Influence of exciton energy on intersubband transition of chirped superlattice GaAs/AlGaAs quantum cascade laser

The influence of exciton energy on intersubband transition was simulated for a chirped supperlattice quantum cascade laser of GaAs/Al_xGa_1-xAs. Exciton energy was modelled as a function of QW width for alloys of various percentages of constituent elements. The results showed that the exciton energy decreased proportionally with increasing QW width. Models were also generated to study exciton energy as a function of the percent alloy contents of Al_xGa_1-xAs barriers for QWs of various widths. Exciton energy showed characteristics of higher discrete energy when QW width was narrower. Transition energy was also simulated from e₁ and e₂ to the 1s exciton state as functions of applied electric field at various QW widths. Our simulation results showed that the transition energy from e₂ to the 1s exciton state increased proportionally to the increasing strength of the electric field. This transition energy was indicative of THz range radiation.     

Calculation of subband breadth of GaAs/AlGaAs superlattice

From the view of electron waving, taking account of the electron wave reflections at the interface between the well and the potential barrier layer we discuss the electronic states above the barriers in a GaAs/AlGaAs superlattice. We present a new method on calculating the breadth of the subband and the calculated breadth of GaAs/AlGaAs superlattice is in good agreement with experimental results.     

Auger decay of X-point excitons in a type II GaAs/AlGaAs superlattice

The origin and characteristics of the cross-interface photoluminescence observed in hydrostatic-pressure-induced, type II GaAs/AlGaAs superlattices is investigated. A low quantum efficiency luminescence feature with an Auger-limited lifetime, as evidenced by the observation of the “hot” Auger electrons recombining across the GaAs direct-gap, was observed. This feature has been found in a set of MOCVD-prepared superlattices, identical, except for the Al-mole-fraction of the barriers. The feature exhibiting Auger recombination is attributed to the recombination of a cross-interface exciton bound to a neutral donor in the AlGaAs. An impurity-bound-exciton seems necessary to explain the over 3-decade purely exponential decays observed in these experiments.     

Phonon heating of two-dimensional exciton gases in GaAs/AlGaAs quantum wells

We report the first measurements of the interaction of non-equilibrium phonons with two-dimensional exciton gases (2DExGs). The rise in the effective temperature of the 2DExG produced by the phonons depends on the width of the quantum well and the exciton sheet density and hence on the ratio τ^?1 (ex-ph)/τ^?1 (ex-ex). The dependence of the effective temperature rise on this ratio is attributed to the non-equilibrium frequency distribution of the phonons incident on the 2DExG.     

Inter-island energy transfer and in-plane exciton migration in AlGaAs/GaAs quantum wells detected by exciton dynamics

We present the results of optical, steady-state and time-resolved studies of photoluminescence and photoluminescence excitation in high-quality Al_0.3Ga_0.7As/GaAs quantum wells in which the presence of large (larger than the exciton radius) atomically flat islands can be inferred, identical to the case of interrupted MBE growth. Migration of excitons towards lower-lying energy states induced by local potential fluctuations and/or progressive localisation has been revealed and the transition rate between quantum well regions 24 to 25 monolayers thick has been derived to be 290 ps⁻¹.     

Temperature dependent time-resolved exciton luminescence in GaAs/AlGaAs quantum wires and dots

Transient photoluminescence of GaAs/AlGaAs quantum wires and quantum dots formed by strain confinement is studied as a function of temperature. At low temperature, luminescent decay times of the wires and dots correspond to the radiative decay times of localized excitons. The radiative decay time can be either longer or shorter than that of the host quantum well, depending on the size of the wires and dots. For small wires and dots (∼ 100 nm stressor), the exciton radiative recombination rate increases due to lateral confinement. Exciton localization due to the fluctuation of quantum well thickness plays an important role in the temperature dependence of luminescent decay time and exciton transfer in quantum wire and dot structures up to at least ∼ 80 K. Lateral exciton transfer in quantum wire and dot structures formed by laterally patterning quantum wells strongly affects the dynamics of wire and dot luminescence. The relaxation time of hot excitons increases with the depth of strain confinement, but we find no convincing evidence that it is significantly slower in quasi 1-D or 0-D systems than in quantum wells.     

Long-range spatial correlations in the exciton energy distribution in GaAs/AlGaAs quantum wells

Variations in the width of a quantum well (QW) are known to be a source of broadening of the exciton line. Using low temperature near-field optical microscopy, we have exploited the dependence of exciton energy on well width to show that in GaAs QWs, these seemingly random well-width fluctuations actually exhibit well-defined order-strong long-range correlations appearing laterally, in the plane of the QW, as well as vertically, between QWs grown one on top of the other. We show that these fluctuations are correlated with the commonly found mound structure on the surface. This is an intrinsic property of molecular beam epitaxial growth.     

Temperature and density dependence of exciton lifetimes in GaAs/AlGaAs multiple quantum wells

The photoluminescence linewidths and excition lifetimes of free excitons in GaAs/AlGaAs multiple quantum wells were systematically investigated as a function of temperature, quantum well width, and carrier density. The experimental results showed that the exciton decay processes were strongly related to the linewidth of the exciton and the exciton binding energy.     

Quantum Monte Carlo simulation of exciton–exciton scattering in a GaAs/AlGaAs quantum well

We present a computer simulation of exciton–exciton scattering in a quantum well. Specifically, we use quantum Monte Carlo techniques to study the bound and continuum states of two excitons in a 10 nm wide GaAs/Al_0.3Ga_0.7As quantum well. From these bound and continuum states we extract the momentum-dependent phase shifts for s-wave scattering. A surprising finding of this work is that a commonly studied effective-mass model for excitons in a 10 nm quantum well actually supports two bound biexciton states. The second, weakly bound state may dramatically enhance exciton–exciton interactions. We also fit our results to a hard-disk model and indicate directions for future work.     

Properties of exciton states in GaAs/AlGaAs quantum wells in the presence of a quasi-two-dimensional electron gas

The changes in binding energy and oscillator strength of the exciton state due to the screening by a quasi-two-dimensional electron gas are calculated self-consistently in the approximation of noninteracting electrons and in the local field approximation. It is shown that the collapse of the bound state occurs at very low concentrations, N _s≈5×10⁹ cm^?2, which is a consequence of the inclusion of the nonlinearity of the response of the system to a Coulomb perturbation. The temperature dependence of the exciton collapse is investigated. The phase diagram of the dissociation of the given bound state is constructed, and the region in which it is possible to observe experimentally the temperature dependence of the exciton collapse is indicated.     

Field-induced lifetime enhancement and ionization of excitons in GaAs/AlGaAs quantum wells

Picosecond and nanosecond luminescence studies of GaAs/AlGaAs quantum wells exposed to electric fields perpendicular to the layers are reported. The drastic red-shift of the photoluminescence with the electric field strength is accompanied by a strong increase of the electron-hole recombination lifetime. These features are most dominant for the wider wells due to the stronger polarization of the confined electron-hole pairs. Our observations are consistent with the model of the Quantum-Confined Stark Effect. In contrast, for high fields in the regime of ∼100 kV/cm field ionization limits the confinement of electrons and holes and leads to a strong decrease of the photoluminescence yield and lifetime with increasing field strength.     

Anomalous influence of magnetic field on the indirect exciton in GaAs/AlGaAs double quantum wells

A study is reported of exciton luminescence in GaAs double quantum wells produced in electric and magnetic fields. It has been found that the indirect-exciton line (IX) behaves anomalously, namely, one observes a magnetic-field-induced low-energy shift of the IX line, and the onset of periodic (≈5 s) fluctuations in the IX-line intensity. Fiz. Tverd. Tela (St. Petersburg) 40, 803–805 (May 1998)     

Time-resolved four-wave-mixing of exciton transitions in GaAs/AlGaAs quantum wells: Novel effects in the lineshape

We investigate coherent exciton transitions in GaAs/Al _x Ga_1–x As quantum wells using subpicosecond four-wave-mixing spectroscopy. In a first part, we show that the four-wave-mixing lineshape deviates considerably from earlier predictions when the detailed structure of the excitons is taken into account, and we study the density dependence and excitation energy dependence in detail. In a second part, we discuss the observation of quantum beats due to the coherent superposition of different excitonic transitions and show how the analysis of the lineshape can yield information about relaxation processes.Dedicated to H.-J. Queisser on the occasion of his 60th birthday     

Suppressed intermixing in InAlGaAs/ AlGaAs/GaAs and AlGaAs/GaAs quantum well heterostructures irradiated with a KrF excimer laser

The influence of gallium arsenide surface modification induced by irradiation with a KrF excimer laser on the magnitude of the quantum well (QW) intermixing effect has been investigated in InAlGaAs/AlGaAs/GaAs QW heterostructures. The irradiation in an air environment with laser pulses of fluences between 60 and 100 mJ/cm² has resulted in the formation of a gallium oxide-rich film at the surface. Following the annealing at 900 °C, up to 35 nm suppression of the band gap blue shift was observed in all the laser irradiated samples when compared to the non-irradiated samples. The origin of suppression has been discussed in terms of stress controlled diffusion. PACS 78.55.Et; 66.30.Lw; 73.21.Fg     

Impurity cyclotron resonance in InGaAs/GaAs superlattice and InGaAs/AlAs superlattice grown on GaAs substrates

Various temperature measurements of cyclotron resonance (CR) under pulsed ultra-high magnetic field up to 160 T were carried out in InGaAs/GaAs superlattice (SL) and InGaAs/AlAs SL samples grown by molecular beam epitaxy on GaAs substrates. Clear free-electron CR and impurity CR signals were observed in transmission of CO₂ laser with wavelength of 10.6 μm. A binding energy of impurities in these SLs was roughly estimated based on the experiment as result, and we found it was smaller than the previous experimental result of GaAs/AlAs SLs and theoretical calculation with a simple model.     

Modeling and experimental study of 780–808-nm AlGaAs/GaAs injection lasers with electron superlattice barriers

Electron superlattice barriers (ESBs) were used in AlGaAs/GaAs injection lasers to improve the electron confinement of the active layer by Bragg reflection of electron waves. The design of a separate-confinement heterostructure (SCH) laser with ESBs operating at 780–808 nm was optimized. Conventional SCH and SCH-ESB were prepared by low-pressure MOCVD epitaxy. Oxide stripe lasers with stripe widths of 100 and 200µm were prepared. The threshold current density of 0.3 kA/cm² and the characteristic temperature constantT ₀=220 K were measured at a wavelength of 808 nm for SCH-ESB lasers with an active-layer thickness of 40 nm and a resonator length of 0.4–0.5 mm. For conventional SCH lasers with the same geometry, a threshold current density of 0.42 kA/cm² andT ₀=160 K were obtained. Experimental results on the low-temperature photoluminescence characterizing ESB regions are presented and are compared with the calculated miniband energy spectrum of the superlattice structure. The leakage currents for ordinary SCH and SCH-ESB lasers were analyzed. Experimental verification of a reduction in the leakage current for SCH-ESB lasers was obtained.     

First-principles study of stability of point defects and their effects on electronic properties of GaAs/AlGaAs superlattice

When the GaAs/AlGaAs superlattice-based devices are used under irradiation environments, point defects may be created and ultimately deteriorate their electronic and transport properties. Thus, understanding the properties of point defects like vacancies and interstitials is essential for the successful application of semiconductor materials. In the present study, first-principles calculations are carried out to explore the stability of point defects in GaAs/Al_0.5Ga_0.5As superlattice and their effects on electronic properties. The results show that the interstitial defects and Frenkel pair defects are relatively difficult to form, while the antisite defects are favorably created generally. Besides, the existence of point defects generally modifies the electronic structure of GaAs/Al_0.5Ga_0.5As superlattice significantly, and most of the defective SL structures possess metallic characteristics. Considering the stability of point defects and carrier mobility of defective states, we propose an effective strategy that Al_As, Ga_As, and Al_Ga antisite defects are introduced to improve the hole or electron mobility of GaAs/Al_0.5Ga_0.5As superlattice. The obtained results will contribute to the understanding of the radiation damage effects of the GaAs/AlGaAs superlattice, and provide a guidance for designing highly stable and durable semiconductor superlattice-based electronics and optoelectronics for extreme environment applications.