Magnetic properties of the cyclic spincluster Fe6:bicine

The magnetic properties of the cyclic compound [Fe₆(bicine)₆] LiClO₄ ^. 2MeOH are reported. The cluster Fe₆(bicine)₆ forms an antiferromagnetically coupled ring structure of Fe ^III ions. The magnetic susceptibility is measured between 2 and 300 K and yields the exchange coupling of J/k _B = - 27.5±0.5 K. The field dependence of the magnetic moment is studied at 3 and 6 K in magnetic fields up to 5 T. The zero-field splitting of the first excited spin states with S = 2 and 3 are determined by ESR at 94 GHz. The intra-molecular interactions of the Fe ^III ions are analyzed and the on-site anisotropy of the Fe ^III due to the ligand-configuration is determined to d /k _B = - 0.633±0.008K. Received 28 October 2002 / Received in final form 22 February 2003 Published online 20 June 2003 RID="a" ID="a"e-mail: bernd@piobelix.physik.uni-karlsruhe.de     

(EC+β +) decay of 130Nd and 140Tb

The available astrophysical S(E) factor data for the reaction ⁷Li (p,α)α at 10 < E < 1000keV exhibit an exponential increase at low energies due to the effects of electron screening. A parametrisation of the data using a non-resonant, direct process and two subthreshold resonances reproduces the data at energies E≥ 100keV, while at lower energies this calculated S _b(E) factor curve for bare nuclides drops below the data, which in turn represent the case of electron-shielded nuclides, i.e. the electron-shielded S _s(E) factor. The comparison between S _b(E) and S _s(E) leads to an electron-screening potential energy U _e = 350eV, which is much higher than the adiabatic limit of 175eV and not understood at present. The deduced value of S _b(0) is considerably smaller than the previously adopted value of 59keV b, significantly increasing the calculated abundance of ⁷Li in big-bang nucleosynthesis. The Trojan-horse method was applied to the reaction ⁷Li (p,α)α to determine the energy dependence of the S _b(E) factor for 10 < E < 370keV, free from the effects of the Coulomb barrier and electron screening. The THM results are close to the calculated S _b(E) curve and suggest that the THM may become a powerful way to obtain improved information on low-energy cross-sections and associated electron-screening effects in a model-independent way. Received: 9 September 2000 / Accepted: 5 December 2000     

Evolution of the N = 20 and N = 28 shell closures in neutron-rich nuclei

The isospin dependence of shell closure phenomena is studied for light neutron-rich nuclei within a microscopic self-consistent approach using the Gogny force. Introducing configuration mixing, ³²Mg is found to be dynamically deformed, although the N = 20 spherical shell closure persists at the mean-field level for all N = 20 isotones. In contrast, the N = 28 spherical shell closure is found to disappear for N - Z≥ 10 whereas deformed shell closures are preserved and lead to shape coexistence in ⁴⁴ S. Configuration mixing shows that the ground state of this nucleus is triaxially deformed. The first 2⁺ excitation energy E_x = 1.46 MeV and the reduced transition probability B(E2;0⁺ _gs→ 2⁺ ₁)= 420 e ² fm ⁴ obtained with our approach are in good agreement with experimental data. Received: 26 July 2000 / Accepted: 30 August 2000     

Study of nucleon spin-dependent properties in the resonance region

In this paper, the spin-dependent structure functions of nucleon g ₁, and photoabsorption cross sections σ_1/2, σ_3/2 and σ_T in the resonance region are estimated based on the constituent quark model and the properties of the five phenomenological Breit-Wigner resonances P ₃₃(1232), S ₁₁(1535), D ₁₃(1520), P ₁₁(1440), and F ₁₅(1680). Our results are compared to the recent E143 data of the polarized structure functions g ₁(W ², Q ²) at points Q ²=0.5 GeV² and Q ²=1.2 GeV² and the data of the total inclusive photoabsorption cross sections. Received: 7 October 1997     

The E1 capture amplitude in 12C(α,γ0) 16O

An excitation function of the ground-state γ₀-ray capture transition in ¹²C (α,γ)¹⁶O at θ_γ = 90^° was obtained in far geometry using six Ge detectors, where the study of the reaction was initiated in inverse kinematics involving a windowless gas target. The detectors observed predominantly the E1 capture amplitude. The data at E = 1.32 to 2.99 MeV lead to an extrapolated astrophysical S factor S _E1(E ₀) = 90±15 keV b at E ₀ = 0.3 MeV (for the case of constructive interference between the two lowest E1 sources), in good agreement with previous works. However, a novel Monte Carlo approach in the data extrapolation reveals systematic differences between the various data sets such that a combined analysis of all available data sets could produce a biased estimate of the S _E1(E ₀) value. As a consequence, the case of destructive interference between the two lowest E1 sources with S _E1(E ₀) = 8±3 keV b cannot be ruled out rigorously. Received: 6 June 2001 / Accepted: 26 July 2001     

The local potential approximation for the Brueckner G-matrix and a simple model of the scalar-isoscalar Landau-Migdal amplitude

The Brueckner G-matrix for a slab of nuclear matter is analyzed in the singlet ^1S and triplet ³ S + ³ D channels. The complete Hilbert space is split into two domains, the model subspace S₀, in which the two-particle propagator is calculated explicitly, and the complementary one, S', in which the local potential approximation is used. This kind of local approximation was previously found to be quite accurate for the ^1S pairing problem. A set of model spaces S ₀(E ₀) with different values of the energy E₀ is considered, E₀ being the upper limit for the single-particle energies of the states belonging to S₀. The independence of the G-matrix on E₀ is assumed as a criterion for the validity of the local potential approximation. It turns out that such an independence holds within few percents for E ₀ = 10-20 MeV, for both channels under consideration. The G-matrix within the local potential approximation is used for justifying a simple microscopic model for the coordinate-dependent scalar-isoscalar component f (r) of the Landau-Migdal amplitude in terms of the free T-matrix. Received: 2 November 2001 / Accepted: 4 January 2002     

Coulomb breakup of 8B and the flux of 8B neutrinos from the Sun

A kinematically complete measurement was made of the Coulomb dissociation of ⁸B nuclei on a Pb target at 83 MeV/nucleon. The cross-section was measured at low relative energies in order to infer the astrophysical S-factor for the ⁷Be(p,γ)⁸B reaction. A first-order perturbation theory analysis of the reaction dynamics including E1, E2, and M1 transitions was employed to extract the E1 strength relevant to neutrino-producing reactions in the solar interior. By fitting the measured cross-section from E _rel = 130 keV to 400 keV, we find S ₁₇(0) = 17.8^+1.4 _-1.2 eV b. Semiclassical 1st-order perturbation theory and fully quantum-mechanical continuum-discretized coupled-channels analyses yield nearly identical results for the E1 strength relevant to solar-neutrino flux calculations, suggesting that theoretical reaction mechanism uncertainties need not limit the precision of Coulomb-breakup determinations of the ⁷Be(p,γ)⁸B S-factor. A recommended value of S ₁₇(0) based on a weighted average of this and other measurements is presented. This recommendation implies a revised value for the theoretical flux of ⁸B solar neutrinos, which is also given.-1 Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"Present address: Kernfysisch Versneller Instituut, Zernikelaan 25, 9747 AA Groningen, The Netherlands; e-mail: davids@kvi.nl     

Determination of the chemical potential and the energy of the ν=1/2 FQHE system for low temperatures

We consider the energy density of a spin polarized ν = 1/2 system for low temperatures. We show that due to the elimination of the magnetic field and the field of the positive background charge in the calculation of the grand canonical potential of Chern-Simons systems through a mean field formalism one gets corrections to the well known equations which determine the chemical potential and the energy from the grand canonical potential. We use these corrected equations to calculate the chemical potential and the energy of the ν = 1/2 system at low temperatures in two different approximations. Received 14 March 2001     

High resolution photoemission spectroscopy study near the Fermi edge for different surfaces prepared on the icosahedral AlPdMn phase

High resolution photoemission measurements performed at low temperatures on a single-grained sample of the AlPdMn icosahedral phase show that the density of states N(E) strongly depends on the nature of the surface. For an ordered quasicrystalline surface, prepared by Ar etching and ultra high vacuum annealing, a dip feature is observed in N(E) near the Fermi level, which energy dependence can be analyzed with a simple square-root power law. By contrast, N(E) varies only little with energy both for a disordered surface and a crystalline surface of the same sample. A sharp Fermi edge is then clearly observed. This shows that the metallic character of the surface of a quasicrystal is strongly reduced when the surface presents a quasicrystalline ordering. Received 19 February 2000 and Received in final form 6 November 2000     

T-band phenomena in 183Re

Abstact: High-spin states in ¹⁸³Re have been studied using the ¹⁷⁶Yb(¹¹B,4n) reaction at 52 and 57 MeV. Two high-K bands have been observed directly by a time-correlated γ-γ coincidence measurement. One of the bands is built on an isomeric K ^π=(25/2)⁺ state at E _x= 1908 keV with a half-life of 0.82(2) ms. The other band, assigned as K ^π=(29/2)⁻ at E _x= 2739 keV, decays to the (25/2)⁺ band. These bands are interpreted as three-quasiparticle structures, π(5/2)⁺[402] &⊗ν(9/2)⁺[624] ⊗ν(11/2)⁺[615] for the (25/2)⁺ band and π(9/2)⁻[514] ⊗ν(9/2)⁺[624] ⊗ν(11/2)⁺[615] for the (29/2)⁻ band. The K ^π= (29/2)⁻ band becomes strongly Coriolis mixed with increasing spin and is gradually changing into a low-K s-band structure. Received: 20 April 1998     

Effective nonlinear optical properties of shape distributed composite media

The effective linear and nonlinear optical properties of metal/dielectric composite media, in which ellipsoidal metal inclusions are distributed in shape, are investigated. The shape distribution function P(L _x, L _y) is assumed to be 2Δ^-2θ(L _x - 1/3 + Δ/3)θ(L _y - 1/3 + Δ/3)θ(2/3 + Δ/3 - L _x - L _y), where θ( ^{. . .} ) is the Heaviside function, Δ is the shape variance and L_i are the depolarization factors of the ellipsoidal inclusions along i-symmetric axes (i = x, y). Within the spectral representation, we adopt Maxwell-Garnett type approximation to study the effect of shape variance Δ on the effective nonlinear optical properties. Numerical results show that both the effective linear optical absorption α ∼ ωIm() and the modulus of the effective third-order optical nonlinearity enhancement |χ⁽³⁾ _e|/χ⁽³⁾ ₁ exhibit the nonmonotonic behavior with Δ. Moreover, with increasing Δ, the optical absorption and the nonlinearity enhancement bands become broad, accompanied with the decrease of their peaks. The adjustment of Δ from 0 to 1 allows us to examine the crossover behavior from no separation to large separation between optical absorption and nonlinearity enhancement peaks. As Δ → 0, i.e., the ellipsoidal shape deviates slightly from the spherical one, the dependence of |χ⁽³⁾ _e|/χ⁽³⁾ ₁ on Δ becomes strong first and then weak with increasing the imaginary part of inclusions' dielectric constant. In the dilute limit, the exact formula for the effective optical nonlinearity is derived, and the present approximation characterizes the exact results better than old mean field one does. Received 10 December 2002 Published online 4 June 2003 RID="a" ID="a"e-mail: lgaophys@pub.sz.jsinfo.net     

Nuclear spins, magnetic moments and α-decay spectroscopy of long-lived isomeric states in 185Pb

Alpha-decay properties of the neutron-deficient isotope ¹⁸⁵Pb were studied at the PSB-ISOLDE (CERN) on-line mass separator using the resonance ionisation laser ion source (RILIS). The nuclei of interest were produced in a 1.4 GeV proton-induced spallation reaction of a uranium graphite target. In contrast to previous studies, two α-decaying isomeric states were identified in ¹⁸⁵Pb. The relative production of the isomers, monitored by their α-counting rates, could be significantly changed when a narrow-bandwidth laser at the RILIS setup was used to scan through the atomic hyperfine structure. Based on the atomic hyperfine structure measurements, along with the systematics for heavier odd-mass lead isotopes, the spin and the parity of these states were interpreted as 3/2^- and 13/2⁺ and their nuclear magnetic moments were deduced. The α-decay energy and half-life value for the I ^π = 13/2⁺ isomer are E _α = 6408(5) keV, T _1/2 = 4.3(2) s, respectively; while for the I ^π = 3/2^- isomer ( T _1/2 = 6.3(4) s) two α-decays with E _α1 = 6288(5) keV, I _α1 = 56(2)% and E _α2 = 6486(5) keV, I _α2 = 44(2)% were observed. By observing prompt α-γ coincidences new information on the low-lying states in the daughter isotope ¹⁸¹Hg was obtained. Received: 7 February 2002 / Accepted: 19 February 2002     

High-spin isomers in 183Os

High-spin states in ¹⁸³Os have been studied by means of in-beam γ-ray spectroscopy. Two isomers with I ^π= ((43/2)⁻) and (43/2)⁺ have been identified at excitation energies of E _x = 5.068 and 5.168 MeV. The half-lives are determined as T _1/2= 27 ± 3 and 24 ± 2 ns. Received: 22 December 1997     

Magnetic reconstructions at the surface of the B2 FeV alloy

We present an ab initio study of the magnetic surface reconstructions of the B2 FeV alloy using a self-consistent tight-binding linearized muffin tin orbital method developed in the atomic spheres approximation. For (001) and (111), the surface reconstruction stabilizes configurations unstable in the bulk alloy. When Fe is at the (001) surface, a c(2×2) in-plane antiferromagnetic order is found to be the ground state with magnetic moments of -2.32 and 2.27. A p(1×1) ↓ ferromagnetic order is displayed in case of V toplayer with a magnetic moment of -1.83. At the (111) surface, we obtain for Fe toplayer two solutions p(1×1)↑ and p(2×1). The configuration p(1×1)↑ is found to be the ground state with a magnetic moment per atom of 2.34. For V toplayer, only the p(1×1) ↓ solution is obtained with a moment of -0.84. In all cases, the Fe-V coupling is always antiparallel like in the bulk. Our results are discussed and compared to experiments. Received 11 August 2000 and Received in final form 8 June 2001     

Quark model study of the η photo-production:

An extensive and systematic study of the recent η photo-production data up to 1.2 GeV is presented within a chiral constituent quark model. A model embodying all known nucleonic resonances shows clear need for a yet undiscovered third S₁₁ resonance in the second resonance region, for which we determine the mass (1.729 GeV) and the total width (183 MeV). Furthermore, we extract the configuration mixing angles, an important property of the quark-quark interaction in the quark model, for the resonances S ₁₁(1535) and S ₁₁(1650), as well as for the resonances D ₁₃(1520) and D ₁₃(1700). Our results agree well with the quark model predictions. In addition, the partial ηN decay widths and/or the photo-excitation helicity amplitudes for the nucleonic resonances S ₁₁(1535), S ₁₁(1650), P ₁₁(1710), P ₁₃(1720), D ₁₃(1520), D ₁₃(1700), D ₁₅(1675), and F ₁₅(1680) are also obtained in this approach. Received: 14 February 2001 / Accepted: 22 June 2001     

Ground-state properties of LiV2O4 and Li1-xZnx(V1-yTiy)2O4

We present susceptibility, microwave resistivity, NMR and heat-capacity results for Li_1-xZn_x(V_1-yTi_y)₂O₄ with 0 ? x ? 0.3 and 0 ? y ? 0.3. For all doping levels the susceptibility curves can be fitted with a Curie-Weiss law. The paramagnetic Curie-Weiss temperatures remain negative with an average value close to that of the pure compound Θ≈ - 36 K. Spin-glass anomalies are observed in the susceptibility, heat-capacity and NMR measurements for both type of dopants. From the temperature dependence of the spin-lattice relaxation rate we found critical-dynamic behavior in the Zn doped compounds at the freezing temperatures. For the Ti-doped samples two successive freezing transitions into disordered low-temperature states can be detected. The temperature dependence of the heat capacity for Zn-doped compounds does not resemble that of canonical spin glasses and only a small fraction of the total vanadium entropy is frozen at the spin-glass transitions. For pure LiV₂O₄ the spin-glass transition is completely suppressed. The temperature dependence of the heat capacity for LiV₂O₄ can be described using a nuclear Schottky contribution and the non-Fermi liquid model, appropriate for a system close to a spin-glass quantum critical point. Finally an ( x / y , T )-phase diagram for the low-doping regime is presented. Received 16 March 2001 and Received in final form 30 October 2001     

Temperature dependences of resistivity and magnetoresistivity for half-metallic ferromagnets

Peculiarities of transport properties of three- and two-dimensional half-metallic ferromagnets are investigated, which are connected with the absence of spin-flip scattering processes. The temperature and magnetic field dependences of resistivity in various regimes are calculated. The resistivity is proportional to T ^9/2 for T < T ^* and to T ^7/2 for T > T ^*, T^* being the crossover temperature for longitudinal scattering processes. The latter scale plays also an important role in magnetoresistance. The contribution of non-quasiparticle (incoherent) states to the transport properties is discussed. It is shown that they can dominate in the temperature dependence of the impurity-induced resistivity and in the tunnel junction conductivity. Received 16 September 2002 / Received in final form 6 November 2002 Published online 31 December 2002     

Lifetimes in the ground-state band and the structure of 118Te

Lifetimes of excited states in ¹¹⁸Te have been measured using the Doppler Shift Attenuation (DSA) and Recoil Distance (RD) methods in the ¹⁰⁹Ag(¹³C, p3n) reaction at a beam energy of 54 MeV. Lifetime values of the ground-state band levels with spins I ^π = 2⁺-16⁺ have been obtained. The excitation energies and B(E2) values are interpreted in the framework of a version of IBFM ( IBM + 2qp) with the maximum boson number exceeding its standard value. A satisfactory agreement with experimental level scheme and B(E2) values for the ground-state band is achieved. Received: 7 June 2001 / Accepted: 7 February 2002