Broadband noncollinear optical parametric amplification without angularly dispersed idler

We report a new scheme for direct generation of broadband angular-dispersion-free mid-IR idler pulses via noncollinear optical parametric amplification when group-velocity matched wavelengths cannot be found and the traditional noncollinear geometry fails to increase the phase-matching bandwidth. The scheme does not require any post-amplification idler angular dispersion compensation. We derive and interpret the condition for broadband amplification and absence of idler angular dispersion. A broadband angular-dispersion-free 2.15 μm idler pulse is generated as an experimental demonstration. We identify the potential of the scheme to generate a broadband 3.5 μm idler, with a bandwidth supporting a sub-two-cycle pulse.     

Generation of ultrashort pulses of electromagnetic radiation in the mid- and far-infrared ranges

Generation of ultrashort pulses of electromagnetic radiation in the range of wavelengths from 3 to 17 μm is experimentally demonstrated using difference-frequency mixing of the signal and idler waves delivered through an optical parametric amplification of a week broadband seed by high-power near-infrared ultrashort laser pulses. Cross-correlation measurements demonstrate that pulses as short as a few cycles of electromagnetic field are produced in the mid- and far-infrared ranges by means of difference-frequency generation.     

Generation of Broadband Near-Infrared (2–2.5 μm) Radiation from an Optical Parametric Amplifier Driven by a Cr:Forsterite Laser Near Dispersion Anomalies of Tuning Curves

Pulses with a spectral width of 450 nm at a wavelength of 2.2 μm are generated in a parametric amplifier based on a type-I BBO crystal pumped by the second harmonic (620 nm) of a Cr:forsterite laser. Such a broadband radiation is obtained in a specific regime of the group velocity matching near the vertical region of the tuning curve. The generated pulses can be compressed to a duration of about 2.5 optical cycles (34 fs) in a medium with positive group-velocity dispersion.     

Self-referenced spectral interferometry for ultrashort infrared pulse characterization

We demonstrate for the first time (to our knowledge) characterization of ultrashort IR pulses by self-referenced spectral interferometry. Both sub-55-fs pulses from 1.4 μm to 2 μm and broadband 2.5-cycle pulses at 1.65 μm (13 fs FWHM) are characterized.     

Asynchronous midinfrared ultrafast optical parametric oscillator for dual-comb spectroscopy

Two asynchronous, broadband 3.3 μm pulse trains with a stabilized repetition-rate difference of up to 5 kHz were generated using an ultrafast optical parametric oscillator. The two oscillation channels, each producing ～100 mW average power, ran essentially independently, and weak non-phase-matched sum-frequency mixing between them provided a timing signal that indicated when the asynchronous pulses coincided. The system has immediate applications in incoherent asynchronous optical sampling and, with additional carrier-envelope-offset stabilization, could be applied to coherent dual-frequency-comb spectroscopy.     

Generation of tunable picosecond pulses in the medium infrared by down-conversion in AgGaS2

Picosecond pulses from a mode-locked Nd:YAG laser and a traveling-wave dye laser are mixed in an AgGaS₂ crystal to generate pulses at the difference frequency. The dye laser is tunable between 1200 nm and 1460 nm resulting in a tuning range of the parametric pulses from 3.9 μm to 9.4 μm. The spectral bandwidth is quite narrow. A value of Δ?=6.5 cm^-1 was measured which is constant over the whole tuning range. Several percent of the Nd:YAG laser photons are converted to infrared photons. Pump pulses of 21 ps give parametric pulses of 8 ps.     

高功率宽调谐输出的多周期极化铌酸锂晶体光学参量振荡器

利用掺杂浓度为5 mol%的掺氧化镁多周期极化铌酸锂晶体实现了高效单谐振的准相位匹配光参量振荡器,所使用的周期极化铌酸锂晶体有6个周期,且以1 μm为间隔,从26.5~31.5 μm. 该光参量振荡器以脉宽为150 ns,重复频率为10 kHz的声光调Q Nd∶YAG激光器为泵浦源,且泵浦光波长为1.064 μm. 通过控制晶体的温度（50~200℃）以及改变晶体的极化周期（26.5~31.5 μm）,可由该光参量振荡器获得2.83~2.89 μm,3.10~3.38 μm,3.57~3.78 μm,3.95~4.12 μm, 4.28~4.46 μm,4.65~4.79 μm的闲频光连续调谐输出. 且当泵浦功率为8.15 W时,在闲频光输出波长为3.33 μm处,获得了最大输出功率2.17 W.     

宽带光学参变啁啾脉冲放大系统的色散控制

在设计宽带光学参变啁啾脉冲放大系统时,对色散源进行了理论分析和讨论。对光学参变啁啾脉冲放大系统的色散量以及各个过程中的高阶色散对脉冲时域和频域特性的影响进行了计算。结果表明展宽器引入了非常大的色散,放大器中信号光相位变化产生的色散较大,参量晶体本身引入的色散相对较小可以忽略不计。输出脉冲宽度主要受二阶色散影响,而三阶和四阶色散主要影响脉冲的波形和信噪比,对频域影响很小。     

Broadband difference frequency mixing between visible and near-infrared pulses for few-cycle pulse generation with stable carrier-envelope phase

Difference frequency generation between broadband visible noncollinear optical parametric amplifier (NOPA) pulses and the fundamental pump laser pulses allows the generation of ultrashort infrared pulses with passively stabilized carrier-envelope phase. A simple prism compressor for the visible NOPA pulses is sufficient to generate few-cycle pulses in the infrared and no additional compression is needed. We theoretically investigate the concept, explain the principles, and demonstrate it for high repetition rate, long pulse durations, and various wavelengths by applying it to a Ti:sapphire and an Yb:KYW-based laser systems. For the latter sub-15 fs phase stable pulses around 1.8 μm with an energy of 100 nJ are obtained at 100 kHz repetition rate.     

Multimillijoule chirped parametric amplification of few-cycle pulses

The concept of optical parametric chirped-pulse amplification is applied to attain pulses with energies up to 8 mJ and a bandwidth of more than 100 THz. Stretched broadband seed pulses from a Ti:sapphire oscillator are amplified in a multistage noncollinear type I phase-matched beta-barium borate parametric amplifier by use of an independent picosecond laser with lock-to-clock repetition rate synchronization. Partial compression of amplified pulses is demonstrated down to a 10-fs duration with a down-chirped pulse stretcher and a nearly lossless compressor comprising bulk material and positive-dispersion chirped mirrors.     

High average power 2 μm generation using an intracavity PPMgLN optical parametric oscillator

An intracavity quasi-phase-matched optical parametric oscillator (OPO) has been developed for the purpose of generating radiation with high average power and high repetition rate in the 2 μm regime. The device is a degenerate OPO based on a 3 mm thick MgO-doped periodically poled LiNbO(3) (PPMgLN) crystal, which is pumped in turn within the cavity by a diode side-pumped, Q-switched 1 μm Nd:YAG laser operating at 10 kHz. Up to 20 W broadband 2 μm radiation can be generated with a compact configuration under the crystal temperature of 115 °C. The beam profile is close to circularly symmetric with M(2) ~ 10.     

High-resolution optical time domain reflectmetry based on a broadband continuous wave multimode laser diode

A broadband light source can be obtained by operating a multimode laser diode with a bias current below threshold. We propose an optical time domain reflectometer for high-resolution with a broadband cw multimode laser. The emission spectrum of the multimode laser diode that affects an interference signal is investigated. With this method, the spatial resolution is measured as 11.5 μm, corresponding to that of 38.3-fs pulses, and a minimum detectable reflectivity < -90 dB is achieved.     

Color center laser pumped by a flashlamp-pumped dye laser

A reliable, pulsed, color center laser is described which provides a pulse energy up to 0.4 mJ in a wavelength range from 2.4 μm to 3.3 μm at a bandwidth below 20 GHz. A simple, broadband, flashlamp-pumped dye laser is used as the pump source. A new transverse pumping scheme of F-centers is described using hydrogenated color center crystal which allows to pump color center lasers with high energy pump pulses.     

Optical parametric generation in CdSiP2

We report efficient generation of picosecond pulses in the near- and mid-IR in the new nonlinear material CdSiP(2) pumped at 1.064 μm by an amplified mode-locked Nd:YVO(4) laser at a 100 kHz repetition rate. By using single-pass optical parametric generation in 8-mm-long crystal cut for type I(e→oo) noncritical phase matching, an average idler power of 154 mW at 6.204 μm together with 1.16 W of signal at 1.282 μm has been obtained for 6.1 W of pump at photon conversion efficiencies of 15% and 23%, respectively. Signal pulse durations of 6.36 ps are measured for 9 ps pump pulses.     

Six-cycle mid-infrared source with 3.8 μJ at 100 kHz

We report on the shortest pulses to date from a mid-IR optical parametric chirped pulse amplification: 67 fs duration with 3.8 μJ energy operating at 3.2 μm. The system is all solid state and diode pumped and operates at 100 kHz with unprecedented power stability of 0.75%rms over 30 min.     

Generation of a mid-infrared broadband polarized supercontinuum in As₂Se₃ photonic crystal fibers

A simplified structure of birefringent chalcogenide As 2 Se 3 photonic crystal fiber(PCF) is designed.Properties of birefringence,polarization extinction ratio,chromatic dispersion,nonlinear coefficient,and transmission are studied by using the multipole method,the finite-difference beam propagation method,and the adaptive split-step Fourier method.Considering that the zero dispersion wavelength of our proposed fiber is about 4 μm,we have analysed the mechanism of spectral broadening in PCFs with different pitches in detail,with femtosecond pulses at a wavelength of 4 μm as the pump pulses.Especially,mid-infrared broadband polarized supercontinuums are obtained in a 3-cm PCF with an optimal pitch of 2 μm.Their spectral width at 20 dB reaches up to 12 μm.In the birefringent PCF,we find that the supercontinuum generation changes with the pump alignment angle.Research results show that no coupling between eigenpolarization modes are observed at the maximum average power(i.e.,37 mW),which indicates that the polarization state is well maintained.     

High-repetition-rate sub-5-fs pulses with 12 GW peak power from fiber-amplifier-pumped optical parametric chirped-pulse amplification

An optical parametric chirped-pulse amplification system delivering pulses with more than 12 GW peak power is presented. Compression to sub-5 fs, 87 μJ and 5.4 fs, 100 μJ is realized at the 30 kHz repetition rate. A high-energy fiber chirped-pulse amplification system operating at 1 mJ pulse energy and nearly transform-limited pulses is used to achieve ultrabroadband amplification in two 2mm beta-barium borate crystals. Precise pulse shaping is used to compress the pulses to a few percentages of their transform limit. Assuming diffraction limited focusing (d<2 μm), peak intensities as high as 10(18) W/cm(2) can be reached.     

High‐energy optical parametric oscillator for the 6 μm spectral range based on HgGa2S4 pumped at 1064 nm

The defect chalcopyrite crystal HgGa₂S₄ has been employed in a 1064‐nm pumped optical parametric oscillator to generate <7 ns long idler pulses near 6.3 μm with energies as high as 3 mJ, tunable in a broad spectral range from 4.5 to 9 μm.     

Frontend light source for short-pulse pumped OPCPA system

We present the development of a light source for generating optically synchronized seed pulses both for the parametric amplifier chain and the pump-laser chain of the Petawatt Field Synthesizer (PFS), which is currently under construction at MPQ. The PFS system aims at delivering waveform-controlled few-cycle laser pulses with PW-scale peak power using optical parametric chirped pulse amplification (OPCPA). Methods of generating the broadband near-infrared (NIR) seed pulses for the OPCPA chain by spectral broadening using few-cycle pulses are presented. We also demonstrate the generation of a supercontinuum spanning up to three octaves (270–1500 nm) using cascaded hollow-core fibers which supports sub-cycle pulse duration.     

A broadband,quasi‐continuous,mid‐infrared supercontinuum generated in a chalcogenide glass waveguide

The production of a broadband supercontinuum spanning from 1.8 μm to >7.5 μm is reported which was created by pumping a chalcogenide glass waveguide with ≈320 fs pulses at 4 μm. The total power was ≈20 mW and the source brightness was 100 that of current synchrotrons. This source promises to be an excellent laboratory tool for infrared microspectroscopy.