Tunable frequency-controlled laser source in the near ultraviolet based on doubling of a semiconductor diode laser

Continuously tunable ultraviolet laser radiation at 397 nm was generated by doubling the output of a semiconductor diode laser. The fundamental radiation was provided by a 150 mW AlGaAs laser diode injected by a low-power AlGaAs laser diode which was frequency stabilized by optical feedback using a new scheme of a miniature external cavity. Second-harmonic generation was produced in a lithium-triborate crystal placed in a compact enhancement cavity. The fundamental radiation was used for sub-Doppler spectroscopy of the Ar I 4s ³ P ⁰ ₀–4p ¹ P ₁ transition at 795 nm; the second-harmonic radiation was used for spectroscopy of the Ca II 4² S _1/2–4² P _1/2 transition at 397 nm.     

Submicron External Electro-optic Measuring System Based on an Electro-optic Solid Immersion Lens

In this paper, all electro-optic solid immersion lens (EOSIL) is introduced, which is made of GaAs. A reflecting external electro-optic measuring system based on the EOSIL is built. With a hemispherical GaAs EOSIL used as the external probe, 0.7 µm spot size is obtained when the wavelength of the probing beam from a laser diode is 1.3 µm and a microscope objective with 0.3 numerical aperture is used. The principle of the measuring system is analyzed by Jones matrix. By using the system, the electrical signals propagating on a microstrip transmission line are successfully measured. The voltage sensitivity about 5 mV/ is measured when 10 kHz sinusoidal electric signal is applied on the microstrip line.     

A tunable light source in the 370 nm range based on an optically stabilized,frequency-doubled semiconductor laser

A tunable harmonic output power of 18 W at a wavelength of =370 nm is obtained by resonance-enhanced frequency doubling of an optically-stabilized semiconductor laser. A commercially available AlGaAs laser diode which emits a maximum power of 10 mW at =740 nm is operated in an extended-cavity configuration. Dispersion prisms are used in the extended cavity to obtain longitudinal-mode selection with low loss of optical power. The output is focussed into an optically isolated high-finesse ring resonator which contains a LiIO₃ crystal for second-harmonic generation. One potential application of this laser source is the optical excitation and laser cooling of ytterbium in an ion trap. In a related demonstration experiment, the frequency-doubled diode laser is applied to excite the =369.5 nm ² S _1/2-² P _1/2 transition of ytterbium ions in a hollow-cathode discharge.     

High-resolution diode-laser spectroscopy on a fast beam of metastable atoms for detecting very rare krypton isotopes

A fast krypton ion beam with an energy of 10 keV is transferred through a mass filter and neutralized in a Rb- (or Cs-) vapour charge exchange cell. The emerging beam of metastable Kr atoms of a selected Kr isotope is collinearly irradiated with a tunable cw GaAlAs diode laser at 811 nm. The spectrum of the 1s ₅–2p ₉ transition covers 10 GHz and consists of one line each for the five stable isotopes of Kr with even mass number and 15 hyperfine structure lines of⁸³Kr. The individual lines are recorded by detecting the fluorescence signal perpendicular to the beams. Photons are guided to the PM tube by diffuse reflection from a high reflectance thermoplastics light collector. Up to 20 photons per atom are emitted by cycling between the two states during the flight time of 1.2 µs through the detector. The observed absorption linewidth of 100 MHz is a combination of laser linewidth and energy uncertainty in the fast atomic beam. In order to achieve maximum isotope selectivity the beam energy has to be adjusted in such a way that the Doppler shifted lines of all isotopes form an optimum pattern for detecting the very rare isotopes⁸¹Kr and⁸⁵Kr in natural environmental samples.     

Actively mode-locked 1.3 and 1.55 μm InGaAsP diode lasers

Active mode-locking of uncoated InGaAsP diode lasers having an external diffraction grating cavity was investigated experimentally. A high frequency r.f. signal and short-duration electrical pulses were used to drive the lasers. The pulse duration was measured by an ultrafast streak camera. Pulses as short as 13 ps at 1.3m and 29 ps at 1.55m were generated at a repetition rate of 1 GHz. The reason for obtaining broader pulses from the 1.55m laser which had the same structure as the 1.3m diode laser is explained.Formerly with GEC Hirst Research Centre, Wembley, Middlesex, UK.     

Integrated nanostrip dipole antennas for coherent 30 THz infrared radiation

We report on the experimental study of infrared nanostrip dipole antennas which are connected to thin-film nanometer Ni-NiO-Ni diodes. The integrated Ni-NiO-Ni diodes are used to detect 30 THz (10 µm) CO₂-laser radiation.The diodes are deposited on 385 µm silicon substrates which are covered with a layer of 1.6 µm SiO₂ on both sides. We have found that in low-power applications 1.6 µm of SiO₂ yields excellent quarter-wave matching layers for wavelengths centered at ₀ = 10.8 µm. By this method 79% of the incident CO₂-laser radiation is transmitted into the Si substrate compared to 48% without SiO₂ layer. The use of SiO₂ quarter-wave matching layers considerably improves the efficiency of infrared nanostrip dipole antennas. This has been confirmed by the study of the laser-induced response of the Ni-NiO-Ni diode detectors as a function of the lengthL of the dipole antenna. Thus, we have observed that the laser-induced response strongly increases for shorter antennas and exhibits a distinct maximum atL=2.8 ± 0.3 µm. For the first time, we have investigated the 30 THz radiation patterns of nanostrip dipole antennas of different lengths. On this occasion, we have observed that the radiation pattern changes when the lengthL of the dipole antenna is varied. This observation indicates that antenna currents propagate on the nanostrip dipole antenna.     

Similarity of plasma conditions of some Ne-like X-ray lasers and their partner Ni-like X-ray lasers

New pump and signal laser sources for difference frequency generation (DFG) at 4 m are described. A laser diode with a 980 nm fiber Bragg grating and a 785 nm Fabry-Perot (FP) laser diode were coupled into an optical fiber and mixed in a periodically poled Mg-doped lithium niobate (PPMgLN ) crystal, resulting in efficient mid-IR DFG. The DFG power was measured to be 0.23 W for a pump power of 5 mW and a signal power of 50 mW with a slope efficiency of 0.92 mW/W². A Doppler-broadened absorption spectrum of N₂O at 2485.2 cm^-1 (3.927 m) was observed in a 0.1 m-long gas cell at a pressure of 133 Pa. The spectral linewidth of the DFG source was estimated to be 161 MHz (FWHM) for an averaging time of 700 ms. Real-time monitoring of N₂O in a multipass cell with an optical path length of 36 m at a concentration level of 1 ppm was demonstrated. PACS 42.62.Fi; 42.72.Ai; 07.57.Hm     

Laser damage in silicon photodiodes

Thermal damage of silicon photodiodes exposed to intense optical radiation is investigated. Damage thresholds of Si photodiodes irradiated by 1.06m laser pulses are reported for values of irradiation time,, ranging from 10^–8 to 1s. Threshold laser irradiation produces visible microscopic damage and a permanent degradation in photoresponse. The loss of responsivity is associated with degradation of the detector diode characteristics due to laser-induced heating. The time and wavelength dependence agree with the predictions of a thermal model which treats a semi-infinite material irradiated by a Gaussian laser beam. The energy density thresholds are independent of for short irradiation times and asymptotically approach a limiting behaviour which increases as for long times. They are given by the empirical relationE ₀=65[1+217/tan^–1(258)^1/2] J cm^–2 for 1.06m radiation. The thresholds at short irradiation times of detectors damaged by 1.06m radiation are about 25 times larger than those of detectors exposed to 0.6943m radiation. The greater susceptibility at 0.6943m is attributed to a larger optical absorption coefficient.     

External short-cavity diode-laser for MIR difference-frequency generation

A compact mid-infrared (MIR) laser system is described applying two single mode diode-lasers as pump and signal sources to generate difference-frequency radiation in AgGaS₂. A spectral tuning range of 71.5 cm^-1 between 4.9–5.1 m with an output power of 100 nW and linewidth of 1.2×10^-2 cm^-1 (3.6 GHz) for the DFG laser system is obtained by mode behavior improvement of the pump source using an external short-cavity. The performance of such an external short-cavity MIR-DFG laser spectrometer is demonstrated by recording the fundamental absorption spectra of carbon monoxide (¹²C¹⁶O) and nitric oxide (¹⁴N¹⁶O) in a 10 cm long cell in order to estimate line-broadening coefficients of CO and NO molecules, which are of general interest in combustion diagnostics . PACS 32.20.-t; 33.20.Ea; 42.60-v; 42.60.Fc; 42.62.-b; 42.62.Fi; 42.68.-w; 42.68.Ca; 42.72.-g; 42.72.Ai     

CO-laser side-band spectrometer: Sub-Doppler heterodyne frequency measurements around 5 µm

We report the realization of a tunable sub-Doppler heterodyne spectrometer with high absolute accuracy, employing side-band generation with a CO laser. The fixed-frequency CO-gas laser, working from 4.7 to 8.4µm, is made partially tunable by the use of microwave side-band generation in a CdTe Electro-Optical Modulator (EOM). This leads to tunable radiation of high spectral purity. We describe the design of the microwave EOM, adapted to the CO laser, its performance and its first application to highly accurate frequency measurements. The side-band radiation is used for sub-Doppler stabilization of the CO laser, while the carrier frequency is mixed with the frequencies of two CO₂ reference lasers. As a first result, we present measurements of OCS transitions in the 4.9µm (61 THz) region, reaching an absolute accuracy of 30 kHz (/ = 5×1O^–10). Further application of our spectrometer to calibration gases will establish a variety of InfraRed (IR) calibration standards with a new quality of accuracy. On visit from: Fachbereich Physik, Humboldt-Universität zu Berlin     

Tunable CW laser oscillation of NdP5O14 at 1.3 μm

Low-threshold tunable cw laser oscillation is achieved at the⁴ F _3/2⁴ I _13/2 transition of NdP₅O₁₄. Continuous tunign over 1.8% of the central wavelenght is possible with 55 mW of absorbed pump power. At gain line maximum near 1.32 , the output power exceeded 1 mW. Pump threshold as low as 8 mW was observed. Reliable cw operation of the 1.3 m NdP₅O₁₄ laser pumped by a 15 mW AlGaAs laser diode is demonstrated.     

Dynamics of the CO2 lower laser levels as measured with a tunable diode laser

A tunable diode laser operating in the 4.3 m region is used to probe a conventional cw CO₂ laser discharge. Vibrational populations in the 10⁰0, 02⁰0, 02²0, and 01¹0 levels of CO₂ are measured under lasing conditions, i.e., in the presence of intense 10.4 and 9.4 m fields. The tunable diode laser is also used to monitor the energy transfer processes between the four levels after the passage of an intense 10.4 m pulse. The detailed information provided by the tunable probe laser enables us to determineseparately all the vibration-vibration (V-V) and vibration-translation (V-T) rate constants of importance in the relaxation of the lower laser levels in CO₂. The V-V rate constants are found to vary from a low value of 4.5×10⁴ s^–1 Torr^–1 for the coupling of 01¹0 to 10⁰0 to a high value of 8.0×10⁵ s^–1 Torr^–1 for the coupling of 01¹0 to 02²0.This work was supported by the National Science and Engineering Research Council of Canada and the Provincial Government of Ontario     

The CO fundamental-band laser as secondary frequency standard at 5 µm

We present a very high-resolution heterodyne spectrometer based on a CO laser which operates down to fundamental-band transitions of the molecule. This allows us to detect saturated absorption signals on these transitions at very low pressure (0.4 Pa) and laser intensity (< 1 mW/cm²), yielding a linewidth of about 250 kHz. With the CO fundamental-band laser stabilized to these saturation signals we have measured the transition frequencies of the fundamental bands of three isotopic species to an accuracy of typically 20 kHz (v/v 3 × 10^–10), referenced to the CO₂ frequency standard. Together with additional frequency measurements of the first hot bands, these provide the first heterodyne frequency data of sub-Doppler accuracy for transitions in low lying bands of CO. They now represent the most accurate secondary frequency standard in the spectral region around 5 µm (60 THz).     

Measurement of the heavy neutrino admixture upper limit from muon capture by3He

The triton energy spectrum of the muon capture reaction µ³Het+_µ where µ³He is the ground state of muonic³He, has been measured by means of a high-pressure ionization chamber in order to investigate a possible heavyv admixture into the µ flavor with high sensitivity. The upper limit of the µ-heavy v_i mixing matrix element squared was obtained to be U_µi²10^–3 for heavy neutrino masses in the range of 25 E_0V75 MeV.     

Ultrahigh-resolution saturation spectroscopy using slow molecules in an external cell

We present the narrowest molecular lines so far recorded in the 10 µm spectral region. A linewidth of 80 Hz (HWHM) has been obtained for theP(39)A ₁ ³ (–) line of OsO₄, by selecting slow molecules (T _eff=0.6 K) in saturation spectroscopy at low laser fields (30 nW) and low pressures (2 × 10^–6 Torr). In these conditions, the contribution of the fast molecules is greatly reduced because of the finite size of the beam. This method, applied previously to methane at 3.39 µm, is used for the first time in an external cell and improves by a factor 8 the best resolution of our spectrometer. Heterodyne detection and double frequency modulation have been necessary to extract a signal at a contrast of only 10^–6. The physical ideas concerning this regime are described and a detailed analysis of the line shape is given.     

Efficient multiple-longitudinally diode laser pumped Nd:YAG slab laser

The operation of an eightfold longitudinally diode laser pumped 1.06m cw Nd:YAG slab laser is demonstrated. The 809 nm diode radiation is focused through a dichroic coating into each laser channel starting from the reflection points of the 1.06m beam in the slab crystal. At an absorbed pump power in the crystal of 2830 mW a maximum cw TEM₀₀ output of 1075 mW was achieved with a corresponding slope efficiency of 42.5%.     

Efficient room-temperature operation of Cr3+-sensitized, flashlamp-pumped, 2μm lasers

Utilizing the results of Cr³⁺ Tm³⁺ transfer efficiency studies, we have demonstrated that yttrium aluminium garnet (YAG) is the preferred host for room-temperature, flashlamp-pumped solid-state lasers operating in the 2.0 µm spectral range. We report data on two different sensitizer-activator combinations in YAG and yttrium scandium gallium garnet (YSGG) laser materials: one is doped with Cr:Tm:Ho and operates on the Ho^{3+ 5}I₇ ⁵I₈ transition at 2.097 µm; the other is doped only with Cr:Tm, which lases on the Tm^{3+ 3}F₄ ³H₆ transition at 2.014 µm. We have achieved a slope efficiency of 5.1% with the Cr:Tm:Ho:YAG laser, which is the highest slope efficiency yet reported for a room-temperature, flashlamp-pumped, 2 µm solid-state laser. We have measured thresholds as low as 38 J and output energies >1.5 J for that system. We also report the first room-temperature operation of an efficient flashlamp-pumped Cr:Tm:YAG laser at 2.014 µm. Thresholds as low as 43 J, output energies exceeding 2 J, and slope efficiencies as high as 4.5% have been achieved. This is an order of magnitude higher than the efficiency previously reported for a 2.01 µm Cr:Tm:YAG laser operated at cryogenic temperatures. These two efficient 2 µm laser systems (Cr:Tm:Ho:YAG and Cr:Tm:YAG) are discussed in terms of their potential for Q-switched operation.     

Amplification of a <Emphasis Type="Italic">Q</Emphasis>-Switched Ho:GdVO<Subscript>4</Subscript> Oscillator in Thulium-Doped Large-Mode-Area Fiber

We report a high peak power, narrow linewidth, stable pulsed Ho:GdVO₄ amplifier based on thuliumdoped fiber, which produces 6.65 W average output power at 2,048 nm and 56.8 kW peak power with 11.7 ns pulse width at 10 kHz repetition rate. We use a simple Q-switched Ho:GdVO₄ laser as a seed laser and a thulium-doped fiber pumped by a 792 nm laser diode as an amplifier. The fiber amplifier provided 6.5 dB gain to the input signal. The spectral linewidth of the Ho:GdVO₄ amplifier remains < 0.5 nm with an M² beam quality of 1.36.     

Computer controlled diode laser spectrometer with a helium evaporation cryostat and spectroscopy of thev 3 vibration of NCO

A computer-controlled diode laser spectrometer for the 1200 to 2500 cm^–1 spectral region is described. The spectrometer has been applied to high resolution spectroscopy of the NCO radical at 5.2 m. The lead-salt diode lasers are cooled to their operating temperature with a temperature adjustable helium evaporation cryostat. Computer-controlled tuning procedures for the frequency tuning of the diode lasers have been developed; they are independent of tables describing the tuning characteristics of the diode lasers. 41 lines of the antisymmetric stretching-vibrationv ₃ of the linear NCO radical have been observed. We were able to detect vibration-rotation transitions in both² _1/2 and² _3/2 fine structure sublevels. These measurements led to the precise determination of additional molecular constants.     

The characteristics of multiple-photon absorption of SF6 molecules cooled in free jet expansion from a pulsed supersonic nozzle

The multiple-photon absorption of pulsed TEA CO₂ laser radiation by SF₆ molecules cooled toT _R40K andT _v160K in the free jet expansion from a pulsed supersonic nozzle has been investigated at energy fluences of 0.1 to 3.0 J·cm^–2.For practically all laser lines which coincide with the linear absorption spectrum of thev ₃ vibrational mode of SF₆ [P(12)...P(28), 10,6 m], the dependence of the absorbed energyE _ab on the exciting energy fluence was found to be steeper than linearE _abⁿ, wheren=(1.1 to 1.8). Considerable increases of the absorption cross sections with increasing energy fluence were observed.The fraction of the molecules interacting with the laser radiation is estimated.