Dasβ-Spektrum des Cs137

Theβ-ray spectrum of Cs¹³⁷ has been measured with an iron-free spectrometer. The energy of the soft component was found to beE ₀=514±2 keV. The parameterk of the hard-component shape factorC _2VA ⁽²⁾ (W)=q ²+kp ² was determined to bek=0.015±0.004. Theβ intensities amount to 6.5% (hard component) and 93.5% (soft component). TheK conversion coefficient of the isomeric transition was measured to beα _K=0.093±0.003, in excellent agreement withSliv's theoretical value.     

Der Zerfall des Mn52m

Mn^52m(T _1/2=21 m) was produced by irradiating iron-foiles with deuterons ofE _d =9 MeV. Coincidences ofγ-rays with the main 1434 keV-transition had been sought for with the aid of a scintillation fast-slow-coincidence circuit. There was no evidence ofγ-lines which had been found earlier byKatoh et al. atγ-energies 700, 940, 1020, 1150, 1370, 1520 keV. If these transitions exist, their relative intensities are less than 0.7% (700 keV) and 0.3% (all others) per decay of Mn^52m.     

TheK-conversion coefficient of the 321 keVE1 transition in Hf177

TheK-conversion coefficient of the 321 keVE1 transition in Hf¹⁷⁷ has been measured by means of an iron free double focusing beta-ray spectrometer, using the internalexternal conversion method. The result obtained for α _K (321)=0.162±0.016 is in disagreement with the theoretical values for pureE1 transition (α _K =0.0154) calculated bySliv andBand. The large anomaly observed in theK-conversion process of the inhibitedE1 transition is compatible with a largeM2 admixture or, more probable with the presence of penetration matrix elements.     

Verzweigungsverhältnisse und Konversionskoeffizienten von angeregten Zuständen des208Tl

The branching ratios of theγ rays of the second and fourth excited states of²⁰⁸Tl have been investigated by coincidence measurements between the α rays of²¹²Bi and subsequent 40keVγ ray. The detectors employed were a silicon surface barrier counter for α particles, and a 1.5 in ×2 mm NaJ (Tl) crystal forγ rays. It has been found that (75.6±3.7)% of all transitions of the 328 keV state and (94±7)% of all transitions of the (492 keV+473 keV) states populate the first excited state of²⁰⁸Tl. The 40 keV state is excited to (3.4±0.3)% by transitions of higher excited states relative to the direct excitation by α particles. The number of α particles with energyE _α = 6.047 MeV and the number of subsequent 40keVγ rays resulted in a conversion coefficient α(40keV)=22.55± 0.46. Similarly coincidence measurements between Tl-x rays and α particles have been used to determine theK- conversion coefficients α_K(328 keV)=0.31±0.03 and α_K(492 keV+ 473keV)=0.100±0.015. The experimental results are in good agreement with the theoretical values ofSliv.     

Der Zerfall des Lu176m

The decay of Lu^176m has been investigated. TheK-conversion coefficient α _K of the 88,3 keV niveau of Hf¹⁷⁶ has been determined to α _K =1,35±0,07. Theβ-branching ratio to the 0+ and 2+ niveau of Hf¹⁷⁶ has been measured by means of aβ-γ-coincidental technique. (60,4±6,1)% of Lu^176m decay into the 2+ niveau and (39,6±6,1)% into the 0+ niveau of Hf¹⁷⁶.K-capture of Lu^176m to Yb¹⁷⁶ was not found. If there is any, it is less than 0,1% of all decays.     

Zerfallsschema und β-Spektrum des MsTh1 (Ra228)

Theβ-spectrum of MsTh1 (Ra²²⁸) has been measured in a proportional counter in 2π — and in 4π-geometry. Comparison of these measurements shows that there are no conversion electrons. Theβ-decay of MsTh 1 therefore leads in all cases to the ground level of MsTh2. The Kurie plot is straight from 15 keV up to the upper energy limit ofE ₀=55±3 keV (logft=5·6). The result has been checked by a search for photons emitted by the MsTh1. Noγ-rays and no X-rays have been found. The measurements had to be made with a relatively large amount of natural Ra²²⁶ in the sources. — The results do not agree with those ofLecoin, Perey, Teillac andRiou, who proposed a complex decay sheme for MsTh1.     

Untersuchung des ZerfallsBi^{212} (ThC)\xrightarrow{\beta }Po^{212} (ThC')\xrightarrow{\alpha }Pb^{208} (ThD) durch (γ, α)-Koinzidenzen

Theγ-spektrum of Po²¹² (ThC′) has been measured by (γ, α)-coincidences with a fast-slow coincidence apparatus. The results are in excellent agreement with the conversion lines found by theLatyshev group. The absoluteγ-intensities have also been determined in order to get spins and parities of the levels by calculating the absolute conversion coefficients. Theβ-intensity leading to the exited states of Po²¹²(ThC′) is estimated to be about one third of that measured byBurde andRozner by (β, α)-coincidences. Threeγ-lines measured byChinaglia andDemichelis by (γ, α)-coincidences do not agree with our results. The 2⁺ assignment of the first exited state is now well established, but for the other levels in the decay scheme there is still some uncertainty concerning spin and level assignment.     

Messungen derK-Konversionskoeffizienten und der Aktivierungsquerschnitte der isomeren Atomkerne Se77m,Se79m,Ge75m und Ge77m

TheK-conversion coefficients α _K of the nuclear isomers Se^77m , Se^79m , Ge^75m and Ge^77m have been measured by detecting theK-röntgen- andγ-radiation from neutron-irradiated Se- and GeO₂-samples with the aid of scintillation counters to be α _K =0.79±0.06, 7.4±0.6, 1.44±0.13, and 1.2±0.6, respectively. In all cases, the values obtained, are in agreement with those taken from the tables ofRose under the assumption of anE3-transition, thus confirming this assignment which was proposed earlier by other authors. In addition, the cross sectionsσ for inducing the activities by slowed down neutrons have been measured to beσ=22±2, 0.40±0.04, 0.20±0.02, and 0.12±0.03 barns, respectively, and are compared with earlier data of several authors.     

Pion-pion interaction andK 2x03C0;x03C0;x03C0;-decay

The enhancement of theK _2π ⁺ -decay compared to theK _2π ⁰ -decay is discussed on the basis of the\(|\mathop {\Delta {\rm I}}\limits^ \to | = \tfrac{1}{2}\)-rule. The enhancement factor is calculated by dispersion methods which yield an expression depending only on the phase shift of the two pion system in theJ=0,I=0,2 state. This expression has been studied in the framework of simple models for the two-pion interaction in order to obtain a survey of the possibilities for the cause of the anomalous large ratioK _2π ⁺ /K _2π ⁰ . Only characteristic cases have been considered and, as far as possible, experimental results of theπ-π-interaction are taken into account.     

Die Messung der β-γ-Winkelkorrelation bei Au198

The energy dependence of theβ ?γ asymmetry coefficient has been measured. No anomaly at lowβ energies as reported by other authors was found. Theξ-approximation holds andε W/p ² Ν ₁₂=0.027±0.007 was obtained. The matrix elements of theβ transition are discussed.     

Nonradiative <Emphasis Type="Italic">S-T</Emphasis> intersystem crossing in α and β chlorine derivatives of naphthalene

The rate constants K _ST ^s of nonradiative S ₁ ? T ₁ ^s transitions to triplet sublevels s in molecules of chlorine derivatives of naphthalene (1,4-dichloro- and monosubstituted α-chloro- and β-chloronaphthalene) have been calculated within the model of vibronically induced spin-orbit (VISO) couplings. The contribution of the spin-orbit couplings in Cl atoms and carbon framework of the molecule to VISO couplings is determined. A dependence of the heavy-atom effect on the constant K _ST ^s in relation to the type of sublevel T ^s and α and β positions of chlorine in the molecule is established and explained.     

Der Zerfall von Er171 und Er165

Theγ-spectrum of a neutronactivated probe of natural Er₂O₃ revealed an additional peak at 55 keV, which was attributed to the characteristicK-Röntgenstrahlung from the decay of Er¹⁶⁵ by measurement of its half-life in a NaJ-wellcrystal. The activation cross section for thermal reactor neutrons for Er¹⁶⁴ (n, γ) Er¹⁶⁵ has been determined to σ _A =20±7 barn. The averaged conversion coefficient of the 111, 116 and 124 keV γ-rays from Er¹⁷¹→Tm¹⁷¹ have been remeasured with scintillation counter equipment.     

Zerfallsschema und Matrixelemente für denβ-Übergang Ag110m→Cd110

Theβ decay Ag^110m→Cd¹¹⁰ has been investigated with a double lens spectrometer and aβ-γ circular-polarization correlation setup. The shape of the 6⁺→6⁺ β spectrum withE ₀=529 keV was found to be allowed, in disagreement with earlier work. The constantA of theβ-γ circular-polarization correlation was measured to beA=0·07±0·02. This implies a ratioX of Fermi to Gamow-Teller contribution to the decay ofX ₁=?0·02±0·03 orX ₂=?10·3 _?4·1 ^+2·3 . Qualitative shell model considerations favor the valueX ₁. Additional information is given for the disintegration schemes of Ag^110m and Ag¹¹⁰.     

Behaviour of some faintK β for elements As(33) to Ru(44)

1. 1.
   It has been shown that the semi-Moseley graphs for theβ ₈,β ₇,β ₆,β ₅,β ₄,β ^?,β ₁₁ ^? andβ ₀ in theK-series for elements over the rangeZ=33 toZ=44 reported byHulubei, Cauchois andManescu become remarkably regular when referred toα ₁ instead ofβ ₁ as the parent line.     
   
   

Suche nach Zweiquantenprozessen beim Zerfall von Xe131m

The decay of Xe^131m was investigated in order to detect nuclear double decay processes, in which the transition energy is distributed either between twoγ-quanta or between oneγ-quantum and oneK-conversion electron or between twoK-conversion electrons. By analyzing the emittedγ-radiation in a two-dimensional way an upper limit of 2.2 · 10^?5 was derived for the ratio of theγγ- toγ-transition probability. An investigation of theγ-spectrum in coincidence withK-quanta yielded an upper limit of 3 · 10^?2 for the rate ofe _Kγ-transitions relative toγ-transitions. The simultaneous emission of twoK-quanta was actually observed. These doubleK-quanta result either from the doubleK-conversion that was sought or from the internal conversion of the internal Compton-effect. For the doubleK-electron emission toγ-emission probability a value of (3.6±0.7) · 10^?3 was obtained. TheK-conversion coefficient and the half-life of Xe^131m were measured to be 32.1±0.4 and 11.94±0.04 d, respectively.     

Untersuchung des Vanadium-52-Zerfalls

Theγ-rays of the decay of V⁵² were investigated with NaJ crystals andγ-γ-cascades had been sought for by a fast-slow coincidence circuit. Threeγ-transitions of energyγ ₁=0,935 (0,14%),γ ₂=1,331 (0,9%),γ ₃=1,531 MeV (0,16%), respectively, in coincidence with the 1,434 MeV transition could be detected. It is concluded that there are four branches of V⁵² β-decay:β ₀=2,47MeV (98,8%, logft=5,1),β ₁=1,53 MeV (0,14%, logft=7,0),β ₂=1,14 MeV (0,9%, logft=5,7),β ₃=0,94 MeV (0,16%, logft=6,1). Spin and parity of V⁵² ground level is concluded to be 3+.     

Concerning internal conversion coefficients in Hf180

The gamma-ray relative intensities from transitions in Hf¹⁸⁰ following the 5.5 hour Hf^180m decay have been measured using a bent-crystal gamma-ray diffraction monochromator and a least-squares fitting technique. From these measurements it was possible to deduce a value for the internal conversion coefficient for the 93.3-keV transition of α _T ⁹³ =4.91±0.23. From previous measurements of conversion electron intensities byEdwards andBoehm and our gamma-ray relative intensities, internal conversion coefficients for all transitions except the 57.5-keV transition were obtained. These coefficients agree well with the previous determinations byEdwards andBoehm, however, our measurements have improved precision, particularly in the case of 501.3-keV transition. The present measurements of α _K for the 215.3-, 332.5-and 443.8-keVE2 transitions are 11% lower than theoretical values while α_K for 93.3 keV E2 transition agrees closely with the theoretical value. These results are in close agreement with the previous measurements ofEdwards andBoehm. The present experimental α_K for the 501-keV transition agrees closely with the theoretical α_K for an E3 multipolarity.     

Die absolute Intensität der durch Elektronenstoß in einer dicken Wolfram-Antikathode erzeugtenL α -Strahlung

The number\(N_{L_\alpha }^{dir} \) (produced) ofL _α -photons produced by electron-bombardment in a thick target of tungsten per incident electron has been measured absolutely with the Ross-filter method and relatively with the crystal-spectrometer method in the energyregion up to the 3.6 times theL _III-ionization energy\(E_{L_{III} } \). The result can be presented in the following empirical form:\(N_{L_\alpha }^{dir} \) (produced)=4π·?·(U ₀?1) ⁿ with ?=0.52·10^?4±5% andn=1.44±0.02\((U_0 = E_0 /E_{L_{III} }< 3.6)\). Out of this the number\(n_{L_{III} } \) ofL _III-ionizations per electron which is slowed down to the energy\(E_{L_{III} } \) within the target, has been evaluated. The computation of\(n_{L_{III} } \) out of the elementary process by usingBethe's non-relativistic formulae for totalL _III-ionization cross sectionQ _L and energy loss-dE/ds is in full agreement with experiment in the region 2<U ₀<3.6, if the constants in\(Q_{L_{III} } \) are chosen as follows:\(B = 4E_{L_{III} } , b_{L_{III} } = 0.25 \cdot 5.89\). By comparison of this result for\(b_{L_{III} } \) with the corresponding value ofb _K in the totalK-ionization cross-sectionQ _K for copper (b _K=0.35·2.26) it is concluded that\(Q_{L_{III} } \) is considerably higher than predicted by theory. The necessary correction factors as e.g. loss ofL _III-ionizations by rediffusion of electrons and portion of indirectly producedL _α -radiation-radiation are determined for tungsten quantitatively.     

Bestimmung des (631)K=1/2, I=1/2-Zustandes im U 239

Theγ-ray spectrometer at the DR 3-reactor at Risø was used to investigate the low energyγ-lines of U 239 which are emitted during neutron-capture in U 238. Very closely lying lines have been found between 500 and 650 keV. The big intensity of the 133 keV line and the lack of other transitions of appropriate energy and intensity point out that this line corresponds to the hinderedE 2-transition from the (631)I=1/2⁺ level to the (622)I=5/2⁺ groundstate. A suggestion was made for the decay possibility of the octupole states at 700 keV found by N.Fiebiger.     

Aufbau eines automatisch arbeitenden π√2-Spektrometers und Untersuchung des Konversionslinienspektrums von In114m und ThB mit Folgeprodukten

An automatically operatedπ√2 spectrometer is described. The regulated current supply is transistorized. With this spectrometer the electron spectra of In^114m and of ThB with daughter products have been investigated. TheK/L ratio of the 191 keV isomeric transition in In^114m was found to be 1·25±0·03, in excellent agreement with the theoretical value ofSliv andBand. In the electron spectrum of ThB and daughter products 46 lines were found betweenB?=1750Г cm andB?=10000Г cm. Some of them are new. Most important is a new weak line atB?=7030Г cm which fixes a new level atE=1·807 MeV in ThC′ (Po²¹²). Simultaneously the earlier reported discrepancy between electron andγ-ray intensities for 1·8 MeV transition energy is resolved. There is anE0 transition of 1·800 MeV while the new line is theK conversion line of a new radiative transition (most probablyM2). A spin ofI=2+ is assigned to the 1·680 MeV level of ThC′. The 0·953 MeV transition from this level isM1, withE0 admixture.