Bipolaronic excitations of interacting electron(hole) gas in one-dimensional lattice model

By developing a diagonalization scheme we observe that the dynamics of interacting electrons or holes locally coupled to dispersionless phonon mode in one-dimensional lattice can be mapped into that of paired electron or hole states (bipolaronic states), which then gives a physically appealing picture of excitation modes of the interacting electron or hole gas. As a result, the bipolaronic model of the interacting electron or hole gas, obtained from Holstein–Hubbard Hamiltonian in one-dimensional lattice, exhibits normalization of the hopping terms and leads to a reduced effective mass of the bipolaron, which essentially gives support to the bipolaronic theory of high T_c superconductivity.     

Effect of Nd on the Superconductivity of Nd1+x Ba2-x Cu3O y with 0.1 ≤ x ≤ 0.35

The effect of Nd substitution at the Ba sites has been studied in Nd_1+x Ba_2-x Cu₃O _y system for 0.1 x 0.35. Orthorhombic to tetragonal structural phase transition occurs at about x = 0.17. With the increase of Nd, the T _c value decreases and T increases, where T is the difference between the onset and critical temperatures and indicates the sharpness of the transition. These changes are explained by ac-susceptibility measurements on Nd_1.1Ba_1.9Cu₃O_7.12 at 0.10 Oe. The susceptibility curves show the presence of about four phases, which are not detectable by X-ray diffraction technique.     

On the preparation and the characterization of superconducting thin films of YBa2Cu3O7−x

The results of our initial efforts to deposit thin films of YBa₂Cu₃O_7−x system on sapphire substrate are described. The deposited films are shiny black in appearance and are of quite uniform chemical composition. The annealed films exhibit zero resistance superconducting transition temperatureT _c(R=0) ranging between 23 K and 30 K.     

Superconductivity in Bi2.2Ca2.8−x Sr x Cu2O y system and effect of rare earth substitution

The oxide system Bi_2.2Ca_2.8−x Sr _x Cu₂O _y has been investigated for superconductivity as a function of Ca/Sr ratio withx=0.7, 1.0, 1.4 and 1.8. All these compositions are found to be superconducting with onset temperature in the range of 80–90 K implying a large homogeneity range between Sr and Ca for the superconductivity to occur in this system. Effect of partial replacement of Bi by rare earths has been studied and it is observed that 20% replacement of Bi by Nd and Eu does not significantly affect the superconducting transition temperature.     

Cluster calculations of the hyperfine properties of copper compounds

Spin-polarized ab-initio cluster procedures are used to investigate the electronic structure of CuO₂-planes in the La₂CuO₄ and YBa₂Cu₃O₇ compounds. In particular, electric field gradients (EFGs) and magnetic hyperfine interaction parameters for the Cu sites were calculated with various theoretical methods. Calculations with density functional theory reproduce the experimentally determined EFGs fairly well while those at the Hartree-Fock level generally yield values which are too large by about 40%. The anisotropic magnetic hyperfine coupling can also be calculated with reasonable accuracy. This revised version was published online in August 2006 with corrections to the Cover Date.     

MuSR技术在凝聚态物理中的应用

缪子自旋弛豫/旋转(MuSR)实验技术利用缪子的自旋,在原子尺度上研究样品内部磁场的静态分布和动态涨落。文章介绍MuSR实验技术在凝聚态物理中的应用,阐述了MuSR在磁性、超导材料中发现的独特信息,包括磁有序、内部磁场分布、具有特定频率范围的自旋涨落,以及在半导体材料中获得杂质的电子状态和位置。这些应用表明 MuSR 对于理解关联电子材料复杂的物理现象及其物理机制具有重要意义。     

Macroscopic quantum tunnelling in the r.f. SQUID with S-c-S point contacts

Summary The experimental results on quantum decay of metastable flux states in the r.f. SQUID containing different S-c-S point contacts as the weak link are compared with various theoretical models. The formulae following from the RSJ model with weak and strong damping and the microscopic treatment of quantum effects in S-c-S junctions are analysed. It is concluded that only the latter theory provides a quantitative agreement with the experimental values.     

Electronic plus phonon-exchange mechanism for high-temperature superconductivity in layered crystals

A general mathematical formulation is developed for calculating the effective electron-electron interaction in layered crystals like YBa₂Cu₃O_7−δ, and for finding the resulting superconducting transition temperatureT _c in such systems within the framework of the conventional BCS pairing arising from various possible excitations in the medium. This differs considerably from the usual case of an effective three-dimensional homogeneous system, and should be relevant in the calculation ofT _c for the new class of high-T _c perovskites in which oxygen deficiencies in Cu-O layers and their distribution in the crystal play a crucial role. The explicit form of the effective interactionV _jj(q _t,ω) in a given layerj in the unit cell of the crystal is found to be determined not only by the true polarization functionπ _j(q _t,ω) of that layer, but also of other layers. The exchange of electronic excitations of a nearby insulating layer by carriers in a conducting layer thus becomes possible to get highT _c, with or without the usual phonon exchange.     

On the pairing interaction in highT c superconductors

It is argued, from the dependence of the critical current density and ofT _c on applied magnetic field, that the pairing interaction in highT _c superconductors must be strongly field-dependent.     

Algebra for fermions with a new exclusion principle

We construct the algebra of the creation and destruction operators for spin 1/2 particles obeying a new exclusion principle which is “more exclusive” than Pauli’s exclusion principle: an orbital state shall not contain more than one particle, whether spin up or spin down. The consequences of this algebra are studied and applications to the Hubbard model in condensed matter physics are indicated. An erratum to this article is available at .     

Investigation of novel highT c superconducting oxides

Our results of microscopic and macroscopic studies of novel highT _c superconductors are discussed. They permit a straightforward comparison of the nature of the superconductivity in 40 K range (La₂CuO₄ type) and 90 K range (YBa₂Cu₃O₇ type) superconductors.     

A two-channel model for transport across high T c bicrystal grain boundary junctions

This paper describes an investigation of the microscopic configuration of the barrier which exists at the boundary in high T _c grain boundary junctions. A model for describing the properties of bicrystal and biepitaxial grain boundary junctions is proposed. Two channels for transport currents are assumed, the supercurrent being carrier by one channel only. The measurable macroscopic parameters of a junction, (critical current density and normal state resistance) are computed in terms of the microscopic parameters that appear in this model. The model well describes major features of the characteristics observed for high T _c bicrystal junctions.     

Even harmonics of AC susceptibility in some sintered pellets of high temperature superconductors

The real (χ′ _n) and imaginary (χ″ _n) parts of even harmonic susceptibility (n⩽6) are measured as a function of external DC field (H _dc) in the field increasing (H↑) and decreasing (H↑) cycle. Hysteresis is observed betweenH↑ andH↓ cycles. In theH↓ cycle, at a field,H _comp=4·2G, bothχ′ andχ″ of all the even harmonics vanish indicating a true cancellation of fields in the intergrain region (H _eff≈0) caused by the balance betweenH _dc and the remanent magnetization of the grains. The position of the extrema and the zero of the various harmonics undergo a shift proportional to the remanent magnetization of the grains at that particular field.     

Reduction dependence of superconductivity in the end-member T′ cuprates

We have recently achieved superconductivity in T′-RE₂CuO₄ (RE: Pr, Nd, Sm, Eu, and Gd), using epitaxial thin films by metal organic decomposition. The key recipes to achieve superconductivity are low-P_O2 firing and subsequent vacuum reduction to minimize the amount of impurity oxygen atoms, which are very harmful to high-T_c superconductivity. In this article, we report our investigation on the reduction dependence of superconductivity of T′-RE₂CuO₄. For thin films, the amount of remnant O_ap atoms is difficult to evaluate but we propose that one good measure for this may be the c-axis lattice constant, which tells us whether the reduction is insufficient or excessive.     

高温超导体中约瑟夫森涡旋流阻的振荡效应

通过数值计算耦合sine-Gordon方程组研究高温超导体中约瑟夫森涡旋的运动,得到约瑟夫森涡旋电压和流阻随平面磁场和驱动电流的变化规律.固定驱动电流,约瑟夫森涡旋电压和流阻随着磁场的增大出现周期性的振荡行为,振荡周期与每层约瑟夫森结中进入一个磁通量子相对应.分析和阐明了产生这种周期性振荡的原因. 关键词： 约瑟夫森涡旋 涡旋格子 高温超导     

Mössbauer study of 1/8 anomaly in La2−x Ba x CuO4

The measurements of Mössbauer effect, magnetic susceptibility and muon spin relaxation have been carried out for the high-T _c superconductor La_2?x Ba _x CuO₄. The intensity of Mössbauer doublet spectrum of the sample of x～1/8 begins to decrease rapidly at a certain temperature T _m, which we define as a magnetic transition temperature T _Möss. This temperature almost agrees with T _μSR determined from muon spin relaxation. The quadrupole doublet disappears at low temperature below T _m but a clearly splitted spectrum is not observed even at 4.2 K, which indicates a peculiar magnetic state with a wide distribution of internal magnetic field. Around x～1/8, the superconducting critical temperature T _c and T _m are competed each other. In conclusion, superconductivity disappears around 1/8 hole concentration and a peculiar magnetic state such as spin density wave appears.     

Infrared detection by Tl?Ba?Ca?Cu?O superconducting films

The response of polycrystalline Tl–Ba–Ca–Cu–O superconducting thin films on short laser pulses has been investigated for radiation between 10 m and 500 m wavelength. Fast signals with time constants less than 1 ns were observed for wavelengths longer than about 100 m whereas for shorter wavelengths only a bolometric signal could be detected.     

Multivariate Image Analysis of Magnetic Resonance Images with the Direct Exponential Curve Resolution Algorithm (DECRA): Part 1: Algorithm and Model Study

Antalek and Windig recently presented a fast method to resolve a series of NMR mixture spectra, where the contribution of the components varies with a decaying exponential [B. Antalek and W. Windig,J. Am. Chem. Soc.118, 10,331–10,332 (1996); W. Windig and B. Antalek,Chemom. Intell. Lab. Syst.37, 241–254 (1997)]. The method was called DECRA (direct exponential curve resolution algorithm). In this paper DECRA will be applied to two series of magnetic resonance images. The signal of one series is based uponT₂relaxation, and the other is based uponT₁relaxation. In order to evaluate the technique, the magnetic resonance images of a phantom where used. A transformation is introduced to enable the application of DECRA to aT₁series of magnetic resonance images. A separate paper in this issue will describe the application of the techniques to magnetic resonance images of the human brain.     

Observation of rf SQUID characteristics in YBCO bulk at 77 K

RF SQUID behaviour due to grain boundary weak links in a bulk YBCO is observed at 77 K using modified commercial rf electronics. Porous samples with lowI _c are found to show this characteristic whereas dense samples with higherI _c do not show SQUID behaviour.V-B modulation characteristic is found to be better when the rf pumping frequency is kept slightly higher than the resonance frequency of the tank circuit. Designing of coil for tank circuit with appropriateQ has been found to be very crucial for seeing the SQUID behaviour. Estimation of parameters such as coupling constant, mutual inductance, inductance and radius of the SQUID loop, have been made and their significance is discussed. Flux noise spectrum of the bulk rf SQUID in flux locked mode is also reported.     

Generic phase diagram of “electron-doped” T′ cuprates

We investigated the generic phase diagram of the electron doped superconductor, Nd_2−xCe_xCuO₄, using films prepared by metal organic decomposition. After careful oxygen reduction treatment to remove interstitial O_ap atoms, we found that the T_c increases monotonically from 24 K to 29 K with decreasing x from 0.15 to 0.00, demonstrating a quite different phase diagram from the previous bulk one. The implication of our results is discussed on the basis of tremendous influence of O_ap “impurities” on superconductivity and also magnetism in T′ cuprates. Then we conclude that our result represents the generic phase diagram for oxygen-stoichiometric Nd_2−xCe_xCuO₄.