Parametric amplification of few-cycle carrier-envelope phase-stable pulses at 2.1 microm

We demonstrate an optical parametric chirped-pulse amplifier producing infrared 20 fs (3-optical-cycle) pulses with a stable carrier-envelope phase. The amplifier is seeded with self-phase-stabilized pulses obtained by optical rectification of the output of an ultrabroadband Ti:sapphire oscillator. Energies of -80 microJ with a well-suppressed background of parametric superfluorescence and up to 400 microJ with a superfluorescence background are obtained from a two-stage parametric amplifier based on periodically poled LiNbO3 and LiTaO3 crystals. The parametric amplifier is pumped by an optically synchronized 1 kHz, 30 ps, 1053 nm Nd:YLF amplifier seeded by the same Ti:sapphire oscillator.     

Timing jitter in a kilohertz regenerative amplifier of a femtosecond-pulse Ti:Al(2)O(3) laser

We measure the timing error of femtosecond pulses amplified by a Ti:sapphire regenerative amplifier at a 1-kHz repetition rate by use of a modified cross-correlation technique. Linearly frequency-chirped amplified pulses are frequency mixed with transform-limited oscillator pulses. A shift in the sum frequency corresponds to the timing error of each amplified pulse relative to the oscillator pulses. The timing error was measured every 6 ms with approximately 1-fs resolution over a measurable range of 400 fs.     

采用飞秒光纤激光同步泵浦的自启动锁模钛宝石激光研究

针对常规连续激光泵浦钛宝石激光振荡器不能自启动锁模的缺点,采用倍频飞秒光纤激光同步泵浦,通过调节振荡器腔长与泵浦腔长匹配,实现了飞秒钛宝石激光的自启动锁模。实验中采用3.4 W的倍频掺镱光纤激光同步泵浦钛宝石激光振荡器,获得了平均功率大于130 mW、重复频率75 MHz、光谱宽度大于47 nm、脉冲宽度17 fs的锁模脉冲输出,不仅能够稳定可靠地实现自启动锁模,解决了常规钛宝石激光振荡器锁模启动的困难,而且还具有同步输出1040,800,520 nm三束飞秒激光的特点,为进一步开展飞秒激光相干合成以及光参量放大等研究提供了优势基础。     

High-average-power kilohertz-repetition-rate sub-100-fs Ti:sapphire amplifier system

We report on a femtosecond Ti:sapphire laser amplifier system that generates pulse energies >5 mJ at a 1-kHz repetition rate. The system consists of regenerative and multipass amplifiers and uses the technique of chirped-pulse amplification. When the system was seeded with 70-fs pulses at 800 nm from a self-mode-locked Ti:sapphire oscillator, amplified pulses of 94-fs duration at a repetition rate of 1 kHz and an average output power of 5.4 W were produced. The amplified pulse-repetition rate is variable from 250 Hz to 3 kHz. Pulse energies of >7.5 mJ were obtained at 500 and 250 Hz.     

Generation of 0.1-TW 5-fs optical pulses at a 1-kHz repetition rate

A compact all-solid-state femtosecond Ti:sapphire oscillator?amplifier system using no grating-based pulse stretcher produces 20-fs, 1.5-mJ pulses at a 1-kHz repetition rate. The pulses are subsequently compressed in a hollow-fiber chirped-mirror compressor. The system delivers bandwidth-limited 5-fs, 0.5-mJ pulses at 780 nm in a diffraction-limited beam.     

Phase-preserving chirped-pulse optical parametric amplification to 17.3 fs directly from a Ti:sapphire oscillator

Phase-stabilized 12-fs, 1-nJ pulses from a commercial Ti:sapphire oscillator are directly amplified in a chirped-pulse optical parametric amplifier and recompressed to yield near-transform-limited 17.3-fs pulses. The amplification process is demonstrated to be phase preserving and leads to 85-microJ, carrier-envelope-offset phase-locked pulses at 1 kHz for 0.9 mJ of pump, corresponding to a single-pass gain of 8.5 x 10(4).     

Nonlinear optics with phase-controlled pulses in the sub-two-cycle regime.

Nonlinear optical effects due to the phase between carrier and envelope are observed with 5 fs pulses from a Kerr-lens mode-locked Ti:sapphire laser. These sub-two-cycle pulses with octave spanning spectra are the shortest pulses ever generated directly from a laser oscillator. Detection of the carrier-envelope phase slip is made possible by simply focusing the short pulses directly from the oscillator into a BBO crystal. As a further example of nonlinear optics with such short pulses, the interference between second- and third-harmonic components is also demonstrated.     

全固态kHz啁啾脉冲飞秒激光放大器

要建造大功率超强激光系统,必须将nJ量级的种子进行放大,以得到mJ量级以及更高能量的激光输出.为达到这个目的,必须使种子能量指数增加,再生腔放大器是实现这一目的的良好途径;同时,为了得到更稳定的激光输出,须采用高重复频率的泵浦源.为此,设计了一种kHz重复频率激光泵浦的再生放大器,使用15 mJ的527 nm的绿光泵浦,得到了约2.3 mJ的800 nm放大激光输出,同时,对其输出激光的光谱特性进行了测量,将带宽为40 nm的种子注入后,得到了光谱带宽约为30 nm激光输出.     

A double-pass optical parametric amplifier seeded by a blue-shifted output of a photonic-crystal fiber

A blue-shifted output of a photonic-crystal fiber, providing a frequency upconversion of femtosecond Ti:sapphire laser pulses, is used to seed a double-pass optical parametric oscillator (OPA). The OPA is based on a BBO crystal, pumped by 65-mW 150-fs second-harmonic pulses of a Ti:sapphire laser. Gain factors in excess of 10³ are demonstrated for such an OPA, yielding tunable light pulses within the range of wavelengths from 420 to 650 nm, a peak power up to 250 kW, and a typical pulse width of about 200 fs at a repetition rate of 100 kHz. PACS 42.81.Gs; 42.81.Qb     

High-power parametric amplification of 11.8-fs laser pulses with carrier-envelope phase control

Phase-stable parametric chirped-pulse amplification of ultrashort pulses from a carrier-envelope phase-stabilized mode-locked Ti:sapphire oscillator (11.0 fs) to 0.25 mJ/pulse at 1 kHz is demonstrated. Compression with a grating compressor and a LCD shaper yields near-Fourier-limited 11.8-fs pulses with an energy of 0.12 mJ. The amplifier is pumped by 532-nm pulses from a synchronized mode-locked laser, Nd:YAG amplifier system. This approach is shown to be promising for the next generation of ultrafast amplifiers aimed at producing terawatt-level phase-controlled few-cycle laser pulses.     

Operation of Kerr-lens mode-locked Ti:sapphire laser in thenon-soliton regime

A Kerr-lens mode-locked Ti:sapphire laser operating in a non-soliton regime is demonstrated. Dispersive wave generation is observed as a result of third order dispersion in the vicinity of zero dispersion. The characteristics of the Ti:sapphire laser operating in a positive dispersion regime are presented, where the oscillator directly generates pulses with duration continuously tunable from 0.37~ps to 2.11~ps, and 36~fs pulses are achieved after extracavity compression. The oscillation is numerically simulated with an extended nonlinear Schr?dinger equation, and the simulation results are in good agreement with the experimental results.     

Compression of long-cavity Ti:sapphire oscillator pulses with large-mode-area photonic crystal fibers

Motivated by the pulse compression challenge of novel long-cavity, high-pulse-energy Ti:sapphire laser oscillators, we report on ~280 nm supercontinuum generation and 4.5-times compression of close to transform limited, high-energy oscillator pulses using different large-mode-area photonic crystal fibers and standard chirped mirrors. As input, we used pulses of a long-cavity Ti:sapphire oscillator with 190 nJ pulse energy, 70 fs pulse length and 3.6 MHz repetition rate. Compressed pulses at the fiber/compressor output had a duration of 15–18 fs with up to 100 nJ pulse energy representing as much as 53 % throughput for the fiber/chirped mirror system. Using transform-limited input pulses, we could use short fiber pieces and thus a simple, low-dispersion chirped mirror compressor comprised of one pair of mirrors.     

Generation of single-cycle THz transients with high electric-field amplitudes

Single-cycle terahertz (THz) transients in the frequency range 0.3-7 THz with electric-field amplitudes of more than 400 kV/cm are generated by four-wave mixing of the fundamental and the second harmonic of 25 fs pulses from a Ti:sapphire amplifier in ionized air. These transients are fully characterized by electro-optic sampling with ZnTe and GaP crystals. One can tune the center frequency of the THz transients by varying the length of the incident pulse. The electric-field amplitude increases linearly with the incident pulse energy.     

Sub-10-fs pulse generation from a blue laser-diode-pumped Ti:sapphire oscillator

Pulses as short as 8.1 fs were generated from a blue laser-diode-pumped Kerr-lens mode-locked Ti:sapphire oscillator, with an average power of 27 m W and a repetition rate of 120.6 MHz. The full width at half-maximum exceeds 146 nm, benefitting from the dispersion management by a combination of a low-dispersion fused silica prism pair and a series of double-chirped mirrors. To the best of our knowledge, this is the first time to generate sub-10-fs pulses from a laser diode directly pumped Ti:sapphire oscillator.     

12-fs pulses from a continuous-wave-pumped 200-nJ Ti:sapphire amplifier at a variable repetition rate as high as 4 MHz

We demonstrate a novel compact femtosecond Ti:sapphire laser system operating at repetition rates from 10 kHz to 4 MHz. The scheme is based on the combination of a broadband cavity-dumped oscillator and a double-pass Ti:sapphire amplifier pumped by a low-noise cw solid-state laser. Amplified pulses with an extremely smooth spectrum, a duration of only 12 fs, and less than 0.25% rms fluctuation are generated in a beam with M2 < 1.2. A maximum pulse energy of 210 nJ and an average output power of as much as 720 mW are achieved. This output energy is sufficient to generate a stable continuum in a sapphire disk.     

钛宝石飞秒激光振荡器的稳定性改善

对钛宝石飞秒激光器脉冲序列的强度和时间的稳定性进行了分析.实验比较了钛宝石飞秒激光器底板有无水冷的条件下,输出锁模脉冲序列的稳定性以及中心波长和光谱宽度的变化.结果表明对钛宝石飞秒激光器底板施加水冷可改善锁模脉冲的稳定性. 关键词： 钛宝石激光器 稳定性 飞秒脉冲     

Spectral phase interferometry for direct electric-field reconstruction of ultrashort optical pulses

We present a novel, self-referencing interferometric technique for measuring the amplitude and the phase of ultrashort optical pulses. The apparatus uses a collinear geometry that requires no moving components. The phase-retrieval procedure is noniterative and rapid and uses only two one-dimensional Fourier transforms. We apply the technique to characterize ultrashort pulses from a mode-locked Ti:sapphire oscillator.     

Piezo-driven deformable mirror for femtosecond pulse shaping

We have developed a deformable, gold-coated mirror based on piezoelectric actuators with 15-micros response time. With 20 independent channels we were able to compress 72-fs pulses from a Ti:sapphire oscillator down to 45 fs in a 4f zero-dispersion compressor arrangement. Spectral interference was used to measure the mirror performance, while the spectral phase interferometry for direct electric field reconstruction (SPIDER) technique was used for the laser pulse characterization.     

Generation of 0.4-keV femtosecond electron pulses using impulsively excited surface plasmons

We demonstrate the generation of 0.4-keV, sub-27 fs electron pulses using low-intensity laser pulses from a Ti:sapphire oscillator through the excitation of surface plasmon waves on a time scale within the plasmon lifetime. Modeling of the ponderomotive electron pulse acceleration yields electron energy spectra that are in excellent agreement with the observed ones. Our work opens a doorway for time-resolved experimentation using low-power, high-repetition rate laser pulses.     

High-power intracavity frequency doubling of a Ti:sapphire femtosecond oscillator

We demonstrate intracavity frequency doubling of a standard femtosecond Ti:sapphire oscillator. The cavity is extended with a pair of focusing mirrors and a 0.5-mm-thick BBO crystal. We achieve a repetition rate of 50 MHz and simultaneously generate 22 mW of 55-fs pulses at 810 nm and 200 mW of 73-fs pulses at 405 nm, which corresponds to 4 nJ per pulse. We create a total of 330-mW, 405-nm light when pumping the Ti:sapphire crystal with 5.7 W from an Ar-ion laser, corresponding to a conversion efficiency of 5.7%. No saturation is found, which implies that higher outputs can be achieved with higher pump rates. Preliminary results from the use of blue pulses as pump in an optical parametric amplifier seeded by pulses from a photonic crystal fiber are presented. Received: 27 January 2003 / Revised version: 27 March 2003 / Published online: 12 May 2003 RID="*" ID="*"Corresponding author. Fax: +45-861/96199, E-mail: tva@chem.au.dk