Energy scaling of a carbon nanotube saturable absorber mode-locked femtosecond bulk laser

We report successful energy scaling of a room-temperature femtosecond Cr⁴⁺: forsterite laser by using a single-walled carbon nanotube saturable absorber (SWCNT-SA). By incorporating a q-preserving multipass cavity, a repetition rate of 4.51?MHz was realized, and the oscillator produced 121?fs, 10?nJ pulses at 1247?nm, with an average output power of 46?mW. To the best of our knowledge, the peak power of 84?kW is the highest generated to date from a SWCNT-SA mode-locked oscillator. Furthermore, energy scaling of a femtosecond multipass-cavity laser, mode-locked using a SWCNT-SA, is demonstrated for the first time.     

Wavelength dependent damage in biological multi-photon confocal microscopy: A micro-spectroscopic comparison between femtosecond Ti:sapphire and Cr:forsterite laser sources

Molecular excitation by the simultaneous absorption of two photons provides intrinsic three-dimensional resolution in laser scanning fluorescence microscopy. Thus induced two-photon absorption and the accompanied multi-photon absorption/ionization not only cause photo-bleaching but also cell damage in the vicinity of the focal point. In this paper, we study the wavelength dependent cell damage induced by high intensity femtosecond near infrared lasers. The study was performed with a Ti:sapphire laser and a Cr:forsterite laser. With a longer output wavelength from a Cr:forsterite laser, multi-photon absorption and auto-fluorescence were found to be significantly suppressed and the destructive plasma formation was found to be greatly reduced. Sustained multi-photon spectra can be observed in most plant specimens with a tightly focused Cr:forsterite laser beam under long term irradiation with more than 100 mW laser average power. In contrast, multi-photon absorption induced destructive plasma formation were frequently observed with a tightly focused Ti:sapphire laser beam within seconds with more than 10 mW laser average power.     

Direct diode-pumped continuous-wave near-inf rared tunable laser operation of Cr(4+):forsterite and Cr(4+):Ca(2)GeO(4)

Continuous-wave tunable laser operation of direct diode-pumped Cr(4+):Mg(2)SiO(4) (Cr:forsterite) and Cr(4+):Ca(2)GeO(4) (cunyite) crystal were demonstrated. Diode-pumped Cr:forsterite was tunable over the 1236-1300-nm spectral range. The maximum output of 10 mW was measured at 1260 nm for 640 mW of pump power absorbed by the crystal. Diode-pumped laser operation of cunyite was also demonstrated over the 1390-1475-nm range. Free-running 20-mW output was centered at 1410 nm.     

自锁模飞秒掺铬的镁橄榄石激光器的实验研究

用波长为1.06μm的Nd:YAG激光器泵浦Cr⁴⁺:forsterite晶体,实现了Cr⁴⁺:forsterite激光器的自锁模飞秒激光运转,在吸收泵浦功率为8W的条件下,得到了脉冲宽度为85fs,中心波长为1246nm,平均输出功率为200mW的稳定锁模输出。     

Efficient, kHz repetition rate, gain-switched Cr:forsterite laser

We have developed a gain-switched room-temperature Cr:forsterite laser operating at repetition rates of between 1 and 34 kHz, and pumped by a continuous wave, Q-switched Nd:YAG laser. With optimised output coupling, an output pulse energy of 52 μJ was measured at 1.5 kHz repetition rate, corresponding to 11% efficiency and 13% slope efficiency. Threshold pulse energy was 53 μJ. Output power of 370 mW was obtained at 10 kHz repetition rate and 4.4 W pump power. Water cooling was not required for repetition rates up to 10 kHz. In a tunable, folded resonator, the Cr:forsterite wavelength tuned between 1173 and 1338 nm. This laser operated with maximum pulse energy of 34 μJ, efficiency of 13%, and power of 307 mW. The laser output was close to diffraction-limited with M² of 1.2. Received: 6 January 1999 / Published online: 29 July 1999     

Two-octave spectral broadening of subnanojoule Cr:forsterite femtosecond laser pulses in tapered fibers

Spectral broadening of femtosecond Cr:forsterite laser pulses is enhanced due to the use of tapered fibers. Supercontinuum generation with unamplified subnanojoule femtosecond Cr:forsterite laser pulses is observed for the first time. With 40-fs 0.6-nJ pulses of 1.25-μm Cr:forsterite laser radiation coupled into a tapered fiber having a taper waist diameter of about 2 μm and a taper waist length of 90 mm, we observed the spectra spanning more than two octaves at the output of the fiber in the regime of anomalous group-velocity dispersion. This result opens the way for the creation of compact femtosecond Cr:forsterite laser plus tapered fiber systems for optical metrology and biomedical applications. Received: 23 October 2001 / Accepted: 16 January 2002 / Published online: 14 March 2002     

Pump-probe nonlinear absorption spectroscopy of molecular aggregates using chirped frequency-shifted light pulses from a photonic-crystal fiber

Photonic-crystal fibers provide efficient nonlinear-optical transformations of femtosecond Cr: forsterite laser pulses, delivering linearly chirped frequency-shifted broadband light pulses optimized for pump-probe nonlinear absorption spectroscopy of molecular aggregates. The blue-shifted output of a photonic-crystal fiber with a spectrum stretching from 530 to 680 nm is used to probe one-and two-exciton bands of thiacarbocyanine J aggregates in a polymer film excited by femtosecond second-harmonic pulses of the Cr: forsterite laser.     

Simultaneous multiwavelength generation from a mode-locked all-solid-state Cr:forsterite laser

We demonstrate a multiple-channel, mode-locked, all-solid-state Cr:forsterite laser. By inserting an etalon into the laser cavity, we have generated 12 phase-locked channels with 9-19-ps pulse width near 1230 nm with 280-mW average output power from a single laser oscillator. By tuning the etalon bandwidth we can shorten the pulse width in a specific channel to 1.8 ps.     

Cr:forsterite laser pumped by broad-area laser diodes

We report the demonstration of a Cr:forsterite laser pumped by broad-area laser diodes producing non-diffraction-limited beams. The use of a thin crystal to reduce losses at the lasing wavelength and of short-wavelength pump diodes reduces the lasing threshold to <500mW .Relatively low output powers (5mW) are obtained, but prospects for increasing the power and achieving mode-locked operation of this laser are good and are discussed.     

Microjoule supercontinuum generation by stretched megawatt femtosecond laser pulses in a large-mode-area photonic-crystal fiber

Microjoule supercontinuum generation is demonstrated using a large-mode-area photonic-crystal fiber (PCF) pumped by an amplified stretched-pulse output of a mode-locked Cr:forsterite laser. A PCF with a mode area of 380 μm² is employed to transform 300-fs Cr:forsterite laser pulses with a peak-power of a few megawatts into a supercontinuum radiation with a spectrum spanning from 700 to 1800 nm and a total energy of 1.15 μJ.     

Spectral superbroadening of subnanojoule Cr:Forsterite femtosecond laser pulses in a tapered fiber

Spectral superbroadening of subnanojoule femtosecond Cr:forsterite laser pulses is demonstrated for the first time in experiments with a tapered fiber. Coupling 40-fs 0.6-nJ pulses of 1.25-μm Cr:forsterite laser radiation into a tapered fiber with a taper waist diameter of about 2 μm and a taper waist length of 90 mm, we observed the spectra spanning more than two octaves at the output of the fiber. These experimental results open new horizons for the creation of compact femtosecond systems based on Cr:forsterite lasers and tapered fibers for optical metrology and biomedical applications.     

Microstructure fibers as frequency-tunable sources of ultrashort chirped pulses for coherent nonlinear spectroscopy

Microstructure fibers are shown to allow the creation of new tunable sources for femtosecond nonlinear spectroscopy. These fibers provide a high efficiency of frequency upconversion of regeneratively amplified femtosecond pulses of a Cr:forsterite laser, permitting the generation of subpicosecond anti-Stokes pulses with a smooth temporal envelope and a linear positive chirp. These pulses from a microstructure fiber were used to measure the spectra of coherent anti-Stokes Raman scattering (CARS) of toluene solution by cross-correlating these pulses with the femtosecond second-harmonic output of the Cr:forsterite laser in boxcars geometry (XFROG CARS). PACS 42.65.Wi; 42.81.Qb     

All-solid-state Cr:forsterite laser generating 14-fs pulses at 1.3 mum

We report the generation of 14-fs pulses at 1.3mum with 80-mW average power at 100-MHz repetition rate by an all-solid-state Kerr-lens mode-locked Cr:forsterite laser. The laser spectrum covers wavelengths of 1230-1580 nm, with a FWHM of 250 nm. Since 1.3-mum wavelengths are close to the zero dispersion wavelength of Cr:forsterite, higher-order dispersion is the main factor limiting pulse durations. We use specially designed and fabricated double-chirped mirrors in combination with high-index PBH71 prisms to compensate for the intracavity dispersion over almost 300 nm.     

Improved stabilization of a 1.3 microm femtosecond optical frequency comb by use of a spectrally tailored continuum from a nonlinear fiber grating

We report significant enhancement (+24 dB) of the optical beat note between a 657 nm cw laser and the second-harmonic generation of the tailored continuum at 1314 nm generated with a femtosecond Cr:forsterite laser and a nonlinear fiber Bragg grating. The same continuum is used to stabilize the carrier-envelope offset frequency of the Cr:forsterite femtosecond laser and permits improved optical stabilization of the frequency comb from 1.0 to 2.2 microm. Using a common optical reference at 657 nm, a relative fractional frequency instability of 2.0 x 10(-15) is achieved between the repetition rates of Cr:forsterite and Ti:sapphire laser systems in 10 s averaging time. The fractional frequency offset between the optically stabilized frequency combs of the Cr:forsterite and Ti:sapphire lasers is +/-(0.024 +/- 6.1) x 10(-17).     

LD end-pumped passively mode-locked Nd:YVO<Subscript>4</Subscript> laser with single-walled carbon nanotubes

We demonstrate a LD end-pumped passively mode-locked Nd:YVO₄ laser using a single-walled carbon nanotubes saturable absorber (SWCNT-SA). The SWCNT wafer was fabricated by electric arc discharge method on quartz substrate with absorption wavelength of 1064 nm. At the absorbed pump of 15.8 W, an output power of 750 mW CW (continuous wave) mode-locked laser pulse was achieved with the repetition of 79.7 MHz, corresponding to optical-optical efficiency of 4.75%.     

Relative carrier-envelope phase dynamics between passively synchronized Ti:sapphire and Cr:forsterite lasers

We observed and measured the relative carrier-envelope phase difference per round trip between synchronized femtosecond Ti:sapphire and Cr:forsterite mode-locked lasers. The relative carrier-envelope phase slip was directly recorded by heterodyning of the Cr:forsterite laser with the supercontinuum from the Ti:sapphire laser. We also obtained another phase relation by superimposing the third harmonic of the Cr:forsterite laser with the second harmonic of the Ti:sapphire laser. In the latter case we obtained a stable beat signal with a signal-to-noise ratio larger than 30 dB and found a dependence of the beat frequency on the cavity length.     

Broadband phase-coherent optical frequency synthesis with actively linked Ti:sapphire and Cr:forsterite femtosecond lasers

We link the output spectra of a Ti:sapphire and a Cr:forsterite femtosecond laser phase coherently to form a continuous frequency comb with a wavelength coverage of 0.57-1.45 microm at power levels of 1 nW to 40 microW per frequency mode. To achieve this, the laser repetition rates and the carrier-envelope offset frequencies are phase locked to each other. The coherence time between the individual components of the two combs is 40 micros. The timing jitter between the lasers is 20 fs. The combined frequency comb is self-referenced for access to its overall offset frequency. We report the first demonstration to our knowledge of an extremely broadband and continuous, high-powered and phase-coherent frequency comb from two femtosecond lasers with different gain media.     

Coherent anti-Stokes Raman scattering microspectroscopy of silicon components with a photonic-crystal fiber frequency shifter

Coherent anti-Stokes Raman scattering (CARS) microspectroscopy of silicon components is demonstrated with pump and probe fields delivered by a mode-locked Cr:forsterite laser and the frequency-shifted soliton output of a photonic-crystal fiber as a Stokes field. CARS microspectroscopy is shown to allow a visualization of microscale features and defects on the surface of silicon wafers, offering much promise for online diagnostics of electronic and photonic silicon chip components.     

High-quality, large-area monolayer graphene for efficient bulk laser mode-locking near 1.25 μm

High-quality monolayer graphene as large as 1.2×1.2?cm² was synthesized by chemical vapor deposition and used as a transmitting saturable absorber for efficient passive mode-locking of a femtosecond bulk solid-state laser. The monolayer graphene mode-locked Cr:forsterite laser was tunable around 1.25?μm and delivered sub-100?fs pulses with output powers up to 230?mW. The nonlinear optical characteristics of the monolayer graphene saturable absorber and the mode-locked operation were then compared with the case of the bilayer graphene saturable absorber.     

54-fs, 1-GW, 1-kHz pulse amplification in Cr:forsterite

30-fs pulses at 1.22 microm are produced by a self-mode-locked Cr:forsterite laser and amplified in a Cr:forsterite regenerative amplifier by a chirped-pulse amplification technique. 54-fs, 1-GW pulses at a 1-kHz repetition rate are obtained.