Formulation of strain gradient plasticity with interface energy in a consistent thermodynamic framework

In this work, the strain gradient formulation is used within the context of the thermodynamic principle, internal state variables, and thermodynamic and dissipation potentials. These in turn provide balance of momentum, boundary conditions, yield condition and flow rule, and free energy and dissipative energies. This new formulation contributes to the following important related issues: (i) the effects of interface energy that are incorporated into the formulation to address various boundary conditions, strengthening and formation of the boundary layers, (ii) nonlocal temperature effects that are crucial, for instance, for simulating the behavior of high speed machining for metallic materials using the strain gradient plasticity models, (iii) a new form of the nonlocal flow rule, (iv) physical bases of the length scale parameter and its identification using nano-indentation experiments and (v) a wide range of applications of the theory. Applications to thin films on thick substrates for various loading conditions and torsion of thin wires are investigated here along with the appropriate length scale effect on the behavior of these structures. Numerical issues of the theory are discussed and results are obtained using Matlab and Mathematica for the nonlinear ordinary differential equations (NODE) which constitute the boundary value problem.This study reveals that the micro-stress term has an important effect on the development of the boundary layers and hardening of the material at both hard and soft interface boundary conditions in thin films. The interface boundary conditions are described by the interfacial length scale and interfacial strength parameters. These parameters are important to control the size effect and hardening of the material. For more complex geometries the generalized form of the boundary value problem using the nonlocal finite element formulation is required to address the problems involved.     

Modelling of the interface between a thin film and a substrate within a strain gradient plasticity framework

Interfaces play an important role for the plastic deformation at the micron scale. In this paper, two types of interface models for isotropic materials are developed and applied in a thin film analysis. The first type, which can also be motivated from dislocation theory, assumes that the plastic work at the interface is stored as a surface energy that is linear in plastic strain. In the second model, the plastic work is completely dissipated and there is no build-up of a surface energy. Both formulations introduce one length scale parameter for the bulk material and one for the interface, which together control the film behaviour. It is demonstrated that the two interface models give equivalent results for a monotonous, increasing load. The combined influence of bulk and interface is numerically studied and it is shown that size effects are obtained, which are controlled by the length scale parameters of bulk and interface.     

A unified residual-based thermodynamic framework for strain gradient theories of plasticity

A unified thermodynamic framework for gradient plasticity theories in small deformations is provided, which is able to accommodate (almost) all existing strain gradient plasticity theories. The concept of energy residual (the long range power density transferred to the generic particle from the surrounding material and locally spent to sustain some extra plastic power) plays a crucial role. An energy balance principle for the extra plastic power leads to a representation formula of the energy residual in terms of a long range stress, typically of the third order, a macroscopic counterpart of the micro-forces acting on the GNDs (Geometrically Necessary Dislocations). The insulation condition (implying that no long range energy interactions are allowed between the body and the exterior environment) is used to derive the higher order boundary conditions, as well as to ascertain a principle of the plastic power redistribution in which the energy residual plays the role of redistributor and guarantees that the actual plastic dissipation satisfies the second thermodynamics principle. The (nonlocal) Clausius-Duhem inequality, into which the long range stress enters aside the Cauchy stress, is used to derive the thermodynamic restrictions on the constitutive equations, which include the state equations and the dissipation inequality. Consistent with the latter inequality, the evolution laws are formulated for rate-independent models. These are shown to exhibit multiple size effects, namely (energetic) size effects on the hardening rate, as well as combined (dissipative) size effects on both the yield strength (intrinsic resistance to the onset of plastic strain) and the flow strength (resistance exhibited during plastic flow). A friction analogy is proposed as an aid for a better understanding of these two kinds of strengthening effects. The relevant boundary-value rate problem is addressed, for which a solution uniqueness theorem and a minimum variational principle are provided. Comparisons with other existing gradient theories are presented. The dissipation redistribution mechanism is illustrated by means of a simple shear model.     

Shakedown analysis for a class of strengthening materials within the framework of gradient plasticity

The classical shakedown theory is extended to a class of perfectly plastic materials with strengthening effects (Hall–Petch effects). To this aim, a strain gradient plasticity model previously advanced by Polizzotto (2010) is used, whereby a featuring strengthening law provides the strengthening stress, i.e. the increase of the yield strength produced by plastic deformation, as a degree-zero homogeneous second-order differential form in the accumulated plastic strain with associated higher order boundary conditions. The extended static (Melan) and kinematic (Koiter) shakedown theorems are proved together with the related lower bound and upper bound theorems. The shakedown limit load problem is addressed and discussed in the present context, and its solution uniqueness shown out. A simple micro-scale structural system is considered as an illustrative example. The shakedown limit load is shown to increase with decreasing the structural size, which is a manifestation of the classical Hall–Petch effects in a context of cyclic loading.     

Analysis of size effects associated to the transformation strain in TRIP steels with strain gradient plasticity

The size dependent strengthening resulting from the transformation strain in Transformation Induced Plasticity (TRIP) steels is investigated using a two-dimensional embedded cell model of a simplified microstructure composed of small cylindrical metastable austenitic inclusions within a ferritic matrix. Earlier studies have shown that within the framework of classical plasticity or of the single length parameter Fleck–Hutchinson strain gradient plasticity theory, the transformation strain has no significant impact on the overall strengthening. The strengthening is essentially coming from the composite effect with a marked inclusion size effect resulting from the appearance during deformation of new boundaries constraining the plastic flow. The three parameters version of the Fleck–Hutchinson strain gradient plasticity theory is used here in order to better capture the effect of the plastic strain gradients resulting from the transformation strain. The three parameters theory incorporates separately the rotational and extensional gradients in the formulation, which leads to a significant influence of the shear component of the transformation strain, not captured by the single-parameter theory. When the size of the austenitic inclusions decreases, the overall strengthening increases due to a combined size dependent effect of the transformation strain and of the evolving composite structure. A parametric study is proposed and discussed in the light of experimental evidences giving indications on the optimization of the microstructure of TRIP-assisted multi-phase steels.     

A unified treatment of strain gradient plasticity

A theoretical framework is presented that has potential to cover a large range of strain gradient plasticity effects in isotropic materials. Both incremental plasticity and viscoplasticity models are presented. Many of the alternative models that have been presented in the literature are included as special cases. Based on the expression for plastic dissipation, it is in accordance with Gurtin (J. Mech. Phys. Solids 48 (2000) 989; Int. J. Plast. 19 (2003) 47) argued that the plastic flow direction is governed by a microstress q_ij and not the deviatoric Cauchy stress σ_ij′ that has been assumed by many others. The structure of the governing equations is of second order in the displacements and the plastic strains which makes it comparatively easy to implement in a finite element programme. In addition, a framework for the formulation of consistent boundary conditions is presented. It is shown that there is a close connection between surface energy of an interface and boundary conditions in terms of plastic strains and moment stresses. This should make it possible to study boundary layer effects at the interface between grains or phases. Consistent boundary conditions for an expanding elastic-plastic boundary are as well formulated. As examples, biaxial tension of a thin film on a thick substrate, torsion of a thin wire and a spherical void under remote hydrostatic tension are investigated.     

On lower order strain gradient plasticity theories

By way of numerical examples, this paper explores the nature of solutions to a class of strain gradient plasticity theories that employ conventional stresses, equilibrium equations and boundary conditions. Strain gradients come into play in these modified conventional theories only to alter the tangent moduli governing increments of stress and strain. It is shown that the modification is far from benign from a mathematical standpoint, changing the qualitative character of solutions and leading to a new type of localization that is at odds with what is expected from a strain gradient theory. The findings raise questions about the physical acceptability of this class of strain gradient theories.     

Interfacial gradient plasticity governs scale-dependent yield strength and strain hardening rates in micro/nano structured metals

The effect of the material microstructural interfaces increases as the surface-to-volume ratio increases. It is shown in this work that interfacial effects have a profound impact on the scale-dependent yield strength and strain hardening of micro/nano-systems even under uniform stressing. This is achieved by adopting a higher-order gradient-dependent plasticity theory [Abu Al-Rub, R.K., Voyiadjis, G.Z., Bammann, D.J., 2007. A thermodynamic based higher-order gradient theory for size dependent plasticity. Int. J. Solids Struct. 44, 2888–2923] that enforces microscopic boundary conditions at interfaces and free surfaces. Those nonstandard boundary conditions relate a microtraction stress to the interfacial energy at the interface. In addition to the nonlocal yield condition for the material’s bulk, a microscopic yield condition for the interface is presented, which determines the stress at which the interface begins to deform plastically and harden. Hence, two material length scales are incorporated: one for the bulk and the other for the interface. Different expressions for the interfacial energy are investigated. The effect of the interfacial yield strength and interfacial hardening are studied by analytically solving a one-dimensional Hall–Petch-type size effect problem. It is found that when assuming compliant interfaces the interface properties control both the material’s global yield strength and rates of strain hardening such that the interfacial strength controls the global yield strength whereas the interfacial hardening controls both the global yield strength and strain hardening rates. On the other hand, when assuming a stiff interface, the bulk length scale controls both the global yield strength and strain hardening rates. Moreover, it is found that in order to correctly predict the increase in the yield strength with decreasing size, the interfacial length scale should scale the magnitude of both the interfacial yield strength and interfacial hardening.     

A finite deformation theory of strain gradient plasticity

Plastic deformation exhibits strong size dependence at the micron scale, as observed in micro-torsion, bending, and indentation experiments. Classical plasticity theories, which possess no internal material lengths, cannot explain this size dependence. Based on dislocation mechanics, strain gradient plasticity theories have been developed for micron-scale applications. These theories, however, have been limited to infinitesimal deformation, even though the micro-scale experiments involve rather large strains and rotations. In this paper, we propose a finite deformation theory of strain gradient plasticity. The kinematics relations (including strain gradients), equilibrium equations, and constitutive laws are expressed in the reference configuration. The finite deformation strain gradient theory is used to model micro-indentation with results agreeing very well with the experimental data. We show that the finite deformation effect is not very significant for modeling micro-indentation experiments.     

On the formulations of higher-order strain gradient crystal plasticity models

Recently, several higher-order extensions to the crystal plasticity theory have been proposed to incorporate effects of material length scales that were missing links in the conventional continuum mechanics. The extended theories are classified into work-conjugate and non-work-conjugate types. A common feature of the former is that existence of higher-order stresses work-conjugate to gradients of plastic strain is presumed and an extended principle of virtual work involving such an additional virtual work contribution is formulated. Meanwhile, in the latter type, the higher-order stress quantities do not appear explicitly. Instead, rates of crystallographic slip are influenced by back stresses that arise in response to spatial gradients of the geometrically necessary dislocation densities. The work-conjugate type and the non-work-conjugate type of theories have different theoretical backgrounds and very unlike mathematical representations. Nevertheless, both types of theories predict the same kind of material length scale effects. We have recently shown that there exists some equivalency between the two approaches in the special situation of two-dimensional single slip under small deformation. In this paper, the discussion is extended to a more general situation, i.e. the context of multiple and three-dimensional slip deformations.     

Stress gradient versus strain gradient constitutive models within elasticity

A stress gradient elasticity theory is developed which is based on the Eringen method to address nonlocal elasticity by means of differential equations. By suitable thermodynamics arguments (involving the free enthalpy instead of the free internal energy), the restrictions on the related constitutive equations are determined, which include the well-known Eringen stress gradient constitutive equations, as well as the associated (so far uncertain) boundary conditions. The proposed theory exhibits complementary characters with respect to the analogous strain gradient elasticity theory. The associated boundary-value problem is shown to admit a unique solution characterized by a Hellinger–Reissner type variational principle. The main differences between the Eringen stress gradient model and the concomitant Aifantis strain gradient model are pointed out. A rigorous formulation of the stress gradient Euler–Bernoulli beam is provided; the response of this beam model is discussed as for its sensitivity to the stress gradient effects and compared with the analogous strain gradient beam model.     

Strain gradient effects on cyclic plasticity

Size effects on the cyclic shear response are studied numerically using a recent higher order strain gradient visco-plasticity theory accounting for both dissipative and energetic gradient hardening. Numerical investigations of the response under cyclic pure shear and shear of a finite slab between rigid platens have been carried out, using the finite element method. It is shown for elastic-perfectly plastic solids how dissipative gradient effects lead to increased yield strength, whereas energetic gradient contributions lead to increased hardening as well as a Bauschinger effect. For linearly hardening materials it is quantified how dissipative and energetic gradient effects promote hardening above that of conventional predictions. Usually, increased hardening is attributed to energetic gradient effects, but here it is found that also dissipative gradient effects lead to additional hardening in the presence of conventional material hardening. Furthermore, it is shown that dissipative gradient effects can lead to both an increase and a decrease in the dissipation per load cycle depending on the magnitude of the dissipative length parameter, whereas energetic gradient effects lead to decreasing dissipation for increasing energetic length parameter. For dissipative gradient effects it is found that dissipation has a maximum value for some none zero value of the material length parameter, which depends on the magnitude of the deformation cycles.     

A separated law of hardening in strain gradient plasticity

This paper presents a separated law of hardening in plasticity with strain gradient effects. The value of the length parameter ℓ contained in this model was estimated from the experimental data for copper. The project supported by the National Natural Science Foundation of China     

On the homogenization of metal matrix composites using strain gradient plasticity

The homogenized response of metal matrix composites（MMC） is studied using strain gradient plasticity.The material model employed is a rate independent formulation of energetic strain gradient plasticity at the micro scale and conventional rate independent plasticity at the macro scale. Free energy inside the micro structure is included due to the elastic strains and plastic strain gradients. A unit cell containing a circular elastic fiber is analyzed under macroscopic simple shear in addition to transverse and longitudinal loading. The analyses are carried out under generalized plane strain condition. Micro-macro homogenization is performed observing the Hill-Mandel energy condition,and overall loading is considered such that the homogenized higher order terms vanish. The results highlight the intrinsic size-effects as well as the effect of fiber volume fraction on the overall response curves, plastic strain distributions and homogenized yield surfaces under different loading conditions. It is concluded that composites with smaller reinforcement size have larger initial yield surfaces and furthermore,they exhibit more kinematic hardening.     

Mechanism-based strain gradient plasticity in C0 axisymmetric element

Non-uniform plastic deformation of materials exhibits a strong size dependence when the material and deformation length scales are of the same order at micro- and nano-metre levels. Recent progresses in testing equipment and computational facilities enhancing further the study on material characterization at these levels confirmed the size effect phenomenon. It has been shown that at this length scale, the material constitutive condition involves not only the state of strain but also the strain gradient plasticity. In this study, C⁰ axisymmetric element incorporating the mechanism-based strain gradient plasticity is developed. Classical continuum plasticity approach taking into consideration Taylor dislocation model is adopted. As the length scale and strain gradient affect only the constitutive relation, it is unnecessary to introduce either additional model variables or higher order stress components. This results in the ease and convenience in the implementation. Additional computational efforts and resources required of the proposed approach as compared with conventional finite element analyses are minimal. Numerical results on indentation tests at micron and submicron levels confirm the necessity of including the mechanism-based strain gradient plasticity with appropriate inherent material length scale. It is also interesting to note that the material is hardened under Berkovich compared to conical indenters when plastic strain gradient is considered but softened otherwise.     

A nonlocal strain gradient plasticity theory for finite deformations

Strain gradient plasticity for finite deformations is addressed within the framework of nonlocal continuum thermodynamics, featured by the concepts of (nonlocality) energy residual and globally simple material. The plastic strain gradient is assumed to be physically meaningful in the domain of particle isoclinic configurations (with the director vector triad constant both in space and time), whereas the objective notion of corotational gradient makes it possible to compute the plastic strain gradient in any domain of particle intermediate configurations. A phenomenological elastic–plastic constitutive model is presented, with mixed kinematic/isotropic hardening laws in the form of PDEs and related higher order boundary conditions (including those associated with the moving elastic/plastic boundary). Two fourth-order projection tensor operators, functions of the elastic and plastic strain states, are shown to relate the skew-symmetric parts of the Mandel stress and back stress to the related symmetric parts. Consistent with the thermodynamic restrictions therein derived, the flow laws for rate-independent associative plasticity are formulated in a six-dimensional tensor space in terms of symmetric parts of Mandel stresses and related work-conjugate generalized plastic strain rates. A simple shear problem application is presented for illustrative purposes.     

Grain boundary interface mechanics in strain gradient crystal plasticity

Interactions between dislocations and grain boundaries play an important role in the plastic deformation of polycrystalline metals. Capturing accurately the behaviour of these internal interfaces is particularly important for applications where the relative grain boundary fraction is significant, such as ultra fine-grained metals, thin films and micro-devices. Incorporating these micro-scale interactions (which are sensitive to a number of dislocation, interface and crystallographic parameters) within a macro-scale crystal plasticity model poses a challenge. The innovative features in the present paper include (i) the formulation of a thermodynamically consistent grain boundary interface model within a microstructurally motivated strain gradient crystal plasticity framework, (ii) the presence of intra-grain slip system coupling through a microstructurally derived internal stress, (iii) the incorporation of inter-grain slip system coupling via an interface energy accounting for both the magnitude and direction of contributions to the residual defect from all slip systems in the two neighbouring grains, and (iv) the numerical implementation of the grain boundary model to directly investigate the influence of the interface constitutive parameters on plastic deformation. The model problem of a bicrystal deforming in plane strain is analysed. The influence of dissipative and energetic interface hardening, grain misorientation, asymmetry in the grain orientations and the grain size are systematically investigated. In each case, the crystal response is compared with reference calculations with grain boundaries that are either ‘microhard’ (impenetrable to dislocations) or ‘microfree’ (an infinite dislocation sink).