75As中子辐射俘获截面的实验测量及蒙特卡罗修正

在四川大学2.5 MV静电加速器上， 用活化法测量了29—1 100 keV 能区中子引起的75As(n， γ)76As反应截面， 并用MCNP 4C程序对实验中由中子的多次散射、 注量率衰减效应等引起的偏差进行了修正， 最后将所得结果与已有数据进行了比较。 We have measured the neutron radiative capture cross section of 75As in the energy range of En=29—1 100 keV using the activation technique at 2.5 MV electrostatic accelerator of Sichuan University. The experimental data were then corrected for multiple scattering and self shielding effects with MCNP 4C code. We also compared our results， with the existing measurement， calculation and evaluated data in ENDF/B Ⅵ.     

间接测量中重放射性核中子俘获截面——替代比率法

s过程中的放射性核素中子俘获截面对天体核合成和核素丰度有重大影响, 在直接测量异常困难的情况下, 替代比率法是获得放射性核素中子俘获截面数据的一种间接新方法。 简单介绍了替代比率法理论, 并简要论述了用替代比率法推导中重核区放射性核素中子俘获截面的可行性。 The radioactive nuclei neutron capture cross section is very important to nuclearsynthesis and nuclide abundance in s process, but it is difficult to be measured directly because of the target production. A new method, surrogate ratio method which is developed from surrogate method, could be used to determine the cross section of radioactive nuclei neutron capture. In this paper, the surrogate ratio method was introduced and the feasibility was discussed to deduce the desired neutron capture cross sections with surrogate ratio method.     

17C反应截面和去中子截面

利用日本理化学研究所的放射性束流线RIPS, 测量了能量为79A MeV的¹⁷C在¹²C反应靶上的反应截面, 并同时得到了¹⁷C的移去1个、2个及3个中子的截面; 分别利用有限力程Glauber模型和少体Glauber模型结合壳模型的谱因子分析了反应截面和移去1个中子截面, 研究了¹⁷C的密度分布、结构和价中子布居. 反应截面和中子移去截面是两个相互独立的量, 通过对两者的分析, 都可以得出¹⁷C由芯核¹⁶C和价中子组成, 并且价中子主要处于d_5/2轨道的结论. 总结了现有的碳同位素的反应截面和相互作用截面的工作.     

The Reaction Cross Section and Neutron Removal Cross Sections of 17C

The reaction cross section, together with the one-, two- and three neutron removal cross sections, of ¹⁷C with the energy of 79A MeV on carbon target were measured using the radioactive beam line RIPS of RIKEN. The reaction cross section and the one-neutron removal cross section were analyzed within the frame of Glauber model. Both the analyses favor the dominant configuration of a ¹⁶C core (2⁺) plus a d_5/2 valence neutron for ¹⁷C. The work for the neutron-rich carbon isotope on the reaction cross section σ_R and the interaction cross section σ_I on ^{12C target are summarized.}     

20MeV以下快中子与56Fe非弹性散射截面的分歧研究

56Fe的非弹性散射截面在核装置中子输运计算中扮演着重要的角色,但无论从实验数据还是从评价数据,非弹性散射截面都存在很大分歧,它的数据直接影响到核装置的设计、建造与运行维护。本工作从实验数据本身出发,深入分析了不同实验室测得的847 keV的γ产生截面的分歧,经转化后补充非弹性散射截面的实验空白能区,并同时利用满足全截面、去弹截面等截面自洽关系的评价方法推荐了高精度的快中子与56Fe的非弹反应截面结果。积分检验表明,新的非弹截面的改进使得评价数据与积分实验结果一致,较CENDL-3.1的评价数据结果有显著改善。Knowledge about the inelastic scattering cross section of 56Fe is very important in neutron transportation calculation. However there are great discrepancies not only between experimental data but also between evaluated data. More detail analysis was performed for inelastic scattering cross section in the fast range up to 20 MeV where there are significant differences among the main evaluated libraries, mainly caused by the different inelastic scattering cross section measurements. The large discrepancies on 56Fe(n, n₁'γ) cross section which could fill the neutron energy blank of the 56Fe(n,inl) were clarified and were converted to the inelastic scattering cross section of 56Fe. And the high-quality results were evaluated by using the unitarity constrain among total cross section, noelastic reaction and other reactions. The integral experiment result indicates that the new evaluated result of inelastic cross section brings greater improvement than that of CENDL-3.1.     

轻丰中子核反应中子集团产生截面的理论研究

采用Boltzmann-Langevin方程研究了能量为35MeV/u的¹⁴Be, ⁸He,⁶He,¹¹Li,¹⁷B,¹¹Be,¹⁹C与¹²C靶的反应,计算了产生中子集团的截面, 发现^14,Be与¹²C靶反应产生⁴n的截面与实验值符合得很好. 通过这几个入射核与¹²C靶形成中子集团截面的对比, 发现核的晕中子越多产生中子集团的截面越大, 晕中子数相同时, 质量数越大产生中子集团的截面越大.中子集团可能主要来自晕核子.     

Maxwellian Averaged Neutron Capture Cross Sections in 56Fe and 57Fe

Measurements of the keV-neutron capture cross sections and radiative γ-ray spectrum of 56Fe and 57Fe are performed based on a 7 Li（p,n）7 Be reaction neutron source. The incident neutron spectrum on a capture sample is measured by means of a time-of-flight （TOF） method with a 6Li-glass detector. The radiative capture 7-rays emitted from an iron CS Fe or 57 Fe） or standard gold （197Au） sample are detected by a large anti-Compton NaI（TI） spectrometer covered with a heavy shield. The capture yields of samples are obtained by applying a pulse-height weighting technique to the corresponding capture γ-ray pulse-height spectrum. The Maxwellian averaged neutron capture cross sections of 56Fe and 5T Fe are derived according to the present capture cross section results.     

12C快中子辐射俘获反应中的共振现象

主要研究中子辐射俘获反应中的共振现象,利用DSD模型计算激发能量在5—25MeV能区的¹²C(n,γ0)反应截面与E_n=9MeV时的角分布.所考虑的反应机制包括复合核俘获、直接和半直接俘获、复弹性和非弹性散射道的辐射俘获.计算表明,矮共振的峰值在激发能量为13MeV处;巨共振的峰值位置在激发能量21MeV处.计算结果与实验符合较好.     

光子穿透系数及同质异能态俘获截面的研究

合理地给出了复合核反应光子穿透系数及同质异能态俘获截面的计算公式,其中包括统计和非统计过程.通过求解级联γ退激过程计算光子穿透系数,既合理地扣除(n,γn)过程,又包括首次γ跃迁至中子分离能B_n以上能级的贡献.以4MeV以下中子和⁵⁹Co及¹⁰³Rh的反应为例,比较用不同方法计算的光子穿透系数,计算同质异能态俘获截面并和实验数据进行比较,最后对结果进行了分析和讨论.     

Boron Neutron Capture Therapy

Physics of Atomic Nuclei - Fundamentals of boron neutron capture therapy of malignant tumors are outlined, and the current status of the development of epithermal-neutron sources on the basis of...     

中子分布弥散度对反应总截面的影响

在引入库仑场修正的Glauber模型基础上,区分入射弹核和靶核中的中子、质子,并考虑有限力程相互作用,发展了一个计算核反应总截面的微观修正模型.如果引入一个核内中子分布弥散度随中子分离能的变化关系,则能较好地解释奇异核(如⁸He,¹¹Li,¹¹Be)反应总截面的反常增加.同时,该修正模型还能在低能到高能的范围内较好地拟会稳定核的反应总截面.     

Analysis of Neutron Double-Differential Cross Section of n＋^14N at 14.2 MeV

Abstract By using a new reaction model for light nuclei, the double-differential cross section of n ^14N reactions at En=14.2 MeV has been analyzed. In the case of n ^14N reactions, the reaction mechanism is very complex, there are over one hundred opened partial reaction channels even at incident energy En=14.2 MeV. In this paper the opened reaction channels are listed in detail. With LUNF code the model calculation is performed to analyze the doubledifferential cross sections of total outgoing neutron. The calculated results agree fairly with the experimental data. The results indicate that the pre-equilibrium mechanism dominates the whole reaction processes, and the recoil egect in light nuclear reactions is essentially important. 5He emission has been considered, but it is only a small contribution to thedouble-differential cross section at incident energy En=14.2 MeV.     

Analysis of Neutron Double-Differential Cross Section of n+14N at 14.2 MeV

By using a new reaction model for light nuclei, the double-differential cross section of n 14N reactions at En = 14.2 MeV has been analyzed. In the case of n 14N reactions, the reaction mechanism is very complex, there are over one hundred opened partial reaction channels even at incident energy En = 14.2 MeV. In this paper the opened reaction channels are listed in detail. With LUNF code the model calculation is performed to analyze the doubledifferential cross sections of total outgoing neutron. The calculated results agree fairly with the experimental data. The results indicate that the pre-equilibrium mechanism dominates the whole reaction processes, and the recoil effect in light nuclear reactions is essentially important. 5He emission has been considered, but it is only a small contribution to the double-differential cross section at incident energy En = 14.2 MeV.     

快中子在Li核上的弹性散射微分截面

用伴随粒子飞行时间法测量了14.7MeV中子在⁶Li和⁷Li核上的弹性散射截面,并用蒙特卡罗方法对中子在样品中的通量衰减、多次散射作了修正.本文工作与他人工作以及理论数据作了比较.给出了截面的勒让德系数;截面实验点总误差在10%到15%之间,其中统计误差为1%-5%.     

Theoretical Analysis of Neutron Double-Differential Cross Section of n+10B at 14.2 MeV

By using a new reaction model for light nuclei, the double-differential cross sections of n+ 10B reactions atEn ＝ 14.2 MeV have been analyzed. In the case of n+10B reactions there are over one hundred opened partial reactionchannels. Besides the sequential particle emissions, there is also the three-body breakup process, in which the kinematicsis classified into four types. In this paper the opened reaction channels are listed in detail with the LUNF code, withwhich the model calculation is performed to analyze the total outgoing neutron double-differential cross sections. All ofthe fittings agree fairly well with the measurements. The calculation results indicate that the pre-equilibrium mechanismdominates the whole reaction processes, and the recoil effect in light nuclear reaction is essentially important.     

Theoretical Analysis of Neutron Double-Differential Cross Section of n ＋^19F at 14.2 MeV

A new light nuclear reaction model has been developed and the double-differential measurements of lp shell nuclei have been analyzed successfully. Now, the application of this model is expanded to 19F of the 2s-ld shell nucleus. The double-differential cross section of total outgoing neutron for n ＋^19F reactions at En=14.2 MeV has been calculated and analyzed, which agrees fairly well with the experimental measurements. In this paper, the contributions from different reaction channels to the double-differential cross sections have been analyzed in detail. The calculations indicate that this light nudear reaction model is also able to be used for the 2s-ld shell nucleus so long as the related level scheme couM be provided sufficiently.     

Theoretical Analysis of Neutron Double-Differential Cross Section of n+11B at 14.2 MeV

A new reaction model for light nuclei is proposed to analyze the measured data, especially for the doubledifferential cross sections. In this paper the calculation with this model is employed to analyze measurements of the total outgoing neutron double-differential cross sections for n+11B reactions at En = 14.2 MeV. The representation of the double-differential cross sections of the second emitted particles is given in detail. The calculation results indicate that the recoil effect in light nuclear reaction is essentially important. The reaction channels are discussed in detail.     

单能中子源中低能成份对活化截面测量的影响

对用单能中子源作活化截面测量时低能中子干扰的影响作了分析研究,并从测量的两种常用中子源T(d,n)⁴He和D(d,n)³He的中子源能谱中验证了这种定性分析.最后给出了两个比较典型的反应⁵⁸Ni(n,P)⁵⁸Co和⁶⁴Zn(,P)⁶⁴Cu反应的截面测量结果.