Investigation of the interaction of subpicosecond KrF laser pulses with a preformed carbon plasma

The interaction of a subpicosecond KrF laser pulse with a preformed carbon plasma of various scale lengths is investigated. Two different interaction geometries are chosen. In the first one the propagation vector of the short pulse has a component along the density gradient of the preformed plasma (angle of incidence is 45°). In the second geometry the propagation direction of the short pulse is perpendicular to the density gradient of the preplasma (angle of incidence is 90°). The emitted soft X-ray spectrum in the wavelength interval from 10 to 700 is observed while changing several parameters of the experiment. It is found that the emission in the short wavelength part under 200 results from the radiation of ions created by collisional heating near the critical density region. The long wavelength part above 200 , enhanced up to a maximal factor of 20, is mainly produced by radiating particles field—ionized up to the He-like carbon state in the high-intensity laser field. The short wavelength part is missing in the case of 90° angle of incidence because there is no interaction with the critical layer that results in an insufficient collisional heating.     

Detailed study of the effect of a short prepulse on soft X-ray spectra generated by a high-intensity KrF* laser pulse

The effect of a short prepulse (0.5 ps) on soft X-ray spectra from a plasma generated by a high intensity KrF* laser pulse (main pulse: 0.5 ps, intensity I _main=5.3×10¹⁵ W/cm²) on flat targets of Al and Cu has been studied in detail. The spectra have been measured as a function of the pulse separation t between the two pulses and the prepulse intensity I _pre. It was found that both the overall emission and the line emission increased with t (at constant I _pre) and with I _pre (at constant t). In particular, lines in the shorter wavelength region had higher intensity. The influence of the prepulse on the line emission of specific transitions in the Al spectra was investigated systematicly. An explanation for the observed effects is given.     

Effects of an ultrashort prepulse on soft X-ray generation from an aluminium plasma produced by femtosecond Ti:Sapphire laser pulses

The influence of a prepulse on soft X-ray emission in the range of 50–200 from an aluminium plasma produced by 130 fs Ti: Sapphire laser pulses with an intensity of 10¹⁴ W/cm² at normal incidence is studied. An ultrashort prepulse with an intensity of 10¹³ W/cm² significantly enhances soft X-ray emission when there is a long time separation ( > 100 ps) between the prepulse and an intense main pulse. It is also observed for the first time that a prepulse with a short pulse time separation can slightly reduce soft X-ray emission, contrary to the previous work done using 248 nm laser pulses. This can be explained qualitatively in terms of the dependence of absorption on the length scale.     

Porous layer effects on soft X-ray radiation emitted from a plasma generated by 130-fs laser pulses irradiating a porous silicon target

Received: 2 May 1997/Revised version: 17 October 1997     

Mechanisms of absorption in pulsed excimer laser-induced plasma

2 . Received: 20 January 1997/Accepted: 23 June 1997     

X-ray spectra from highly ionized dense plasmas produced by ultrashort laser pulses

Hydrogen-like and helium-like X-ray spectra (between 7.1 and 8.2 , i.e., 1500 to 17.50 eV, respectively) from solid aluminium targets irradiated with high intensity (up to 10¹⁷ W/cm²) subpicosecond (0.7 ps) laser pulses have been measured. The spectra show that the resonance lines are very broad and very asymmetric. Evidence for a Doppler-shifted reabsorption of the resonance line emission has been found. The spectra have been simulated by a computer code for the calculation of spectral-line intensities and linewidths. Electron densities exceeding the critical density have been estimated for different laser intensities by comparing the observed and simulated intensity ratio of different dielectronic satellite lines. From the X-ray spectra generated byp- ands-polarized radiation fat different laser intensities, the thresholds for the formation of hydrogen-like and helium-like ions have been determined.     

Generation of high order optical harmonics from solid surfaces

Received: 26 November 1998     

Influence of strong laser fields on the inverse bremsstrahlung collision frequency

A new model is described for the absorption of laser light by a plasma. Two issues important for high laser intensity are considered: changes in the electron velocity distribution and the absorption non-linearity. The effects of anisotropy and non-Maxwellian distribution function are analysed with a hard sphere model. It is shown that anisotropy alters the electron-ion collision frequency by an amount which depends on the ratio of the temperatures in direction of and perpendicular to the laser field.The effect of high laser intensity is considered assuming Coulomb collisions, and a new expression obtained for the collision frequency as a function of quiver velocity. It will be shown that the result is in agreement with the Spitzer result in the case of small fields and with the result of Catto and Speziale in the case of very strong fields, but shows an unexpected maximum of the collision frequency in an intermediate regime.     

Ultrashort X-ray pulses

In this paper, we discuss recent advances in ultrashort-pulse X-ray technology. Femtosecond laser-plasma based X-ray sources can now generate sub-pico-second soft X-ray pulses, with photon energies from 10 eV to 10⁶ eV, and with a high conversion efficiency of incident laser light to broadband X-rays. Recent advances in high-speed X-ray detectors and soft X-ray optics make it practical to use such sources as experimental tools for time-resolved X-ray science. Other possible generation techniques, such as laser-electron-beam scattering, promise to further expand the experimental capabilities in this area.     

Generation of magnetic fields by the non-stationary ponderomotive force of electromagnetic waves in plasmas with streaming electrons

It is shown that the non-stationary ponderomotive force of large amplitude electromagnetic waves in plasmas with streaming electrons can spontaneously create magnetic fields. The present result may account for the magnetic fields in laser-produces plasmas, in cosmic plasmas, as well as in galactic and inter-galactic spaces.     

Line-emission enhancement in laser-ablated carbon plasmas

The role of recombination and charge-exchange processes in enhancing the line emission of various ionic species of laser-ablated carbon in the presence of helium and argon are presented.     

Prospects of “water-window” X-ray emission from subpicosecond laser plasmas

Soft-X-radiation in the “water-window” region (23.3–43.6 ?) mainly from carbon laser plasmas generated by subpicosecond (700 fs) 0.248-μm laser pulses is studied as a function of angle of incidence and intensity (up to 10¹⁸ W/cm²) for p-polarized laser light. Furthermore, comparison is made between plasmas generated from massive and foil targets. Numerical calculations are performed using a hydrocode coupled to X-ray line and continuum emission calculations including radiation transport. The optimized conditions to achieve maximum water-window X-ray emissivity and, in particular, carbon Lyman-α line emission are investigated. In addition, analytical scalings are presented. These theoretical results are essentially confirmed by previous experiments. It is found that at optimized conditions, picosecond or subpicosecond laser plasma X-ray sources with a power of the order of 1–10 GW in a spectral window of 1 ? could be developed. Received: 6 August 1998 / Final version: 6 August 1999 / Published online: 30 November 1999     

Flight range of the particulate in a laser-plasma generated soft X-ray chamber

Some closed expressions for the flight ranges of the spherical particle ejected from a laser-produced plasma target in buffer gas are given as a function of its initial velocity, diameter, and some parameters of the properties for gas and particle material. It is shown that when estimating the ranges of the particulates generated from the laser target, the decline of viscosity with the decrease of the gas pressure has to be considered. Received: 3 March 2000 / Accepted: 28 March 2000 / Published online: 5 July 2000     

High-order optical harmonic generation from solid surfaces

During the interaction of an intense ultrashort laser pulse with solid targets, a thin layer of surface plasma is generated in which the density drops to the vacuum level in a distance much shorter than the wavelength. This sharp plasma-vacuum boundary performs an oscillatory motion in response to the electromagnetic forces of the intense laser light. It is shown that the generation of reflected harmonics can be interpreted as a phase modulation experienced by the light upon reflection from the oscillating boundary. The modulation side-bands of the reflected frequency spectrum correspond to odd and even harmonics of the laser frequency. Retardation effects lead to a strong anharmonicity for high velocities of the plasma-vacuum boundary. As a result, harmonic generation is strongly enhanced in the relativistic regime of laser intensities.Prof. F. P. Schäfer on the occasion of his 65th birthday.     

Instabilities in laser-produced carbon plasma expanding in a nonuniform magnetic field

The laser-produced carbon plasma expanding in an ambient atmosphere in the presence of an inhomogeneous magnetic field has been studied by emission spectroscopy and fast photography. A double-peak structure is observed in the temporal profile of CII and CIII transition. A sudden increase in delay observed in the second peak when the plasma expands in the concave region of a magnetic field is attributed to Rayleigh–Taylor instability in a magnetic field. An estimate of the growth rate of the instability inferred using intensity and velocity profile of the expanding plasma is reported. Received: 26 August 1999 / Revised version: 3 January 2000 / Published online: 20 September 2000     

An incoherent sub-picosecond X-ray source for time-resolved X-ray-diffraction experiments

Ultrashort bursts of K _α X-ray radiation were generated from fs-laser-produced plasmas. A complete experimental characterization of the X-ray source in terms of spectral, spatial, and temporal properties was performed. The pulse width of the K _α burst is shorter than 250 fs. The time-resolved evolution of a shock wave launched by a synchronized laser pulse in InSb was investigated. The transient change of the rocking curve yields detailed information on the structural changes. Received: 29 June 2000 / Published online: 22 November 2000     

Simulations on false gain in recombination-pumped soft-X-ray lasers

-1 in the case of plasmas with short active medium lengths. The false gain in the case of fiber targets is found to be of equal magnitude to that for slabs in the case of plasmas with less than 0.1 cm active medium lengths. Calculations for slab targets predict that adopting a tolerance of ±1 cm^-1 for gain will severely restrict the time and the active medium length of the plasma that can be used for error-free observations, while those for fiber targets are found to be considerably relaxed. The effects of false gain in the 54.2 Å Na Balmer α laser is also investigated, again revealing the importance of this phenomena under optimum gain conditions. Received: 10 December 1996/Revised version: 12 March 1997     

Low-energy ion emission from a xenon gas-puff laser-plasma X-ray source

We have measured low-energy ion emission from a gas-puff laser-plasma X-ray source. The ions may cause the degradation of the condenser mirror of the extreme ultra-violet projection lithography system. A 0.7 J in 8 ns Nd:YAG laser at 1.06 μm was focused onto the xenon gas-puff target with an intensity of ∼10¹² W/cm². The silicon (111) plates, placed at a distance of 32 mm from the laser-interaction region, were exposed with the xenon ions. The average ion energy was measured to be less than 50 eV with a Faraday-cup detector placed close to the silicon plates. The xenon deposition occurred in the silicon plates with a depth of less than 40 nm. The deposition density was measured with a quadrupole secondary ion mass spectrometer to be 10²¹ /cm³ after 1500 laser shots. The energy-conversion efficiency from the laser energy into the ions is ∼0.1%/4 π sr/shot. For the lithography system, if we can remove such ion bombardment completely using novel techniques such as electro-magnetic devices or gas flow curtain techniques, the lifetime of the condenser mirror will be extended significantly. Received: 20 November 2000 / Published online: 9 February 2001     

Spectroscopic studies of laser-produced plasmas formed in CO and CO2 using 193, 266, 355, 532 and 1064 nm laser radiation

The wavelength dependence of laser-produced breakdown in air, CO and CO₂ has been studied using the four Nd:YAG harmonics (266 nm, 355 nm, 532 nm and 1064 nm) and the ArF-excimer laser (193 nm). Breakdown thresholds at these wavelengths are reported for air, CO and CO₂. A significant reduction in the breakdown thresholds for both CO and CO₂ is apparent when comparing 193 nm with the four Nd:YAG harmonics. This reduction is attributed to the resonance-enhanced two-photon ionization of metastable carbon atoms generated in the laser focus at the ArF-laser wavelength. In addition to reporting breakdown thresholds, the laser-produced plasmas in CO and CO₂ are characterized in terms of plasma temperatures and electron densities which are measured by time-resolved emission spectroscopy. Electron densities range from 9 × 10¹⁷ cm^–3 to 1 × 10₁₇ cm^–3. Excitation temperatures range from 22 000 K at 0.2 µs to 11 000 K at 2 µs. Ionization temperatures range from 22 000 K at 0.1 µs to 16 000 K at 2 µs. Evidence is presented to indicate that, like ArF-laser-produced plasmas, Nd:YAG-laser-produced plasmas formed in CO and CO₂ are in or near a state of Local Thermodynamic Equilibrium (LTE) soon after their formation.     

Absorption of subpicosecond ultraviolet laser pulses in high-density plasma

The absorption of 250 fs KrF laser pulses incident on solid targets of aluminum, copper and gold has been measured for normal incidence as a function of laser intensity in the range of 10¹²–10¹⁴ W cm^–2 and as a function of polarization and angle of incidence for the intensity range of 10¹⁴–2.5×10¹⁵ W cm^–2. As the intensity increases from 10¹² W cm^–2 the reflectivity at normal incidence changes from the low-intensity mirror reflectivity value to values in the range of 0.5–0.61 at 10¹⁴ W cm^–2. For this intensity maximum absorption of 63–80% has been observed for p-polarized radiation at angles of incidence in the range of 54°–57°, increasing with atomic number. The results are compared with the expected Fresnel reflectivity from a sharp vacuum-plasma interface with the refractive index given by the Drude model and also to numerical calculations of reflectivity for various scale length density profiles. Qualitative agreement is found with the Fresnel/Drude model and quantitative agreement is noticed with the numerical calculations of absorption on a steep density profile with normalized collision frequencies, v/, in the range of 0.13–0.15 at critical density and normalized density gradient scale lengths, L/₀, in the range of 0.018–0.053 for a laser intensity of 10¹⁴ W cm^–2.At 2.5×10¹⁵ W cm^–2 a small amount of preplasma is present and maximum absorption of 64–76% has been observed for p-polarized radiation at angles of incidence in the range of 45°–50°.Dedicated to Prof. Dr. Rudolf Wienecke on the occasion of his 65^th birthdayOn leave from: Department of Electrical Engineering, University of Alberta, Edmonton, T6G 2G7, Canada