measuring- and delayed-rf-coincidences. A half-life ofT _1/2=6(1) ns was obtained for the level at 1578.1 keV. This experimental result confirms the 9/2⁺ assignment and the proton 1g_9/2 single-particle character of this state. Experimental M2 transition strengths in^85,87Rb are compared with predictions of the shell model and the particle-core coupling model.This work was partly supported by the Bulgarian National Research Foundation.     

The effects of collisional quenching on degenerate four-wave mixing

We report a theoretical and experimental investigation of the effects of collisional quenching on resonant degenerate four-wave mixing (DFWM). Using single-mode laser radiation, peak signal intensity measurements were performed on an isolated line in the A – X transition of NO. By using appropriate mixtures of N₂ and CO₂ as buffer gases, we varied the collisional quenching rate over several orders of magnitude while maintaining a fixed total collisional dephasing rate. The mixtures had approximately 100 Torr total pressure and were at room temperature. For I/I _sat approximately equal to 0.02, DFWM intensities were found to be less affected by variations in quench rate than were laser-induced fluorescence (LIF) intensities (I and I _sat are the pump laser and one-photon saturation intensities, respectively). Moreover, for I/I _sat roughly equal to 0.5, DFWM intensities were observed to be nearly independent of quench rate. The results are compared to two theoretical predictions, with good agreement observed. Both theories indicate that the minimum sensitivity of DFWM to quenching occurs near I/I _sat1.     

New phenomena in homoepitaxial growth of metals

The growth of Pt(111) by Pt vapour deposition is studied by He diffraction as a function of substrate temperature and deposition rate. At a deposition rate of about 2.5×10^–2 monolayers/second several growth modes are observed: layer-by-layer (2D-) growth at 450 KT _s800 K, multilayer (3D-) growth at 340 KT _s450 K and reentrant layer-by-layer (2D-) growth at T _s340 K. The observed growth modes and in particular the reentrant 2D-growth are shown to be characteristic of growing Pt(111) under clean conditions, i.e. not influenced by contaminants. The influence of the intra- and interlayer mass transport on the growth mode is discussed in the light of experimental and simulation results. The 3D-growth mode is attributed to the existence of an activation barrier which suppresses the descent of adatoms from the top of the growing adatom islands onto the lower terraces. The barrier can be overcome by thermal adatoms at T _s450 K enabling interlayer mass transport which leads to 2D-growth. The reentrant 2D-growth occurs due to a break down of this barrier for small, irregularly shaped islands.     

Phenomenological wave functions for the massA=14 system and a consistent description of beta decay observables

A set of phenomenological wave functions has been derived to describe the¹⁴N ground state and the isospin triplet consisting of the¹⁴C ground state, the first excited state of¹⁴N at 2.313 MeV and the¹⁴O ground state. Elastic and inelastic electron scattering form factors, the magnetic moment of the¹⁴N ground state and the shape factors in the ^± decay have been employed in a multiparameter fitting procedure to determine the amplitudes of the wave functions inL-S coupling. The inclusion of the beta decay observables in the fit has become possible for the first time since exact formulas for the shape factor in higher order do exist. The set of wave functions deduced exhibit predominately anL=0 contribution for the 0⁺; 1 states andL=1 and 2 contributions of nearly equal weight for the 1⁺; 0 state. It was observed that the inclusion of the shape factors allowed a more stringent determination of the amplitudes compared to previous attempts reported in the literature and led in the case of the 0⁺; 1 states to wave functions that show a small but noticeable difference within the isospin triplet. Besides the observables used for the fit, the radiative width (M1) of the 2.313 MeV state in¹⁴N can be described quite well with the derived wave functions, and in addition it has become possible to predict the pathological largeft ^– value of the¹⁴C decay and theft ⁺ value of the¹⁴O decay precisely. The wave functions are also applied to calculate the¹⁴N(, ⁺) cross section.Dedicated to Prof. Dr. P. Kienle on the occasion of his 60th birthday. Supported by the German Federal Minister for Research and Technology (BMFT) under contract number 06DA 184I     

Isomeric transitions between shape coexisting states in iodine isotopes withA=115, 119 and 121

Applying delayed- r.f. coincidences and generalized centroid-shift analysis, nanosecond isomers in some odd-A iodine isotopes are studied in-beam. The reactions¹⁰⁶Cd(¹²C,p2n) and^116,118Sn(⁶Li,3n) have been used. The following half-lives were determined:T _1/2(565 keV)=0.50±0.10 ns andT _1/2(837 keV) =0.90±0.20 ns in¹¹⁵I,T _1/2(687 keV)=5.50±0.50 ns andT _1/2(2418 keV)=4.0±0.50 ns in¹¹⁹I as well asT _1/2(812 keV)=0.35±0.20 ns andT _1/2(445 keV)<0.10 ns=">¹²¹I. A systematics of the absolute probabilities for the transitions deexciting theg _9/2 9/2⁺ and _11/2 11/2 ₁ ^– band heads in^115–125I is presented and discussed.Partly supported by the Bulgarian National Research Foundation under contracts PH14, and PH31 and Kernforschungszentrum Karlsruhe, Stabsabteilung Internationale Beziehungen     

X-rays from antiprotonic3He and4He

Antiprotonic X-rays from the helium isotopes have been observed at pressures of 36, 72, 375 and 600 mbar. The antiproton beam from LEAR with momenta of 309 and 202 MeV/c has been stopped at these pressures using the cyclotron trap. The X-rays were detected with Si (Li) and intrinsic Ge semiconductor detectors. Absolute X-ray yields were determined and the strong-interaction 2p shifts and the 2p and 3d broadenings measured to be _2p=(–17±4) eV, _2p=(25±9) eV and _3d=(2.14 ±0.18) meV for ¯p³He and _2p=(-18±2) eV, _2p =(45±5) eV and _3d=(2.36±0.10) meV for ¯p⁴He.The efforts of the LEAR staff and the help of P. Gauss from the CERN Cryogenic Group as well as the technical assistance of M. Dröge and M. Stoll are gratefully acknowledged. This work is part of the Ph.D. of one of us (M.S.), University of Karlsruhe (1987), KfK report no. 4222.     

Neutron scattering study of the two-dimensional spinS=1/2 square-lattice Heisenberg antiferromagnet Sr2CuO2Cl2

We have carried out a neutron scattering investigation of the static structure factorS(q _2D ) (q _2D is the in-plane wave vector) in the two-dimensional spinS=1/2 square-lattice Heisenberg antiferromagnet Sr₂CuO₂Cl₂. For the spin correlation length we find quantitative agreement with Monte Carlo results over a wide range of temperature. The combined Sr₂CuO₂Cl₂-Monte Carlo data, which cover the length scale from 1 to 200 lattice constants, are predicted without adjustable parameteres by renormalized classical theory for the quantum nonlinear sigma model. For the structure factor peakS(0), on the other hand, we findS(0) ² for the reduced temperature range 0.16<T/2 _s <0.36, whereas current theories predict that at low temperaturesS(0)T ^{2 2}. This discrepancy has important implications for the interpretation of many derivative quantities such as NMR relaxation rates. In the ordered phase, we have measured the temperature dependence of the out-of-plane spin-wave gap. Its low-temperature value of 5.0 meV corresponds to an XY anisotropyJ _XY /J=1.4×10^–4. From measurements of the sublattice mangetization we obtain =0.22±0.01 for the order parameter exponent. This may either reflect tricricality as in La₂CuO₄, or it may indicate finite-size two-dimensional XY behavior as suggested by Bramwell and Holdsworth. As in theS=1 system K₂NiF₄, the gap energy in Sr₂CuO₂Cl₂ scales linearly with the order parameter up to the Néel temperature. We also reanalyze static structure factor data for K₂NiF₄ using the exact low temperature result for the correlation length of Hasenfratz and Niedermayer and including the Ising anisotropy explicitly. Excellent agreement between experiment and theory is obtained for the correlation length, albeit with the spin-stiffness _s reduced by 20% from the spin-wave value. As in Sr₂CuO₂Cl₂ we find thatS(0) ² for the reduced temperature range 0.22<T/2 _s <0.47.     

Positron mobility in polyethylene in the 60–400 K temperature range

We have determined the positron mobility (₊) in polyethylene samples (67.2% crystalline, glass transition temperatureT _g=151 K) in the 64–400 K temperature range by Doppler shift measurements. A method based on the simulataneous observation of two lines from¹³³Ba and¹³⁷Cs radioactive sources together with the positron annihilation line, was employed to measure the Doppler shift of the 511 keV line as a function of the electric field applied to the samples. With this method we were able to measure at the same time the drift velocity of positrons and theS parameter. This parameter is very important in the interpretation of the mobility trend in samples where the positron states change with temperature. The positron mobility was corrected for positronium formation. ₊ at 64 K is 31.7±0.8 cm² V^–1 s^–1 then decreases up to 123 K, increases at 148 K and decreases again up to 170 K (₊=26.9±0.8 cm² V^–s^–). This sharp change in mobility is centred around the glass transition temperature of our samples. Then the mobility remains almost constant up to 230 K. From 250 K to 377 K, ₊ increases and reaches the value of 38.4±1.0 cm² V^–1s^–1. The corrected experimental data were well fitted by a simple model taking into account scattering and a thermally activated process (hopping mechanism).     

Nuclearg-factors of the 1229 and 2911 keV isomers in143Nd

Nuclearg-factors of the 1229 keV 13⁺/2 and 2911 keV 21⁺/2 level and the half-life of the 1229 keV level have been measured to beg(1229)=0.058(5),g(2911)=0.69(12) andT _1/2 (1229)=6.79(2) ns. The experimental g-factors show that the 1229 keV level has a dominant configuration of (f _7/23^–), and the 2911 keV level has an almost pure (f _7/27^–), configuration.The authors would like to thank the crew of CYRIC for the operation of the cyclotron.     

Deep bandtail states picosecond intensity-dependent carrier dynamics of GaN epilayer under high excitation

Picosecond carrier dynamics of deep bandtail states (3.1 eV) in an unintentionally n-doped GaN epilayer at room temperature under high excitation densities (i.e., N ₀ = 1.0× 10¹⁹– 1.1× 10²⁰ cm^–3) have been investigated with nondegenerate femtosecond pump–probe (267/400 nm) reflectance ( R/R ₀). All R/R ₀ traces possess a 2 ps buildup time that represents an overall time for the initial non-thermal carrier population to relax towards the continuum extremes and then into the probed tail states. We observe a saturation of R/R ₀ initial (first 10 ps) recovery rate _i at a density of 5– 6×10¹⁹ cm^–3 close to the Mott transition threshold obtained from time-integrated PL measurements. Such a saturation phenomenon has been identified as the trap-bottleneck due to the bandtail states and deep traps. As N ₀ is further increased, _i accelerates due to the onset of Auger recombination as the trap-bottleneck becomes effective. The best fit by the Auger model for N ₀ in the range of the mid-10¹⁹–10²⁰ cm^–3 yields an Auger coefficient of C _a 5.0× 10^–30 cm⁶ s^–1.     

Test of the Pauli exclusion principle for nucleons and atomic electrons by accelerator mass spectrometry

The Pauli exclusion principle was tested by searching with accelerator mass spectrometry for non-Paulian atoms with three electrons in theK-shell and for non-Paulian nuclei with three protons or three neutrons in the nuclear 1 s_1/2 shell. For non-Paulian atoms of and the following limits have been obtained: and . For non-Paulian nuclei of and with three protons or three neutrons, respectively, in the nuclear 1 s_1/2 shell the following limits have been measured: for a range of proton separation energies of between 0 and 50 MeV and for neutron separation energies between 0 and 32 MeV. The result for⁵Li is used to deduce a limit for the probability ²/2 of finding two colliding protons in the symmetric state with respect to exchange to be ²/2<>^–32.Dedicated to Prof. Dr. P. Kienle on the occasion of his 60th birthday. Supported by the BMFT     

Au diffusion in α-Ti

The solubility and diffusion of Au in -Ti have been studied in a 823–1023 K temperature range using the Rutherford backscattering technique. For this purpose we have implanted Au into -Ti samples. Our results show that the solubility of Au varies between 0.2 and 0.35 at.%. In addition, we found that the diffusion coefficients follow a normal Arrhenius behavior with Q=260 kJ/mol and D _o=1.9×10^–5 m²/s¹. These values are typical for a substitutional diffusion mechanism.     

Measurements of magnetic moments of Tc isotopes and the hyperfine field of Tc in Fe and Ni

We report measurements of nuclear magnetic resonance on oriented nuclei (NMR-ON) on⁹⁴Tc (I=7⁺,T _1/2=4.9 h),⁹⁵Tc (I =9/2⁺,T _1/2=20 h) and⁹⁶Tc (I =7⁺,T _1/2=4.3 d) in Fe and on⁹⁵Tc and⁹⁶Tc in Ni. In order to elucidate the discrepancies on the hyperfine field of TcFe in the literature, the resonances were measured with high precision as a function of the external magnetic field B_ext up to 2.0 T. In addition, TDPAC measurements were performed on⁹⁹TcFe at T=300 K and 13 K. TheT=0 K hyperfine fields of Tc in Fe and Ni were determined to be –314(3) kG and –51.8(5) kG, respectively. The g-factors of⁹³Tc,⁹⁴Tc,⁹⁵Tc,⁹⁶Tc and⁹⁹Tc(E=181 keV;I =5/2⁺) are redetermined as g(⁹³Tc)=1.405(14), g(⁹⁴Tc)=0.731(7),g(⁹⁵Tc)=1.321(13), g(⁹⁶Tc)=0.727(7), g(⁹⁹Tc)=1.390(17).We wish to thank E. Smolic and G. Seewald for experimental help. This work was funded by the German Federal Minister for Research and Technology (BMFT) under the contract number 06TM353/TP 4, by the Deutsche Forschungsgemeinschaft (DFG) under the contract numbers Ha 1282/3-1,2, and, partly, by the Kernforschungszentrum, Karlsruhe.     

Precision measurement of antiprotonic hydrogen and deuterium X-rays

X-rays from antiprotonic hydrogen and deuterium have been measured at low pressures. Using the cyclotron trap, a 105 MeV/c antiproton beam from LEAR was stopped with an efficiency of 86% in 30 mbar hydrogen gas in a volume of only 100 cm³. The X-rays were measured with Si(Li) detectors and a Xe-CH₄ drift chamber. The strong interaction shift and broadening of the Lyman transition and the spin-averaged 2p width in antiprotonic hydrogen was measured with unprecedented accuracy. The triplet component of the ground state in antiprotonic hydrogen was determined for the first time.The authors would like to thank the LEAR staff for their efforts in providing the antiproton beam. The help of P. Gauss from the CERN cryogenic group and of P. Zettwoch from the PS workshop is gratefully acknowledged. We wish to thank K.-P. Wieder for his help with the drawings. This work is part of the Ph.D. thesis of one of us (K.H., University of Karlsruhe, 1990).