Magnetization and neutron diffraction studies on FeCrP

Crystal structure and magnetic behaviour of FeCrP have been investigated using magnetization and neutron diffraction measurements. FeCrP crystallizes in orthorhombic FeZrP type structure (P_nma space group,Z = 4) in which Cr atoms occupy the pyramidal site and Fe atoms occupy the tetrahedral site with total preference. Structural parameters including positional parameters have been refined. The refined values of positional parameters for Fe and Cr are quite different from those in FeZrP. The nature of magnetization-temperature curve is suggestive of antiferromagnetic nature withT _N = 280 (±10) K. Preliminary analysis of neutron diffraction pattern at 13 K is indicative of a rather complicated magnetic structure.     

Magnetic order in the Shastry-Sutherland model

We investigate the influence of energetic disorder, viscous damping and an external field on the electron transfer (ET) in DNA. The double helix structure of the λ-form of DNA is modeled by a steric oscillator network. In the context of the base-pair picture two different kinds of modes representing twist motions of the base pairs and H-bond distortions are coupled to the electron amplitude. Through the nonlinear interaction between the electronic and the vibrational degrees of freedom localized stationary states in the form of standing electron-vibron breathers are produced which we derive with a stationary map method. We show that in the presence of additional energetic disorder the degree of localization of such breathers is enhanced. It is demonstrated how an applied electric field initiates the long-range coherent motion of breathers along the bases of a DNA strand. These moving electron-vibron breathers, absorbing energy from the applied field, sustain energetic losses due to the viscous friction caused by the aqueous solvent as well as the impact of a moderate amount of energetic disorder. Moreover, it is illustrated that with the choice of the amplitude and frequency of the external field, the breather can be steered to a desired lattice position achieving control of the ET. Received 5 July 2002 Published online 29 November 2002     

Magnetic order in the two-dimensional compass-Heisenberg model

A Green-function theory for the dynamic spin susceptibility in the square-latticespin-1/2 antiferromagneticcompass-Heisenberg model employing a generalized mean-field approximation is presented.The theory describes magnetic long-range order (LRO) and short-range order (SRO) atarbitrary temperatures. The magnetization, Néel temperature T _N , specific heat, anduniform static spin susceptibility χ are calculated self-consistently. As the mainresult, we obtain LRO at finite temperatures in two dimensions, where the dependence ofT _N on the compass-modelinteraction is studied. We find that T _N is close to theexperimental value for Ba₂IrO₄. The effects of SRO are discussed in relation to thetemperature dependence of χ.     

Magnetic field induced order in quasi-one-dimensional systems

We investigate possible ordered phases in a magnetic field in quasi-one-dimensional conductors (Q1D$Q1D$). Long ago [I.E. Dzyaloshinskii, E.I. Kats, JETP 28 (1969) 178] we found that sufficiently strong external magnetic field leads to instability of the Fermi state with an arbitrarily weak repulsion between the particles. In the present communication we generalize this idea and provide more details to assign a physical meaning to such a state. We show that without umklapp processes the found instability corresponds to antiferromagnetic (spin density wave) order, whereas umklapp processes favor to Cooper pairing.     

Magnetic order in TbNiAl and TbCuAl intermetallic compounds

Polycrystalline samples of the ternary intermetallics TbNiAl and TbCuAl are investigated by means of magnetization and neutron diffraction measurements. When Cu replaces Ni in the crystal structure, the magnetic behaviour is shown to be totally different, although both elements are non-magnetic. Analysis of the neutron spectra by the Rietveld refinement method gives evidence that TbNiAl orders antiferromagnetically whereas TbCuAl becomes ferromagnetic. Frustrated spins at the Tb atoms are found only in the TbNiAl compound. Their alignment changes at a second magnetic transition. The magnetic structures and the transition temperatures are discussed.     

Magnetic order in TbNiAl and TbCuAl intermetallic compounds

Polycrystalline samples of the ternary intermetallics TbNiAl and TbCuAl are investigated by means of magnetization and neutron diffraction measurements. When Cu replaces Ni in the crystal structure, the magnetic behaviour is shown to be totally different, although both elements are non-magnetic. Analysis of the neutron spectra by the Rietveld refinement method gives evidence that TbNiAl orders antiferromagnetically whereas TbCuAl becomes ferromagnetic. Frustrated spins at the Tb atoms are found only in the TbNiAl compound. Their alignment changes at a second magnetic transition. The magnetic structures and the transition temperatures are discussed.     

Magnetic order in the pseudogap phase of high-Tc superconductors

One of the leading issues in high-T(c) superconductors is the origin of the pseudogap phase in underdoped cuprates. Using polarized elastic neutron diffraction, we identify a novel magnetic order in the YB(2)Cu(3)O(6+) system. The observed magnetic order preserves translational symmetry of the lattice as proposed for orbital moments in the circulating current theory of the pseudogap state. To date, it is the first direct evidence of a hidden order parameter characterizing the pseudogap phase in high-T(c) cuprates.     

Magnetic order induced birefringence and critical behaviour of the long range order parameter in NiO

The optical linear magnetic birefringence of single-domain NiO crystals was measured at temperatures above and below the antiferromagnetic phase transition. The analysis of the experimental data yield a Néel temperature of T_N = (523.7 ± 0.2)K and a critical exponent β = 0.325^+0.01_-0.02 which determines the temperature behaviour of the magnetic long range order parameter $\text{S}\text{?}\text{～ (}\text{1?T}\text{T}{}_{\mathrm{N}}\text{)}{}^{\mathrm{\beta }}$. This critical behaviour of S? is found to be continued to temperatures well below T_N.     

Magnetic order in lightly doped La2-xSrxCuO4

We study long wavelength magnetic excitations in lightly doped La2-xSrxCuO4 (x相似文献   

Magnetic order and transport in the heavy-fermion system CeCuAu

We report on extensive elastic neutron scattering to determine the wave vector of the magnetic order in CeCu_6-xAu_x single crystals for x > 0.1. For all values of x investigated (0.2, 0.3, 0.5, 1.0) we find long-range incommensurate antiferromagnetic order with an ordering vector (0.625 0.275) for x =0.2, nearly unchanged for x =0.3, and (0.59) for x =0.5, staying roughly the same for x =1.0. In addition, short-range correlations are observed for x =0.2, reminiscent of those found previously for x =0.1. The ordered magnetic moment is found to increase rapidly for small x, and more slowly for the larger x values. The increase of the specific-heat anomaly at the ordering temperature with x is in qualitative accord with this behavior. Finally, data of the electrical resistivity for current flow along the three crystallographic directions are presented, showing a clear signature of the magnetic order. A theoretical interpretation of the interplay of magnetic order and transport in terms of (i) the partial suppression of the Kondo effect by the staggered magnetization and (ii) the anisotropic band structure induced by the staggered field is shown to account well for the data, provided the ordering vector is close to 2 k F, where k F is a typical Fermi momentum. Received: 20 February 1998 / Accepted: 17 April 1998     

Magnetic order and spin dynamics in ferroelectric HoMnO3

Hexagonal HoMnO3 is a frustrated antiferromagnet (T(N)=72 K) ferroelectric (T(C)=875 K) in which these two order parameters are coupled. Our neutron measurements of the spin-wave dispersion for the S=2 Mn3+ on the layered triangular lattice are well described by a two-dimensional nearest-neighbor Heisenberg exchange J=2.44 meV, and an anisotropy D that is 0.28 meV above the spin-reorientation transition at 40 K and 0.38 meV below. For H parallel c the magnetic structures and phase diagram have been determined, and reveal additional transitions below 8 K where the ferroelectrically displaced Ho3+ ions are ordered magnetically.     

Magnetic response of mesoscopic superconducting rings with two order parameters

The magnetic response and fluxoid transitions of superconducting aluminum rings of various sizes, deposited under conditions likely to generate a layered structure, show good agreement with a two-order-parameter Ginzburg-Landau model. For intermediate couplings, we find metastable states that have different phase winding numbers around the ring in each of the two order parameters. Those states, previously theoretically predicted, are analogous to fractional vortices in singly connected samples with two-order-parameter superconductivity. Larger coupling locks the relative phase so that the two order parameters are only manifest in the temperature dependence of the response. With increasing proximitization, this signature gradually disappears.     

Magnetic order and crystal field effects in the Ce deuterides

The f.c.c. dideuterides CeD_2+x, for various D/Ce concentrations between 1.95 and 2.91, and PrD_1.95 have been investigated by susceptibility measurements between 1.4 and 400 K and by magnetization measurements up to 35T at 1.4 K. For the first time, it is shown that CeD_1.95 and PrD_1.95 order antiferromagnetically below T_N equal to 6.2 and 2.3 K, respectively. Due to the occupation of the octahedral sites for D/Ce above 1.95, the AF order in CeD_2.00 is destroyed down to 1.4 K. From the experiments the ground state of the Ce³⁺ ions is inferred to be quartet Γ₈ for all D/Ce compositions between 1.95 and 2.91. This agrees with the electronic band structure calculations by various authors, from which the tetrahedral hydrogen is concluded to be negative, whereas the octahedral hydrogen is found to be neutral.