Application of a phase conjugate Brillouin cavity for the generation of a train of short laser pulses

Summary An oscillator and a regenerative amplifier have been realized using a phase conjugate mirror in the amplifier laser cavity. The phase conjugate mirror, via stimulated Brillouin scattering, acts as a modulator owing to its time-depending reflectivity. A pulse-forming network applied to the amplifier increases the discharging time which contributes to get an output beam formed by a train having four short pulses. The shortest pulse was 2 ns FWHM long.     

Phase Conjugation with Picosecond Pulses in BaTi03

The self-pumped phase conjugate signal of picosecond laser pulses is observed. The width of the incident laser pulses is about 1.5 ps and their repetition rate is 82 MHz. The wavelength of the pulses can be tuned in the range from 710 nm to 850 nm. The pulse character of the conjugate signal is determined by an autocorrelator. The quality of the conjugate pulses is found to be good by the well-known phase distorter method.     

Pulse synthesis in the single-cycle regime from independent mode-locked lasers using attosecond-precision feedback

We report the synthesis of a nearly single-cycle (3.7?fs), ultrafast optical pulse train at 78?MHz from the coherent combination of a passively mode-locked Ti:sapphire laser (6?fs pulses) and a fiber supercontinuum (1-1.4?μm, with 8?fs pulses). The coherent combination is achieved via orthogonal, attosecond-precision synchronization of both pulse envelope timing and carrier envelope phase using balanced optical cross-correlation and balanced homodyne detection, respectively. The resulting pulse envelope, which is only 1.1 optical cycles in duration, is retrieved with two-dimensional spectral shearing interferometry (2DSI). To our knowledge, this work represents the first stable synthesis of few-cycle pulses from independent laser sources.     

Characterisation of a train of subpicosecond laser pulses by fringe resolved autocorrelation measurements

Fringe resolved autocorrelation functions generated by a train of subpicosecond laser pulses from a synchronously pumped ring dye laser were recorded. By comparison with calculated correlation functions one can not only derive the pulse duration of the center pulse, but also draw conclusions about the quasicontinuous background or satellite pulses of lower intensity.     

High-energy long-pulse Nd:YAG picosecond laser

A long train of actively mode-locked pulses is obtained from a negative feedback controlled Nd:YAG laser. The 70s pulse train contains up to 0.1 J energy and the duration of the picosecond pulses is 120 ps. The laser is operated at a repetition rate of 20 Hz. ActiveQ-control of the cavity generates a short pulse train of duration 50 to 70 ns. An excellent peak-to-background intensity ratio of the correlation function for the picosecond pulses in the train of 5×10³ is reported.     

Interferometric autocorrelation of an attosecond pulse train in the single-cycle regime

We report on the direct observation of the phase locking of the attosecond pulse train (APT) via interferometric autocorrelation in the extreme ultraviolet region. APT is formed with Fourier synthesis of high-order harmonic fields of a femtosecond laser pulse. Time-of-flight mass spectra of N+, resulting from the Coulomb explosion of N2 absorbing two photons of APT, efficiently yield correlated signals of APT. The measured autocorrelation trace exhibits that the duration of the pulse should be only 1.3 periods of the extreme ultraviolet carrier frequency. A few interference fringes within the short pulse duration clearly show two types of symmetry, which ensure the phase locking between pulses in APT.     

Generation of chirp-free picosecond pulses

The frequency spectrum of moderately chirped laser pulses depends upon the portion of the beam which is accepted by the spectrometer. Observation of the development of the chirp in a mode-locked pulse train allows to determine the small incipient chirp of early pulses. A product, bandwidth times pulse duration, of 0.47 ± 0.03 is consistently observed for single pulses switched from a passively mode-locked Nd-glass system.     

Carrier envelope phase noise in stabilized amplifier systems

At present most laser systems for generating phase-stabilized high-energy pulses are chirped pulse amplifier systems that involve the selection and subsequent amplification of pulses from a phase-stabilized seed oscillator. We investigate the effect of the picking process on the carrier envelope phase stability and how the phase noise of the picked pulse sequence can be estimated from the phase noise properties of the seed oscillator. All noise components from the original pulse train above the picking frequency are aliased into the picked pulse train and therefore cannot be neglected.     

Simple technique for generating trains of ultrashort pulses

A simple method for generating trains of high-contrast femtosecond pulses is proposed and demonstrated: a linearly polarized, frequency-chirped laser pulse is passed through a multiple-order wave plate and a linear polarizer. It is shown theoretically that this arrangement forms a train of laser pulses, and in experiments the production of a train of approximately 100 pulses, each of 200 fs duration, is demonstrated. In combination with an acousto-optic programmable dispersive filter this technique could be used to generate and control pulse trains with chirped spacing. Pulse trains of this type have widespread applications in ultrafast optics.     

Experimental Study of Double XeCl Laser with a Phase-conjugate Stimulated Scattering Cavity

SupportedbytheNationalNatureScienceFoundationofChina.1.Intr0ducti0nExcimcrlasersareonekindofthemostefficientsourcesofUVcoherentlight.Theyareusedinmanyficldssuchasn2atcrialpr0ccssing[lJ,photolitography['J,laserfusion[3Jetal..Inmany0ftheseapplicationstheshort-x`,avelcngthexcimerlaserswith1aserbeamsofhighqua1ityarenecessary.Mostoftheexci113crlasersi1regcncra11yfedbydischargecircuitswhichpumpthegasvol-umebutcausedischargeinstabiliticsinthedischargevolume['1j.Thislastphenomenonisduetothepresen…     

Multi-terawatt laser system generating 12-fs pulses at 100 Hz repetition rate

We have developed a laser system generating high peak-power ultrashort pulses based on the chirped pulse amplification of a Ti:sapphire laser. The pulse duration of the laser is reduced to 12 fs, owing to the successful compensation of gain narrowing during amplification with novel optics. The pulse energy and the repetition rate are 40 mJ and 100 Hz, respectively, as a consequence of sufficient energy extraction from a laser medium in the final stage of a multipass amplifier chain, which is designed to balance focusing with a thermal lens against defocusing with convex mirrors without cryogenic cooling for Ti:sapphire crystals. The laser pulses delivered from this laser system are suitable for generating an intense attosecond pulse train in a vacuum ultraviolet or extreme ultraviolet region.     

高次谐波产生阿秒极紫外和X光脉冲研究新进展

 近年来在可见光谱范围内已经把激光脉冲压缩到接近一个光学周期(2～3 fs)的物理极限,几fs的时间分辨精度可以描述分子化学反应过程,但是要探测远小于可见光周期的电子跃迁过程则需要阿秒(as)量级的光脉冲。利用脉冲间具有相同载波包络相位的阿秒脉冲序列能把可见光波段的光学频率梳向极紫外波段扩展;利用电子和离子碰撞复合过程短于一个光周期这个时间窗,通过测量激光场椭圆极化率对电子轨迹的微扰实现了as精度的分辨率;通过测量碰撞复合过程中的高能电子的辐射谱可以重构阿秒X光脉冲以及探测强场下束缚态和连续态电子动力学。     

Angular distributions of CH3I fragment ions under the irradiation of single pulse and trains of ultrashort laser pulses

The angular distribution of CH₃I is investigated experimentally using a single Fourier transform-limited laser pulse and a pulse train, where a 90-fs 800-nm linearly polarized laser field with a moderate intensity of 2.8×10¹³ W/cm² is used. The dynamic alignment is demonstrated in a single pulse experiment. Moreover, a pulse train is used to optimize the molecular alignment, and the alignment degree is almost identical to that with the single pulse. The results are analysed by using chirped femtosecond laser pulses, and it demonstrates that the structure of pulse train rather than its effective duration is crucial to the molecular alignment.     

Noise amplification during supercontinuum generation in microstructure fiber

Supercontinua generated by femtosecond pulses launched in microstructure fiber can exhibit significant low-frequency (<1-MHz) amplitude noise on the output pulse train. We show that this low-frequency noise is an amplified version of the amplitude noise that is already present on the input laser pulse train. Through both experimental measurements and numerical simulations, we quantify the noise amplification factor and its dependence on the supercontinuum wavelength and on the energy and duration of the input pulse. Interestingly, the dependence differs significantly from that of the broadband white-noise component, which arises from amplification of the input laser shot noise.     

Simple electro-optic technique to generate temporally flat-top laser pulses

A simple technique is presented to generate temporally flat-top shaped laser pulses using electro-optic modulator (Pockels cell). It involves splitting of input laser pulse into two halves of equal intensity and then stacking together with appropriate optical delay to get a temporally flat-top laser pulse. It also allows generation of other pulse shapes by varying the relative intensity, delay, and phase between two halves of the input laser pulse. Temporally flat-top laser pulses of duration ~ 9 ns have been generated using ~ 7 ns duration incident laser pulses from a flash lamp pumped Q-switched Nd:glass laser oscillator. The rise and fall-time of the shaped pulse is limited by speed of electro-optic switch (Pockels cell), which is ~ 2 ns in the present case.     

周期量级激光脉冲作用下原子电离不对称性研究

应用不对称性参量对周期量级强激光脉冲下原子电离分布的反演不对称性进行了定量分析.采用非微扰的散射理论解析方法和三个激光模式模拟超短脉冲,研究不对称性参量随激光强度、包络位相和脉冲宽度的变化.计算表明,这种不对称性是随着波包的绝对位相以正弦形式变化而变化,其最大不对称程度依赖于脉冲强度和脉冲宽度.随着激光强度的提高,不对称性参量是先降低到最小值然后增加.对脉冲宽度相对长、有几个周期量级的高强度激光,其不对称性具有显著的特点.因此,提高脉冲强度有助于对包络绝对位相变化的观察.     

Mode-locked fiber laser with a manganese-doped cadmium selenide saturable absorber

We demonstrate the generation of mode-locked pulses in an erbium-doped fiber laser(EDFL) by using a new manganese-doped cadmium selenide quantum-dots-based saturable absorber. The laser produces a soliton pulse train operating at 1561.1 nm with a repetition rate of 1 MHz, as the pump power is varied from 113 to 250 m W.At the maximum pump power, we obtain the pulse duration of 459 ns with a signal-to-noise ratio of 50 dB.     

Design and construction of Q-switched Nd:YAG laser system for LIBS measurements

A passive, Q-switched pulsed, Nd:YAG laser system was designed and built, which can provide a potential compact robust laser source for portable laser induced breakdown spectroscopy systems.The developed laser system operates at 1064 nm. Each laser shot contains a train of pulses having maximum total output energy of 170 mJ. The number of pulses varies from 1–6 pulses in each laser shot depending on the pump energy. The pulse width of each pulse ranges from 20 to 30 ns. The total duration of the output pulse train is within 300 μs. The multi-pulse nature of the laser shots was employed to enhance the LIBS signal. To validate the system, LIBS measurements and analysis were performed on ancient ceramic samples collected from Al-Fustat excavation in Old Cairo. The samples belong to different Islamic periods in Egypt history. The results obtained are highly indicative that useful information can be provided to archeologists for use in restoring and repairing of precious archeological objects.     

三色圆偏振激光组合脉冲驱动氦原子产生椭圆偏振的阿秒脉冲

我们提出利用频率为ω,3ω和强度较弱的2ω组成的三色圆偏振激光组合脉冲驱动氦原子能够得到椭偏率较大的阿秒脉冲链的一种方法.通过强场近似方法,计算了氦原子在两色和三色圆偏振激光组合脉冲驱动下发射高次谐波谱及其合成阿秒脉冲链,比较了氦原子(初态为s态)在这两种情况下发射高次谐波谱的特点及其合成阿秒脉冲链椭偏率的大小,结果发现,在反旋的两色ω,3ω激光脉冲基础上加入了频率为2ω的第三色激光脉冲联合作用到氦原子上,所得到的阿秒脉冲链的椭偏率相对于双圆场情况下有所增加,通过调整ω,3ω激光的强度比,并且选择适当的第三色激光的强度,对初态为s态的原子,仍能够得到具有较大椭偏率的阿秒脉冲链.     

Dual-wavelength synchronously mode-locked Nd:CNGG laser

We have experimentally demonstrated a dual-wavelength synchronously mode-locked Nd:CNGG laser based on the semiconductor saturable absorber mirror technique. Mode locking was achieved simultaneously on two gain bands of the crystal that have a central wavelength separation of 2.4 nm. The fundamental mode-locked pulse train has a repetition rate of 88 MHz and pulse duration of 5 ps, with an average output power of approximately 90 mW. Autocorrelation measurements show that each of the synchronously mode-locked pulses consists of a train of quasi-periodic beat pulses with a 660 fs pulse width and a 0.63 THz repetition rate.